Exploring ICD and Dynamic Interference by Free Electron Lasers
|
|
- Tyler Jesse Spencer
- 6 years ago
- Views:
Transcription
1 Exploring ICD and Dynamic Interference by Free Electron Lasers Lorenz Cederbaum Theoretische Chemie Physikalisch-Chemisches Institut Universität Heidelberg
2 Exploring Intermolecular Coulombic Decay by Free Electron Lasers or How energy deposited by FEL on one site in a medium can be transferred fast to the surrounding
3 How does an isolated excited ion decay?
4 How does an isolated excited ion decay?
5 How does an isolated excited ion decay?
6 ICD L.S. Cederbaum, J. Zobeley, and F. Tarantelli, PRL 79, 4778 (1997) * A + B A + B + + e ICD is a general phenomenon Hydrogen bonded clusters (H 2 O) n, (HF) n van der Waals clusters Ne n, Ne n Ar m, MgNe, CaNe,... even He 2 quantum dots Ultrafast process fs regime Faster with more neighbors Source of LEE biological relevance
7 ICD in water L. S. Cederbaum, J. Zobeley and F. Tarantelli, PRL 79, 4778 (1997). I. B. Müller and LSC, J. Chem. Phys. 125, (2006). O. Vendrell, S. Stoychev and LSC, Chem. Phys. Chem. 11, 1006 (2010).
8 ICD in water Dimer: T. Jahnke, R. Dörner et al., Nature Phys. 6, 139 (10) Electron-ion coincidence experiments Large clusters: M. Mucke, U. Hergenhahn et al., Nature Phys. 6, 143 (10) Sum of electron energy experiments
9 electrons ICD-electrons ICD-electrons KER Photoelectron spectrum ICD generates lowenergy electrons in water exactly in the energy range where electrons are known to cause DNA strand breaks by dissociative attachment.
10 ICD in H-bonded H systems S.D. Stoychev, A.I. Kuleff, and L.S. Cederbaum, JACS 133, 6817 (2011)
11 ICD in H-bonded H systems S.D. Stoychev, A.I. Kuleff, and L.S. Cederbaum, JACS 133, 6817 (2011)
12 ICD in van der Waals clusters R. Santra, J. Zobeley, L. S. Cederbaum, and N. Moiseyev, Phys. Rev. Lett. 85, 4490 (2000). R. Santra, J. Zobeley, and L. S. Cederbaum, Phys. Rev. B 64, (2001). N. Sisourat, N. V. Kryzhevoi, P. Kolorenc, S. Scheit and L. S. Cederbaum, Nature Phys. (2010).
13 Ionization and double-ionization spectra of atomic Ne and Ne 2 dimer In Ne 2 dimer: 'one-site' Ne 2+ Ne 'two-site' Ne + Ne +
14
15 Interatomic Coulombic decay in Ne n clusters R. Santra, J. Zobeley, and L. S. Cederbaum, Phys. Rev. B 64, (2001).
16 Exploring ICD by free electron lasers Ph. Demekhin, S. Stoychev, A. Kuleff, and L.S. Cederbaum, PRL 107, (2011).
17 ICD by FEL For ICD: Ph. Demekhin et al., PRL 107, (2011). For Auger in isolated atom: E. P. Kanter et al., PRL 107, (2011).
18 Exploring ICD by free electron lasers At least two photons are needed for the ICD process. ω = ev
19 Exploring ICD by free electron lasers Integral yield of Ne + ion pairs Comparison of yields for a pulse of central frequency ω = ev (two-photon process) and a pulse doubling the central frequency, ω = ev (one-photon process). Same peak intensity.
20 Electron spectra for different pulse durations and intensities
21 Exploring ICD by free electron lasers Contributions to the electron spectrum. There are strong interference effects between the ICD electrons and those produced by direct ionization of the two Ne atoms.
22 Exploring ICD by free electron lasers Measuring the individual contribution of ICD. Total electron spectrum that measured 30 fs after pulse maximum.
23 Exploring ICD by free electron lasers In a laser field at resonant frequency the potential energy surfaces of the initial state and of the excited state possess a light-induced conical intersection even for a diatomic [1]. If decay processes (like ICD) are involved, the surfaces become complex and their intersections are light-induced DICES (Doubly Intersecting Complex Energy Surfaces) [2]. 1 M. Sindelka, N. Moiseyev, and L.S. Cederbaum, J. Phys. B 44, (2011). 2 L.S. Cederbaum, Y.-C. Chiang, P.V. Demekhin, and N. Moiseyev, PRL 106, (2011).
24 Theory Ansatz for the total WF Nuclear WP propagation Molecular Hamiltonian matrix
25 Summary Enhancement of ICD by strong fields: Two-photon absorption is more efficient than one-photon absorption of double frequency (traditional scheme) Sequential two-photon absorption by one subunit competes with the absorption of two photons by two different subunits Coherent superposition of these two-photon ionization mechanisms: two physical mechanisms two different timescales Measurement of the spectrum after a time delay will allow to identify the individual contributions and determine ICD
26 Dynamic Interference Bound-Continuum Scenario Ph.V. Demekhin and L.S. Cederbaum, Phys. Rev. Lett. 108, (2012). For model ion: K. Toyota et al., Phys. Rev. A 76, (2007). Bound-Bound Scenario Ph.V. Demekhin and L.S. Cederbaum, submitted (2012) arxiv: v1.
27 Bound-Continuum Scenario Weak Field What happens if the field becomes more intense? Field Peak Intensity Total wavefunction
28 Exact photoelectron spectrum of the H atom ω = ev 2 2 gt () = exp( t / τ ) ω IP = 40 ev
29 How to understand the surprising findings? To simplify the exact equations we introduce approximations and verify them. Rotating wave approximation Local approximation Stationary phase approximation
30 Local approximation Ground state amplitude in the local approximation AC Stark Shift and ionization rate
31 Local approximation Photoelectron spectrum
32 Stationary phase approximation Stationary phase condition and the spectrum
33 Dynamic Interference Physical meaning of the stationary phase The dressed ground state follows the pulse and electrons of the same energy emitted at different times interfere with each other. The interference pattern is controlled by the shape of the pulse. Easily generalizable to many electron systems.
34 Bound-Bound Scenario Weak Field The initial (I) and intermediate (R) states are coupled resonantly by the field. Here, for stronger fields, the coupling of the states via the laser pulse is responsible for the shift of the dressed levels as a function of time.
35 Dynamic interference in the two-photon ionization of H Electron spectra Ansatz for the total WF
36 Dynamical coupling of resonances 2x2 Hamiltonian Decoupled resonances scenario Spectrum
37 Dynamic interference in the two-photon ionization Physical meaning The two dressed levels ± > = ( I > ± R > )/ 2 are degenerate at low intensity and repel each other at higher intensity. This repulsion follows the pulse and electrons of the same energy emitted at different times interfere with each other.
38 Summary Dynamic interference is a general consequence of the nature of laser pulses, and it is fundamental to the spectroscopy of strong laser fields. Whenever the field-induced couplings between electronic states of a system and hence the energies of the resonantly dressed states possess the time dependence provided by the pulse, the phenomenon of dynamic interference takes place. This is always the case at high laser frequencies. Where can it be seen: Single-photon ionization (due to AC Stark effect) Two-photon ionization (due to resonant coupling) Resonant auger decay (due to resonant coupling) X-ray photoemission (resonant coupling or AC Stark effect)
39 Jürgen Zobeley ICD Robin Santra ICD Simona Scheit dynamics Imke Müller microsolvation cluster Vitali Averbukh decay widths Kirill Gokhberg RICD Spas Stoychev ICD following Auger Nicolas Sisourat He dimer Acknowledgements External collaboration - Theory External collaboration - Experiment Christian Buth XeF n Hans-Dieter Meyer CAP & CAP/CI Thomas Sommerfeld CAP/CI Alex Kuleff electron dynamics Nayana Vaval Propagators/CAP Nikolai Kryshevoi He droplets Ying-Chih Chiang cascades Philipp Demekhin ICD/Dyn. Interfer. Francesco Tarantelli computational techniques Perugia/Italia Nimrod Moiseyev Ne 2 dynamics Haifa/Israel U. Hergenhahn München/BESSY R. Dörner Frankfurt P. Lablanquie Paris E. Rühl Berlin K. Ueda Sendai
40 Extra material
41 Controllability of the dynamic interference
42 Dynamic interference in He Total AC Stark shift:
43 Dynamic interference in the resonant Auger decay N. Rohringer and R. Santra Ph. V. Demekhin and L. S. Cederbaum
NONLINEAR PROCESSES IN THE EXTREME ULTRAVIOLET REGION USING THE FEL
NONLINEAR PROCESSES IN THE EXTREME ULTRAVIOLET REGION USING THE FEL FERMI@ELETTRA A. Dubrouil, M. Reduzzi, C. Feng, J. Hummert, P. Finetti, O. Plekan, C. Grazioli, M. Di Fraia, V. Lyamayev,A. LaForge,
More informationDetecting ultrafast interatomic electronic processes in media by fluorescence
FAST TRACK COMMUNICATION OPEN ACCESS Detecting ultrafast interatomic electronic processes in media by fluorescence To cite this article: André Knie et al 2014 New J. Phys. 16 102002 View the article online
More informationLETTER. Site- and energy-selective slow-electron production through intermolecular Coulombic decay
doi:10.1038/nature12936 Site- and energy-selective slow-electron production through intermolecular Coulombic decay Kirill Gokhberg 1,Přemysl Kolorenč 2, Alexander I. Kuleff 1 & Lorenz S. Cederbaum 1 Irradiation
More informationarxiv: v2 [physics.atom-ph] 19 Mar 2012
Kinetic Energy Release in Fragmentation Processes following Electron Emission: A time dependent approach Ying-Chih Chiang 1, Frank Otto 1, Hans-Dieter Meyer 1, Lorenz S. Cederbaum 1 1 Theoretische Chemie,
More informationX-Ray Probing of Atomic and Molecular Dynamics in the Attosecond Limit
X-Ray Probing of Atomic and Molecular Dynamics in the Attosecond Limit Produce high order harmonics (soft x-rays) and use them for ultrafast time-resolved femtosecond dynamics experiments and attosecond
More informationMulti-electron coincidence spectroscopy: double photoionization from molecular inner-shell orbitals
Journal of Physics: Conference Series OPEN ACCESS Multi-electron coincidence spectroscopy: double photoionization from molecular inner-shell orbitals To cite this article: Y Hikosaka et al 2014 J. Phys.:
More informationICPEAC XXX, Carins, Australia. Nonlinear resonant Auger spectroscopy in CO using an x-ray pump-control scheme 2017/07/31
ICPEAC XXX, Carins, Australia Nonlinear resonant Auger spectroscopy in CO using an x-ray pump-control scheme Song-Bin Zhang Shaanxi Normal University, Xi an, China 2017/07/31 Acknowledgements Victor Kimberg
More informationarxiv: v1 [physics.atom-ph] 4 May 2017
Observation and Control of Laser-Enabled Auger Decay arxiv:1705.01812v1 [physics.atom-ph] 4 May 2017 D. Iablonskyi, 1 K. Ueda, 1, Kenichi L. Ishikawa, 2, 3 A. S. Kheifets, 4 P. Carpeggiani, 5 M. Reduzzi,
More informationSfb 658 Colloquium 11 May Part II. Introduction to Two-Photon-Photoemission (2PPE) Spectroscopy. Martin Wolf
Sfb 658 Colloquium 11 May 2006 Part II Introduction to Two-Photon-Photoemission (2PPE) Spectroscopy Martin Wolf Motivation: Electron transfer across interfaces key step for interfacial and surface dynamics
More informationCorrelated electronic decay following intense nearinfrared ionization of clusters
Journal of Physics: Conference Series PAPER OPEN ACCESS Correlated electronic decay following intense nearinfrared ionization of clusters To cite this article: Bernd Schütte et al 2015 J. Phys.: Conf.
More informationOn the nature and origin of di-cationic, charge-separated species formed in liquid water upon X-ray irradiation
On the nature and origin of di-cationic, charge-separated species formed in liquid water upon X-ray irradiation Stephan Thürmer, 1 Milan Ončák, 2 Niklas Ottosson, 3 Robert Seidel, 4 Uwe Hergenhahn, 5 Stephen
More informationarxiv: v1 [physics.atm-clus] 12 Aug 2013
Nuclear wave packet quantum interference in the intense laser dissociation of the D + molecule Gábor J. Halász, Ágnes Vibók, Department of Information Technology, University of Debrecen, H- Debrecen, PO
More informationICD - THE DECAY WIDTHS I
CD - THE DECAY WDTHS 1 st ORDER THEORY AND GENERAL CHARACTERSTCS Přemysl Kolorenč nstitute of Theoretical Physics, Charles University in Prague CD Summer School Bad Honnef September 1 st 5 th P. Kolorenč
More informationSupporting information for Metal-semiconductor. nanoparticle hybrids formed by self-organization: a platform to address exciton-plasmon coupling
Supporting information for Metal-semiconductor nanoparticle hybrids formed by self-organization: a platform to address exciton-plasmon coupling Christian Strelow, T. Sverre Theuerholz, Christian Schmidtke,
More informationAuger electron and x-ray emission from high-z few-electron ions
Auger electron and x-ray emission from high-z few-electron ions S. Fritzsche MPI für Kernphysik Heidelberg and GSI Darmstadt 4th August 2007 Main goal for studying high-z ions is the better understanding
More informationMulti-Dimensional IR Spectroscopy of Acetic Acid Dimers and Liquid Water
Multi-Dimensional IR Spectroscopy of Acetic Acid Dimers and Liquid Water N. Huse 1, J. Dreyer 1, E.T.J.Nibbering 1, T. Elsaesser 1 B.D. Bruner 2, M.L. Cowan 2, J.R. Dwyer 2, B. Chugh 2, R.J.D. Miller 2
More informationAn Investigation of Benzene Using Ultrafast Laser Spectroscopy. Ryan Barnett. The Ohio State University
An Investigation of Benzene Using Ultrafast Laser Spectroscopy Ryan Barnett The Ohio State University NSF/REU/OSU Advisor: Linn Van Woerkom Introduction Molecular spectroscopy has been used throughout
More informationAtomic structure and dynamics
Atomic structure and dynamics -- need and requirements for accurate atomic calculations Analysis and interpretation of optical and x-ray spectra (astro physics) Isotope shifts and hyperfine structures
More informationICD - THE DECAY WIDTHS II
ICD - THE DECAY WIDTHS II BEYOND WIGNER-WEISSKOPF Přemysl Kolorenč Institute of Theoretical Physics, Charles University in Prague ICD Summer School Bad Honnef September 1 st 5 th P. Kolorenč (Charles University
More informationHigh-energy collision processes involving intense laser fields
High-energy collision processes involving intense laser fields Carsten Müller Max Planck Institute for Nuclear Physics, Theory Division (Christoph H. Keitel), Heidelberg, Germany EMMI Workshop: Particle
More information31 st International Free Electron Laser Conference
FHI-BERLIN ASG at CFEL MAX-PLANCK-GESELLSCHAFT 3 st International Free Electron Laser Conference 3 rd - 8 th August, 009 BT Convention Centre Liverpool, UK Evidence for Position Based Entanglement in Auger
More informationAtomic double slit: Coherence transfer through excitation and (Auger) decay processes. S. Fritzsche, Kassel University Göteborg, 3rd June 2006
Atomic double slit: Coherence transfer through excitation and (Auger) decay processes S. Fritzsche, Kassel University Göteborg, 3rd June 2006 Experiments with double slits (Feynman-Lectures 1962) Interference
More informationLecture on: Multiphoton Physics. Carsten Müller
Lecture on: Multiphoton Physics Carsten Müller Institut für Theoretische Physik I, Heinrich-Heine-Universität Düsseldorf Max-Planck-Institut für Kernphysik, Heidelberg IMPRS-QD Annual Event, MPIK, Heidelberg,
More informationInterference effects on the probe absorption in a driven three-level atomic system. by a coherent pumping field
Interference effects on the probe absorption in a driven three-level atomic system by a coherent pumping field V. Stancalie, O. Budriga, A. Mihailescu, V. Pais National Institute for Laser, Plasma and
More informationSpectroscopies for Unoccupied States = Electrons
Spectroscopies for Unoccupied States = Electrons Photoemission 1 Hole Inverse Photoemission 1 Electron Tunneling Spectroscopy 1 Electron/Hole Emission 1 Hole Absorption Will be discussed with core levels
More informationSUPPLEMENTARY INFORMATION
DOI: 10.1038/NCHEM.1680 On the nature and origin of dicationic, charge-separated species formed in liquid water on X-ray irradiation Stephan Thürmer, 1 Milan Ončák, 2 Niklas Ottosson, 3 Robert Seidel,
More informationInterface identification by non-local autoionization transitions
ARTICLE www.rsc.org/[journal] [journal name] Interface identification by non-local autoionization transitions Silko Barth, a Simon Marburger, a Sanjeev Joshi, a Volker Ulrich, a Oliver Kugeler a,b and
More informationResonances in Chemical Reactions : Theory and Experiment. Toshiyuki Takayanagi Saitama University Department of Chemistry
Resonances in Chemical Reactions : Theory and Experiment Toshiyuki Takayanagi Saitama University Department of Chemistry What is Chemical Reaction? Collision process between molecules (atoms) containing
More informationAttosecond-correlated dynamics of two electrons in argon
PRAMANA c Indian Academy of Sciences Vol. 82, No. 1 journal of January 2014 physics pp. 79 85 Attosecond-correlated dynamics of two electrons in argon V SHARMA 1,,NCAMUS 2, B FISCHER 2, M KREMER 2, A RUDENKO
More informationViolation of electronic optical selection rules in x-ray emission by nuclear dynamics: Time-dependent formulation
Violation of electronic optical selection rules in x-ray emission by nuclear dynamics: Time-dependent formulation S. A. Malinovskaya* and L. S. Cederbaum Physikalisch-Chemisches Institut, Theoretische
More informationStrong Field Quantum Control. CAMOS Spring Meeting 2012 o
Strong Field Quantum Control CAMOS Spring Meeting 2012 o p Motivation & Outline Motivation: Want to control molecular dynamics and develop control based spectroscopy 1. Controlling Molecular Dissociation
More informationJahn-Teller Intersections of Potential Energy Surfaces: A Paradigm for Nonadiabatic Excited-State Dynamics
Jahn-Teller Intersections of Potential Energy Surfaces: A Paradigm for Nonadiabatic Excited-State Dynamics Horst Köppel Horst.Koeppel@pci.uni-heidelberg.de Theoretische Chemie Physikalisch-Chemisches Institut
More informationModels for Time-Dependent Phenomena. I. Laser-matter interaction: atoms II. Laser-matter interaction: molecules III. Model systems and TDDFT
Models for Time-Dependent Phenomena I. Laser-matter interaction: atoms II. Laser-matter interaction: molecules III. Model systems and TDDFT Manfred Lein, TDDFT school Benasque 22 p. Outline Laser-matter
More informationarxiv:physics/ v2 20 Mar 2004
mpact of nteratomic Electronic Decay Processes on Xe4d Hole Decay in the Xenon Fluorides Christian Buth, Robin Santra, and Lorenz S. Cederbaum Theoretische Chemie, Physikalisch-Chemisches nstitut, Ruprecht-Karls-Universität
More informationAarhus University Denmark
Participant presentation: Aarhus University Denmark Lars Bojer Madsen Department of Physics and Astronomy Henrik Stapelfeldt Department of Chemistry MEDEA Kick-off MBI, Berlin January 19-20, 2015 Alignment
More informationand states of CH 2 Non-adiabatic effects in the à 2 B 2 through coupling vibrational modes Journal of Physics: Conference Series Related content
Journal of Physics: Conference Series PAPER OPEN ACCESS Non-adiabatic effects in the à B and states of CH F + through coupling vibrational modes To cite this article: Rudraditya Sarkar 016 J. Phys.: Conf.
More informationLooking into the ultrafast dynamics of electrons
Looking into the ultrafast dynamics of electrons G. Sansone 1,2,3 1) Dipartimento di Fisica Politecnico Milano, Italy 2) Institute of Photonics and Nanotechnology, CNR Politecnico Milano Italy 3) Extreme
More informationWP-3: HHG and ultrafast electron imaging
WORKPACKAGE WP-3: HHG and ultrafast electron imaging Coordinators: P. Salières (CEA), A. Assion (FEMTO, Spectra Physics Vienna) Period: Start Month 4 End Month 48 Leading Participants (Orange in the picture):
More informationAMO at FLASH. FELs provide unique opportunities and challenges for AMO physics. due to essentially three reasons:
Experience at FLASH AMO at FLASH FELs provide unique opportunities and challenges for AMO physics due to essentially three reasons: AMO at FLASH 1. huge integrated flux dilute samples Highly charged ions
More informationNonlinear Optics (WiSe 2015/16) Lecture 12: January 15, 2016
Nonlinear Optics (WiSe 2015/16) Lecture 12: January 15, 2016 12 High Harmonic Generation 12.1 Atomic units 12.2 The three step model 12.2.1 Ionization 12.2.2 Propagation 12.2.3 Recombination 12.3 Attosecond
More informationAnalysis of the ultrafast dynamics of the silver trimer upon photodetachment
J. Phys. B: At. Mol. Opt. Phys. 29 (1996) L545 L549. Printed in the UK LETTER TO THE EDITOR Analysis of the ultrafast dynamics of the silver trimer upon photodetachment H O Jeschke, M E Garcia and K H
More informationProbing Matter: Diffraction, Spectroscopy and Photoemission
Probing Matter: Diffraction, Spectroscopy and Photoemission Anders Nilsson Stanford Synchrotron Radiation Laboratory Why X-rays? VUV? What can we hope to learn? 1 Photon Interaction Incident photon interacts
More informationarxiv: v1 [physics.atom-ph] 9 Jan 2018
Normal Auger processes with ultrashort x-ray pulses in Neon Raymond Sullivan, 1, Junteng Jia, 3,4 Álvaro Vázquez-Mayagoitia, 4 and Antonio Picón 1 Western Illinois University, Macomb, IL 61455 Argonne
More informationAttosecond Science. Jon Marangos, Director Extreme Light Consortium, Imperial College London
Attosecond Science Jon Marangos, Director Extreme Light Consortium, Imperial College London Electron Orbit in Bohr Model T orbit 150 as for H ground state Electron Motion In most matter electrons are in
More informationMultiphoton Multielectron Ionization of Rare Gas Atoms under FEL Radiation (An attempt at interpreting existing experimental data from FLASH)
Multiphoton Multielectron Ionization of Rare Gas Atoms under FEL Radiation (An attempt at interpreting existing experimental data from FLASH) Hamburg Oct. 8 10, 2008 P. Lambropoulos in collaboration with
More informationTwo-center resonant photoionization in slow atomic collisions & strong laser fields
Two-center resonant photoionization in slow atomic collisions & strong laser fields A.B. Voitkiv,1 J. Fedyk,2 S.F. Zhang,3 X. Ma3 and C. Müller1 Institut für Theoretische Physik I, Uni Düsseldorf 2 Physikalisch-Chemisches
More informationModels for Time-Dependent Phenomena
Models for Time-Dependent Phenomena I. Phenomena in laser-matter interaction: atoms II. Phenomena in laser-matter interaction: molecules III. Model systems and TDDFT Manfred Lein p.1 Outline Phenomena
More informationPhoton Interaction. Spectroscopy
Photon Interaction Incident photon interacts with electrons Core and Valence Cross Sections Photon is Adsorbed Elastic Scattered Inelastic Scattered Electron is Emitted Excitated Dexcitated Stöhr, NEXAPS
More informationLecture 12. Electron Transport in Molecular Wires Possible Mechanisms
Lecture 12. Electron Transport in Molecular Wires Possible Mechanisms In Lecture 11, we have discussed energy diagrams of one-dimensional molecular wires. Here we will focus on electron transport mechanisms
More informationBackground and Present Status from AMO Instrument Team
Background and Present Status from AMO Instrument Team 1. Team Organization. 2. Proposed Scientific Plan. 3. The First Experiment. 4. Future Plan. Historical Facts April 2004: LCLS puts out a call for
More informationMechanism of Tunneling in Interacting Open Ultracold Few-Boson Systems. Abstract
Mechanism of Tunneling in Interacting Open Ultracold Few-Boson Systems Axel U. J. Lode, Alexej I. Streltsov, Ofir E. Alon, and Lorenz S. Cederbaum arxiv:1005.0093v1 [cond-mat.quant-gas] 1 May 2010 Theoretische
More informationSUPPLEMENTARY INFORMATION
Fig. S1: High-Harmonic Interferometry of a Chemical Reaction A weak femtosecond laser pulse excites a molecule from its ground state (on the bottom) to its excited state (on top) in which it dissociates.
More informationMany-particle fragmentation processes in atomic and molecular physics new insight into the world of correlation
Nuclear Instruments and Methods in Physics Research B 233 (2005) 3 11 www.elsevier.com/locate/nimb Many-particle fragmentation processes in atomic and molecular physics new insight into the world of correlation
More informationThe Mechanism of Excimer Formation: An Experimental and Theoretical Study on the Pyrene Dimer: Supplementary Material
Electronic Supplementary Material (ESI) for Physical Chemistry Chemical Physics. This journal is the Owner Societies 2017 The Mechanism of Excimer Formation: An Experimental and Theoretical Study on the
More informationULTRAFAST LASER CONTROL. Of IONIZATION. Fundamentals And Applications. Thomas Baumert. Institut fuer Physik der Universitaet Kassel, GERMANY
ULTRAFAST LASER CONTROL Fundamentals And Applications Of IONIZATION Thomas Baumert Institut fuer Physik der Universitaet Kassel, GERMANY H. Baumann: first permanent Laser Sculpture / since Documenta 6
More informationAcademic qualifications. Research experience. Research programs
Nicolas SISOURAT born 1981, september 7 Associate Professor e-mail: nicolas.sisourat@upmc.fr Tel. : 00 33 1 44 27 62 78 Fax. : 00 33 1 44 27 62 26 Laboratoire de Chimie Physique-Matière et Rayonnement
More informationModels for Time-Dependent Phenomena
Models for Time-Dependent Phenomena I. Phenomena in laser-matter interaction: atoms II. Phenomena in laser-matter interaction: molecules III. Model systems and TDDFT Manfred Lein p. Outline Phenomena in
More informationarxiv: v1 [physics.atm-clus] 9 Sep 2014
Phys. Rev. A 90, 022515 (2014) Interatomic-Coulombic-Decay induced recapture of photoelectrons in Helium Dimers P. Burzynski 1, F. Trinter 1, J. B. Williams 1, M. Weller 1, M. Waitz 1, M. Pitzer 1, J.
More informationXMDYN: Modeling radiation damage of XFEL irradiated samples
XMDYN: Modeling radiation damage of XFEL irradiated samples 16.09.2014 Zoltan Jurek, Beata Ziaja, Robin Santra Theory Division, Center for Free-Electron Laser Science, DESY Outline > Introduction modeling
More informationX-Ray transitions to low lying empty states
X-Ray Spectra: - continuous part of the spectrum is due to decelerated electrons - the maximum frequency (minimum wavelength) of the photons generated is determined by the maximum kinetic energy of the
More informationElectronic structure of correlated electron systems. Lecture 2
Electronic structure of correlated electron systems Lecture 2 Band Structure approach vs atomic Band structure Delocalized Bloch states Fill up states with electrons starting from the lowest energy No
More informationMagnetic Binding and Cyclotron Transitions of the Ions: Applications to Laboratory and Astrophysically Strong Magnetic Fields
Magnetic Binding and Cyclotron Transitions of the Ions: Applications to Laboratory and Astrophysically Strong Magnetic Fields Victor G Bezchastnov victor@tcpciuni-heidelbergde Theoretische Chemie Physikalisch-Chemisches
More informationQuantum Feedback Stabilized Solid-State Emitters
FOPS 2015 Breckenridge, Colorado Quantum Feedback Stabilized Solid-State Emitters Alexander Carmele, Julia Kabuss, Sven Hein, Franz Schulze, and Andreas Knorr Technische Universität Berlin August 7, 2015
More informationLaser-controlled Molecular Alignment and Orientation. Marc Vrakking FOM Institute AMOLF
Laser-controlled Molecular Alignment and Orientation Marc Vrakking FOM Institute AMOLF Summer School Cargese - Tuesday August 19 th 2008 Contents What is molecular alignment resp. orientation, and why
More informationRichard Miles and Arthur Dogariu. Mechanical and Aerospace Engineering Princeton University, Princeton, NJ 08540, USA
Richard Miles and Arthur Dogariu Mechanical and Aerospace Engineering Princeton University, Princeton, NJ 08540, USA Workshop on Oxygen Plasma Kinetics Sept 20, 2016 Financial support: ONR and MetroLaser
More informationDensity-matrix theory for time-resolved dynamics of superconductors in non-equilibrium
Max Planck Institute for Solid State Research Density-matrix theory for time-resolved dynamics of superconductors in non-equilibrium co-workers and papers: (1) (2) (3) (4) Dirk Manske A. Knorr (TU Berlin),
More informationPhysics and Chemistry with Diatomic Molecules Near Absolute Zero. Tanya Zelevinsky & ZLab Columbia University, New York
Physics and Chemistry with Diatomic Molecules Near Absolute Zero Tanya Zelevinsky & ZLab Columbia University, New York Pupin Labs @ Columbia E. Fermi I. I. Rabi 10 What is Ultracold? MK kk 7 6 5 4 3 2
More informationMolecular alignment, wavepacket interference and Isotope separation
Molecular alignment, wavepacket interference and Isotope separation Sharly Fleischer, Ilya Averbukh and Yehiam Prior Chemical Physics, Weizmann Institute Yehiam.prior@weizmann.ac.il Frisno-8, Ein Bokek,
More informationCoherence Vibrations and Electronic Excitation Dynamics in Molecular Aggregates and Photosynthetic Pigment-Proteins
VILNIUS UNIVERSITY Coherence Vibrations and Electronic Excitation Dynamics in Molecular Aggregates and Photosynthetic Pigment-Proteins L. Valkunas Department of Theoretical Physics, Faculty of Physics,
More informationTime-dependent density functional theory
Time-dependent density functional theory E.K.U. Gross Max-Planck Institute for Microstructure Physics OUTLINE LECTURE I Phenomena to be described by TDDFT LECTURE II Review of ground-state DFT LECTURE
More informationChapter 9: Multi- Electron Atoms Ground States and X- ray Excitation
Chapter 9: Multi- Electron Atoms Ground States and X- ray Excitation Up to now we have considered one-electron atoms. Almost all atoms are multiple-electron atoms and their description is more complicated
More informationEntangled Photon Generation via Biexciton in a Thin Film
Entangled Photon Generation via Biexciton in a Thin Film Hiroshi Ajiki Tokyo Denki University 24,Apr. 2017 Emerging Topics in Optics (IMA, Univ. Minnesota) Entangled Photon Generation Two-photon cascade
More informationMatthias Lütgens, Frank Friedriszik, and Stefan Lochbrunner* 1 Concentration dependent CARS and Raman spectra of acetic acid in carbon tetrachloride
Electronic Supplementary Material (ESI) for Physical Chemistry Chemical Physics. This journal is the Owner Societies 2014 SUPPORTING INFORMATION Direct observation of the cyclic dimer in liquid acetic
More informationNo. 2 lectronic state and potential energy function for UH where ρ = r r e, r being the interatomic distance and r e its equilibrium value. How
Vol 12 No 2, February 2003 cfl 2003 Chin. Phys. Soc. 1009-1963/2003/12(02)/0154-05 Chinese Physics and IOP Publishing Ltd lectronic state and potential energy function for UH 2+* Wang Hong-Yan( Ψ) a)y,
More informationCore Level Spectroscopies
Core Level Spectroscopies Spectroscopies involving core levels are element-sensitive, and that makes them very useful for understanding chemical bonding, as well as for the study of complex materials.
More informationUltrafast 2D Spectroscopy of Photosynthetic Light-Harvesting Complexes
Ultrafast 2D Spectroscopy of Photosynthetic Light-Harvesting Complexes PETAR LAMBREV PREAMBLE LASERS IN LIFE SCIENCE LASERS IN MEDICINE AND LIFE SCIENCE, SZEGED 2017 2 Preamble LASERS IN MEDICINE AND LIFE
More informationMicroscopic Modelling of the Optical Properties of Quantum-Well Semiconductor Lasers
Microscopic Modelling of the Optical Properties of Quantum-Well Semiconductor Lasers Stephan W. Koch Department of Physics Philipps University, Marburg/Germany OVERVIEW - Outline of Theory - Gain/Absorption
More informationVibrational Autoionization in Polyatomic molecules
Vibrational Autoionization in Polyatomic molecules S.T. Pratt Annu. Rev. Phys. Chem. 2005. 56:281-308 2006. 12. 4. Choi, Sunyoung 1 Schedule 12/4 (Mon) - Introduction - Theoretical background 12/6 (Wed)
More informationComputational and spectroscopic investigation of 7-azaindole: Solvation and intermolecular interactions
Computational and spectroscopic investigation of 7-azaindole: Solvation and intermolecular interactions Michael Kamrath, Krista Cruse, Nathan Erickson, Molly Beernink Abstract We report results of an experimental
More informationOkinawa School in Physics 2017 Coherent Quantum Dynamics. Cold Rydberg gases
Okinawa School in Physics 2017 Coherent Quantum Dynamics Cold ydberg gases 1. Basics of ydberg atoms 2. ydberg atoms in external fields. ydberg-ydberg interaction Wenhui Li Centre for Quantum Technologies
More informationLorentz meets Fano spectral line shapes: A universal phase and its laser control
Lorentz meets Fano spectral line shapes: A universal phase and its laser control Christian Ott 1, Andreas Kaldun 1, Philipp Raith 1, Kristina Meyer 1, Martin Laux 1, Jörg Evers 1, Christoph H. Keitel 1,
More informationAuthor(s): Niikura, Hiromichi; Wörner, Hans Jakob; Villeneuve, David M.; Corkum, Paul B.
Research Collection Journal Article Probing the Spatial Structure of a Molecular Attosecond Electron Wave Packet Using Shaped Recollision Trajectories Author(s): Niikura, Hiromichi; Wörner, Hans Jakob;
More informationNuclear Effects in Electron Capture into Highly Charged Heavy Ions
Nuclear Effects in Electron Capture into Highly Charged Heavy Ions W. Scheid 1,A.Pálffy 2,Z.Harman 2, C. Kozhuharov 3, and C. Brandau 3 1 Institut für Theoretische Physik der Justus-Liebig-Universität
More information8 Quantized Interaction of Light and Matter
8 Quantized Interaction of Light and Matter 8.1 Dressed States Before we start with a fully quantized description of matter and light we would like to discuss the evolution of a two-level atom interacting
More informationThe broad topic of physical metallurgy provides a basis that links the structure of materials with their properties, focusing primarily on metals.
Physical Metallurgy The broad topic of physical metallurgy provides a basis that links the structure of materials with their properties, focusing primarily on metals. Crystal Binding In our discussions
More informationTHz experiments at the UCSB FELs and the THz Science and Technology Network.
THz experiments at the UCSB FELs and the THz Science and Technology Network. Mark Sherwin UCSB Physics Department and Institute for Quantum and Complex Dynamics UCSB Center for Terahertz Science and Technology
More informationExercises 16.3a, 16.5a, 16.13a, 16.14a, 16.21a, 16.25a.
SPECTROSCOPY Readings in Atkins: Justification 13.1, Figure 16.1, Chapter 16: Sections 16.4 (diatomics only), 16.5 (omit a, b, d, e), 16.6, 16.9, 16.10, 16.11 (omit b), 16.14 (omit c). Exercises 16.3a,
More informationPIs: Louis DiMauro & Pierre Agostini
Interaction of Clusters with Intense, Long Wavelength Fields PIs: Louis DiMauro & Pierre Agostini project objective: explore intense laser-cluster interactions in the strong-field limit project approach:
More informationRevival Structures of Linear Molecules in a Field-Free Alignment Condition as Probed by High-Order Harmonic Generation
Journal of the Korean Physical Society, Vol. 49, No. 1, July 2006, pp. 337 341 Revival Structures of Linear Molecules in a Field-Free Alignment Condition as Probed by High-Order Harmonic Generation G.
More informationGroup Members: Your Name In Class Exercise #6. Photon A. Energy B
Group Members: Your Name In Class Exercise #6 Shell Structure of Atoms Part II Photoelectron Spectroscopy Photoelectron spectroscopy is closely related to the photoelectric effect. When high energy photons
More informationQuantum superpositions and correlations in coupled atomic-molecular BECs
Quantum superpositions and correlations in coupled atomic-molecular BECs Karén Kheruntsyan and Peter Drummond Department of Physics, University of Queensland, Brisbane, AUSTRALIA Quantum superpositions
More informationAtomic Quantum number summary. From last time. Na Optical spectrum. Another possibility: Stimulated emission. How do atomic transitions occur?
From last time Hydrogen atom Multi-electron atoms This week s honors lecture: Prof. Brad Christian, Positron Emission Tomography Course evaluations next week Tues. Prof Montaruli Thurs. Prof. Rzchowski
More informationAtomic Physics 3 rd year B1
Atomic Physics 3 rd year B1 P. Ewart Lecture notes Lecture slides Problem sets All available on Physics web site: http:www.physics.ox.ac.uk/users/ewart/index.htm Atomic Physics: Astrophysics Plasma Physics
More informationNon-equilibrium spin systems - from quantum soft-matter to nuclear magnetic resonance
Non-equilibrium spin systems - from quantum soft-matter to nuclear magnetic resonance Igor Lesanovsky Daejeon 24/10/2017 Postdocs Federico Carollo Carlos Espigares Perez Ricardo Gutierrez Alexander Karabanov
More informationPHOTO-DISSOCIATION OF CO 2 GAS BY USING TWO LASERS
Proceedings of the 3rd Annual ISC Research Symposium ISCRS 9 April 14, 9, Rolla, Missouri PHOTO-DISSOCIATION OF CO GAS BY USING TWO LASERS Zhi Liang MAE department/zlch5@mst.edu Dr. Hai-Lung Tsai MAE department/tsai@mst.edu
More informationClusters in intense x-ray pulses from 100 nm to.7 nm
Clusters in intense x-ray pulses from 100 nm to.7 nm Linac Coherent Light Source, SLAC National Accelerator Laboratory Outline: Introduction and motivation Spectroscopy of clusters Single shot imaging
More informationNuclear isomers in intense electromagnetic fields
Nuclear isomers in intense electromagnetic fields Adriana Pálffy Max Planck Institute for Nuclear Physics, Heidelberg, Germany SDANCA 15 Sofia, October 8th, 2015 Max Planck Institute in Heidelberg Light-nuclei
More informationAMO physics with LCLS
AMO physics with LCLS Phil Bucksbaum Director, Stanford PULSE Center SLAC Strong fields for x-rays LCLS experimental program Experimental capabilities End-station layout PULSE Ultrafast X-ray Summer June
More informationApplicability of atomic collisional ionization cross sections in plasma environment
Applicability of atomic collisional ionization cross sections in plasma environment Viktoriia Isaenko,Voronezh State University, Russia CFEL Theory Division September 6, 2018 Abstract Secondary ionization
More informationModule 4 : Third order nonlinear optical processes. Lecture 28 : Inelastic Scattering Processes. Objectives
Module 4 : Third order nonlinear optical processes Lecture 28 : Inelastic Scattering Processes Objectives In this lecture you will learn the following Light scattering- elastic and inelastic-processes,
More information