Photochemical Processes in Organized Molecular Systems
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1 Photochemical Processes in Organized Molecular Proceedings of the Memorial Conference for the late Professor Shigeo Tazuke Yokohama, Japan September 22-24, 1990 Editor-in-Chief Kenichi Honda Tokyo Institute ofpolytechnics Executive Editors Noboru Kitamura Research Development Corporation of Japan Hiroshi Masuhara Osaka University Co-Editors Tomiki Ikeda Masahiko Sisido Tokyo Institute of Technology Mitchell A. Winnik University of Toronto 1991 NORTH-HOLLAND AMSTERDAM LONDON NEW YORK TOKYO
2 XI TABLE OF CONTENTS Preface The Memorial Conference for the Late Professor Shigeo Tazuke Group Photograph of the Conference Professor Shigeo Tazuke Acknowledgements v vi vii viii x Chapter I: PHOTOINDUCED ELECTRON AND ENERGY TRANSFER PROCESSES Ultrafast Laser Photolysis Investigations on the Photoinduced Electron Transfer and Dynamics of Transient Ion Pairs N. Mataga 3 Dynamics of Photoinduced Electron Transfer in Solution LR. Gould, R.H. Young and S. Fand 19 Control of Electron Transfer Rates by Motions of Atoms and Molecules J.R. Miller 41 Fluorescence Probes Based on Adiabatic Photochemical Reactions W. Rettig, R. Fritz and J. Springer 61 Multicomponent Fluorescence Decay Analysis in Intramolecular Excimer Formation with Dipyrenylalkanes K.A. Zachariasse, G. Duveneck, W. Kühnle, U. Leinhos and P. Reynders 83 Excitation Hopping between Two Identical Chromophores Attached to Both Ends of Alkanes T. Ikeda, B. Lee and S. Tazuke 101
3 xii Picosecond Dynamics of Dyes in Heterogeneous Environments K. Yoshihara and K. Kemnitz 117 Chapter II: PHOTOREDOX REACTIONS IN SOLUTION Intramolecular, Photochemical Electron and Energy Transfer TJ. Meyer 133 Intramolecular Electron Transfer and Energy Transfer in Bimetalated Compounds T. Ohno, K. Nozaki and M.-A. Haga 151 Solvent Effect on Electron-Transfer Quenching of *Ru(bpy) H.-B. Kim, N. Kitamura and S. Tazuke 163 Photosensitized Reactions by [Re(bpy)(CO)3X] C. Pac, S. Kaseda, K. Ishii, S. Yanagida and O. Ishitani 177 Magnetic Field Effects on Photoinduced Electron Transfer and the Succeeding Processes in Organized Molecular Assemblies T. Matsuo, H. Nakamura, S. Usui, H. Yonemura and A. Uehata 187 Highly Specific Isomerization of Aromatic Olefin Radical Cations Produced by Photosensitized Electron Transfer K. Tokumaru, Y. Kuriyama, T. Arai, I.K. Lednev, R. Akaba and H. Sakuragi 199 Photoinduced Single Electron Transfer Fragmentation and Cyclization Reactions. Medium and Interfacial Effects D.G. Whitten, C. Chesta, X. Ci, M.A. Kelle«and V.W.W. Yam 213
4 Xlll Chapter III: PHOTOCHEMISTRY IN ORGANIZED MOLECULAR SYSTEMS Luminescence Spectroscopy and Polymer Chemistry F.C. De Schryver 239 Fluorescence Studies of Hydrophobie Polymers in Water: Phase Transitions in Aqueous Poly-(N-Isopropylacrylamide) Solutions F. M. Winnik 257 Polymer Diffusion in Latex Films M. A. Winnik, Y. Wang and C.-L. Zhao 275 Steady State Intrinsic Fluorescence Studies of Block Copolymer Micelles D.A. Ylitalo, A.S. Yeung and C.W. Frank 295 Interfacial Characteristics of Doped Polymer Films: Total Internal Reflection Fluorescence Spectroscopic Study A. Itaya and H. Masuhara 315 Energy Transfer and Migration in Polymer LB Films M. Yamamoto, S. Ito and S. Ohmori 329 Regulation of Liquid Crystalline Alignment Change by Photochromic Molecular Films K. Ichimura 343 Synthetic Design of Liquid Crystals for Directional Electron Transport M.A. Fox and H.-L. Pan 359 Diffuse Reflectance Laser Photolysis of Adsorbed Molecules F. Wilkinson and R. Beer 377 Chapter IV: TOWARD INTEGRATED MOLECULAR SYSTEMS Photochromism of Diarylethenes with Heterocyclic Rings M. Irie 399
5 xiv Photo-Induced and Electrochemical Redox Molecular T. Shimidzu, T. Iyoda, H. Segawa and K. Honda 411 Information Storage Using Photoelectrochemical Hybrid Z.F. Liu, K. Hashimoto and A. Fujishima 427 Electroluminescence in Organic Thin Films T. Tsutsui, C. Adachi and S. Saito 437 Electron-Phonon Interaction in Photochemical Hole Burning in Porphyrin-Polymer K. Horie 451 Photo-Electric Conversion with Langmuir-Blodgett Films M. Fujihira 463 Fractals and Excitation Transfer in Molecular Assemblies I. Yamazaki, N. Tamai and T. Yamazaki 483 Microphotoconversion: Exploratory Chemistry by Laser and Microfabrication H. Masuhara 491 Micrometer Photochemical Dynamics in Organized Molecular N. Kitamura and H. Masuhara 509 Appendix; The Title of Contributed Posters 525 Author Index 531 Subject Index 533
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