Theoretical approach to estimate radiation damage within FEL irradiated samples. Beata Ziaja
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1 Theoretical approach to estimate radiation damage within FEL irradiated samples Beata Ziaja Hasylab, DESY Hamburg and INP, Krakow Prague, November 2006
2 I. Mechanisms 2
3 Radiation damage Contribution of different processes to radiation damage strongly depends on radiation wavelength 3
4 Radiation damage by VUV photons Basic processes contributing: photoionizations (from outer shells) and collisional ionizations, elastic scatterings of electrons on atoms/ions long-range Coulomb interactions of charges with external and internal fields heating of electrons by inverse bremsstrahlung modification of atomic potentials by electron screening and ion environment recombination (3-body recombination) short range electron-electron interactions 4
5 Radiation damage by VUV photons Also other processes may contribute: sequential ionization, e.g. Xe Xe*, Xe* Xe+ multiphoton ionization many-body recombination ionization by internal electric field (at the edge of the sample)... 5
6 Radiation damage by VUV photons Specific interactions in detail: plasma effects 6
7 Plasma created by VUV photons Example: 7
8 Plasma created by VUV photons 8
9 Plasma created by VUV photons 9
10 Plasma created by VUV photons 10
11 Plasma created by VUV photons 11
12 Plasma created by VUV photons 12
13 Radiation damage by VUV photons Specific interactions in detail: inverse bremsstrahlung 13
14 Inverse bremsstrahlung 14
15 Inverse bremsstrahlung 15
16 Inverse bremsstrahlung Classical impact model cannot be applied in case of cold photoelectrons, as bmax< bmin 16
17 Inverse bremsstrahlung Quantum emission or absorption of n photons [Kroll, Watson]: 17
18 Inverse bremstrahlung Field strength parameter, s: 18
19 Electron screening and ion environment Example: Sample of Xe atoms before ionization (neutral) after ionization, if electrons stayed inside (ion potential screened by electrons) after ionization, if some electrons escaped (ion potential barriers overlap) 19
20 Radiation damage by X-ray photons Other processes than in VUV case give dominant contribution to radiation damage: inner and outer shell ionizations. No inverse bremsstrahlung. Warm/hot plasma is created. 20
21 Radiation damage by X-ray photons Basic processes contributing: photoionizations (from outer and inner shells with subsequent Auger decays) and collisional ionizations, elastic scatterings of electrons on atoms/ions long-range Coulomb interactions of charges with internal fields modification of atomic potentials by electron screening and ion environment recombination (3-body recombination) short range electron-electron interactions Compton scattering No inverse bremsstrahlung at these radiation wavelengths! 21
22 Radiation damage by X-ray photons Specific interactions in detail: photo- and collisional ionizations 22
23 Photoionizations 23
24 Auger effect 24
25 Collisional ionizations by electrons Primary ionization (photo- and Auger) Secondary ionization Photons Electrons 25
26 Collisional ionization by electrons Two energy regimes of electrons released by X-ray photons: 26
27 II. Models 27
28 How to model radiation damage within irradiated samples? 28
29 Particle approach 29
30 Particle approach Advantages: first-principles model transparent algorithm no complex numerics Disadvantages: High computational costs which scale with the number of participating particles statistical errors 30
31 Particle approach Methods: stochastic Monte-Carlo method deterministic Molecular Dynamics simulations Particle-in-Cell method 31
32 Particle approach Example: MC code for modelling Auger-electron cascade in diamond 32
33 Particle approach Example: MC code for modelling Auger-electron cascade in diamond 33
34 Particle approach Example: MC code for modelling Auger-electron cascade in diamond 34
35 Particle approach Example: MC code for modelling Auger-electron cascade in diamond Results: spatio-temporal evolution of electron cascade Electron range: 35
36 Particle approach Example: MC code for modelling an Auger-electron cascade in diamond 36
37 Transport approach Evolution of larger systems described in terms of collective density function: 37
38 Transport approach 38
39 Transport approach Methods: Semiclassical Boltzmann equation Hydrodynamic models 39
40 Transport approach 40
41 Transport approach 41
42 Working with Boltzmann equations Plasma physics Applied mathematics Solid state physics Atomic physics Algorithm Contributing physical processes Boltzmann solver 42
43 Why to use statistical Boltzmann approach? first-principle approach single-run method computational costs do not scale with number of atoms Disadvantage: requires advanced numerical methods 43
44 Transport approach Example: Boltzmann solver for radiation damage within Xe clusters irradiated by VUV FEL photons 44
45 Hydrodynamic models Reduced form of Boltzmann equations: simplifying assumptions applied (e.g. only collective transport component of velocity treated, thermalisation of electrons assumed, local force equilibrium assumed) - standard tool for plasma simulations 45
46 Conclusions, questions and outlook Understanding of radiation damage within FEL irradiated samples important for theory and experiment Description of radiation damage more complicated in case of irradiation with VUV photons that with X-ray photons Choice of the method for modelling the radiation damage depends on the size and structure of the sample: (particle method for smaller, complex samples; transport method for large samples of regular structure) 46
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