Optical Bessel-like Beams with Engineered Axial Phase and Intensity Distribution

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1 JLMN-Journal of Laser Micro/Nanoengineering Vol. 3, No. 3, 08 Optical Bessel-like Beams with Engineered Axial Phase Intensit Distribution Sergej Orlov, Alfonsas Juršėnas, Ernestas Nacius Center for Phsical Sciences Technolog, Industrial laborator for photonic technologies, Sauletekio av. 3, Vilnius, Lithuania Bessel beams are known for their propert of maintaining propagation-invariant transverse intensit distribution. The true Bessel beams has unlimited energ, however the experimental realiation of limited energ Bessel-like beams provides almost diffraction-free beams over a certain distance. These beams are applicable to microfabrication, particle manipulation etc. where long narrow intense beam is needed. A tpe of laser beams that maintains narrow intensit peak for long distances are often called optical needles. In this paper we propose a construction of an "optical needle" using a superposition of vector Bessel beams for flexible engineering of axial intensit profile. We investigate both theoreticall experimentall generation of various optical beams of different axial profiles, lengths, beam widths etc. We use a spatial light modulator as a to model of an optical element to shape the spatial spectrum of the beam. Moreover, we demonstrate distortions introduced into the optical needle b a planar interface between two dielectric media: spherical aberration astigmatism due to the nonero inclination angle discuss was to correct them. DOI: 0.96/jlmn Kewords: Bessel beam, focal line engineering, diffraction, spatial light modulator, nondiffracting beams, planar interface, laser microproecessing.. Introduction Laser beam shaping is an important technique used in modern laser beam applications such as light sheet microscop, microfabrication photopolimerisation to name a few. In situations where the same pattern is needed over long propagation distance it is advantageous to use nondiffracting beams. One of them is Bessel beam [], which exhibits a long focal line with high length to width ratio []. Due to this propert it can be perceived as an optical needle. Optical needle beams are advantageous to use in applications such as fabrication of long canals in bulk material, trapping man particles simultaneousl [-4]. In some cases the microfabrication process is sensitive to the polariation structure of the laser beam. Nonhomogeneous polariations like aimuthal or radial have been shown to affect the efficienc of laser drilling procedure [5,6]. The polariation control of optical needle could also increase the speed of the laser microprocessing of the materials will be discussed in this publication as an additional degree of freedom in the use of vectorial Bessel beams. A multitude of different beam shaping methods can be used in order to experimentall obtain complex focal structures. One of the approaches is to use the spatial light modulator (which is a dnamic optical element but requires adjustments to the design in order to be flexibl used for high laser power applications), another example is geometrical phase elements (which are static but can sustain high laser power used in microfabrication applications), an example is given in [7]. In this work we present the formation of optical needle b superimposing man monochromatic vector Bessel beams to achieve desired axial intensit distribution. We anale the generation of various optical needles with different axial intensit profiles. In order to test our theoretical results we compare our simulated beam intensit profiles with experimentall obtained ones. The experiment is conducted using spatial light modulator as beam spatial spectrum alternator. Furthermore we numericall demonstrate a method for compensating the axial intensit distortions caused b focusing the laser beam trough air-dielectric interface.. Control of an axial intensit of vector Bessel beams In this chapter we introduce the vector description of Bessel beams [8] a method of controlling the intensit distribution in the propagation direction of the beam [9,0].. Vector Bessel beams Consider an ideal monochromatic scalar Bessel beam complex amplitude [] ψ ( ρφ,, ) = J ( k ρ)exp(imφ + i k ), () m m ρ ρ, here J m -Bessel function of order m, ρφ,, -circular clinder spatial coordinates, k k - transverse longitudinal of the wave vector k, m -topological charge. The scalar description can be extended to a full vector solution (denoted here as M N ) of Maxwell s equations in the free space using [8,] M = ( aψ m ), N = M, () k vector solutions M, N are mutuall orthogonal b the definition. The vector a enforces here vectorial boundar 44

2 JLMN-Journal of Laser Micro/Nanoengineering Vol. 3, No. 3, 08 conditions that solutions M, N should obe []. Therefore the choice of a directl influences the polariation of the resulting electromagnetic field. For instance, with a = e x the field represented b the M solution is a vector Bessel beam, which is linearl polaried in the direction ik M = i kej0( kρρ) + e sin( ϕ) kρj( kρρ) e (3) For a = e the electromagnetic field represented b the N solution is also a linearl polaried in the direction vector Bessel beam J ( kρρ ) kρ N = ex x k ρ ( ρρ ) ( ρ) ( ρ) J k k J k k ρ ρ ρ ρ + e J0 ( kρ ρ ) k + x, (4) ρ ρ J k kρ ik + ike e ρ here ex, e, e- Cartesian unit vectors. An analsis of Eqs. (3,4) reveals that under tight focusing conditions, i.e. large numerical apertures, the longitudinal component of the electric field becomes larger.. Control of the axial intensit We can express linearl polaried electromagnetic fields from Eqs. (3,4) close to the axis ( ρ 0 ) as ( ) M ρ = e, (5) ik 0 ik e k + k ρ ik N( ρ 0) = e e. (6) k For the sake of brevit we will consider now a smmetrical mode, which is a sum of TM TE modes, see Eqs. (5, 6). The axial intensit control of a linearl polaried Bessel beam superposition is achieved as follows. Let us assume a continuous representation of the axial beam profile via the spatial beam spectrum + i A( K ) ( ) K = f e d π (7) here f( ) is a desired axial beam profile. We assume, that k = k0 + K, where k 0 is a carrier wave vector. If k >> K, we can rewrite (7) as a Fourier transform 0 Ψr () = A( k) ψr (; k) dk, (8) where ψr (; ) is a smmetric combination of M(; r ) k N(; r k ). Thus, the monochromatic superposition of Bessel beams in Eq. (8) enables us to opticall engineer the axial intensit distribution f( ) of a Bessel-like optical beam. We note, that the case of a discreet Fourier transform for scalar beams with a Talbot effect was presented elsewhere [9,0]. k 3. Focusing through an air-dielectric interface Focusing of the laser beam in the presence of an airdielectric interface results in appearance of optical field distortions like spherical aberration, astigmatism coma. Some of them are present onl when the optical beam enters the second media perpendicularl to the interface, another do appear when the beam enters the media at an angle []. We note that usuall Zernike polnomials are used to classif characterie optical aberrations [3]. Here we aim for a more general approach, where we compensate all possible aberrations due to the dielectric interface without the exact classification of them using Zernike polnomials. We assume that the focusing sstem is an aplanatic lens use Ref. [] as a guidance in our further derivations. Fig. Focusing of beam E inc trough air-dielectric interface using aplanatic lens L, the focusing angle in air is denoted θ in the dielectric medium θ with refractive index n. The focal field inside the dielectric material can be expressed as an integral over spatial angles of the plane waves [] π θmax s p E t = C { t ( θ)[ V( θ, φ) φ] φ + t ( θ)[ V( θ, φ) θ] θ } 0 0 i( kxx+ k) + ik e sin( θ ) cos( θ ) dθ dφ, (9) s p ikf t, t are Fresnel coefficients [], C = ikfe π is a constant, f - focal length of an aplanatic lens, θ, θ, φ angles of the plane wave components, see Fig., ˆ θ ˆ, ˆ θ, φ - spherical unit vectors, V - denotes the spatial spectra of the vector beam a linear combination of N ( θ, φ) M ( θ, φ) - angular spectra of the solutions from Eq. (3,4). An analsis of the expression (9) reveals that main causes for the distortions of the initial field after entering the second medium is due to Fresnel coefficients due to the the Snell s law, which changes the angular dispersion of the optical beam. Fig. Dependenc of the ratio t / t on angles θ refractive index n of the dielectric medium. We plot now the ratio t / t of the Fresnel coefficients for s- p- polariation as a function of angles refractive indices of the second medium, see Fig.. We can observe a rather large region in the parameter space θ,n, where the polariation structure of the spatial spectra won t be significantl affected b the interface itself be- 45

3 JLMN-Journal of Laser Micro/Nanoengineering Vol. 3, No. 3, 08 cause t / t. In this region the distortion in the engineered profile will be caused mainl b the Snell s law. The can be accounted for b adjusting the angular dispersion of the entering optical beam using the interchange of variables θ θ V( φθ, ) V( φθ, ), see Eq. (9). After aforementioned substitution we obtain the following expression π θmax s p E t = C { t ( θ)[ V( θ, φ) φ] φ + t ( θ)[ V( θ, φ) θ ] θ } 0 0 i( kxx+ k) + ik e sin( θ ) cos( θ ) dθ dφ. (0) Expressions in Eqs. (9, 0) can be numericall evaluated, so we choose an axial distribution described b a function f ( ) L L L L Π is a boxcar =Π( ) +Π( ), where ( ) (or a rectangular) function, L is its length, L L are positions. The intensit profiles in the longitudinal plane (x,) along with the intensit profiles of a spatial spectra are depicted in the Fig. 3. In this case, we use a slightl another axial intensit pro- f ( ) =Π L L present a comparison of two file ( ) cases with different angles between the optical axis the interface, see Fig. 4. We observe that the spatial spectra can be readjusted in order to ensure the expected length of the optical needle bot for the case on ero incidence angle for non-ero. Nevertheless, we do observe that the transverse distribution (computed along the red dashed line) is asmmetricall distorted, when focusing into the medium with non-ero incidence angle. Fig. 3 Intensit distribution of an optical needle with a two-step axial profile in the longitudinal plane (on the right) for two cases: first line direct focusing onto the interface, second line direct focusing but with corrections applied. Intensit distribution in the Fourier plane for both cases (on the left). The refractive index n =.8, the position of the interface is denoted b a red line (=0), expected length L of the optical needle is denoted b green vertical lines. The maximal angle in the spatial spectra isθ max = 45. On the left side of the interface (<0) (see Fig. 3) a reflected beam is observed in both cases. We note, that in the case of direct focusing onto the interface, the first rectangular profile is enlarged, shifted into the material its shape is somehow distorted. However, when the spatial spectra is modified to account for the presence of the interface, the expected axial profile is restored. 3. Focusing into medium under an angle Let us consider a case when the angle α between the optical axis of the beam the normal to the interface is nonero. Expressions for the electric field in this case can be found from the Eq. (0) b appling the rotation transformation to the incident field modifing the spatial spectra, so the k-vectors are properl transformed. More details on this procedure is out of the scope of this report, but details can be found in Ref. []. Fig. 4 Intensit distribution of an optical needle with a step-like axial profile in the longitudinal plane (first row) for two cases: direct focusing but with corrections applied for angles α = 0, 5. Second row, intensit distributions on the red dotted line for two cases depicted above. The position of the interface is denoted b a red line (=0), expected length L of the optical needle is denoted b green vertical lines. The maximal angle in the spatial spectra is θ max = 45. The refractive index of the second medium n = Experimental results 4. Setup of the experiment Numerical simulations were verified experimentall using an optical setup depicted in Fig. 5, where the spatial light modulator (SLM) was used to alter the spatial spectrum of the beam. The procedure is as follows:. A linearl polaried exped light beam (at the wavelength of 53 nm) reaches the matrix of the SLM at angle of incidence of ero degrees.. It is reflected from the liquid crstal mask of the SLM, where the phase mask encodes both amplitude phase spatial distribution. The 4f lens sstem (lenses L L3) is used to transfer the spectral image from the SLM to a lens L4. 3. The lens L4 makes a Fourier transform of the beam generated on the SLM. The sie of the liquid crstal mask of the SLM (x s, s ) focal length of the Fourier lens f 4 determine spatial frequencies f x f, which can be achieved in the setup. 4. Knowing the window of spatial frequencies (f x, f ), one can relate them to the maximal values of transverse wave vectors k x, k via k = πf. The pixel sie dx d of the SLM determines the pixel sie dkx dk of the spatial spectrum 46

4 JLMN-Journal of Laser Micro/Nanoengineering Vol. 3, No. 3, 08 Fig. 5 Experimental setup: CW laser, lenses (L-L5), objectives (OB OB), spatial light modulator (PLUTOVIS-006-A, HOLOEYE Photonics AG) CCD camera. Fig. 6 Intensit distributions of two experimentall observed optical needles with different lengths: L = -0. mm L = 0. mm (left) L = -0.6 mm L = 0.6 mm (right). Note that due to magnification scale is 6 times bigger. Fig. 7 Comparison of numericall calculated experimentall observed axial intensit profiles of beams: L = -0. mm L = 0. mm (left) L = -0.6 mm L = 0.6 mm (right). Fig. 8 Intensit distribution of numericall simulated (left) experimentall observed (right) optical needles in the transverse planes in the plane = 0 mm, L = -0. mm L = 0. mm. picture, which we obtain from Eqs. (7,8). 5. The complex valued spatial spectrum has to be encoded to a phase-onl picture, suitable for our SLM. The amplitude modulation is implemented here b using a checkerboard mask method, where groups of four phase-onl pixels emulate a single pixel with arbitraril chosen amplitude phase [4]. In this method the amplitude A of the com- Aexp iϕ is encoded as the sum of two plex amplitude ( ) different phases for a 4x4 checkerboard: ϕ = ϕ arccos A ϕ = ϕ+ arccos A. 6. Thus, a desired beam profile is generated in the focal region of the lens L4. It is captured recorded afterwards b the imaging sstem. A moving linear translation stage with mounted imaging sstem is moved along axis. 7. While the stage moves, the transverse intensit data at different distances from focal plane is imaged onto the CCD matrix of the camera, this image is recorded processed after-wards b a personal computer. Our optical sstem achieves transverse magnification of approximatel x7.4 a longitudinal magnification of approximatel x6. (boxcar) ( ) 4. Experiments with controllable axial intensit Optical needles with various potentiall interesting axial intensit profiles can be easil formed using the method described in section.. We start b a rectangular function f ( ) = Π L with different lengths L. Such needles can have different axial profiles, lengths, beawidths etc. The start of the rectangular function is at L = - L/ the end is at the L = L/, so that L = L L, we can control beam length in the direction. An example of two needles with different lengths are depicted in the Fig. 6. The figure 7 presents comparison of the maximum axial intensit distribution over the propagation distance between the numerical simulation (blue curve) experiment (red curve). Although, the intensit modulation peaks observed experimentall not alwas actuall match intensit modulation in the numericall modelled curves, which could be attributed to the use of the discretied SLM grid. We observe a ver similar intensit growth deca locations speed. In overall, a relativel good agreement between our numerical expectations experimental results is observed. Both axial profiles closel match numerical curves for the axial intensit distribution, see Fig. 7. A comparison of the transverse intensit distributions at the same plane = 0 mm is presented in the Fig. 8. Once again, it is clearl seen that the degree of conformit between numerical modelling experimental results is quite high. 4.3 Experiments with more complex axial profiles Lastl, we anale more complex axial profiles. For the start we anale creation of the profile, which was alread presented in the section 3 the two step-like function L+ L L3 + L4 f( ) =Π L L +Π L 4 L 3. () This particular profile consists of two different length boxcars. We have also analed more elaborate axial intensit profile containing two exponentials, one rising another falling: L+ L f( ) = exp [( L) ] Π L L L3 + L4 + exp [ ( L3) ] Π L4 L3. () Experiment numerical simulation results depicting the axial intensit are presented in the figure 9. Our numerical expectations are compared with our experimental results in the same Figure. Here, numerical expectations are show in 47

5 JLMN-Journal of Laser Micro/Nanoengineering Vol. 3, No. 3, 08 Fig. 9 Intensit distribution of experimentall obtained numerical calculated optical needles on the axis. Parameters are L = -0.5 mm, L = -0. mm, L3 = 0. mm, L4 = 0.5 for the two step function (left) L = -0.5 mm, L = -0. mm, L3 = 0. mm, L4 = 0.5 (right) for two adjacent exponential profiles. beams, with independent axial intensit profiles, axial positions amplitudes. Moreover, we have also discussed in great detail theoretical methods, which would let us compensate the spherical aberration, some astigmatism related effects due to the focusing the beam to the sample with non-ero angles of incidence. Those effects become more important nowadas in such applications like manufacturing high-aspect-ratio through-silicon vias, see Ref. [5]. These theoretical considerations will be also important in the near future while adapting techniques presented in this short report for the actual laser microprocessing of transparent materials. Further results on this approach together with an experimental implementation of the concept using geometrical phase elements (produced b Altechna R&D using birefringent nanogratings inscribed in the glass volume, see Refs. [7,6] for more details) will be presented elsewhere. Acknowledgements Fig. 0 Two-dimensional intensit distribution of the structures represented in the Fig.. Fig. Three-dimensional view of intensit distribution depicted in the Fig. (left picture). the blue, our experimental measurements are depicted in red, see Fig. 9. We note, that we have observed interference between two adjacent optical needles, which distorts the axial intensit profile near the focal plane (=0.0 mm). Our preliminar analsis reveals, that this is happening due to the phsical limitations of our experimental sstem the dimensions of the liquid crstal matrix in the SLM are too big to properl represent the fine phase modulation in the spatial spectrum. A two dimensional view on the intensit distributions can be found in the Figure 0. Lastl, a three dimensional representation of the intensit isosurfaces is depicted for this complex structure in Fig.. Using this experimental setup we were able to control not onl to the individual on-axis intensit distribution of an optical needle, but also the individual axial position of each individual optical needle their relative amplitudes in a superposition of man individual beams. 5. Conclusions discussions In conclusion, we have presented a flexible technique, which enables us to create experimentall controlled axial intensit distributions of linearl polaried optical needles. We have briefl discussed a creation of complex axial structures, which contains a number of individual optical This research is funded b the European Social Fund according to the activit Improvement of researchers qualification b implementing world-class R&D projects of Measure No LMT-K-7 References [] J. Durnin: J. Opt. Soc. Am. A, 4 (987) 65. [] M. Duocastella, C.B. Arnold: Laser Photonics Rev., 6 (0) 607. [3] R. Yang, R. Li: J. Quant. Spectrosc. Radiat. Transf., 78 (06) 30. [4] R. Stoian, M.K. Bhuan, G. Zhang, G. Cheng, R. Meer, F. Courvoisier: Adv. Opt. Techn. 7 (08) 65. [5] H. Misawa, S. Juodkais: 3D Laser Microfabrication Principles Applications Edited b. (Wile- VCH; 006). [6] R. Osellame, G. Cerullo, R. Ramponi: Femtosecond Laser Micromachining: Photonic Microfluidic Devices in Transparent Materials. (Springer Science & Business Media; 0). [7] M. Beresna, M. Gecevičius, P.G. Kaansk, T. Gertus: Appl. Phs. Lett., 98 (0) 00. [8] J.A. Stratton: Electromagnetic theor. (John Wile & Sons; 007). [9] M. Zamboni-Rached: Opt. Express, (004) 400. [0] M. Zamboni-Rached: Opt. Express, 4 (005). [] P.M. Morse, H. Feshbach: Methods of theoretical phsics. (Technolog Press; 946). [] L. Novotn, B. Hecht: Principles of nano-optics. (Cambridge universit press; 0). [3] G. D. Love: Appl. Opt. 36 (997) 57. [4] A. Dudle, R. Vasileu, V. Beli, N. Khilo, P, Ropot, A. Forbes: Opt. Commun., 85 (0) 5. [5] F. He, J. Yu, Y. Tan, W. Chu, C. Zhou, Y. Cheng, K. Sugioka: Sci. Rep. 7 (07) [6] (Received: June 4, 08, Accepted: October 5, 08) 48

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