Optical Remote Sensing with DIfferential Absorption Lidar (DIAL)

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1 Optcal emote esg wth DIffeetal Absopt Lda DIAL Pat : Theoy hstoph eff IE Uvesty of oloado & OAA/EL/D/Atmosphec emote esg oup uest lectue fo AE-659 Lda emote esg U oulde Octobe 8 0

2 Outle DIAL ccept A shot hstoy of DIAL DIAL equat Pecs & accuacy of DIAL eteval Dual-DIAL techque

3

4 Atmosphec gases measued wth DIAL H O O 3 O O O H 3 H 4 O Hg VOs Volatle Ogac ompouds Toluee ezee

5 Fst DIAL measuemets chad M. chotlad The fathe of DIAL 964 Measued vetcal pofles of wate vapo by themally tug a uby lase ad the wate vapo absopt le at m. Oly 4 yeas afte vet of uby lase!

6 Majo mlestes the hstoy of DIAL Mama: Ivet of the lase humate & Mezes: Fst Aboe DIAL colum O 3 owell: Fst automous DIAL LAE H 0 DIAL E- acaft pace-based DIAL Peset?? chotlad: Fst H O DIAL measuemets Mege: Fst O 3 DIAL owell: Fst aboe H O DIAL

7 DIAL equat abs mol Tot Tot L wth d A 0 exp d d d m X X X L L exp exp exp gle scatteg elastc backscatte LIDA equat: Take ato of LIDA equats fo le ad le wavelegths λ ad λ : umbe desty of csttuet

8 DIAL equat l l l wth X E d d d d d d m X X = dffeetal geometcal facto = dffeetal backscatte E = dffeetal extct X = tefeg csttuets

9 How to choose a appopate absopt le fo DIAL exp 0 d Extct of le wavelegth due to absopt by csttuet must be ethe too small o too lage. Absopt too stg Absopt too weak λ λ λ λ est pecs whe: max 0 max d. emsbeg & odley 978

10 How to choose a appopate absopt le fo DIAL max Example: Oze max d. 0 Fo m O 3 O 3 80 ppbv O 3 max o. O 3 0 O 3 8 m 3 ad max.830 3km: m λ 88 m λ 99 m

11 Pecs of DIAL measuemets mple back of the evelope calculat: Eve modest pecs of 5% eques hgh. ca be ceased by aveagg /le sgals tme- ad age-wse. 400! 5% 0.05 : l Example wth wth j j j : t ad t t ce statstcs Poss

12 Accuacy of DIAL measuemets X E d d d d d d m X X l l l Accuacy affected by: How well s absopt coss sect kow? Impope coect of sgal sets e.g. backgoud lght eometcal facto dffeet fo λ ad λ Dffeetal backscatte & extct ot popely coected Itefeg speces ot take to accout

13 Accuacy of DIAL measuemets Dffeetal geometcal facto: d l d ; Effect of dffeetal geometcal facto O 3 eteval

14 Accuacy of DIAL measuemets 3 Dffeetal backscatte & extct: d d l E aylegh Aeosol aylegh Aeosol λ 88 m Fo oze DIAL eteval backscatte ad extct coect s ecessay due to lage Δλ. λ 99 m β Aeosol ad α Aeosol have to be detemed fom le sgal data ad wavelegth depedece of β ad α have to be guessed.

15 Accuacy of DIAL measuemets 4 β Aeosol smulat O 3 eteval smulat Wg assumpts about aeosol paametes ca toduce sgfcat eos O 3 eteval!

16 Dual-DIAL ccept λ λ λ 3 DIAL wavelegth pas: λ / λ ad λ / λ 3

17 Dual-DIAL mmzes aeosol tefeece * * * * 0 ' ' / : / : ' ' l l l l fo E pa DIAL pa DIAL wth E d d d d o coect of dffeetal aeosol effects eeded ad esdual eos ae small. Howeve pecs of DIAL eteval s degaded.

18 Dual-DIAL mmzes aeosol tefeece O 3 eteval smulat

19 elected efeeces DIAL hstoy sldes 5-6 chotlad. M. 974: Eos the Lda Measuemet of Atmosphec ases by Dffeetal Absopt J. Appl. Meteool humate M... T. Mezes W.. at ad D.. McDougal 98: Lase Absopt pectomete: emote Measuemet of Toposphec Oze Appl. Opt Pel J. ad. Mege 98: Oze Mtog the Toposphee ad Lowe tatosphee: Evaluat ad Opeat of a oud-ased Lda tat J. eophys. es Mege. J.. Acellet ad J. Pel 985: Lda Measuemets of Oze Vetcal Pofles Appl. Opt owell E. V.. Ismal W.. at 998: Dffeetal Absopt Lda DIAL Measuemets fom A ad pace Appl. Phys Ismal. E. V. owell. A. Feae. A. Koo M.. layt V.. ackett ad P.. ussell 000: LAE Measuemets of Aeosol ad Wate Vapo Pofles Dug TAFOX J. eophys. es. 05 D How to choose a DIAL absopt le? sldes 9-0 emsbeg E. E. ad L. L. odley 978: Aalyss of Dffeetal Absopt Lda fom the pace huttle Appl. Opt Aeosol coect & DUAL-DIAL sldes 4-8 owell E. V.. Ismal ad. T. hpley 985: Ultavolet DIAL measuemets of O3 pofles egs of spatally homogeeous aeosols Appl. Opt Wag Z. H. akae H. Hu ad J. Zhou 997: Thee-Wavelegth Dual Dffeetal Absopt Lda Method fo tatosphec Oze Measuemets the Pesece of Volcac Aeosols Appl. Opt

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