What we know about Francium. University of Science and Technology of China Hefei, China July 2018 Luis A. Orozco
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1 What we know about Francium University of Science and Technology of China Hefei, China July 2018 Luis A. Orozco
2 The slides are available at:
3 FrPNC Collaboration (Summer 2017) Seth Aubin; College of William and Mary, USA. John A. Behr, Matt R. Pearson, Alexander Gorolov, Mukut R. Kalita; TRIUMF, Canada. Victor V. Flambaum; University of New South Wales, Australia. Eduardo Gómez; Universidad Autónoma de San Luis Potosí, México. Gerald Gwinner SPOEKESPERSON M. Kossin, T. Hucko; University of Manitoba, Canada. Luis A. Orozco; University of Maryland, USA. Yanting Zhao; Shanxi University, Taijuan, China. Work supported by NRC, TRIUMF, and NSERC from Canada, DOE, and NSF from the USA, and CONACYT from Mexico.
4 The weak interaction
5 Rutherford discovered two kinds of radioactive rays (α, β), the second are electrons Ernest Rutherford
6 Beta Decay: Lise Meitner and Otto Hann (1911), Jean Danysz (1913), and James Chadwick (1914) measured the beta decay spectrum and see a continuum of energies. 210 Bi
7 Theory of beta decay by Fermi (1934) treats the process as if it were spontaneous emission Enrico Fermi
8 Spontaneous emission excited> excited> photon ground> ground> Beta decay neutron> proton> electron neutron> (anti)neutrino proton>
9 Parity non conservation
10 Nature (the weak interaction) lacks P symmetry Purcell and Ramsey say it should be tested T. D. Lee and C. N Yang point to the weak interaction Three experiments show that the weak interaction violates P: Wu, Lederman, and Telegdi lead the three efforts. The Columbia-NBS experiment by Wu, Ambler, Hayward, Hoppes and Hudson studied β decay of cobalt (σ p).
11 β decay 60 Co Wu, Ambler, Hayward, Hoppes, and Hudson; Columbia, National Bureau of Standards (ahora NIST). They look at the correlation between the nuclear spin nuclear σ and the electron momentum p! σ Parity is maximally violated in the weak interaction. p!
12 Feynman diagram of beta decay of a neutron. The W - is very heavy (about a Rb atom), so the interaction is short range, There are three carriers of the interaction: W + W - and Z 0.
13 The weak interaction in atomic physics
14 Coulomb, spin-orbit, etc. H atomic = H 0 + H PV Parity violating. (1958 Zel dovich) The new Hamiltonian induces a perturbation on the eigenstates: ϕ 0 Ψ = ϕ 0 + The ground state of alkali: ϕ n H ϕ PV 0 E 0 E ϕ n n Forbidden transitions (e.g. E1 between S states) become allowed n Ψ = ns 1/ 2 + δ np 1/ A Ψ i r Ψ f 0
15 H PV = G F H NSI PV 2 (κ 1iγ 5 κ nsd,i σ n α)δ(r) H NSD PV Nuclear spin independent Interaction: Coherent over all nucleons. Measurement increases as Z 3, from Q weak, S> and P> Nuclear spin dependent interaction: Only from valence nucleons. Measurement increases as Z 8/3 Main contribution from anapole moment for heavy nuclei.
16 A. Weiss
17 How to extract weak charge Q w from Cs experiment? e e Z 0 q q Electron-quark parity violating interaction (exchange of virtual Z 0 boson) Neutron density function Electronic sector: Extraction of weak the charge: Theoretical calculation of PNC amplitude Measured value Safranova
18 Measure APNC and compare to predictions of the SM and study if the weak interaction gets affected by the presnece of lots of nucleons. Use a heavy atom (Buchiats) as the measurements scale faster than Z 3 and Z 8/3
19
20 Francium
21 Discovery as a product of actinium decay 1939
22 Margarite Perey, first row left, Radium Institute, Paris~1939
23 Fr Z=87; A= and neutron rich 221 (TRIUMF) Radioactive ( 212 Fr: τ 1/2 =20min; 209 Fr: τ 1/2 =1 min) Make it and trap it. Simple atomic structure, quantitatively understandable We want to use it as a laboratory to study the weak interaction through the signature of parity non-conservation.
24 How did we make Fr at Stony Brook? Z Chart of the Nuclei Fr 210 product Gold Target 18 O projectile O + Au Fr 215 neutrons N
25 A Brief History of Francium at Stony Brook : Construction of 1 st production and trapping apparatus. 1995: Produced and Trapped Francium in a MOT : Laser spectroscopy of Francium. 2,000 atoms Fr MOT : High efficiency trap. 2003: Spectroscopy. 2004: Lifetime of 8S level. 2007: Magnetic moment 210 Fr. 250,000 atoms Fr MOT
26 Spectroscopy studies of francium Ideal cold sample of trapped atoms (no Doppler broadening) Energy levels Excited state lifetimes (transition matrix elements) Hyperfine splittings (wavefunctions at the nucleus) Quantitative comparisons to ab initio calculations. Nuclear structure studies (nuclear magnetization).
27 Francium Atomic Energy Levels 8S 1/2 6D state 7P 3/2 506nm 718nm 7P 1/2 817nm 7S 1/2
28 8s atomic lifetime measurement and theory Uncertainty ± 0.7% a) Safronova et.al. b) Dzuba et.al. c) Johnson et.al. d) Dzuba et.al. e) Marinescu et.al. f) Theodosiou et.al. g) Biemont et.al. h) Van Wijngaarden et.al.
29 Spin independent APNC
30 APNC in Cesium at Boulder 1997 Wieman (Boulder) 0.35% measurement from an experiment in one isotope of Cesium. The most accurate test of the standard model with atomic physics. Follows the suggestion of the Bouchiats to use heavy atoms. Uses interference with a Stark Induced transition to enhance the signal. Uses atomic beams optically pumped Uses a cavity enhancing the 6S to 7S transition.
31
32 Spin dependent APNC
33 The Anapole Moment History 1958 Zel dovich, Vaks 1980 Khriplovich, Flambaum 1984 Khriplovich, Flambaum, Shuskov 1995 Fortson (Seattle) bound from an experiment Thallium 1997 Wieman (Boulder) 15% measurement from an experiment in one isotope of Cesium
34 Does weak N-N interaction change in heavy nuclei? isoscalar isovector
35 The dream in francium isoscalar isovector
36 1.- Define handedness of the apparatus by the coordinate system (ie RF B M 1 B DC ) 2.- Create superposition to interfere and enhance PNC signal: A total = A PC PNC M 1 ± A E1 3.- Measure rate of transition through resonance fluorescence. Rate A total Change handedness of apparatus + Signal A total 2 Atotal 2 Expected signal with 450 V/m 5.- Repeat. A E1! = 0.01 rad /s
37
38 Principle of the measurement (AM 1 ± AE1 )t c Ξ ± = N sin 2! AM 1t c AE1t c S = Ξ + Ξ N sin 2! 2! 2 Control phase of different interactions Ground state hyperfine splitting Fr ~46 GHz, Z=87 Rb ~6.834 GHz, Z=37
39 Oscillations and sensitivity test 1.0 P M1 Rabi oscillations (50 Hz) with 10 5 Rb atoms in blue detuned (20 nm) dipole trap interaction time (ms) P At 37.5 ms, add a second microwave source with 10 4 attenuation, change of the phase. 0 π/3 2π/3 π 4π/3 5π/3 2π relative phase (rad)
40 Signal Noise = 2Ω E1Δt N = 2 Number of atoms = N ~ 10 6 Ω E1 ~ 10 mrad Interaction time = Δt ~ 0.1s
41 The Francium Trapping Facility at TRIUMF
42 ISAC I hall at TRIUMF, Francium Trapping Facility
43 High efficiency capture MOT
44 Commissioning of Apparatus: Trapped atoms: ~ 10 5 to 10 6 now 10 7 Efficiency ~ 1% now higher. Trap lifetimes ~ 30s
45 Measurements at TRIUMF
46 Need to understand the atom and the nuclear properties that enter for the calculation: Charge radius. Magnetization radius. Measure the scalar (alpha) and vector (beta) polarizabilities for the Stark induced transition.
47 Isotope Shift Mass Shift Field Shift Reduced mass (easy) Electronic correlations (difficult) Finite size Nucleus Point Nucleus
48 King plot
49 Results (1) 190 (100) GHz amu
50 Nuclear Magnetization
51 Hyperfine Interaction: Interaction of electron with the magnetic moment of nucleus. Hyperfine Anomaly: ε quantifies the effect of the finite size of the nucleus. A S,P [ρ]= hyperfine coefficient hyperfine splitting francium ρ=nuclear magnetization distribution 7P 1/2 7S 1/2 radial distribution πh 9/2 νf 5/2 radius (fm)
52 HF Anomaly N Normalized R HFS (A) g f 5/2 p 3/2 m f 5/2 f 5/2 h 9/2 f 5/2 p 1/2 Green: Nuclear Structure Theory Blue and Red: Measurements Two isomers for 206 g and m i 13/ A
53
54 8S 1/2 F=U F=L Not detected Excitation at 1012 nm Not detected 7P 3/2 7P 1/2 7S 1/2 F=U F=L Detection at 817 nm
55 King plot two-photon vs D1 shifts relative to 213 Fr D1 (10 6 MHz amu) Fr 208 Fr 211 Fr 209 Fr Residuals S 1/2 8S 1/2 (10 6 MHz amu) 0.2 Residuals
56 Comparison of the slope from the King plot Experiment: ± Theory: ± Next step DC Stark Shift for the 7S to 8S transition in Fr. We have the results in Rb
57
58
59 Isotope shifts of 206,207,213 Fr with respect to 209 Fr measured to within a few MHz in two transitions. Changes in the charge radius. 7P 1/2 splitting measured for 206,207,209,213, 221 Fr to a few khz for the Hyperfine anomaly. Changes in the magnetization radius. DC Startk shift observed, but now need to measure it in controlled environment
60
61
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