List of publications. 56. X. Lin, N. Nilius*, J. Phys. Chem. C 112 (2008) Self assembly of MgPc molecules on FeO thin films

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1 List of publications N. Nilius*, V. Ganduglia-Pirovano, V. Brazdova, M. Kulawik, J. Sauer, H-J. Freund, Phys. Rev. Lett. 100 (2008) Counting electrons transferred through a thin alumina film into Au chains 48. H. M. Benia, P. Myrach, N. Nilius*, New J. Phys. 10 (2008) Photon emission spectroscopy of thin MgO films with the STM: From a tip-mediated to an intrinsic emission characteristic 49. V. Simic-Milosevic, N. Nilius*, H.-P. Rust, H.-J. Freund, Phys. Rev. B 77 (2008) Band gap modulations in non-stoichiometric V 2 O 3 thin films probed by scanning tunnelling spectroscopy 50. M. Baron, D. Stacchiola, S. Ulrich, N. Nilius, S. Shaikhutdinov, H.-J. Freund, U. Martinez, L.Giordano, G. Pacchioni, Chem. Phys. C. 112 (2008) The role of the atomic structure of thin SiO 2 films on adsorption of Au and Pd atoms. 51. S. Ulrich, N. Nilius*, H.-J. Freund, L. Giordano, G. Pacchioni, ChemPhysChem. 9 (2008) Evidence for a size-selective adsorption mechanism on oxide surfaces: Pd and Au atoms on SiO 2 /Mo(112) 52. V. Simic-Milosevic, M. Heyde, N. Nilius, T. König, H.-P. Rust, M. Sterrer, T. Risse, H.-J. Freund, L. Giordano, G. Pacchioni, J. Amer. Chem. Soc. 130 (2008) Au Dimers on Thin MgO(001) Films: Flat and Charged or Upright and Neutral? 53. S. Benedetti*, P. Torelli, S. Valeri, H. M. Benia, N. Nilius*, G. Renaud, Phys. Rev. B 78 (2008) Relaxation via dislocation formation of thin MgO films on Mo(001) 54. L. Giordano, G. Pacchioni*, J. Goniakowski, N. Nilius*, E. D. L. Rienks, H.-J. Freund, Phys. Rev. Lett. 101 (2008) Charging of Metal Adatoms on Ultrathin Oxide Films: Au and Pd on FeO/Pt(111) 55. N. Nilius*, V. Simic-Milosevic, J. Phys. Chem. C 112 (2008) Adsorption of Single Magnesium Phthalocyanine Molecules on V 2 O 3 Thin Films 56. X. Lin, N. Nilius*, J. Phys. Chem. C 112 (2008) Self assembly of MgPc molecules on FeO thin films 57. Y. Romanyshyn, S. Guimond, H. Kuhlenbeck, S. Kaya, R.P. Blum, H. Niehus, S. Shaikhutdinov, V. Simic Milosevic, N. Nilius, H.-J. Freund, M. V. Ganduglia-Pirovano, R. Fortrie, J. Döbler, J. Sauer, Top. Catal. 50 (2008) 106 Selectivity in Methanol Oxidation as Studied on Model Systems Involving Vanadium Oxides. 58. T. Risse, S. Shaikhutdinov, N. Nilius, M. Sterrer, H.-J. Freund, Acc. Chem. Res. 41 (2008) 949 Gold Supported on Thin Oxide Films: From Single Atoms to Nanoparticles 59. V. Simic-Milosevic, M. Heyde, X. Lin, T. König, H.-P. Rust, M. Sterrer, T. Risse, N. Nilius*, H-J. Freund, L. Giordano, G. Pacchioni*, Phys. Rev. B 78 (2008) Charge-induced formation of linear Au clusters on thin MgO films

2 S. Ulrich, N. Nilius*, H.-J. Freund, U. Martinez, L. Giordano, G. Pacchioni, Phys. Rev. Lett. 102 (2009) Tailoring the adsorption properties of inert oxide film by inserting controlled anchor sites 61. N. Nilius*, V. Ganduglia-Pirovano*, V. Brazdova, V. Simic-Milosevic, J. Sauer, H.-J. Freund, New J. Phys. 11 (2009) Nucleation of gold atoms on V 2 O 3 thin films 62. S. Ulrich, N. Nilius*, H.-J. Freund, U. Martinez, L. Giordano, G. Pacchioni, Surf. Sci. 603 (2009) Realization of an atomic sieve: Silica on Mo(112) 63. E. D. L. Rienks, N. Nilius*, H.-J. Freund, L. Giordano, G. Pacchioni, J. Goniakowski, Phys. Rev. B 79, (2009). Zero-bias conductance anomaly of a FeO-bound Au atom triggered by CO adsorption 64. X. Lin, N. Nilius*, H.-J. Freund, M. Walter, P. Frondelius, K. Honkala, H. Häkkinen, Phys. Rev. Lett. 102, (2009). Quantum well states in two-dimensional gold clusters on MgO thin films 65. P. Myrach, N. Nilius*, H.-J. Freund, J. Phys. Chem. C 113 (2009) Alkali earth nano-particles on MgO thin film: Growth and optical properties 66. N. Nilius, Surf. Sci. Rep. 64 (2009) Properties of oxide thin films and their adsorption behavior studied by scanning tunneling microscopy and conductance spectroscopy 67. U. Martinez, J.-F. Jerratsch, N. Nilius,* L. Giordano, G. Pacchioni, H.-J. Freund, Phys. Rev. Lett. 103, (2009) Modifying the adsorption properties of silica thin films via work function control 68. J.-F. Jerratsch, N. Nilius,* H.-J. Freund, U. Martinez, L. Giordano, G. Pacchioni, Phys. Rev. B 80, (2009) Lithium incorporation into a silica-mo(112) thin film H. M. Benia, P. Myrach, N. Nilius*, H.-J. Freund, Surf. Sci. 604 (2010) 435. Structural and electronic characterization of the MgO/Mo(001) interface using STM 70. H.-J. Freund, N. Nilius, T. Risse, S. Shaikhutdinov, M. Sterrer, Jahresbericht der Max-Planck- Gesellschaft 2009 Ultradünne Oxidschichten auf Metallsubstraten: eine interessante Materialkombination 71. N. Nilius*, V. Ganduglia-Pirovano, V. Brazdova, M. Kulawik, J. Sauer, H-J. Freund, Phys. Rev. B 81 (2010) Electronic properties and charge state of gold monomers and chains adsorbed on alumina thin films on NiAl(110) 72. J.-F. Jerratsch, N. Nilius,* D. Topwal, U. Martinez, G. Pacchioni, H.-J. Freund, ACS-Nano 4 (2010) 863 Stabilizing Monomeric Iron Species in a Porous Silica/Mo(112) Film 73. B. Yang, X. Lin, H. J. Gao, N. Nilius,* H.-J. Freund, J. Chem. Phys. C 114 (2010) 8997

3 CO Adsorption on thin MgO films and single Au adatoms: An STM study 74. Xiao Lin, Niklas Nilius,* Martin Sterrer, Pekka Koskinen, Hannu Häkkinen, Hans-Joachim Freund, Phys. Rev. B 81 (2010) Characterizing the periphery atoms of Au islands on MgO thin films 75. H. M. Benia, P. Myrach, A. Gonchar, T. Risse, N. Nilius,* H.-J. Freund, Phys. Rev. B 81 (2010) (R). Electron trapping in dislocation lines of an MgO/Mo(001) film 76. X. Lin, B. Yang, H.-M. Benia, P. Myrach, M. Yulikov, A. Aumer, M. A. Brown, M. Sterrer, O. Bondarchuk, E. Kieseritzky, J. Rocker, T. Risse, H-J. Gao, N. Nilius,* H-J. Freund, J. Am. Chem. Soc. 132 (2010) Charge-mediated adsorption behavior of CO on MgO-supported Au clusters 77. P. Myrach, N. Nilius,* S. V. Levchenko,* A. Gonchar, T. Risse, K.-P. Dinse, L. A. Boatner, W. Frandsen, R. Horn, H.-J. Freund, R. Schlögl, M. Scheffler, ChemCatChem 2 (2010) 854. Li-doped MgO: Temperature dependent morphology, magnetic and optical properties H.-J. Freund, N. Nilius, T. Risse, S. Schauermann, T. Schmidt, ChemPhysChem 12 (2011) 79. New Measurement Techniques in Surface Science 79. Philipp Myrach, Niklas Nilius,* Hans-Joachim Freund, Phys. Rev. B 83 (2011) Photon mapping of individual Ag particles on MgO/Mo( N. Nilius T. Risse, S. Schauermann, S. Shaikhutdinov, M. Sterrer, H.-J. Freund, Top. Catal. 54 (2011) 4. Model Studies in Catalysis 81. X. Shao, P. Myrach, N. Nilius,* H.-J. Freund, Umberto Martinez, Stefano Prada, Livia Giordano, Gianfranco Pacchioni,* Phys. Rev. B 83 (2011) Strain-induced formation of thin mixed-oxide films 82. X. Shao, P. Myrach, N. Nilius,* H.-J. Freund, J. Phys. Chem. C 115 (2011) Growth and Morphology of Calcium-Oxide Films grown on Mo(001): An STM study 83. Jan-Frederick Jerratsch, Xiang Shao, Niklas Nilius,* Hans-Joachim Freund, Cristina Popa, M. Veronica Ganduglia-Pirovano, Asbjörn M. Burow, Joachim Sauer,* Phys. Rev. Lett. 106 (2011) Electron localization in defective ceria films: An STM and DFT study 84. M. A. Brown, Y. Fujimori, F. Ringleb, X. Shao, F. Stavale, N. Nilius, M. Sterrer, H.-J. Freund, J. Amer. Chem. Soc. 133 (2011) Oxidation of Au by surface OH Nucleation and electronic structure of gold on hydroxylated MgO(001) 85. Bing Yang, Xiao Lin, Niklas Nilius,* Hans-Joachim Freund, J. Phys. Chem. C 115 (2011) 3404 Role of the V 2 O 3 (0001) defect structure on the adsorption characteristics of Au adatoms 86. S. Benedetti, P. Myrach, S. Valeri, N. Nilius,* H.-J. Freund, Phys. Rev. B 83 (2011) Growth and Morphology of Metal Clusters on MgO/Mo(001): A comparative STM and diffraction study 87. S. Benedetti, N. Nilius,* I. Valenti, P. Myrach, S. Valeri, H.-J. Freund, J. Phys. Chem. C 115 (2011) 3684.

4 Spontaneous oxidation of Mg adatoms at defect sites in the MgO surface 88. Y. Pan, S. Benedetti, N. Nilius,* H.-J. Freund, Phys. Rev. B 84 (2011) Tailoring the electronic structure of a metal by a monolayer oxide film: MgO on Au(111) 89. X. Shao, S. Prada, L. Giordano, G. Pacchioni, N. Nilius,* H.-J. Freund, Angew. Chem. Int. Ed. 50 (2011) Tailoring the Shape of Metal Ad-particles by Doping the Oxide Support 90. S. Benedetti,* N. Nilius,* P. Torelli, G. Renaud, H.-J. Freund, S. Valeri, J. Phys. Chem. C 115 (2011) Competition between Polar and Nonpolar Growth of MgO Thin Films on Au(111) 91. X. Shao, J.-F. Jerratsch, N. Nilius,* H.-J. Freund, Phys. Chem. Chem. Phys. 13 (2011) Probing the f states of Ceria by tunneling spectroscopy N. Nilius, S. M. Kozlov, J.-F. Jerratsch, M. Baron, X. Shao, S. Shaikhutdinov, H.-J. Freund, F. Viñes, K. M. Neyman, ACS Nano 6 (2012) Polar step edges in a CeO 2 (111) surface 93. Xiang Shao, Niklas Nilius,* Hans-Joachim Freund, J. Am. Chem. Soc. 134 (2012) Li/Mo co-doping of CaO films: A means to tailor the equilibrium shape of Au deposits 94. F. Stavale. Niklas Nilius,* Hans-Joachim Freund, New J. Phys. 14 (2012) Cathodoluminescence spectroscopy of near-surface centres in Cr doped MgO(001) thin films by Scanning Tunnelling Microscopy 95. Yi Pan, Stefania Benedetti, Sergio Valeri, Claudine Noguera, Livia Giordano, Jacek Goniakowski,* Niklas Nilius*, J. Phys. Chem. C 116 (2012) Compensating edge polarity: A means to alter the growth orientation of MgO nanostructures on Au(111) 96. Bing Yang, Xiao Lin, Yi Pan, Niklas Nilius,* Hans-Joachim Freund, Catherine Hulot, Anne Giraud, Siegfried Blechert, Sergio Tosoni, Joachim Sauer, J. Am. Chem. Soc. 134 (2012) Stabilizing gold adatoms by thiophenyl derivates: A possible route towards metal redispersion 97. Xiang Shao, Niklas Nilius, Hans-Joachim Freund, Phys. Rev. B 85 (2012) Crossover from 2D to 3D Au particle-shapes on CaO films of different thickness 98. S. M. Kozlov, F. Viñes, N. Nilius, S. Shaikhutdinov, K. M. Neyman, J. Phys. Chem. Lett. 2012, 3, Absolute Surface Step Energies: Accurate Theoretical Methods Applied to Ceria Nanoislands 99. Yi Pan, Bing Yang, Catherine Hulot, Siegfried Blechert, Niklas Nilius,* Hans-Joachim Freund, Phys. Chem. Chem. Phys. 31 (2012) Role of lattice-gas atoms on the adsorption behaviour of thioether molecules 100. F. Stavale, X. Shao, N. Nilius,* H.-J. Freund, S. Prada, L. Giordano,* G. Pacchioni, J. Am. Chem. Soc. 134 (2012) Donor Characteristics of Transition-Metal-Doped Oxides: Cr-Doped MgO versus Mo-Doped CaO

5 101. N. Nilius, S. Shaikhutdinov, M. Sterrer, D. Menzel, H.-J. Freund, Chemical Energy Storage, R. Schlögl (Ed.), De Gruyter Verlag 2012 Model Systems in Catalysis for Energy Economy 102. Fernando Stavale, Leandro Pascua, Niklas Nilius,* Hans-Joachim Freund, Phys. Rev. B 86 (2012) From embedded nano-islands to thin films: Topographic and optical properties of europium-oxide on MgO(001) films 103. Fernando Stavale, Niklas Nilius, Hans-Joachim Freund, Appl. Phys. Lett. 101 (2012) Probing the luminescence of single Eu 2 O 3 nanoislands on MgO(001) with Scanning Tunneling Microscopy 104. Xiang Shao, Yi Cui, Wolf-Dieter Schneider, Niklas Nilius,* Hans-Joachim Freund, J. Phys. Chem. C 116 (2012) Two-dimensional lithium islands grown on CaO(001) thin films 105. L. Lichtenstein, M. Heyde, S. Ulrich, N. Nilius*, H.-J. Freund, J. Phys.: Condens. Matter 24 (2012) Probing the properties of metal-oxide interfaces: Silica films on Mo and Ru supports 106. S. Benedetti, F. Stavale, J. Goniakowski, N. Nilius*, Adv. Funct. Materials (in press) Self-organization effects of metal nano-particles on the MgO/Mo(001) coincidence lattice Niklas Nilius,* Stefania Benedetti, Yi Pan, Philipp Myrach, Claudine Nogera, Jacek Goniakowski*, Phys. Rev. B (in press) Probing polar properties of (111)-type MgO islands at the local scale Fernando Stavale, Niklas Nilius,* Hans-Joachim Freund, Surf. Sci. (in press) Lithium-molybdate nanostructures grown on the Mo(001) surface 109. S. Schauermann, N. Nilius, S. Shaikhutdinov, H.-J. Freund, Acc. Chem. Res (in press) Nanoparticles for Heterogeneous Catalysis: New Mechanistic Insights (* corresponding author)