ASSESSMENT OF THE GEISA AND GEISA/IASI SPECTROSCOPIC DATA QUALITY: trough comparisons with other public database archives
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1 ASSESSMENT OF THE GEISA AND GEISA/IASI SPECTROSCOPIC DATA QUALITY: trough comparisons with other public database archives N. Jacquinet-Husson, N.A. Scott, A. Chédin, R. Armante Laboratoire de Météorologie Dynamique Atmospheric Radiation Analysis Group Ecole Polytechnique 91128, Palaiseau, France
2 OUTLINE I) II) III) IV) V) DATABASES OVERVIEW DATABASE FORMATS UPDATING SPECTROSCOPIC PARAMETERS: examples of issues 1) Updating of H2O in GEISA (and GEISA/IASI-03) 2) Differences between GEISA (GEISA/IASI-03) and HITRAN04 3) Differences between GEISA(GEISA/IASI-03) and MIPAS-03 EVALUATION OF THE IMPACT OF SPECTROSCOPIC ARCHIVE DIFFERENCES ON RADIATIVE TRANSFER SIMULATIONS CONCLUDING COMMENTS
3 Data bases involved in comparisons GEISA Jacquinet-Husson et al. Proc. of the 13th International TOVS Study Conference, Sainte-Adèle, Canada, 28 Oct-4 Nov and GEISA/IASI-03 HITRAN-04 Jacquinet-Husson et al. JQSRT 95 (2005) Rothman et al. JQSRT 96 (2005) MIPAS Dedicated Spectroscopic Database Flaud et al. Atm. And Ocean Optics, 16 (2003) Evaluation of the differences in contents and subsequent radiative transfer modelling impacts
4 DATABASES OVERVIEW
5 The GEISA-2003 system Gestion et Etude des Informations Spectroscopiques Atmosphériques Management and Study of Atmospheric Spectroscopic Information Three SUB-DATABASES Line transition parameters database 42 molecules (96 isotopic species) 1,668,371 entries between 0 and 35,877 cm-1 Absorption cross-sections database IR: 32 molecular species (mainly CFC s) UV/Visible : 11 molecular species Aerosol data archive and softwares ASSOCIATED MANAGEMENT SOFTWARES (For each sub-database)
6 SUMMARIZED CONTENTS OF HITRAN-04 AND GEISA-03 INDIVIDUAL LINE LISTS Molecule H2O CO2 O3 N2O CO CH4 O2 NO SO2 NO2 NH3 PH3 HNO3 OH HF HCl HBr HI ClO OCS H2CO O NO+ GEISA-03 # lines HITRAN specific HITRAN specific HITRAN-04 # lines Molecule C2H6 CH3D C2H2 C2H4 GeH4 HCN C3H8 C2N2 C4H2 HC3N HOCl N2 CH3Cl H2O2 H2S HCOOH COF2 SF6 C3H4 HO2 ClONO2 HOBr CH3OH GEISA-03 # lines HITRAN-04 #l ines isotope of CH GEISA specific GEISA specific 2577 GEISA specific 1405 GEISA specific 2027 GEISA specific Supl GEISA specific Supl. HITRAN specific 4358 HITRAN specific 19899
7 GEISA/IASI-03 database general context GEISA/IASI-03 database: extraction (spectral range cm-1) and partial update of GEISA-03 Spectroscopic database Maintained and developed with the purpose of assessing the IASI measurements capabilities, within the ISSWG, in the frame of the CNES/EUMETSAT European Polar System (EPS) preparation, by simulating high resolution radiances and/or using experimental data. IASI mainly designed for operational meteorological soundings with a very high level of accuracy. Measurement technique based on passive IR remote sensing using an accurately calibrated Fourier Transform Spectrometer operating in the µm spectral range Continuous update Associated interest for AIRS IASI : Infrared Atmospheric Sounding Interferometer AIRS : Advanced InfraRed Sounder ISSWG : IASI Sounding Science Working Group CNES : Centre National d Etude Spatiales, France EUMETSAT : EUropean organization for the exploitation of METeorological SATellites
8 MIPAS Dedicated Spectroscopic Database MIPAS (Michelson Interferometer for Passive Atmospheric Sounding) experiment operating on board the ENVISAT satellite since March 2002 Recording emission limb sounding spectra at cm-1 (unapodized) in the spectral range cm-1 Starting from HITRAN-96 and GEISA-97, and updated in 2001 and 2003 with specific spectroscopic studies or from spectroscopic studies prior to their publications 32 molecules retained from the HITRAN list (O, NO+, HOBr, C2H4, CH3OH, H2CO, CH3OH discarded) Molecular line parameters updated for: H2O, CO2, O3,N2O, CH4,NO2,HNO3,HOCl,COF2 Validation through ATMOS and MIPAS recorded spectra
9 DATABASE FORMATS
10 GEISA-03 Line Transitions Records A-J fields (A) (B) (C) (D) (E) (F) (G) (I) (J) Mainly specific of GEISA management software Wavenumber (cm-1) of the line associated with the vibro-rotational transition. Intensity of the line (cm molecule-1 at 296K). Lorentzian collision halfwidth (cm-1 atm-1 at 296K). Energy of the lower transition level (cm -1). Transition quantum identifications for the lower and upper levels of the transition Temperature dependence coefficient n of the halfwidth Identification code for isotope. Identification code for molecule. Internal GEISA code for data identification. K-Q fields in the GEISA format (K) (L) (M) (N) (O) (P) (Q) Mainly HITRAN-01 format inter-compatibility related Molecule number as in HITRAN Isotope number as in HITRAN Transition probability (in debye2) Self broadening pressure halfwidth (HWHM) (cm -1atm-1) at 296K (for water) Air pressure shift of the line transition (cm -1atm-1) at 296K Accuracy indices for wavenumber, intensity and halfwidth Indices for lookup of references for wavenumber, intensity and halfwidth
11 GEISA-03 Line Transitions Records (following) R-U fields in the GEISA/IASI format Mainly IASI specific (R) Temperature dependence coefficient n of the air pressure shift (A ) Estimated accuracy (cm-1) on the line position (B ) Estimated accuracy on the intensity of the line in (cm -1/(molecule.cm-2) (C ) Estimated accuracy on the air collision halfwidth (HWHM) (cm-1atm-1) (F ) Estimated accuracy on the temperature dependence coefficient n of the air broadening HW (O ) Estimated accuracy on the air pressure shift of the line transition (R ) Estimated accuracy on the temperature dependence coefficient n of the air pressure shift Water specific (N ) (S) (S ) (T) (T ) (U) (U ) Estimated accuracy on the self broadened (HWHM) (cm Temperature dependence coefficient n of the self broadening halfwidth Estimated accuracy on the temperature dependence coefficient n of the self broadening HW Self pressure shift of the line transition (cm Estimated accuracy on the self pressure shift of the line transition (cm Temperature dependence coefficient n of the self pressure shift Estimated accuracy on the temperature dependence coefficient n of the self pressure shift ) 209 Characters record
12 HITRAN-04 Line Transition Records 160-character records of the HITRAN-04 line-by-line section M I ν S R A air self E air air V V Q' Q Ierr Iref * g' g Molecule number Isotopologue number Vacuum wavenumber cm-1 Intensity cm-1/(molecule cm-2) at 296K Weighted square of the transition moment Debye 2 Einstein A-coefficient s-1 Air-broadened half-width HWHM at 296K (cm-1atm-1) Self-broadened half-width HWHM at 296K (cm-1atm-1) Lower-state energy cm-1 Temperature-dependence exponent for air Air pressure-induced line shift cm-1atm-1 at 296K Upper-state global quanta Lower-state global quanta Upper-state local quanta Lower-state local quanta Uncertainty indices Reference indices Flag Availability of program and data for the case of line mixing Statistical weight of the upper state Statistical weight of the lower state
13 MIPAS Line Transition Records The format of the MIPAS database as well as the numbering of the molecules and of the isotopic species is the same as in HITRAN-96 and HITRAN-2K
14 UPDATING OF SPECTROSCOPIC PARAMETERS: examples of issues
15 1) Updating of H2O in GEISA and GEISA/IASI-03
16 H2O GEISA/IASI-03 updating and alternative archive RAL/ EUMETSAT cm-1 Log intensity ( cm.molecule-1) Log intensity ( cm.molecule-1) Toth s (2000, 2002) cm-1 Wavenumber ( cm-1 ) Choice for GEISA/IASI-03 update Wavenumber (cm-1) Alternative choice for GEISA/IASI-03 update
17 H2O updating in GEISA/IASI-03: TOTH VS RAL Halfwidths (%) Intensity (%)
18 2) DIFFERENCES BETWEEN GEISA (GEISA/IASI-03) and HITRAN-04
19 H2O Intensity Differences GEISA/IASI 03 (Toth s data) and HITRAN 04 comparisons for air-broadened half-widths (HW) and intensities (I) % 10 cm-1 HW Average % 10 cm-1 Intensity Average difference (I H04 I G03) / (I H04 max + I G03 max)*2*100 difference (HW H04 HW G03) / Wavenumber (cm-1) Intensity average (cm-1/(molecule cm-2) Difference (%) Difference (%) Halfwidths average (cm-1 atm-1) (HW H04 max + HW G03 max)*2*100 Wavenumber (cm-1)
20 CO2 Intensity Differences Intensity average (cm-1/ molecule cm-2) New data for GIA-03 LTS LPMA Wavenumber ( cm-1) cm-1) % 10 cm-1 Intensity Average difference Number of lines Wavenumber ( Difference (%) Log intensity ( cm.molecule-1) GEISA/IASI 03 and HITRAN 04 comparisons for intensities (I H04 I G03) / (I H04 max + I G03 max)*2*100 Wavenumber ( cm-1)
21 O3 Intensity Differences New data for GIA-03 GSMA,LPMA LPPM (LISA), LTS, NASA (Langley), JPL Number of lines Log intensity (cm.molecule-1) GEISA/IASI 03 and HITRAN 04 comparisons for intensities Wavenumber (cm-1 ) Difference (%) HITRAN more Complete MIPAS data? Intensity average (cm-1/ molecule cm-2) Wavenumber (cm-1 ) % 10 cm-1 Intensity Average difference (I H04 I G03) / (I H04 max + I G03 max)*2*100
22 N2O Collision Half-Width Differences Number of lines New data for GIA-03 Wavenumber (cm-1) Wavenumber (cm-1 ) Difference (%) Halfwidths average (cm-1 atm-1) Log intensity (cm.molecule-1) GEISA/IASI 03 and HITRAN 04 comparisons for air-broadened half-widths % 10 cm-1 HW Average difference (HW H04 HW G03) / (HW H04 max + HW G03 max)*2*100
23 3) DIFFERENCES BETWEEN GEISA (GEISA/IASI-03) and MIPAS-03
24 H2O Intensity Differences
25 H2O Collision Half-Width Differences
26 CO2 Collision Half-Width Differences
27 O3 Intensity Differences
28 Evaluation of the Impact of Spectroscopic Archive Differences on Radiative Transfer Simulations
29 Spectroscopic data involved in comparisons GEISA/IASI ,001 cm-1 14 molecules: H2O, CO2, O3, N2O, CO, CH4, O2, NO, SO2, NO2, HNO3, OCS, C2H2, N2 MIPAS database 597 2,503 cm-1 Version pf3.1 HITRAN-04 extractions in GEISA/IASI and MIPAS databases common spectral intervals 6 Molecular species selected for comparisons, i.e.: H2O, CO2, O3, N2O, CO, CH4
30 IASI Radiative Transfer Modelling Overall Approach Five atmospheric profiles; mean of each of 5 air mass class the Thermodynamic Initial Guess Retrieval (TIGR) data set, in its latest version, a climatological library of about 2300 representative atmospheric situations selected by statistical methods from 80,000 radiosonde reports [Chédin et al., 1985; Achard, 1991; Chevallier et al., 1998]. Mc Clatchey profiles Three IASI spectral Bands: cm-1; cm-1; cm-1 4A (Automatized Atmospheric Absorption Atlas); fast and accurate line-by-line radiative transfer model [N.A. Scott and A. Chédin, 1981; Tournier et al. 1995; Chéruy et al. 1995] or STRANSAC line-by-line and layer-by-layer model, in their latest 2000 version [N.A. Scott, 1974] Mean thermodynamic Parameters for each TIGR air-mass
31 Spectroscopy issues and IASI sounding Channels Selection (H2O exemple) IASI Stransac-2000 simulations with RAL or TOTH spectroscopy
32 HITRAN and GEISA H2O DIFFERENCE IMPACT STRANSAC-2000 IASI Simulation Tropical TIGR-2000 atmosphere
33 HITRAN and GEISA O3 DIFFERENCE IMPACT STRANSAC-2000IASI Simulation Tropical TIGR-2000 atmosphere
34 HITRAN and GEISA N2O DIFFERENCE IMPACT STRANSAC-2000IASI simulation Tropical TIGR-2000 atmosphere
35 IASI 4A-2000 Band-1 Simulation TIGR-2000 Mean latitude 2
36 IASI 4A-2000 Band-2 Simulation TIGR-2000 Polar 2
37 IASI 4A-2000 Band-3 Simulation TIGR-2000 Tropical
38 CONCLUDING COMMENTS
39 Remaining spectroscopy related problems Some conclusions of validation exercises, using e.g. : the 4A-00/LMD Model, in the case of IASI radiative transfer modelling The water vapour spectroscopic parameters: still need to be validated; The water vapour continuum: more tuning to be done when more validation data (especially with high water vapor content) become available; The freons bands at 850 and 920 cm -1: refine the temperature dependence; O3 in the 9.6 micron region: the spectroscopic parameters still need to be validated; Some CO2 Q branches: further improvement/tuning of the line mixing
40 GEISA/IASI Present Operational Use GEISA and GEISA and registerme
41 GEISA/IASI Future Operational Use GEISA/IASI and associated facilities are being implemented on the Ether (CNRS/IPSL) Products and Services Centre (CPS) Effective fall 2006 Ether Products and Services Centre Facilities: measurement data from French laboratories, as well as from many international centres, forecasts such as Potential Vorticity, modelling results, downloadable procedures, browse images, on-line processing software (which can be activated through the Ether interface
42 IASI INSTRUMENT STATUS IASI Level 1 Cal/Val activities GEISA/IASI used as the reference spectroscopic database It is expected that validation can be achieved using a Line by line RTM (4A will be used for validation at 3 wavenumbers in each 3 bands)
43 ACKNOWLEDGMENTS to CNES and EUMETSAT for their Encouragements and Supports
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