American Physical Society Division of Fluid Dynamics Meeting, San Antonio, TX, November 23 25, 2008.
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1 American Physical Society Division of Fluid Dynamics Meeting, San Antonio, TX, November 23 25, TURBULENT MIXING DUE TO RAYLEIGH-TAYLOR INSTABILITY David Youngs AWE Aldermaston UNITED KINGDOM British Crown Copyright 2008 / MOD 1
2 OUTLINE OF TALK What is Rayleigh-Taylor instability and where does it occur? The fundamental case growth of a single sinusoidal mode Self-similar turbulent mixing Constant acceleration, influence of initial conditions, internal structure, variable acceleration Examples of more complex flows Break-up of a dense layer, a simple (ICF) implosion Concluding remarks Will give some historical background and show some experimental results Will discuss major advances recently made using 3D simulation ( and scope for further work) similarities to turbulent shear flow implications for engineering modelling (RANS models) 2
3 What is Rayleigh-Taylor (RT) instability? Note: pressure gradient from heavy to light in both cases First publication, Rayleigh (1883) Became an important research topic after the paper of G.I. Talyor (1950) (related process Richtmyer-Meshkov instability occurs when shock waves pass through perturbed interfaces) 3
4 A broad set of vital applications Astrophysics Atmosphere / Ocean t=5000s Rayleigh-Taylor instability traced by cirrus clouds (Picasa Web) Instability and clumping in SN1987A. Müller et al. Astronomy and Astrophysics (1991) Geological flows (e.g. oil trapping in salt-domes) wide range of distance and time scales, wide range of density ratios 4
5 Inertial Confinement Fusion (ICF) nanosecond time-scale Amendt et al. Physics of Plasmas (2002) degradation of capsule performance. Focus of the present talk will be high-reynolds no. mixing at initially sharp interfaces. Flows may be compressible, but turbulence Mach no. (u/c) is low most key aspects of the RT process can be understood via incompressible experiments and simulations. 5
6 3D simulation has greatly enhanced our understanding of RT turbulence during the past decade log E(k) energy -5/3 ~ k (Kolmogorov spectrum) ILES/LES DNS log(k) experimental dissipation wavenumber achievable grid resolution DNS: Direct Numerical Simulation needed to understand the effect of Reynolds No. LES: Large Eddy Simulation best approximation to high-reynolds No. mixing in more complex flows ( explicit sub-grid-scale dissipation model or high-wavenumber 6 dissipation Implicit in the numerical scheme: ILES)
7 DNS for simple problems High resolution 3D simulation (LES) for more complex problems As computer power increases the LES should get closer and closer to the full scale applications calibration / validation Engineering models Applications 7
8 Historical Development (in the West) s Main focus on evolution of a single sinusoudal mode ( small amplitude linear growth large amplitude non-linear growth) (see review paper by David Sharp, PhysicaD,1984 full references given at end of PDF file) 1980s Present day Emphasis changed to understanding turbulent mixing ( evolution of mixing from random multimode perturbations) ( note contrast with turbulent shear flow e.g. mixing layer - Liepmann & Laufer (1947) : self-similar turbulent mixing Brown & Rosko (1974) : coherent structures ) 8
9 Single mode Rayleigh-Taylor instability 2D simulation at density ratio 1 / 2 = Atwood number: A= 1 2 linear nt a=a e, n= 0 2 Ag non-linear h b bubble h s spike dh dt early time: exponential growth (19 th C theory for interfacial waves with sign of 1-2 reversed) late-time: bubbles rise with velocity: V~ Ag Atwood No. close to 1 : Equation due to Layzer (1955) gives a good approximation to the b bubble velocity V= : 2 E 1 E Ag- where E=exp - 2 dv 6 V 6 hb dt Low Atwood No. : More complex behaviour, Ramaprahbu et al. (2006) - 3D simulations 9
10 Multimode initial perturbations 2D simulation Apply Layzer equation to a range of wavelengths (similar technique used by G. Birkhoff, Los Alamos report, 1954) =4 h b initial amplitude = 0.01 =2 =1 =0.5 =0.25 time bubble competition experiments of Emmons et al
11 Experiments used for Rayleigh-Taylor turbulence (1980 onwards) accelerated tank static tank light heavy remove barrier heavy light Cambridge U Chelyabinsk-70 AWE, LLNL Chelyabinsk-70, U Arizona water/gas channel, h b =f(t) where t=x/u U U splitter plate heavy light U Texas A&M U 11
12 Rocket-Rig RT experiment - AWRE Foulness,1980s, (see, Read,1984) N 2 He mixing layer: Brown and Rosko, JFM, (1974) length scale increases by vortex pairing Compressed SF 6 Pentane 2 33ms 53ms 79ms h s (spike) h b (bubble) length scale increases by bubble competition 12
13 Experiments show increase in length scale as mixing evolves if mixing is self-similar, dimensional analysis suggests mixing zone width W f gt The Rocket-rig experiments showed hb gt where and h s /h b a slowly increasing function of / 1 2 very simple pattern for the amount of mixing h b penetration of dense fluid (bubble distance) h s penetration of light fluid (spike distance) More recent Linear Electric Motor experiments at LLNL, (Dimonte & Schnieder,1996) gave ~ 0.05, Texas A&M =0.07 Also similar results from experiments performed by Kucherenko s group at Chelyabinsk-70 (Kucherenko et al., 1991) 13
14 LOSS OF MEMORY OF INITIAL CONDITIONS (Youngs 1984) If the initial surface consists of small random short wavelength perturbations then, after a short time: dominant length scale» viscous scale dominant length scale increases by mode coupling expect loss of memory of the initial conditions to occur (as assumed in turbulent shear flow, Townsend, 1976*) unique value of It was noted that mixing would be enhanced if long-wavelength initial perturbations with sufficiently high amplitudes were present. However, before high-resolution 3D simulation was feasible it was thought that loss of memory of initial conditions would apply to low end of the observed range of values * was known at the time that shear layer growth varied from experiment to experiment 14
15 TURMOIL MILES ( 1 / 3 = 3) 720 x 600 x 600 meshes (simple explicit compressible code run at low Mach no) Short wavelength initial perturbations : random combination of Fourier modes: wavelengths:- 4 x to 8 x, amplitude s.d.: x t = 0.8 t = 2.0 t = 3.8 Calculations performed on the AWE Cray XT3 (8000 processing elements). For these calculations: 360 processors for 24 hours 15
16 h b 2 W f1f2 dx, hb 3.3W f 1= f, f fluid volume fractions averaged over a horizontal layer h s (spike) h b (bubble) h b X (3 calculations with different random numbers) Dimonte, Youngs et al, 2004: for 7 ILES methods, 512x256x256 meshes X=Agt 2 16
17 Cabot & Cook,LLNL, 2006: DNS TURMOIL (ILES) 720x600x600 Re hh 2 hb b 4Ah b b DNS suggests that may increase slowly with Re some uncertainty in high Re limit. TURMOIL shows similar limiting behaviour to the much higher resolution DNS. 17
18 For the ideal situation of small random perturbations a range of both LES and DNS results have all given values of much less than observed need to assume that in experiments low levels of initial long wavelength perturbations have enhanced mixing. A model for enhanced self-similar growth was proposed by Inogamov(1999): Long wavelength initial perturbations with amplitude wavelength, up to size of experiment. Note similarity to Birkhoff s arguement In mathematical terms 2 3 s.d of surface =, where = P(k)dk with P(k) ~ 1/k have used here: wavelengths up to 1 2 box width and = box width (a very small value) 18
19 long wavelength perturbations h b X h b short wavelength perturbations h b X X=Agt 2 19
20 The results suggest that low levels of long-wavelength initial perturbations are the explanation of the higher observed growth rates. (note recent experiments, Kucherenko et.al, 2003, have indicated a lower ~0.04) Experiments are finite: The basic problem is not mixing at an infinite plane boundary with finite s.d. (this should asymptote to ~0.025) but mixing in a finite domain of size L, with low levels of perturbations with wavelengths up to size L. Then expect influence of initial conditions to persist throughout the duration of the experiment. Similar conclusion apply to turbulent shear flows (influence of upstream conditions) W.K.George, Freeman Scholar Lecture, ASME Fluids Engineering Meeting,
21 A simple quatitative model for the dependence on initial conditions 0 k+ k Initial perturbation at wavelength : a = P(k )dk Perturbation due to mode-coupling = k-k (invariant) d dominant scale at time t, then (approximately) d nt 1 2 a e where n= b d 0 Then h ~ 2 ln 2 Agt d 2 Ag Suggests weak logarithmic dependence in initial conditions (more quantitative argument given by Dimonte, 2004) 21
22 Important Implications for Engineering Modelling {RANS models, one-point closure models e.g. (k,) model} Given set of model coefficients a given value of - does not capture the dependence on initial conditions (also applies to shear flow modelling W. K. George) velocity field due to long wavelength initial perturbation will enhance mixing at late-time (not captured in one-point closure models) current region of turbulent mixing 22
23 Solution adopted here Note that, for a given experimental series, assuming = a const., works quite well (weak dependence on initial conditions) Derive model coefficient sets for a range of values of, using 3D LES (or DNS) results for enhanced self-similar mixing (Inogamov) Use LES for simplified versions of the real problems, with estimates of realistic initial conditions, to estimate the appropriate effective for a given application. 23
24 The 3D simulations also give much detailed information on the internal structure for ICF important to know the amount of molecular mixing molecular mixing parameter f f 1 2 f f 2 1 f f Ramaprabhu & Andrews, 2004 (Expt A=7.5 x 10-4 ) mean volume fraction short wavelength perturbations long wavelength perturbations 24
25 Measurements of molecular mixing parameter: Malcolm Andrews group at Texas A&M Lvis Sc= D L diff 2 Sc=700 (brine/water) Pr=Sc=7 (cold/hot water) Sc=0.7 (gases) Combining passive scalar and reacting scalar experiments at multiple equivalence ratios provide a measure of the volume fraction variance, Meuschke et al (2008) Measurement of molecular mixing demonstrates a large influence of Schmidt number at small Re, but tending toward saturation at high Re ~10 4 a challenge for DNS. Note similarity to jet mixing, Dimotakis (2000) mixing transition at Re =U/ = 1-2 x Re h 25
26 Power spectra: w (vertical velovity), u&v (horizontal velocity) and (density) u,v w -5/3 Cabot&Cook, DNS -5/3 fit Experiment, Dalziel et al. (1999) TURMOIL, ILES DNS and ILES show similar behaviour for velocity spectra at low wavenumber. DNS/ILES/Experiment all show spectra for slightly 26 flatter than k-5/3
27 Departures from Kolmogorov s k -5/3 law (see also O. Poujade, 2006) Both DNS and LES velocity spectra show some asymmetry at high-wavenumbers suggests buoyancy effects persist at high-wavenembers (some evidence for this from TAMU experiments) Corrections to the k -5/3 law have been proposed, for slowly varying turbulence (Yoshizawa,1994: Woodruff &Rubinstein, 2006) 2/3-5/3 2/3-7/3 D K N Dt E(k)=C k C k +..., Now for RT mix with constant g 3 u ~ t But expect to get more extreme variations than this 27
28 Have so far assumed, acceleration, g = a constant not very realistic approximation in many applications (e.g supernova explosion, ICF implosion). g ~ t g~1/t highly likely to occur (the LLNL Linear Electric Motor experiments did consider variable g) Antoine Llor, CEA (2004) has advocated studying self-similar RT mixing problems, also O. Poujade APS-DFD 2008: n n+2 g=ct h b = nact Very useful for extended validation of the one-point closure models. Also interesting to look at power spectra g ~ t ~ t 3 : g ~ 1/t ~ 1/t expect more extreme variations in time than many other types of turbulent flow 28
29 Finally some more complex RT flows will be considered: (a) Break-up of a dense fluid layer due to Rayleigh-Taylor instability. (b) A simplified spherical implosion Will show that ILES currently makes an essential contribution to engineering model validation model used here : multiphase flow equations +turbulent diffusion terms + decay of concentration fluctuations (a type of RANS model) 29
30 BREAK-UP OF A DENSE FLUID LAYER DUE TO RAYLEIGH-TAYLOR INTABILITY 2 =1 H 1 =1.5 or 10 H 2 =1 g x dimensionless time 2H L = Ag t H (Atwood no. or Boussinesq scaling) A= Initial perturbations at lower boundary P(k) ~ 1/k 3 (as before) Corresponding low Atwood no. experiments, Jacobs & Dalziel (2005) 30
31 1 / 2 =1.5, 3D simulation, sections for fluid 2 volume fraction 1 / 2 =10, 3D simulation, sections for fluid 2 volume fraction =1 =2.5 =4 =10 31 mixing time scale is confirmed by experiments of Jacobs & Dalziel (2005)
32 Mean fluid volume fractions (averaged over horizontal layers) for 1 / 2 =10 =4 =10 fr x, depth x, depth 1D engineering model uses coefficient set for =
33 A simple spherical implosion (dimensionless units) I relevant to Inertial Confinement Fusion Perturbation spectrum, P(k)~ 1, s.d.= k2 max. wavelength = shell thickness = 1.0 p =0.1 Outer radius = 12 Perfect gas equations of state =5/3 = 0.05, p = 0.1 Outer radius= 10 D.L.Youngs and R.J.R.Williams, (2008) applied pressure on outer boundary 33
34 1D Lagrangian calculation RM RM:Richtmyer-Meshkov RT : Rayleigh-Taylor RT RT RM RT RM Note influence of initial conditions more complex: initial spectrum +amplification due to first shock + spherical convergence set initial perturbations for late stage mixing 34
35 3D SIMULATION THE SPHERICAL IMPLOSION 1D 3D 3D square patch perturbed by Fourier modes 1D Calculate sector 2 8, 2 8 Spherical polar mesh, Lagrangian in r-direction, 1D Lagrangian regions at origin and at outer boundary. 35
36 t = 2.0 t = 2.4(~max compression) t = 2.8 2D sections through the 3D simulation (standard mesh) 36
37 Comparison of 3D results with 1D model Mixing zone limits: radii for which f1 = 0.01, D engineering model uses:coefficients for = 0.07 (influence of initial conditions greater here) 37
38 Distributions at time=3 f1f 2 f1 f2 3D simulation for a simplified problem like this is used to tune the engineering model constants for a more complex application 38
39 CONCLUDING REMARKS During the last decade 3D simulation and more detailed experimental diagnostics has led to major advances in our understanding of RT mixing. Interesting range of self-similar cases for further investigation enhanced growth due to longwavelength perturbations, variable acceleration, effect of density ratio. Influence of initial conditions is an extremely important issue. Needs to be allowed for both in the engineering modelling and comparison with experiment. The related process RM mixing has been less well studied via 3D simulation. For self-similar mixing h=a Ut, where U = change in interface velocity due to a shock. Many of the same issues arise as for RT mixing. 39
40 Thanks to Ken Read, Vic Smeaton, Keith Burrows vvvv(rocket- Rig experimental team at AWRE) Malcolm Andrews (LANL) Guy Dimonte (LANL) Stuart Dalziel (Cambridge U) Paul Linden (UCSD-was at Cambridge U) QUESTIONS? 40
41 References 1.Lord Rayleigh (1883) Investigation of the character of the equilibrium of an incompressible heavy fluid of variable density, Proc. London Math. Soc., 14, G. I. Taylor (1950) The instability of liquid surfaces when accelerated in a direction perpendicular to their planes, Proc. Roy. Soc. of London, A201, E. Müller, B. Fryxell & D. Arnett (1991) Instability and clumping in SN1987A. Astron. Astrophysics, 251, P. Amendt et al. (2002) Indirect-drive noncryogenic double-shell ignition targets for the National Ignition Facility: design and analysis, Phys. Plasmas, 9, D. H. Sharp (1984), An overview of Rayleigh-Taylor instability, Physica D, 12, H. W. Liepmann & J. Laufer (1947) Investigations of free turbulent mixing NACA Technical Note No G. L. Brown & A. Roshko (1974 ) On density effects and large structure in turbulent mixing layers, J. Fluid Mech., 64, D. Layzer (1955) On the instability of superposed fluids in a gravitational field, Astrophysical J., 122, P. Ramaprabhu et al. (2006) Limits of the potential flow approach to the single-mode Rayleigh-Taylor problem, Phys. Rev E, 74, (10 pages). 10. G. Birkhoff (1954) Taylor instability and laminar mixing, Los Alamos report, LA H. W. Emmons, C. T. Chang & B. C. Watson (1960) Taylor instability of finite surface waves, J. Fluid Mech., 7, K. I. Read (1984) Experimental Investigation of turbulent mixing by Rayleigh-Taylor instability, Physica D, 12, G. Dimonte & M. Schneider (2000) Density ratio dependence of Rayleigh-Taylor mixing for sustained and impulsive acceleration histories, Phys. Fluids, 12, Yu. A. Kucherenko et al. (1991) Experimental study of the gravitational turbulent mixing self-similar mode, in proceedings of the Third International Workshop on the Physics of Compressible Turbulent Mixing ( IWPCTM3). 13. D. L. Youngs (1984) Numerical simulation of turbulent mixing by Rayleigh-Taylor instability, Physica D, 12,
42 14. A. A. Townsend (1976) The structure of turbulent shear flow (second edition), Cambridge University Press. 15. G. Dimonte, D.L.Youngs et al. (2004) A comparative study of the turbulent Rayleigh-Taylor instability using highresolution three-dimensional numerical simulations: the alpha- group collaboration, Phys. Fluids, 16, W. H. Cabot & A. W. Cook (2006) Reynolds number effects on Rayleigh-Taylor instability with possible implications for type-1a supanovae, Nature Physics, 2, N. Inogamov, The role of Rayleigh-Taylor and Richtmyer-Meshkov instabilities in astrophysics: an introduction, Astrophys. Space Phys. 10, (1999) 18 Yu. A. Kucherenko et al. Experimental investigation into the self-similar mode of mixing of different density gases in the Earth's gravitational field, Laser and Particle Beams, 21, , (2003) 19. W. K. George (2008) Is there an asymptotic effect of initial and upstream conditions on turbulence, Freeman Scholar Lecture, Proceedings of ASME Fluids Engineering Meeting, Aug 10-14, Ramaprabhu & M. J. Andrews, Experimental investigation of Rayleigh-Taylor mixing at small Atwood number, J. Fluid Mech. 502, (2004) 21. N. J. Meuschke et al. (2008) Measurements of molecular mixing in a high Schmidt number Rayleigh-Taylor mixing layer, submitted to J. Fluid Mech. 22. P. E. Dimotakis (2000) The mixing transition in turbulent flows, J. Fluid Mech., 409, S. B. Dalziel. P. F. Linden & D. L. Youngs (1999) Self-similarity and internal structure of turbulence induced by Rayleigh-Taylor instability, J. Fluid Mech., 399, O. Poujade (2006), Rayleigh-Taylor turbulence is nothing like Kolmogorov turbulence in the self-similar regime, Phys. Rev. Lett, 97, A. Yoshizawa (1994). Nonequilibrium effect of the turbulent-energy-production process on the inertial range sprctrum, Phys. Rev. E, 49, S. L. Woodruff & R. Rubinstein (2006), Multiple-scale perturbation analysis of slowly evolving turbulence, J. Fluid Mech., 565, A Llor (2003) Bulk turbulent transport and structure in Rayleigh-Taylor, Richtmyer-Meshkov and variable acceleration instabilities, Laser and Particle Beams, 21, J. Jacobs, & S. B. Dalziel (2005), Rayleigh-Taylor Instability in Complex Stratifications, J Fluid Mech, 542, D.L.Youngs and R.J.R.Williams (2008), Turbulent mixing in spherical implosions, Int. J. Numer. Meth. Fluids. 56,
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