Plasma-beryllium interactions in ITER: research needs

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1 Plasma-beryllium interactions in ITER: research needs G. De Temmerman a, With contributions from M.J. Baldwin b, D. Anthoine a, K. Heinola c, A. Jan a, I. Jepu d, J. Likonen e, S. Lisgo a C.P. Lungu d, C. Porosnicu d, and R.A. Pitts a a ITER Organization, Route de Vinon-sur-Verdon, CS 90046, St Paul Lez Durance, France b Centre for Energy Research, University of California at San Diego, San Diego, USA c University of Helsinki, P.O. Box 64, Helsinki, Finland d National Institute for Laser, Plasma and Radiation Physics, Bucharest-Magurele, Romania e VTT Technical Research Centre of Finland, P.O. Box 1000, FIN VTT, Finland ITER is the Nuclear Facility INB no This paper explores physics processes during the plasma operation of the tokamak; nevertheless the nuclear operator is not constrained by the results of this paper. The views and opinions expressed herein do not necessarily reflect those of the ITER Organization. 1

2 Content Status of the ITER site and construction Brief reminder about ITER plasma-facing components Some key Be-related research questions Be migration T retention Thermal outgassing Dust 2

3 Worksite progress PF Coil Facility Cryoplant Construction underway 400 kv switchyard Transformers Storage area 2 Storage area 3 Assembly Hall Construction underway Contractors area Cryostat Workshop Preparatory works Cleaning facility Tokamak Complex Construction underway Magnet Conversion Power Construction underway Batching plant Headquarters extension Preparatory works Cooling systems ITER IO Headquarters Storage area 1 Preparatory works Control Building (Aerial Photo April 2016) 3

4 Worksite progress 4

5 Tokamak Complex Resting on 493 seismic pads, the reinforced concrete B2 slab bears the ton Tokamak Complex. Concrete casting of the B2 slab was finalized on August 27, Diagnostic Building (left) B1 level slab now complete; installation of interior walls and reinforcement for BioShield ongoing. 5

6 Assembly Hall Before being integrated in the machine, the components will be prepared and pre-assembled in this 6,000 m2, 60-metre high building. The Assembly Hall will be equipped with a double overhead travelling crane with a lifting capacity of 1,500 tons, whose installation is scheduled in June. 6

7 Assembly hall Four crane girders (46m-long) for the double overhead travelling crane delivered 7

8 Cryoplant Foundation works are ongoing on what will be the largest cryoplant in the world. The ITER Cryoplant will distribute liquid helium and nitrogen to various machine components (supraconducting magnets, thermal shield, cryopumps, etc). The cryoplant s cold boxes are currently being equipped with internal components by Air Liquide in Grenoble, France. 8

9 ITER plasma-facing materials Beryllium Be Blanket module ~700m 2 beryllium First wall Low Z- good plasma compatibility Good oxygen getter Good thermal conductivity Tungsten Divertor ~150m 2 tungsten Low sputtering yield highest melting point (3422C) 9

10 Z (m) The plasma-wall interaction challenge B2-Eirene simulations (A.S. Kukushkin) 6 i-dib m_ipp D-Flux 4 (10 20 m -2 s -1 ) Heat R (m) MW.m -2 steady-state 1-10GW.m -2 (ms) Particles m -2 s -1 (10 5 A.m -2 ) E ion <50eV 10

11 Accumulated divertor fluence (m -2 ) High particle fluences expected in ITER Very high particle fluxes expected in ITER divertor ~10 24 m -2 s -1 Limited number of experiments can reach those conditions TCV JET ITER Accumulated over 5000 discharges Discharge duration (s) What is the influence of such high fluences on materials properties? 11

12 Full tungsten divertor 54 divertor assemblies (~9 tonnes each) Bakeable to 350 C Implementation of individual monoblock shaping under discussion 12

13 Reminder: full-w divertor ITER has a close-fitting and shaped first wall q dep (MW m -2 ) q dep Q dep (MW/m 2 ) (MW m -2 ) Q dep (MW/m 2 ) Peaking in erosion pattern expected, magnitude being estimated 13

14 First wall erosion in ITER ITER WALL Be erosion from plasma exposure during normal operations start-up on the high- and low-field sides main chamber charge-exchange neutral particle loads close-fitting, shaped wall geometry- potential for co-deposition on first wall 14

15 First wall erosion in ITER ITER WALL Be erosion from plasma exposure during normal operations start-up on the high- and low-field sides main chamber charge-exchange neutral particle loads close-fitting, shaped wall geometry- potential for co-deposition on first wall Regions of particular interest include: the upper target area (quasi-double null operations)- BM8 and BM9 BM11 and BM18 where plasma contact is though to be concentrated (interaction of 2 nd separatrix with PFC) 15

16 Migration modeling Method: Use state-of-the-art codes linking predicted: plasma background solutions (SOLPS), global impurity transport in the plasma (DIVIMP) PFC surface evolution due to erosion/redeposition (WALLDYN) Calculate the time evolution of the surface composition of PFCs Study sensitivity to different background plasmas Computational grids out to the walls but only 2D so far Wall elements 16

17 Predicted co-deposition rates Low far-sol plasma density case High far- SOL plasma density case Predicting about 3-19g of Be eroded from first wall and rede-posited elsewhere 17

18 T-retention in ITER and inventory limits T retention is limited by nuclear license: 1kg of in-vessel T Minimize environmental release during accidents T-retention in ITER largely driven by co-deposition of T with Be Estimated from WALLDYN for wide range of plasma scenarios Be migration in ITER K. Schmid et al, NF, 55 (2015) 18

19 T-retention in ITER and inventory limits T retention is limited by nuclear license: 1kg of in-vessel T Minimize environmental release during accidents T-retention in ITER largely driven by co-deposition of T with Be Estimated from WALLDYN for wide range of plasma scenarios Be migration in ITER T-limit could be reached in discharges (400s-long Q=10 discharges) NB: major uncertainty lies in the ITER SOL plasma parameters Deposition occurs mainly in the divertor (baffle regions) K. Schmid et al, NF, 55 (2015) 19

20 Global tritium measurements Closed T fuelling system for ITER: Calorimetry (T decay) used to monitor transfer from material subaccounts (sub-systems within T loop) PVT method to measure injection and exhaust Bakeout (240C FW, 350C divertor) for T recovery from PFM No knowledge of where the tritium is trapped. Local measurements provide additional information and help constrain simulations 20

21 Local tritium measurement (1/2) Tritium and deposit monitor being designed for local measurements Laser-induced desorption for retention Lock-in thermography for co-deposit thickness FOV of T/deposition monitor Focus is on inner divertor baffle where most of the deposition is expected to occur FOV~ 50x10cm Desorbed species detected by RGA/QMS Can be used at the end of operation day How to ensure full desorption from the co-deposit using laser heating? 21

22 Local tritium measurement (2/2) Experimental investigations of laser-induced desorption of D from Be Be co-deposits: Yu et al Bulk Be implanted with D: Keroack et al 10ms laser pulse 25ns laser pulse In both cases, significant release only when close or above melting J.H. Yu et al, JNM 438 (2013) D. Keroack et al., JNM (1994) Effect of longer pulse durations and multiple heating pulses? 22

23 T removal in ITER Outgassing by baking is the main technique for tritium removal from plasma-facing components 23

24 T removal in ITER Outgassing by baking is the main technique for tritium removal from plasma-facing components First wall baking at 240C Hot water through cooling system 24

25 T removal in ITER Outgassing by baking is the main technique for tritium removal from plasma-facing components Divertor baking at 350C Hot gas circulated in cooling pipes Needs draining and drying of cooling lines Takes about 100hrs for draining/heating and then cooling Bake frequency/duration not specified yet. Under investigation 25

26 M.J. Baldwin, R.P. Doerner, Nucl. Fusion 54 (2015) Efficiency of T removal by baking Previous investigations point out to possible reduced bake efficiency Effect of layer thickness, succession of bake cycles Recent results from JET beryllium co-deposits PISCES-B results JET results J. Likonen et al, this conference How to extrapolate those results to ITER to assess T removal efficiency? 26

27 Assessing efficiency of thermal outgassing PISCES, JET, NIPLRP (Romania) Experimental TDS data TMAP7 Different deposition conditions, heating rates, Modeling of experimental data Consistent model for different data Understand similarities and differences between different samples Input from WALLDYN Use of JET/PISCES models Extrapolation to ITER Range of efficiency depending on model 27

28 TMAP7 modeling: PISCES TMAP7 developed at INEEL to simulate diffusion/trapping in materials Model developed by Baldwin et al fit a wide range of experimental PISCES data for Be co-deposits TMAP7 model of PISCES data Model extended to TDS data of JET codeposits (J. Likonen, PSI2016) Ramp and hold experiments: different ramp rates and hold time at 350C Diffusion coef. and recombination rates similar to Baldwin et al Assume a homogeneous D profile Trap energy and occupancy used as free parameters M.J. Baldwin et al, Nucl. Fusion 54 (2014) M.J. Baldwin, R.P. Doerner, Nucl. Fusion 54 (2015) 28

29 Desorption flux (m -2 s -1 ) Temperature (C) TMAP7 modeling: JET data Simulated data from 3 samples annealed under different conditions Samples from tile 1 apron TMAP7 results 6x K/min ramp rate 15 hrs hold time at 350C x x x x x10 18 JET sample TMAP7 Temperature Time (s) 0 29

30 Desorption flux (m -2 s -1 ) Temperature (C) TMAP7 modeling: JET data Simulated data from 3 samples annealed under different conditions Samples from tile 1 apron TMAP7 results 1.0x x x x x K/min ramp rate 15 hrs hold time at 350C JET sample 12 TMAP7 Temperature Time (s) 30

31 Desorption flux (m -2 s -1 ) Temperature (C) TMAP7 modeling: JET data Simulated data from 3 samples annealed under different conditions Samples from tile 1 TMAP7 results 3x x K/min ramp rate 5 hrs hold time at 350C JET sample 6 TMAP7 Temperature x Time (s) 31

32 TMAP7 modeling: JET data Simulated data from 3 samples annealed under different conditions See talk by J. Likonen Good agreement obtained with 3 traps at ; 1.1 and 1.4eV Relative occupancy of traps dependent on sample location (and probably conditions during plasma exposure) First two traps correspond well with those observed on PISCES codeposits (0.8 and 1eV) High energy trap appears in JET: effect of impurities? Data for thicker films would be benefitial Temperature history of tile also needed Provides good basis for first extrapolation to ITER 32

33 Remaining T (%) Remaining T fraction (%) 100 Assessing efficiency of 350C bake TMAP simulations using 2 sets of assumptions PISCES model with 1 trap (T dep >100C) JET co-deposit model (sample 12, 3 traps) 623K 603K 583K 513K 50 microns 1 trap model Effect of temperature and thickness 2 weeks 1 week Time (hrs) weeks Temperature increase PISCES model C 240C 20 JET model 350C 240C Layer thickness ( m) 240C bake very inefficient. 350C more efficient At 350C, efficiency decreases very quickly with thickness 33

34 Remaining T fraction Remaining T fraction Efficiency of LID (1/2) Results for single pulse heating LID for T=1000K LID for 10 m thick layer Thickness ( m) 1s 0.5s 0.1s 0.05s 0.01s Pulse duration 1ms 5ms 50ms 100ms 500ms Temperature (K) Desorption efficiency decreases drastically with increasing thickness For a 10 m film, only 25% D removed for a 1s pulse Increasing temperature strongly increases desorption efficiency 34

35 Remaining D fraction Trapped D (m -2 ) Temperature (K) Efficiency of LID (2/2) Different combinations of pulse number/pulse duration investigated Total heating time kept constant 1.0 d=10 m T=1500K 1.0x pulse 500ms 10 pulses 50ms 50 pulses 10ms 8.0x x x10 22 Trapped D Temperature Time (s) 2.0x Time (s) Final desorbed fraction only depends on the total heating time and is independent on the heating scenario (multiple pulses vs single pulse) 35

36 Need for improved diffusion/trapping data Diffusion/trapping modeling also used to assess efficiency of detritration from tokamak waste Large uncertainties in existing diffusion/trapping/recombination rates D recombination rate on Be Diffusion coef. D in Be Understanding the discrepancies between those values would ease extrapolations to ITER 36

37 Be dust: what does it look like? Very little (if any) existing data from relevant experiments Dust from JET-ILW still to be analyzed, no delamination yet Some data from QSPA (but remember: at higher plasma pressure) Dust on QSPA exposed target Most probable dust size from existing experiments is <10 microns (but large size distribution) Early ITER operation phases will bring lots of information Important that sampling/analyses can be done during those phases 37

38 Summary/Outlook Good progress being made on beryllium erosion data Tritium retention estimates bound to uncertainties on SOL plasma Work ongoing to refine the T-removal strategy and develop local T measurement techniques Important to obtain accurate data for T trapping, diffusion and recombination from bulk Be and Be co-deposits Information on Be dust from relevant experiments is needed to refine current assumptions 38

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