Spin-orbit interaction at interfaces: from Rashba states to chiral spin textures
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1 Spin-orbit interaction at interfaces: from Rashba states to chiral spin textures Stefan Blügel Peter Grünberg Institut and Institute for Advanced Simulation Spetses Spin-Orbit Coupling in Surface or Interface States 08. June 2015
2 Spin-Orbit Coupling v spin-orbit coupling has fascinating realizations and ramifications in solids Examples: o Rashba Effect o Dresselhaus Effect o Topological & Chern Insulator o Magnetic Anisotropy o Dzyaloshinskii-Moriya Interaction o Chiral magnets and skyrmions o Spin-Orbit Torque o Anomalous & Spin Hall Effect & Edelstein Effect o Quantum & Topological Spin Hall Effect o Spin-Relaxation (Elliot-Yafet, Dyakonov-Perel) June 11, 2015 Folie 2
3 Spin-Orbit Coupling v spintronics spin-orbitronics Examples: o Rashba Effect o Dresselhaus Effect o Topological & Chern Insulator o Magnetic Anisotropy o Dzyaloshinskii-Moriya Interaction o Chiral magnets and skyrmions o Spin-Orbit Torque o Anomalous & Spin Hall Effect & Edelstein Effect o Quantum & Topological Spin Hall Effect o Spin-Relaxation (Elliot-Yafet, Dyakonov-Perel) June 11, 2015 Folie 3
4 Outline v Aim: Space inversion asymmetry + Spin-orbit coupling + Lack of time inversion symmetry = chiral spin textures at metal surfaces à topologically protected spin-structures June 11, 2015 Folie 4
5 Mitglied der Helmholtz Gemeinschaft Thanks! Bernd Zimmermann Vasile Caciuc Nicolae Atodiresei Phivos Mavropoulos Gustav Bihlmayer Juba Bouaziz Samir Lounis Eugene Chulkov Pedro Echenique STM groups Frank Freimuth Yuriy Mokrousov PES groups Ø Matthias Bode Ø Oliver Rader Ø Thomas Michely Ø Carlo Carbone Ø Roland Wiesendanger SOCSIS, Spetses, June Ø Philip Hofmann Bertrand Dupé Stefan Heinze June 11, 2015 Folie 5
6 Tiny tiny SOC brings us to Spetses degenerate states k (r) =a k (r) k (r) =a k (r) e ik r e ik r E(k) ν k June 11, 2015 Folie 6
7 Tiny tiny SOC brings us to Spetses degenerate states Usually: k (r) = a k (r) + b k (r) e ik r a 2 1 k (r) = a k(r) b k(r) e +ik r b 2 1 b 2 : Ellio1- Yafet parameter H SOC = (r) L S E F E(k) n n Δ soc Perturba<on theory: b 2 nk = X 0 h nk (L S) "# 0 n0 k i 2 (E n 0 nk E n0 k) Fermi surface hot- spots k June 11, 2015 Folie 7
8 Fermi surface hot spots for Anisotropy of b 2 (ŝ) bcc W (Z=74) hcp Os (Z=76) details matter! B. Zimmermann et al., PRL 109, (2012) June 11, 2015 Folie 8
9 Tiny tiny SOC brings us to Spetses degenerate states Usually: k (r) = a k (r) + b k (r) e ik r a 2 1 k (r) = a k(r) b k(r) e +ik r b 2 1 b 2 : Ellio1- Yafet parameter Additional fun: Lifting degeneracies by breaking time and space inversion symmetry! June 11, 2015 Folie 9
10 Spin-Orbit Coupling: Space Inversion Symmetry Elemental solids (Cu, Si, Al.) For a given band ν the following two states have the same energy Proof: time reversal space inversion June 11, 2015 Folie 10 q.e.d.
11 Space inversion symmetry broken Time reversal + space inversion symmetry: (GaAs, InSb, interfaces, surfaces,...) Time reversal only!, Effective spin-orbit ( magnetic ) field Ω: Time reversal symmetry: I. Zˇuti ć, J. Fabian, and S. Das Sarma, Rev. Mod. Phys. 76, 323 (2004). June 11, 2015 Folie 11
12 The functional forms of Ω(k): Symmetry Analysis J. Fabian June 11, 2015 Folie 12
13 Axis of spin-rotation Spin Splitting at constant E (Energy) k y <110> <110> <110> <110> k y <001> <001> k x k x Rashba type Inversion Asymmetry by surface, interface, heterostructure Dresselhaus type Inversion Asymmetry in crystal structure June 11, 2015 Folie 13
14 1 st evidence: Au(111) Surface Theory PES Experiment surface states E F bulk states Lashell et al., PRL 77, 3419 (1996) Reinert et al., PRB 63, (2001) June 11, 2015 Folie 14
15 Semi-metal Bi(111): Theory Without Spin-Orbit Interaction With Spin-Orbit Interaction Yu.M. Koroteev, G. Bihlmayer, J.E. Gayone, E.V. Chulkov, S. Blügel, P.M. Echenique, and PH. Hofmann, PRL 93, (2004) see Poster Aguilera June 11, 2015 Folie 15
16 La(0001) and Lu(0001) Surface 11L dhcp La(0001) 12L hcp Lu(0001) O. Krupin et al. New J. Phys. 11, (2009) (GGA), all relaxed with SOC position of surface state at Γ in good agreement with experiment no detectable Rashba spin-orbit splitting for these surface states Z(La)=57; Z(Lu)=71; Z(Au)=79 June 11, 2015 Folie 16
17 La & Lu(0001) surface states: charge densities Lu: SS M point Lu: SS Γ La: SS Γ Bandstructure Lu(0001) Without SOC O. Krupin et al. New J. Phys. 11, (2009) Rashba-Spin-Orbit Splitting around point! (at M-point 0 due to symmetry) M June 11, 2015 Folie 17
18 La & Lu(0001) surface states: charge densities Bandstructure Lu(0001) With SOC O. Krupin et al. New J. Phys. 11, (2009) June 11, 2015 Folie 18
19 Magnetic Surface: Gd(0001) Surface state as for La(0001) or Lu(0001) But: Spin-splitted by exchange field (acts as Zeeman) June 11, 2015 Folie 19
20 Rashba-Effect at magnetic surfaces Surface electrons moving in a E field: 1 H = p 2 + α Rσ ( p E ) 2m H R Dispersion relation: 2 ( ) 2 ( ε k = ± α σ ) ( ) k R k E 2m Magnetic Surfaces: Dispersion relation: Exchange splitting 1 ± IM 2 2 (, ) 2 1 ( ε α ( k = ± ± ) M k IM RM k 2m 2 E) June 11, 2015 Folie 20
21 Gd(0001) Surface State Dispersion Exp. hν=36 ev T=80 K Theory Small Rashba-Spin-Orbit splitting at Γ-point (majority spin) Exp: O. Krupin, S. Gorovikov, J.E. Pietro, K. Döbrich, G. Kaindl, and K. Starke PRB 71, (2005) June 11, 2015 Folie 21
22 O on Gd(0001): Surface States Gd-(S) O Gd-(S) Gd-(S-1) June 11, 2015 Folie 22
23 Electrons at Surfaces E k -k June 11, 2015 Folie 23
24 Where does the SOC come from? Example: Rashba effect E k -k Spin-Orbit Strength (Z) Asymmetry of Ψ Orbital (s,p.d ) June 11, 2015 Folie 24
25 Where does the SOC come from? Example: Rashba effect Spin-Orbit Strength (Z) Atom Asymmetry of Ψ Orbital (s,p.d ) V (r) r 1 2mc 2 r V r L S Muffin-Tin Sphere June 11, 2015 Folie 25
26 Where does the SOC come from? Example: Rashba effect Atom V (r) r 1 2mc 2 r V r L S Rashba splitting (% of full value) Rashba splitting as function of radius of the sphere in which SOC is taken into account for Au(111) Sphere radius [a.u.] sphere radius (a.u.) 0.99 Muffin-Tin Sphere June 11, 2015 Folie 26
27 SOC+Inversion-asymmetry Example: Rashba effect Contribution of Individual layer to Rashba splitting Atom V (r) r 1 2mc 2 r V r L S 0 S-0 S-1 S-2 S-3 S-4 S-5 layer (S = surface) S S-1 S-2 S-3 S-4 S-5 Layer (S=Surface) 0% contribution of individual layer contribution of the idividual layers sphere radius (a.u.) 20% June 11, 2015 Folie 27 Rashba splitting (% of total) Rashba splitting (% of full value) 20 40% Au(111) 60 Rashba splitting as function of radius of the sphere in which SOC is taken into account for Au(111) 60% Au(111) 100
28 Rashba-Hamiltonian Electrons moving in a E field: 2D electron gas (in xy-plane) ψ ( ) ( k, r ) = 1 Ω ei k r ( ) > E(k) = 2 2m k 2 June 11, 2015 Folie 28
29 Mitglied der Helmholtz Gemeinschaft STS : Fe on Cu(111) Ill*tlsYOlsl.BlOsssl B 'S- -60 HI% \8~'17 <~ Distance (A) ' 1. (A) Constant otan( A x , current Aimage Fig. Fe adatomi (B) Solid line: average of three cross section Crommie etal, Science 218 ) onof the Fe adatom. the Cu(111) surface (V= 0.02 volt, I the center of the Fe adatom image in (A). Dashed line: na). Thefapparent height through the adatom is -0.9 A. The concentric rings surrounding the Fe adatomr 1 to the Cross section (the datawas fit only up to 18 A from th are standing waves due to the scattering of surface state electrons with of the adatom). = 1.0 sharp drop in di/dv at the surface state band June 11, 2015 Folie 29 shows the dil/dv spectrum measured with for imaging, the Fe adatoms did not
30 Rashba-Hamiltonian Electrons moving in a E field: ψ 2D electron gas (in xy-plane) 1 ik r ( k, r ) = e ( ) > ( ) Ω E Δ R Momentum k Δk x June 11, 2015 Folie 30
31 Mitglied der Helmholtz Gemeinschaft STS : Fe on Cu(111) Ill*tlsYOlsl.BlOsssl B Where 'S- is the second length scale due to spin orbit interaction -60 HI% \8~'17 <~ ? 0 20 Distance (A) ' 1. (A) Constant otan( A x , current Aimage Fig. Fe adatomi (B) Solid line: average of three cross section Crommie etal, Science 218 ) onof the Fe adatom. the Cu(111) surface (V= 0.02 volt, I the center of the Fe adatom image in (A). Dashed line: na). Thefapparent height through the adatom is -0.9 A. The concentric rings surrounding the Fe adatomr 1 to the Cross section (the datawas fit only up to 18 A from th are standing waves due to the scattering of surface state electrons with of the adatom). = 1.0 sharp drop in di/dv at the surface state band June 11, 2015 Folie 31 shows the dil/dv spectrum measured with for imaging, the Fe adatoms did not
32 Standing waves at defect scattering E E B k k -k k -B Incoming states + reflected states June 11, 2015 Folie 32
33 Standing waves at defect scattering Fermi Surface Au(111) Scattering States E Γ M K E Γ June 11, 2015 Folie 33
34 Semi-metal Bi(110): Theory J.I. Pascual, G. Bihlmayer, Yu.M. Koroteev, H.-P. Rust, G. Ceballos, M. Hansmann, K. Horn, E.V. Chulkov, S. Blügel, P.M. Echenique, and Ph. Hofmann, PRL 93, (2004) June 11, 2015 Folie 34
35 Spin-dependent Interference: Bi(110) STM Scan Fourier TransF. J.I. Pascual, G. Bihlmayer, Yu.M. Koroteev, H.-P. Rust, G. Ceballos, M. Hansmann, K. Horn, E.V. Chulkov, S. Blügel, P.M. Echenique, and Ph. Hofmann, PRL 93, (2004) June 11, 2015 Folie 35
36 Scattering theory for magnetic adatom " Rashba Hamiltonian H = 1 2m * P2 + α R (σ x P y σ y P x ) " Dyson eq.: G = G 0 + G 0 tg 0 Surface " Surface Green function G D G 0 = e iβ G ND " Scattering Amplitude t = 1 ( m * e2iδ 1) e iβ G ND G D t = t 0! t 0! t t LDOS = 1 π ImG M = 1 π ImTr σ G June 11, 2015 Folie 36
37 Application: Adatoms on Au(111) surface LDOS(r) = 1 π Im ( (G G + G G )(t + t ) ) D D ND ND M z (r) = 1 π Im ( (G G G G )(t t ) ) D D ND ND STM M r (r) = 2 π Im ( G (t t )G ) D ND M z (r) 1 ( r k 1 cos(2k 1 r) + k 2 cos(2k 2 r) ) Surface June 11, 2015 Folie 37
38 Application: Adatoms on Au(111) surface LDOS(r) = 1 π Im ( (G G + G G )(t + t ) ) D D ND ND M z (r) = 1 π Im ( (G G G G )(t t ) ) D D ND ND STM M r (r) = 2 π Im ( G (t t )G ) D ND M r (r) 1 ( r k 1 sin(2k 1 r) k 2 sin(2k 2 r) ) Surface June 11, 2015 Folie 38
39 Mitglied der Helmholtz Gemeinschaft Three-dimensional Spin texture E=EF=410 mev Lounis, Bringer, Blügel, PRL108, (2012) June 11, 2015 Folie 39
40 Skyrmionic spin texture E=E F =410 mev high Result at E F Radius~70Å low June 11, 2015 Folie 40
41 Mitglied der Helmholtz Gemeinschaft Skyrmionic spin texture Bogdanov, Hubert, JMMM 195, 182 (1999) Rößler et al. Nature 442, 797 (2006) Mühlbauer et al. Science 323, 929 (2008) high Radius~70Å low June 11, 2015 Folie 41
42 Mitglied der Helmholtz Gemeinschaft Complex Skyrmionic spin texture Bogdanov, Hubert, JMMM 195, 182 (1999) Rößler et al. Nature 442, 797 (2006) Mühlbauer et al. Science 323, 929 (2008) high Radius~70Å low June 11, 2015 Folie 42
43 Asymptotic behavior Distance from the adatom (Å) First nodes: wave length ~ 20 Å cos(2k F R) and λ = 2π = λ F 2k F 2 ~ 40 2 node Phase switch: ~ 60 Å cos(2k so R) λ and λ = so 2 ~ 120 Å 2 Å June 11, 2015 Folie 43
44 Interference of two skyrmionic waves M total = M k1 + M k Distance from the adatom (Å) M k1 k 1 ( cos(2k 1 r), sin(2k 1 r),0) k 1 = k + k so k 2 = k k so M k2 k 2 ( cos(2k 2 R),sin(2k 2 R),0) June 11, 2015 Folie 44
45 Scattering at two adatoms (Heisenberg) A. Fert & P. M. Levy, PRL 44, 1538 (1980). June 11, 2015 Folie 45
46 Rashba scattering at two adatoms Structure inversion asymmetric magnetism (SIA) E B k (Heisenberg) A. Fert & P. M. Levy, PRL 44, 1538 (1980). June 11, 2015 Folie 46
47 Dzyaloshinskii-Moriya Interaction (DMI): Structure inversion asymmetric magnetism (SIA) E B k (Heisenberg + Dzyaloshinskii-Moriya) June 11, 2015 Folie 47
48 Dzyaloshinskii-Moriya Interaction: Structure inversion asymmetric magnetism (SIA) E B k (Heisenberg) (Heisenberg A. Fert & P. M. + Dzyaloshinskii-Moriya) Levy, PRL 44, 1538 (1980). Example: Au(111) D y 12 (R) = ~ 2 apple sin(2kso R) sin(2k F R) m 2 + k so cos(2k so R)SI(2k F R) R 2R J. Bouaziz, M. d. Santos Dias, A. Ziane,, S. Blügel, S. Lounis June 11, 2015 Folie 48
49 Dzyaloshinskii-Moriya Interaction: Structure inversion asymmetric magnetism (SIA) D y k so k so E B k R x (Heisenberg) (Heisenberg A. Fert & P. M. + Dzyaloshinskii-Moriya) Levy, PRL 44, 1538 (1980). Example: Au(111) D y ~ 2 h sin(2kf R) sin(2k so R) ij = m 2 R 2R i + k so cos(2k so R) SI(2k F R) J. Bouaziz, M. d. Santos Dias, A. Ziane,, S. Blügel, S. Lounis June 11, 2015 Folie 49
50 DMI: Long range interaction DMI due to Rashba effect i R ij j Au(111) 1 1 Au(111) Reinert et al., PRB 63, (2001) Interaction D y ij [mev] R ij [Å] June 11, 2015 Folie 50
51 DMI: Long range interaction DMI due to Rashba effect 1 1 Au(111) Interaction D y ij [mev] R ij [Å] Reinert et al., PRB 63, (2001) D y ij = ~ 2 m 2 R h sin(2kf R) sin(2k so R) 2R June 11, 2015 Folie 51 Bouaziz, Blügel, Lounis i + k so cos(2k so R) SI(2k F R)
52 Real Fermi surface bcc W (Z=74) SOCSIS, Bernd Zimmermann Spetses, June June 11, 2015 Folie 52
53 Exchange and DMI in Pd/Fe/Ir(111) Top view of Fe Fe J 12 = 16.4 mev Ir Pd D 12 = -1.1 mev Bauer, Kiselev, Crum, Schweflinghaus, Bouhassoune, Bouaziz, Lounis, Blügel June 11, 2015 Folie 53
54 Exchange and DMI in 2Pd/Fe/Ir(111) Top view of Fe Fe Pd J 12 = 12.7 mev Ir D 12 = -1.4meV Bauer, Kiselev, Crum, Schweflinghaus, Bouhassoune, Bouaziz, Lounis, Blügel June 11, 2015 Folie 54
55 Dzyaloshinskii-Moriya Interaction o Well-known interaction in many TM oxides, chalcogenides.. Bulk inversion asymmetric (BIA) systems (non-centrosymmetric crystals): e.g. α-fe 2 O 3, MnCO 3, CrF 3. Antiferromagnets show weak ferromagnetism Anisotropic Superexchange Interaction + SOC o Metals : most metals bcc, fcc, hcp.. exceptions: B20 compounds, Spin glasses A. Fert & P. M. Levy, PRL 44, 1538 (1980). June 11, 2015 Folie 55
56 Bulk inversion asymmetric magnets E(c) FM/AFM L> R> c Dzyaloshinskii-Moriya Interaction June 11, 2015 Folie 56
57 Spin textures at surfaces skyrmions magnetism spin-orbit coupling inversion asymmetry chiral spin spirals Dzyaloshinskii-Moriya interaction Nature 465, 901 (2010) Nat. Phys. 7, 713 (2011) chiral domain walls magnon dispersion Nature 447, 190 (2007) PRL 88, (2002) PRB 78, (2008) PRL 102, (2009) PRL 104, (2010) June 11, 2015 Folie 57
58 Spin-Orbit Interaction + Structure Inversion Asymmetry Break of inversion symmetry P(z) P(-z) Magn. Film Substrate with large SOC Dzyaloshinskii-Moriya Interaction But how large?? Which direction (sign)?? What about the metallic systems?? June 11, 2015 Folie 58
59 Skyrmions for Spintronics Chiral magnetism in thin films, but not too thin (min 3 layers) Try find small but not too small skyrmions 3-5 nm Above room temperature and zero magnetic field Fit to the field of spintronics: injection, transport, detection, manipulation at reasonable fields and currents Metallic magnetism Albert Fert, Vincent Cross and João Sampaio, Nature Nanotechnology 8, 152 (2013) June 11, 2015 Folie 59
60 Role of Dzyaloshinskii-Moriya Interaction in Dimensions Micromagnetic energy functional: Z E(m) = A rm 2 + D (rm m)+m K m B m ê z dr 2 R 2 Exchange Dzyaloshinskii-M Anisotropy Ext. Field Stretching transformation: m(r)! m (r) =m( r) 2D: Skyrmion Z apple A E( )= 2 rm 2 + D (rm m)+m K m B m ê 2 z dr 2 R Z 2 E( )= A rm 2 + D (rm m)+ 2 m K m 2 B m ê z dr 2 SOCSIS, R 2 Spetses, June June 11, 2015 Folie 60
61 Role of Dzyaloshinskii-Moriya Interaction in Dimensions Micromagnetic energy functional: Z E(m) = A rm 2 + D (rm m)+m K m B m ê z dr 2 R 2 Exchange Dzyaloshinskii-M Anisotropy Ext. Field Stretching transformation: m(r)! m (r) =m( r) 1D: Domain Wall Z apple A E( )= rm 2 + D (rm m)+ m K m B m ê z dr R Z E( )= A rm 2 + D (rm m)+ 2 m K m 2 B m ê z dr 2 SOCSIS, R 2 Spetses, June June 11, 2015 Folie 61
62 Continuum theory of chiral magnetic skyrmions Theoretical prediction: T. Skyrme: Proc. Roy. Soc. A 260, 127 (1961) A.N. Bogdanov & D. A.Yablonski: Sov. Phys. JETP 68, 101 (1989). A.N. Bogdanov, A. Hubert: JMMM 138, 255 (1994) U. Rössler, A.N. Bogdanov, C. Pfleiderer, Nature 442, 797 (2006). Micromagnetic energy functional: Z E(m) = A rm 2 + D (rm m)+m K m B m ê z dr 2 R 2 Exchange Dzyaloshinskii-M Anisotropy Ext. Field min E{m} of continuous vector field m with unit sphere S 2 = {m 2 R 3 : m =1} è Topological concepts Smooth Mapping R 2! S 2 June 11, 2015 Folie 62
63 Conclusion Ø Many things are unknown and ready to discover Ø E.g. Manipulation and control of topological solitons by external fields Ø Topological, anomalous and thermal Hall effects in static skyrmion lattices Ø Spin orbit torque and damping in chiral magnets Ø Large Skyrmions we can describe in Berry phase physics and materials parameters for micromagnetic models Ø Small skyrmions we may treat completely from abinitio Ø Medium scale skyrmions not-adiabatic but too large of DFT. June 11, 2015 Folie 63
64 Continuum theory of chiral magnetic skyrmions E(m) = Z Mathematical analysis predicts: R 2 A rm 2 + D (rm m)+m K m B m ê z dr 2 Ø Dzyaloshinskii-Moriya Interaction (DMI) à new valley in topologically non-trivial sector of energy landscape Ø Sectors are separated by an energy barrier (topological protection) Ø Theorem: For D 0, for each (D, A) there is a B-field, B 0.8 D 2 /A, at which an isolated chiral skyrmions stabilizes Ø Diameter: R S A/D Ø Critical T : T c D 2 /A Rößler, Leonov, and Bogdanov, J. Phys.: Conf. Series 303, (2011) Melcher Proc. R. Soc. A 470, 0394 (2014) June 11, 2015 Folie 64
65 Thanks! June 11, 2015 Folie 65
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