PRINCIPLES OF NONLINEAR OPTICAL SPECTROSCOPY
|
|
|
- Thomas Quinn
- 6 years ago
- Views:
Transcription
1 PRINCIPLES OF NONLINEAR OPTICAL SPECTROSCOPY Shaul Mukamel University of Rochester Rochester, New York New York Oxford OXFORD UNIVERSITY PRESS 1995
2 Contents 1. Introduction 3 Linear versus Nonlinear Spectroscopy 3 Time- versus Frequency-Domain Techniques 5 Resonant versus Off-Resonant Response 7 2..Quantum Dynamics in Hilbert Space 75 Time-Evolution Operator with Time-Independent Hamiltonians 75 Propagation with Time-Dependent Hamiltonians: Time Ordering 23 The Time Evolution Operator Revisited 25 The Interaction Picture 26 The Magnus Expansion 30 Green Functions and Causality 31 Projection Operators, Reduced Equations of Motion, and Effective Hamiltonians 34 ; Appendix 2A: Linear Vector Spaces and Operators The Density Operator and Quantum Dynamics in Liouville Space 45 Basic Definitions: Pure and Mixed States 45 The Reduced Density Operator: The Truth But Not the Whole Truth 49 Time Evolution of the Density Operator 50 Liouville Space and Tetradic Notation 55 Time Evolution Operator in Liouville Space 59 The Interaction Picture 61 The Magnus Expansion 63 Liouville Space Green Functions 64
3 XIV CONTENTS Projection Operators and the Reduced Density Operator: Effective Liouville Operators 67 The Classical Liouville Equation and the Wigner Representation 68 Concluding Comments Quantum Electrodynamics, Optical Polarization, and Nonlinear Spectroscopy 79 The Minimal Coupling Hamiltonian and the Radiation-Matter Interaction 79 The Power-Zienau Transformation and the Multipolar Hamiltonian 83 The Coupled Field and Matter Equations of Motion and the Semiclassical Hamiltonian 88 The Coupled Maxwell-Liouville Equations 92 Optical Measurements and the Polarization 95 Appendix 4A: Transverse and Longitudinal Vector Fields 104 Appendix 4B: The Multipolar Expansion of the Polarization and Magnetization 706 Appendix 4C: Green Function Solution of the Maxwell Equation Nonlinear Response Functions and Optical Susceptibilities 777 Correlation Function Expressions for the Response Functions of a Small Particle 777 Liouville Space Pathways in the Time Domain 118 Liouville Space Pathways in the Frequency Domain 720 Nonlocal Expressions for the Optical Response of Extended Systems, 725 Nonlinear Response in Momentum (k) Space 124 Optical Response of a Homogeneous Medium of Noninteracting Particles 727 Time versus Frequency Domain Techniques 128 Why Liouville Space? 757 Appendix 5A: Wavefunction versus Density-Operator Formulation of the Nonlinear Response 755 Appendix 5B: Calculating the Response Functions Using the Heisenberg Representation The Optical Response Functions of a Multilevel System with Relaxation 143 Linear Response and the Kramers-Kronig Relations 144
4 CONTENTS XV Eigenstates Revisited: Linear Response in Liouville Space 747 Response Functions of a Multilevel Manifold with Relaxation 149 The Nonlinear Response Functions Calculated Using the Wavefunction in Hilbert Space 759 The Nonlinear Response Functions Calculated Using the Heisenberg Equations of Motion 760 The Anharmonic Oscillator Picture for the Optical Polarization 765 X l3) with a Realistic Population-Relaxation Matrix 767 Homogeneous, Inhomogeneous, and Intermediate Dephasing 769 Examples of Single-Frequency Techniques 775 Appendix 6A: Reduced Equations of Motion for the Density Operator 776 Appendix 6B: The Optical Bloch Equations Semiclassical Simulation of the Optical Response Functions 187 Linear Response of a Two Electronic Level System: Semiclassical Simulations and Phase Averaging 189 Moments of the Linear Absorption 795 Hilbert versus Liouville Space Representation of the Third-Order Response Function 796 Semiclassical Simulations of the Nonlinear Response in Liouville Space: Phase Averaging 799 The Static Limit: Inhomogeneous Broadening and Spectral Diffusion 207 Appendix 7A: The Coherence Green Function 204 Appendix 7B: Derivation of Eqs. (7.19) The Cumulant Expansion and the Multimode Brownian Oscillator Model 209 The Condon Approximation for the Optical Response of a Two-Level System 270 The Cumulant Expansion 272 The Spectral Density and Its Symmetries 214 Coupling to Harmonic Vibrations 277 The Multimode Brownian Oscillator Model 227 Additional Applications of the Cumulant Expansion 235 The Inhomogeneous Cumulant Expansion and Semiclassical Simulations 239 Optical Susceptibilities of a Multilevel System Interacting with a Medium with an Arbitrary Timescale 243
5 XVI CONTENTS Appendix 8A: The Cumulant Expansion for F(z u x 2, T 3, T 4 ) 248 Appendix 8B: Absorption and Emission Lineshapes: The Stokes Shift 250 Appendix 8C: Brownian Oscillator Parameters for a Polar Solvent 253 Appendix 8D: Classical Correlation Functions and the Wiener-Khinchin Theorem 255 Appendix 8E: Relation between Classical Correlation Functions and Response Functions Fluorescence, Spontaneous-Raman, and Coherent-Raman Spectroscopy 267 Absorption of a Quantum Field 262 Spontaneous Light Emission Spectroscopy 265 Frequency Domain SLE 267 Fluorescence and Raman Spectroscopy 277 Resonant Coherent Raman Spectroscopy 279 Appendix 9A: Spontaneous Light Emission with Spectral Diffusion and Vibrational Relaxation Selective Elimination of Inhomogeneous Broadening: Photon Echoes 289 Classification of Time-Domain Resonant Four-Wave Mixing Techniques 295 Two- and Three-Pulse Photon Echo Spectroscopies 299 Impulsive Photon Echoes 507 Brownian Oscillator Analysis of Impulsive Photon Echoes: From Quantum Beats to Spectral Diffusion 304 Spontaneous Light Emission Using Phase-Locked Pulses 570 Appendix 10A: Accumulated Photon Echoes 574 Appendix 10B: Accumulated Photon Echoes with Incoherent Light Sources Resonant Gratings, Pump-Probe, and Hole-Burning Spectroscopy 527 Resonant, Non-Time-Ordered, Four-Wave Mixing 323 Partial Control over Time Ordering: Phase-Locked Transient Gratings 324 Sequential Pump-Probe Spectroscopy 326 Impulsive Pump-Probe Spectroscopy and Quantum Beats 328 Hole-Burning Spectroscopy 336 Three-Pulse Phase-Locked Pump-Probe Absorption 339
6 CONTENTS XVii Macroscopic versus Microscopic Interference 340 Fourier Transform Relationships Wavepacket Dynamics in Liouville Space: The Wigner Representation 345 Liouville Space-Generating Function for the Linear Response 346 Generating Functions for Nonlinear Response: Liouville Space Pathways 347 Classical Simulation of Nuclear Wavepackets: Phase-Averaging Revisited 349 Semiclassical Equations of Motion for the Liouville Space Generating Functions 557 Reduced Dynamics of Liouville Space Paths: The Multimode Brownian Oscillator Model 356 Reduced Equations of Motion for Liouville Space Wavepackets 357 The Doorway-Window Representation of the Nonlinear Response Function 359 Appendix 12A: Eigenstate Expansion of the Liouville Space-Generating * Functions 364 Appendix 12B: The Doorway-Window Picture in the Frequency Domain: Vibronic State Representation Wavepacket Analysis of Nonimpulsive Measurements 369 The Doorway-Window Picture for Well Separated Pulses 373 The Snapshot Spectrum and Related Limiting Cases 377 Nuclear Wavepackets for the Overdamped Brownian Oscillator 385 Semiclassical Picture of Pump-Probe Spectroscopy in a Three-Electronic-Level System 393 Appendix 13A: Wavepacket Representation of Pump-Probe Spectroscopy with Frequency Dispersed Detection 407 Appendix 13B: Wavepacket Representation of Transient Grating with Heterodyne Detection Off-Resonance Raman Scattering 411 Dynamic Approach to Coherent Raman Scattering 414 The Multimode Brownian Oscillator Model 422 Effective Hamiltonian for Raman Scattering 424 Fourier Transform Relationships 430 Beyond Raman Scattering: Multidimensional Off-Resonant Spectroscopy of Liquids 432
7 XViii CONTENTS Appendix 14A: The Doorway State and the Effective Hamiltonian H eff : Derivation of Eqs. (14.33) Polarization Spectroscopy: Birefringence and Dichroism 445 Rotational Contribution to the Nonlinear Response Function 447 Vibrational Contribution to Heterodyne-Detected Transient Grating 450 The Polarization-Dependent Grating Signal 451 Off-Resonant Birefringence and Dichroism 455 Appendix 15A: Solution of the Rotational Fokker-Planck Equation Nonlinear Response of Molecular Assemblies: The Local-Field Approximation 461 Phenomenological Approach to the Nonlinear Response in Real Space: Local-Field and Cascading Corrections 462 The Local-Field Approximation in k Space 466 Microscopic Derivation of the LFA: The Driven Anharmonic Oscillator 469 Local Field Expressions for Optical 'Susceptibilities of Homogeneous Systems Many-Body and Cooperative Effects in the Nonlinear Response 479 Green Function Expression for the Optical Response of Molecular Nanostructures with Arbitrary Geometry 483 Factorized Approximations for the Green Function Solution 488 Anharmonic Oscillator Real Space Expression for the Optical Response beyond the LFA 491 Green Function Expression for the Four-Wave Mixing Signal Including Radiative Decay 493 Optical Susceptibilities of Periodic Structures in k Space 496 Signatures of Cooperativity: Two-Exciton Resonances and Enhanced Nonlinear Susceptibilities in Molecular Aggregates 498 Exciton-Population Variables and Exciton Transport 507 Discussion 575 Appendix 17A: Exciton Dephasing and Relaxation Processes 576 Appendix 17B: Scattering (2T) Matrix Expression for the Two-Exciton Green Function 575 Appendix 17C: Green Function Solution of the Nonlinear Response 520 Index 525
Modern Optical Spectroscopy
Modern Optical Spectroscopy With Exercises and Examples from Biophysics and Biochemistry von William W Parson 1. Auflage Springer-Verlag Berlin Heidelberg 2006 Verlag C.H. Beck im Internet: www.beck.de
ATOMIC AND LASER SPECTROSCOPY
ALAN CORNEY ATOMIC AND LASER SPECTROSCOPY CLARENDON PRESS OXFORD 1977 Contents 1. INTRODUCTION 1.1. Planck's radiation law. 1 1.2. The photoelectric effect 4 1.3. Early atomic spectroscopy 5 1.4. The postulates
5.74 Introductory Quantum Mechanics II
MIT OpenCourseWare http://ocw.mit.edu 5.74 Introductory Quantum Mechanics II Spring 2009 For information about citing these materials or our Terms of Use, visit: http://ocw.mit.edu/terms. p. 10-0 10..
LIST OF TOPICS BASIC LASER PHYSICS. Preface xiii Units and Notation xv List of Symbols xvii
ate LIST OF TOPICS Preface xiii Units and Notation xv List of Symbols xvii BASIC LASER PHYSICS Chapter 1 An Introduction to Lasers 1.1 What Is a Laser? 2 1.2 Atomic Energy Levels and Spontaneous Emission
MOLECULAR SPECTROSCOPY
MOLECULAR SPECTROSCOPY First Edition Jeanne L. McHale University of Idaho PRENTICE HALL, Upper Saddle River, New Jersey 07458 CONTENTS PREFACE xiii 1 INTRODUCTION AND REVIEW 1 1.1 Historical Perspective
5.74 Introductory Quantum Mechanics II
MIT OpenCourseWare http://ocw.mit.edu 5.74 Introductory Quantum Mechanics II Spring 9 For information about citing these materials or our Terms of Use, visit: http://ocw.mit.edu/terms. Andrei Tokmakoff,
Fundamentals of Spectroscopy for Optical Remote Sensing. Course Outline 2009
Fundamentals of Spectroscopy for Optical Remote Sensing Course Outline 2009 Part I. Fundamentals of Quantum Mechanics Chapter 1. Concepts of Quantum and Experimental Facts 1.1. Blackbody Radiation and
Elements of Quantum Optics
Pierre Meystre Murray Sargent III Elements of Quantum Optics Fourth Edition With 124 Figures fya Springer Contents 1 Classical Electromagnetic Fields 1 1.1 Maxwell's Equations in a Vacuum 2 1.2 Maxwell's
5.74 Introductory Quantum Mechanics II
MIT OpenCourseWare http://ocw.mit.edu 5.74 Introductory Quantum Mechanics II Spring 009 For information about citing these materials or our Terms of Use, visit: http://ocw.mit.edu/terms. Andrei Tokmakoff,
Correlation spectroscopy
1 TWO-DIMENSIONAL SPECTROSCOPY Correlation spectroscopy What is two-dimensional spectroscopy? This is a method that will describe the underlying correlations between two spectral features. Our examination
P. W. Atkins and R. S. Friedman. Molecular Quantum Mechanics THIRD EDITION
P. W. Atkins and R. S. Friedman Molecular Quantum Mechanics THIRD EDITION Oxford New York Tokyo OXFORD UNIVERSITY PRESS 1997 Introduction and orientation 1 Black-body radiation 1 Heat capacities 2 The
Optical Characterization of Solids
D. Dragoman M. Dragoman Optical Characterization of Solids With 184 Figures Springer 1. Elementary Excitations in Solids 1 1.1 Energy Band Structure in Crystalline Materials 2 1.2 k p Method 11 1.3 Numerical
Charge and Energy Transfer Dynamits in Molecular Systems
Volkhard May, Oliver Kühn Charge and Energy Transfer Dynamits in Molecular Systems Second, Revised and Enlarged Edition WILEY- VCH WILEY-VCH Verlag GmbH & Co. KGaA Contents 1 Introduction 19 2 Electronic
Preface. Preface to the Third Edition. Preface to the Second Edition. Preface to the First Edition. 1 Introduction 1
xi Contents Preface Preface to the Third Edition Preface to the Second Edition Preface to the First Edition v vii viii ix 1 Introduction 1 I GENERAL THEORY OF OPEN QUANTUM SYSTEMS 5 Diverse limited approaches:
Wolfgang Demtroder. Laser Spectroscopy. Basic Concepts and Instrumentation. Second Enlarged Edition With 644 Figures and 91 Problems.
Wolfgang Demtroder Laser Spectroscopy Basic Concepts and Instrumentation Second Enlarged Edition With 644 Figures and 91 Problems Springer Contents 1. Introduction 1 2. Absorption and Emission of Light
Third-order nonlinear time domain probes of solvation dynamics
Third-order nonlinear time domain probes of solvation dynamics Taiha Joo, Yiwei Jia, Jae-Young Yu, Matthew J. Lang, and Graham R. Fleming Department of Chemistry and the James Franck Research Institute,
Lecture cycle: Spectroscopy and Optics
Lecture cycle: Spectroscopy and Optics Thu. 13:00-15:00 / Room 1.003 15.11.2017 (Staudinger) Mischa Bonn Light-matter interaction overview I 30.11.2017 Mischa Bonn Light-matter interaction overview II
Principles of Nuclear Magnetic Resonance in One and Two Dimensions
Principles of Nuclear Magnetic Resonance in One and Two Dimensions Richard R. Ernst, Geoffrey Bodenhausen, and Alexander Wokaun Laboratorium für Physikalische Chemie Eidgenössische Technische Hochschule
Quantum optics. Marian O. Scully Texas A&M University and Max-Planck-Institut für Quantenoptik. M. Suhail Zubairy Quaid-i-Azam University
Quantum optics Marian O. Scully Texas A&M University and Max-Planck-Institut für Quantenoptik M. Suhail Zubairy Quaid-i-Azam University 1 CAMBRIDGE UNIVERSITY PRESS Preface xix 1 Quantum theory of radiation
Principles of Nuclear Magnetic Resonance Microscopy
Principles of Nuclear Magnetic Resonance Microscopy Paul T. Callaghan Department of Physics and Biophysics Massey University New Zealand CLARENDON PRESS OXFORD CONTENTS 1 PRINCIPLES OF IMAGING 1 1.1 Introduction
CONTENTS. 2 CLASSICAL DESCRIPTION 2.1 The resonance phenomenon 2.2 The vector picture for pulse EPR experiments 2.3 Relaxation and the Bloch equations
CONTENTS Preface Acknowledgements Symbols Abbreviations 1 INTRODUCTION 1.1 Scope of pulse EPR 1.2 A short history of pulse EPR 1.3 Examples of Applications 2 CLASSICAL DESCRIPTION 2.1 The resonance phenomenon
TWO-DIMENSIONAL RAMAN SPECTROSCOPY N. Y , USA. (Received 28 June 1998)
Laser Chem., 1999, Vol. 19, pp. 109-116 Reprints available directly from the publisher Photocopying permitted by license only (C) 1999 OPA (Overseas Publishers Association) N.V. Published by license under
MESOSCOPIC QUANTUM OPTICS
MESOSCOPIC QUANTUM OPTICS by Yoshihisa Yamamoto Ata Imamoglu A Wiley-Interscience Publication JOHN WILEY & SONS, INC. New York Chichester Weinheim Brisbane Toronto Singapore Preface xi 1 Basic Concepts
C.W. Gardiner. P. Zoller. Quantum Nois e. A Handbook of Markovian and Non-Markovia n Quantum Stochastic Method s with Applications to Quantum Optics
C.W. Gardiner P. Zoller Quantum Nois e A Handbook of Markovian and Non-Markovia n Quantum Stochastic Method s with Applications to Quantum Optics 1. A Historical Introduction 1 1.1 Heisenberg's Uncertainty
Introduction to Modern Quantum Optics
Introduction to Modern Quantum Optics Jin-Sheng Peng Gao-Xiang Li Huazhong Normal University, China Vfe World Scientific» Singapore* * NewJerseyL Jersey* London* Hong Kong IX CONTENTS Preface PART I. Theory
List of Comprehensive Exams Topics
List of Comprehensive Exams Topics Mechanics 1. Basic Mechanics Newton s laws and conservation laws, the virial theorem 2. The Lagrangian and Hamiltonian Formalism The Lagrange formalism and the principle
Laser Physics OXFORD UNIVERSITY PRESS SIMON HOOKER COLIN WEBB. and. Department of Physics, University of Oxford
Laser Physics SIMON HOOKER and COLIN WEBB Department of Physics, University of Oxford OXFORD UNIVERSITY PRESS Contents 1 Introduction 1.1 The laser 1.2 Electromagnetic radiation in a closed cavity 1.2.1
Spin Dynamics Basics of Nuclear Magnetic Resonance. Malcolm H. Levitt
Spin Dynamics Basics of Nuclear Magnetic Resonance Second edition Malcolm H. Levitt The University of Southampton, UK John Wiley &. Sons, Ltd Preface xxi Preface to the First Edition xxiii Introduction
Linear and nonlinear spectroscopy
Linear and nonlinear spectroscopy We ve seen that we can determine molecular frequencies and dephasing rates (for electronic, vibrational, or spin degrees of freedom) from frequency-domain or timedomain
Statistical Mechanics
Franz Schwabl Statistical Mechanics Translated by William Brewer Second Edition With 202 Figures, 26 Tables, and 195 Problems 4u Springer Table of Contents 1. Basic Principles 1 1.1 Introduction 1 1.2
Preface Introduction to the electron liquid
Table of Preface page xvii 1 Introduction to the electron liquid 1 1.1 A tale of many electrons 1 1.2 Where the electrons roam: physical realizations of the electron liquid 5 1.2.1 Three dimensions 5 1.2.2
Nanoscale Energy Transport and Conversion A Parallel Treatment of Electrons, Molecules, Phonons, and Photons
Nanoscale Energy Transport and Conversion A Parallel Treatment of Electrons, Molecules, Phonons, and Photons Gang Chen Massachusetts Institute of Technology OXFORD UNIVERSITY PRESS 2005 Contents Foreword,
5.74 Introductory Quantum Mechanics II
MIT OpenCourseWare http://ocw.mit.edu 5.74 Introductory Quantum Mechanics II Spring 009 For information about citing these materials or our Terms of Use, visit: http://ocw.mit.edu/terms. Andrei Tokmakoff,
QUANTUM MECHANICS. Franz Schwabl. Translated by Ronald Kates. ff Springer
Franz Schwabl QUANTUM MECHANICS Translated by Ronald Kates Second Revised Edition With 122Figures, 16Tables, Numerous Worked Examples, and 126 Problems ff Springer Contents 1. Historical and Experimental
Coherence Vibrations and Electronic Excitation Dynamics in Molecular Aggregates and Photosynthetic Pigment-Proteins
VILNIUS UNIVERSITY Coherence Vibrations and Electronic Excitation Dynamics in Molecular Aggregates and Photosynthetic Pigment-Proteins L. Valkunas Department of Theoretical Physics, Faculty of Physics,
11.6. TWO-DIMENSIONAL CORRELATION SPECTROSCOPY
Andrei Tokmakoff, MIT Department of Chemistry, 6/5/009 p. -54.6. TWO-DIMENSIONAL CORRELATION SPECTROSCOPY Our examination of pump-probe experiments indicates that the third-order response reports on the
Ultrafast Spectroscopy of Semiconductors and Semiconductor Nanostructures
Springer Series in Solid-State Sciences 115 Ultrafast Spectroscopy of Semiconductors and Semiconductor Nanostructures Bearbeitet von Jagdeep Shah erweitert 1999. Buch. xvi, 522 S. Hardcover ISBN 978 3
NPTEL
NPTEL Syllabus Nonequilibrium Statistical Mechanics - Video course COURSE OUTLINE Thermal fluctuations, Langevin dynamics, Brownian motion and diffusion, Fokker-Planck equations, linear response theory,
Lasers and Electro-optics
Lasers and Electro-optics Second Edition CHRISTOPHER C. DAVIS University of Maryland III ^0 CAMBRIDGE UNIVERSITY PRESS Preface to the Second Edition page xv 1 Electromagnetic waves, light, and lasers 1
12. Quantum-classical theory of linear and non-linear spectroscopy
12. Quantum-classical theory of linear and non-linear spectroscopy In the quantum-classical formalism, we treat the electric field classically as in eq. 10-17 or Appendix B. The electric field becomes
Multidimensional femtosecond coherence spectroscopy for study of the carrier dynamics in photonics materials
International Workshop on Photonics and Applications. Hanoi, Vietnam. April 5-8,24 Multidimensional femtosecond coherence spectroscopy for study of the carrier dynamics in photonics materials Lap Van Dao,
Survey on Laser Spectroscopic Techniques for Condensed Matter
Survey on Laser Spectroscopic Techniques for Condensed Matter Coherent Radiation Sources for Small Laboratories CW: Tunability: IR Visible Linewidth: 1 Hz Power: μw 10W Pulsed: Tunabality: THz Soft X-ray
STOCHASTIC PROCESSES IN PHYSICS AND CHEMISTRY
STOCHASTIC PROCESSES IN PHYSICS AND CHEMISTRY Third edition N.G. VAN KAMPEN Institute for Theoretical Physics of the University at Utrecht ELSEVIER Amsterdam Boston Heidelberg London New York Oxford Paris
Electron spins in nonmagnetic semiconductors
Electron spins in nonmagnetic semiconductors Yuichiro K. Kato Institute of Engineering Innovation, The University of Tokyo Physics of non-interacting spins Optical spin injection and detection Spin manipulation
Investigations of amplitude and phase excitation profiles in femtosecond coherence spectroscopy
JOURNAL OF CHEMICAL PHYSICS VOLUME 114, NUMBER 2 8 JANUARY 21 Investigations of amplitude and phase excitation profiles in femtosecond coherence spectroscopy Anand T. N. Kumar, Florin Rosca, Allan Widom,
Solid State Physics. GIUSEPPE GROSSO Professor of Solid State Physics, Department of Physics, University of Pavia, and INFM
Solid State Physics GIUSEPPE GROSSO Professor of Solid State Physics, Department of Physics, University of Pisa, and INFM GIUSEPPE PASTORI PARRAVICINI Professor of Solid State Physics, Department of Physics,
Highenergy Nuclear Optics of Polarized Particles
Highenergy Nuclear Optics of Polarized Particles Vladimir G. Baryshevsky Research Institute for Nuclear Problems Belarusian State University 1> World Scientific NEW JERSEY LONDON SINGAPORE BEIJING SHANGHAI
CLASSICAL ELECTRICITY
CLASSICAL ELECTRICITY AND MAGNETISM by WOLFGANG K. H. PANOFSKY Stanford University and MELBA PHILLIPS Washington University SECOND EDITION ADDISON-WESLEY PUBLISHING COMPANY Reading, Massachusetts Menlo
Two-color Transient Grating Spectroscopy of a Two-level System
Two-color Transient Grating Spectroscopy Bull. Korean Chem. Soc. 23, Vol. 24, No. 8 69 Two-color Transient Grating Spectroscopy of a Two-level System Kyungwon Kwak, Minhaeng Cho, * Graham R. Fleming, *,
Principles of Magnetic Resonance
С. Р. Slichter Principles of Magnetic Resonance Third Enlarged and Updated Edition With 185 Figures Springer-Verlag Berlin Heidelberg New York London Paris Tokyo Hong Kong Contents 1. Elements of Resonance
EE 223 Applied Quantum Mechanics 2 Winter 2016
EE 223 Applied Quantum Mechanics 2 Winter 2016 Syllabus and Textbook references Version as of 12/29/15 subject to revisions and changes All the in-class sessions, paper problem sets and assignments, and
EQUATION LANGEVIN. Physics, Chemistry and Electrical Engineering. World Scientific. With Applications to Stochastic Problems in. William T.
SHANGHAI HONG WorlrfScientific Series krtonttimfjorary Chemical Physics-Vol. 27 THE LANGEVIN EQUATION With Applications to Stochastic Problems in Physics, Chemistry and Electrical Engineering Third Edition
Many-Body Problems and Quantum Field Theory
Philippe A. Martin Francois Rothen Many-Body Problems and Quantum Field Theory An Introduction Translated by Steven Goldfarb, Andrew Jordan and Samuel Leach Second Edition With 102 Figures, 7 Tables and
Optically polarized atoms. Marcis Auzinsh, University of Latvia Dmitry Budker, UC Berkeley and LBNL Simon M. Rochester, UC Berkeley
Optically polarized atoms Marcis Auzinsh, University of atvia Dmitry Budker, UC Berkeley and BN Simon M. Rochester, UC Berkeley 1 Chapter 6: Coherence in atomic systems Exciting a 0ö1 transition with z
Matter-Radiation Interaction
Matter-Radiation Interaction The purpose: 1) To give a description of the process of interaction in terms of the electronic structure of the system (atoms, molecules, solids, liquid or amorphous samples).
Harald Ibach Hans Lüth SOLID-STATE PHYSICS. An Introduction to Theory and Experiment
Harald Ibach Hans Lüth SOLID-STATE PHYSICS An Introduction to Theory and Experiment With 230 Figures Springer-Verlag Berlin Heidelberg New York London Paris Tokyo Hong Kong Barcelona Budapest Contents
PROTEIN NMR SPECTROSCOPY
List of Figures List of Tables xvii xxvi 1. NMR SPECTROSCOPY 1 1.1 Introduction to NMR Spectroscopy 2 1.2 One Dimensional NMR Spectroscopy 3 1.2.1 Classical Description of NMR Spectroscopy 3 1.2.2 Nuclear
Professor Dr. Wolfgang Demtröder
Wolfgang Demtröder Laser Spectroscopy Basic Concepts and Instrumentation Third Edition With 710 Figures,16 Tables 93 Problems and Hints for Solution 13 Professor Dr. Wolfgang Demtröder Universität Kaiserslautern
PHYSICS OF SEMICONDUCTORS AND THEIR HETEROSTRUCTURES
PHYSICS OF SEMICONDUCTORS AND THEIR HETEROSTRUCTURES Jasprit Singh University of Michigan McGraw-Hill, Inc. New York St. Louis San Francisco Auckland Bogota Caracas Lisbon London Madrid Mexico Milan Montreal
NANO/MICROSCALE HEAT TRANSFER
NANO/MICROSCALE HEAT TRANSFER Zhuomin M. Zhang Georgia Institute of Technology Atlanta, Georgia New York Chicago San Francisco Lisbon London Madrid Mexico City Milan New Delhi San Juan Seoul Singapore
Optical coherence spectroscopy in solution: Determining the system-bath correlation function
Optical coherence spectroscopy in solution: Determining the system-bath correlation function Lewis D. Book a, David C. Arnett b and Norbert F. Scherer a a Department of Chemistry and The James Franck Institute,
Control and Characterization of Intramolecular Dynamics with Chirped Femtosecond Three-Pulse Four-Wave Mixing
106 J. Phys. Chem. A 1999, 103, 106-1036 Control and Characterization of Intramolecular Dynamics with Chirped Femtosecond Three-Pulse Four-Wave Mixing Igor Pastirk, Vadim V. Lozovoy, Bruna I. Grimberg,
Quantum Mechanics: Fundamentals
Kurt Gottfried Tung-Mow Yan Quantum Mechanics: Fundamentals Second Edition With 75 Figures Springer Preface vii Fundamental Concepts 1 1.1 Complementarity and Uncertainty 1 (a) Complementarity 2 (b) The
Multi-Dimensional IR Spectroscopy of Acetic Acid Dimers and Liquid Water
Multi-Dimensional IR Spectroscopy of Acetic Acid Dimers and Liquid Water N. Huse 1, J. Dreyer 1, E.T.J.Nibbering 1, T. Elsaesser 1 B.D. Bruner 2, M.L. Cowan 2, J.R. Dwyer 2, B. Chugh 2, R.J.D. Miller 2
Advanced Quantum Mechanics
Advanced Quantum Mechanics Rajdeep Sensarma sensarma@theory.tifr.res.in Quantum Dynamics Lecture #2 Recap of Last Class Schrodinger and Heisenberg Picture Time Evolution operator/ Propagator : Retarded
ELECTROMAGNETICALLY INDUCED TRANSPARENCY
14 ELECTROMAGNETICALLY INDUCED TRANSPARENCY J.P. Marangos Quantum Optics and Laser Science Group Blackett Laboratory, Imperial College London, United Kingdom T. Halfmann Institute of Applied Physics Technical
Electronic and Optoelectronic Properties of Semiconductor Structures
Electronic and Optoelectronic Properties of Semiconductor Structures Jasprit Singh University of Michigan, Ann Arbor CAMBRIDGE UNIVERSITY PRESS CONTENTS PREFACE INTRODUCTION xiii xiv 1.1 SURVEY OF ADVANCES
LECTURES ON QUANTUM MECHANICS
LECTURES ON QUANTUM MECHANICS GORDON BAYM Unitsersity of Illinois A II I' Advanced Bock Progrant A Member of the Perseus Books Group CONTENTS Preface v Chapter 1 Photon Polarization 1 Transformation of
Contents. Part I Fundamentals of Lasers 1 Introduction... 3
Contents Part I Fundamentals of Lasers 1 Introduction... 3 2 Basic Optics... 9 2.1 Introduction...... 9 2.2 TheWaveEquation... 9 2.3 Linearly Polarized Waves.... 13 2.4 Circularly and Elliptically Polarized
Diode Lasers and Photonic Integrated Circuits
Diode Lasers and Photonic Integrated Circuits L. A. COLDREN S. W. CORZINE University of California Santa Barbara, California A WILEY-INTERSCIENCE PUBLICATION JOHN WILEY & SONS, INC. NEW YORK / CHICHESTER
Contents. 1 Basic Equations 1. Acknowledgment. 1.1 The Maxwell Equations Constitutive Relations 11
Preface Foreword Acknowledgment xvi xviii xix 1 Basic Equations 1 1.1 The Maxwell Equations 1 1.1.1 Boundary Conditions at Interfaces 4 1.1.2 Energy Conservation and Poynting s Theorem 9 1.2 Constitutive
Design strategies for pulse sequences in multidimensional optical spectroscopies
JOURNAL OF CHEMICAL PHYSICS VOLUME 115, NUMBER 11 15 SEPTEMBER 2001 Design strategies for pulse sequences in multidimensional optical spectroscopies C. Scheurer a) and S. Mukamel b) Department of Chemistry,
THEORY OF MAGNETIC RESONANCE
THEORY OF MAGNETIC RESONANCE Second Edition Charles P. Poole, Jr., and Horacio A. Farach Department of Physics University of South Carolina, Columbia A Wiley-lnterscience Publication JOHN WILEY & SONS
Optics, Light and Lasers
Dieter Meschede Optics, Light and Lasers The Practical Approach to Modern Aspects of Photonics and Laser Physics Second, Revised and Enlarged Edition BICENTENNIAL.... n 4 '':- t' 1 8 0 7 $W1LEY 2007 tri
Nonlinear Optics (WiSe 2015/16) Lecture 12: January 15, 2016
Nonlinear Optics (WiSe 2015/16) Lecture 12: January 15, 2016 12 High Harmonic Generation 12.1 Atomic units 12.2 The three step model 12.2.1 Ionization 12.2.2 Propagation 12.2.3 Recombination 12.3 Attosecond
Spectral Broadening Mechanisms
Spectral Broadening Mechanisms Lorentzian broadening (Homogeneous) Gaussian broadening (Inhomogeneous, Inertial) Doppler broadening (special case for gas phase) The Fourier Transform NC State University
Handbook of Stochastic Methods
C. W. Gardiner Handbook of Stochastic Methods for Physics, Chemistry and the Natural Sciences Third Edition With 30 Figures Springer Contents 1. A Historical Introduction 1 1.1 Motivation I 1.2 Some Historical
Model Answer (Paper code: AR-7112) M. Sc. (Physics) IV Semester Paper I: Laser Physics and Spectroscopy
Model Answer (Paper code: AR-7112) M. Sc. (Physics) IV Semester Paper I: Laser Physics and Spectroscopy Section I Q1. Answer (i) (b) (ii) (d) (iii) (c) (iv) (c) (v) (a) (vi) (b) (vii) (b) (viii) (a) (ix)
Topics for the Qualifying Examination
Topics for the Qualifying Examination Quantum Mechanics I and II 1. Quantum kinematics and dynamics 1.1 Postulates of Quantum Mechanics. 1.2 Configuration space vs. Hilbert space, wave function vs. state
Observation of the waveform of accumulated photon echoes in a dye-doped polymer film by use of an interferometer
1768 J. Opt. Soc. Am. B/Vol. 16, No. 10/October 1999 Yoda et al. Observation of the waveform of accumulated photon echoes in a dye-doped polymer film by use of an interferometer Takuya Yoda, Takao Fuji,
FUNDAMENTALS OF POLARIZED LIGHT
FUNDAMENTALS OF POLARIZED LIGHT A STATISTICAL OPTICS APPROACH Christian Brosseau University of Brest, France A WILEY-INTERSCIENCE PUBLICATION JOHN WILEY & SONS, INC. New York - Chichester. Weinheim. Brisbane
Spectral Broadening Mechanisms. Broadening mechanisms. Lineshape functions. Spectral lifetime broadening
Spectral Broadening echanisms Lorentzian broadening (Homogeneous) Gaussian broadening (Inhomogeneous, Inertial) Doppler broadening (special case for gas phase) The Fourier Transform NC State University
The Physics of Nanoelectronics
The Physics of Nanoelectronics Transport and Fluctuation Phenomena at Low Temperatures Tero T. Heikkilä Low Temperature Laboratory, Aalto University, Finland OXFORD UNIVERSITY PRESS Contents List of symbols
1. Transition dipole moment
1. Transition dipole moment You have measured absorption spectra of aqueous (n=1.33) solutions of two different chromophores (A and B). The concentrations of the solutions were the same. The absorption
Contents Classical and Quantum Interference and Coherence Quantum Interference in Atomic Systems: Mathematical Formalism
1 Classical and Quantum Interference and Coherence... 1 1.1 ClassicalInterferenceandOpticalInterferometers... 2 1.1.1 Young sdoubleslitinterferometer... 2 1.1.2 First-OrderCoherence... 4 1.1.3 WelcherWegProblem...
Wolfgang Demtroder. Molecular Physics. Theoretical Principles and Experimental Methods WILEY- VCH. WILEY-VCH Verlag GmbH & Co.
Wolfgang Demtroder Molecular Physics Theoretical Principles and Experimental Methods WILEY- VCH WILEY-VCH Verlag GmbH & Co. KGaA v Preface xiii 1 Introduction 1 1.1 Short Historical Overview 2 1.2 Molecular
Andrei V. Pisliakov, Tomáš Manal, and Graham R. Fleming
Two-dimensional optical three-pulse photon echo spectroscopy. II. Signatures of coherent electronic motion and exciton population transfer in dimer two-dimensional spectra Andrei V. Pisliakov, Tomáš Manal,
Quantum Physics II (8.05) Fall 2002 Outline
Quantum Physics II (8.05) Fall 2002 Outline 1. General structure of quantum mechanics. 8.04 was based primarily on wave mechanics. We review that foundation with the intent to build a more formal basis
Absorption-Amplification Response with or Without Spontaneously Generated Coherence in a Coherent Four-Level Atomic Medium
Commun. Theor. Phys. (Beijing, China) 42 (2004) pp. 425 430 c International Academic Publishers Vol. 42, No. 3, September 15, 2004 Absorption-Amplification Response with or Without Spontaneously Generated
Nonlinear Optics. Second Editio n. Robert W. Boyd
Nonlinear Optics Second Editio n Robert W. Boyd Preface to the Second Edition Preface to the First Edition xiii xv 1. The Nonlinear Optical Susceptibility 1 1.1. Introduction to Nonlinear Optics 1 1.2.
Frequency- and Time-Domain Spectroscopy
Frequency- and Time-Domain Spectroscopy We just showed that you could characterize a system by taking an absorption spectrum. We select a frequency component using a grating or prism, irradiate the sample,
Lecture 0. NC State University
Chemistry 736 Lecture 0 Overview NC State University Overview of Spectroscopy Electronic states and energies Transitions between states Absorption and emission Electronic spectroscopy Instrumentation Concepts
Theoretical Photochemistry WiSe 2016/17
Theoretical Photochemistry WiSe 2016/17 Lecture 8 Irene Burghardt burghardt@chemie.uni-frankfurt.de) http://www.theochem.uni-frankfurt.de/teaching/ Theoretical Photochemistry 1 Topics 1. Photophysical
As a partial differential equation, the Helmholtz equation does not lend itself easily to analytical
Aaron Rury Research Prospectus 21.6.2009 Introduction: The Helmhlotz equation, ( 2 +k 2 )u(r)=0 1, serves as the basis for much of optical physics. As a partial differential equation, the Helmholtz equation
Elementary Lectures in Statistical Mechanics
George DJ. Phillies Elementary Lectures in Statistical Mechanics With 51 Illustrations Springer Contents Preface References v vii I Fundamentals: Separable Classical Systems 1 Lecture 1. Introduction 3
Femtosecond nonlinear coherence spectroscopy of carrier dynamics in porous silicon
JOURNAL OF APPLIED PHYSICS 98, 083508 2005 Femtosecond nonlinear coherence spectroscopy of carrier dynamics in porous silicon Lap Van Dao a and Peter Hannaford Centre for Atom Optics and Ultrafast Spectroscopy,
F.G. Major. The Quantum Beat. The Physical Principles of Atomic Clocks. With 230 Illustrations. Springer
F.G. Major The Quantum Beat The Physical Principles of Atomic Clocks With 230 Illustrations Springer Contents Preface Chapter 1. Celestial and Mechanical Clocks 1 1.1 Cyclic Events in Nature 1 1.2 The
BY TEMPORALLY TWO-DIMENSIONAL
Laser Chem., 1999, Vol. 19, pp. 35-40 Reprints available directly from the publisher Photocopying permitted by license only (C) 1999 OPA (Overseas Publishers Association) N.V. Published by license under
Chem 442 Review of Spectroscopy
Chem 44 Review of Spectroscopy General spectroscopy Wavelength (nm), frequency (s -1 ), wavenumber (cm -1 ) Frequency (s -1 ): n= c l Wavenumbers (cm -1 ): n =1 l Chart of photon energies and spectroscopies
Classical Electrodynamics
Classical Electrodynamics Third Edition John David Jackson Professor Emeritus of Physics, University of California, Berkeley JOHN WILEY & SONS, INC. Contents Introduction and Survey 1 I.1 Maxwell Equations