Aerosol submodel MADE: New developments
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1 Slide 1 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 Aerosol submodel MADE: New developments Christopher Kaiser, Johannes Hendricks, Mattia Righi Deutsches Zentrum für Luft- und Raumfahrt (DLR) Institut für Physik der Atmosphäre, Oberpfaffenhofen, Germany
2 Slide 2 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 Motivation (Lauer et al., ACP, 2007; Righi et al., EST, 2011) Radiative forcing due to ship emissions - Order of magnitude: 2 several -100 mw/m (?) - large uncertainty - dominated by indirect aerosol effect pubs.acs.org
3 Slide 3 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 Motivation (Lauer et al., ACP, 2007; Righi et al., EST, 2011) Radiative forcing due to ship emissions - Order of magnitude: 2 several -100 mw/m (?) - large uncertainty - dominated by indirect aerosol effect New MADE feature Consideration of coarse particle interactions more realistic description of the atmospheric aerosol influence on cloud condensation nuclei (CCN) concentration? pubs.acs.org
4 Slide 4 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 The MESSy aerosol submodel MADE (Binkowski and Shankar, JGR, 1995; Ackermann et al., AE, 1998; Lauer et al., ACP, 2005) Calculation of number and mass concentrations
5 Slide 5 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 The MESSy aerosol submodel MADE-in (Aquila et al., 2011) Calculation of number and mass concentrations
6 Slide 6 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 The MESSy aerosol submodel MADE3 (Kaiser et al., in preparation, 2013) Calculation of number and mass concentrations
7 Slide 7 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 The MESSy aerosol submodel MADE3 Processes 1. Chemical equilibration (Metzger et al., JGR, 2002; Metzger et al., ACP, 2006) NH3 NH4+ _ HNO3 NO3 _ HCl Cl SOA prec. POM H2O(a) Coarse particles: flux limit (similar to Pringle et al., GMD, 2010)
8 Slide 8 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 The MESSy aerosol submodel MADE3 Processes 1. Chemical equilibration 2. Condensation of H2SO4
9 Slide 9 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 The MESSy aerosol submodel MADE3 Processes 1. Chemical equilibration 2. Condensation of H2SO4 3. Nucleation from H2SO4/H2O (Vehkamäki et al., JGR, 2002)
10 Slide 10 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 The MESSy aerosol submodel MADE3 Processes 1. Chemical equilibration 2. Condensation of H2SO4 3. Nucleation from H2SO4/H2O 4. Coagulation
11 Slide 11 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 MADE3 vs. MADE Box model: emissions in marine background
12 Slide 12 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 MADE3 vs. PartMC-MOSAIC (Riemer et al., JGR, 2009; Zaveri et al., JGR, 2008) MADE3 PartMC-MOSAIC Aerosol representation modal, deterministic particle-resolved, stochastic Aerosol chemistry equilibrium, flux limited dynamical Target application 3D, global, longterm 0/1D, local, episodes
13 Slide 13 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 MADE3 vs. PartMC-MOSAIC Box model: emissions in marine background
14 Slide 14 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 MADE3 vs. PartMC-MOSAIC Box model: emissions in marine background
15 Slide 15 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 MADE3 vs. PartMC-MOSAIC Box model: emissions in marine background
16 Slide 16 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 MADE in MESSy2 3D: reference run MESSy2 MESSy1
17 Slide 17 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 MADE in MESSy2 3D: reference run MESSy2 MESSy1
18 Slide 18 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 To Do - Understand/Reduce MADE-observation discrepancies in MESSy2 - Implement MADE3 in MESSy2 (emissions partitioning, inclusion of HCl in simplified chemistry) - Gather observational data for evaluation (focus: marine boundary layer, coarse particles) - Test/Implement interactive aerosol couplings (radiation, clouds) Comments welcome!
19 Slide 19 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 Thanks to: Valentina Aquila Nicole Riemer Patrick Jöckel Robert Sausen Axel Lauer Holger Tost Swen Metzger Rahul Zaveri and more colleagues at DLR
20 Slide 20 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 Additional material
21 Slide 21 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 Definition: Schwebteilchen in einem Gas(gemisch) Wichtige Prozesse: - Emission - Nukleation - Koagulation - Kondensation/ Verdampfung - Sedimentation - Auswaschen Brasseur, Prinn, Pszenny: Atmospheric Chemistry in a Changing World. Springer, 2003 Aerosole
22 Slide 22 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 Aerosol chemistry: Kinetics 1. Gas diffusion to the particle 2. Transport through the interface 3. (Solvation in the liquid phase) 4. Diffusion within the particle 5. Reaction within the particle
23 Slide 23 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 Aerosolrepräsentation in Klimamodellen: Der modale Ansatz Annahmen: - Lognormalverteilung für die Teilchenzahldichte in jeder Mode Nt dn = exp d ln D 2π ln σ ln D ln D g 2 ln σ 2 2 Dg: Median-Durchmesser (geometrischer Mittelwert) Nt : Teilchenzahldichte σ : Geometrische Standardabweichung - Gleiche Zusammensetzung für alle Teilchen einer Mode - Konstante Standardabweichung
24 Slide 24 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 Klimawirkung des globalen Schiffsverkehrs: Aerosol-Effekte Forster et al., IPCC AR4 (WG1), 2007
25 Slide 25 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 Stand der Forschung: Klimawirkung des globalen Schiffsverkehrs Aerosol, direkt Aerosol, indirekt Eyring et al., Atmos. Environ., 2010 Treibhausgase
26 Slide 26 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 Stand der Forschung: Klimawirkung des globalen Schiffsverkehrs Standardkraftstoff Righi et al., Environ. Sci. Tech., 2011 schwefelarme Kraftstoffe
27 Slide 27 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 Strahlungsantrieb gesamt Forster et al., IPCC AR4 (WG1), 2007
28 Slide 28 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 Stand der Forschung: Klimawirkung des globalen Schiffsverkehrs Fuglestvedt et al., EST, 2009
29 Slide 29 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 Aerosolrepräsentation in EMAC (am DLR): Prozesse in MADE(-IN) Lauer et al., ACP, 2005
30 Slide 30 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 Aerosolrepräsentation in EMAC (am DLR): Integration von MADE(-IN) Axel Lauer
31 Slide 31 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 MADE3 vs. MADE Box model: emissions in marine background
32 Slide 32 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 MADE3 vs. PartMC-MOSAIC Box model: emissions in marine background
33 Slide 33 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 MADE3 in MESSy2 3D: reference run
34 Slide 34 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 MADE3 in MESSy2 3D: reference run
35 Slide 35 > MADE: New developments > C. Kaiser et al. ck_made_new_devel_ odp > June 14, 2013 Erste Ergebnisse: Boxmodelltests von MADE-IN 4 Testkonfigurationen: - urban - Hintergrund kontinental - marine Grenzschicht - freie Troposphäre
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