Continuous observation of aerosols in East Asia using a ground based lidar network (AD NET)

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1 International Workshop on Air Quality in Asia, Hanoi, Vietnam. June 24th 26th, 2014 Continuous observation of aerosols in East Asia using a ground based lidar network (AD NET) Nobuo Sugimoto, Tomoaki Nishizawa, Atsushi Shimizu, Ichiro Matsui, Yoshitaka Jin National Institute for Environmental Studies, Japan

2 Contents Asian Dust and aerosol lidar observation Network (AD Net) ( lidar.nies.go.jp/ad Net/) AD Net lidars and data analysis methods Applications of AD Net data Improvement of lidars and data analysis methods Multi wavelength Raman lidar/ High Spectral Resolution Lidar Development of aerosol component analysis method On going studies

3 AD Net Ulaanbaatar Sainshand Zamynuud Takikawa Tsukuba 1996 Nagasaki 2001 Beijing 2001 Thailand 2002 Lanzhou + Hefei + Beijing* + Niigata Seoul* Sendai Toyama** Daejeon Matsue* Tsukuba* Fukuoka** Jeju Osaka Tokyo Chiba Nagasaki Fukue* AD Net is a contributing network to WMO GAW program Phimai* Shenzhen + Hedo** Lidar specification (532,1064)+ (532) * (532 Raman)+ (532,1064)+ (532) ** (355,532 Raman)+ (355,532,1064)+ (355,532) (355,532 HSRL)+ (355,532,1064)+ (532,1064) +Cooperative stations without realtime data sharing

4 Lidars in AD Net ( ) 2β+1δ (+1α) lidar α: extinction, β: backscattering, δ: depolarization

5 Dust 1β+1δ algorithm March 21 31, 2004 Beijing Dust Spherical aerosol particles Air pollution Method for estimating the extinction coefficients of dust and spherical aerosols using the depolarization ratio

6 Height (km) 18 0 Standard near realtime AD Net data products (updated every hour) Nagasaki June 2014 Attenuated backscattering coefficient at 532 nm Volume depolarization ratio at 532 nm Up to this morning Attenuated backscattering coefficient at 1064 nm Height (km) 9 0 Dust extinction coefficient at 532 nm Spherical aerosol extinction coefficient at 532 nm Also provided in NetCDF format

7 Applications of AD Net data Epidemiological studies of the effects of aerosols (Asian dust) on human health Data assimilation of Asian dust Aerosol climatology

8 Dust Pollution epidemiological studies of the effect of Asian dust on human health Significant effect of Asian dust is reported, for example, in asthma hospitalizaion in children, etc. Daily near surface ( m) extinction estimates for dust and spherical aerosols 2011

9 Ratio of PM2.5 to Extinction Coefficient as a function of relative humidity for Asian dust and air pollution aerosols (a) Asian dust case (b) Air pollution case Near surface lidar extinction coefficient ( m) and PM2.5 at the nearest air pollution monitoring stations are used.

10 Asian dust study using 4D Var data assimilation NIES lidar network (3) 4DVAR data assimilation of Asian dust using the NIES lidar network data (Yumimoto et al. 2007, 2008) Comparison of the assimilated dust transport model with CALIPSO data (Hara et al. 2009) Please see the publication list at lidar.nies.go.jp/~cml/english/publicationse.html

11 AD Net is evolving into a continuously operated advanced multi parameter lidar network Addition of Raman detection channel to current AD Net lidars for independent extinction coefficient measurements (1α+2β+1δ lidar) Development of multi wavelength Raman lidars and High Spectral Resolution Lidars (HSRLs) (2α+3β+2δ lidars) Development of the aerosol component analysis algorithm for multi parameter lidars

12 Aerosol component analysis method Measured parameters Mie polarization lidar +Raman 1β+1δ 2β+1δ 1α+2β+1δ Multi wavelength Raman and HSRL 2α+3β+2δ Derived aerosol components non spherical (dust) spherical non spherical (dust) spherical fine (sulfate, etc.) spherical coarse (sea salt) non spherical (dust) weak absorption fine (sulfate, etc.) weak absorption coarse (sea salt) strong absorption fine (black carbon) Müller s inversion method Microphysical parameters (SSA, effective radius, etc.)

13 Aerosol component retrieval (1α+1β+1δ) Sulfate, etc. Dust Assumption: External mixture of 4 components at each layer Optical properties for each aerosol component are prescribed (e.g., size dist., lidar ratio etc ) Black carbon Sulfate etc.: moderate-absorption / spherical (small-size) Dust : moderate absorption / non-spherical (large-size) Sea-salt : weak-absorption / spherical (large-size) Black carbon : strong-absorption / spherical (small-size) 1 (532)+1 (532)+1 (532) data measured with HSRL and MSL on Apr were used in the analysis. The aerosol properties at 532 nm used in 2 +1 algorithm were used.

14 Development of a multi wavelength high spectral resolution lidar 2α+3β+2δ HSRL system 532nm HSRL nm receiver 355nm HSRL receiver PMT (532nm) PMT (355nm) Etalon APD (1064nm)

15 Raman lidar 2α+3β+2δ Raman lidar at Kyushu University

16 On going studies Data assimilation of multi parameter lidars To develop data assimilation method for aerosol components and to construct aerosol reanalysis data set in East Asia Development of aerosol retrieval algorithms and validation methods for EarthCARE ATLID(355nm HSRL:1α+1β+1δ) (scheduled for launch in 2016) Our target includes establishing compatibility of different lidar (+radiometer) observations based on the aerosol component analysis method (+data assimilation).

17 The project on data assimilation of multi wavelength Raman (or HSR) lidars! Grant in Aid for Scientific Research(S) Integrated Disciplines (Environmental science) Five dimensional data assimilation of aerosol based on integrated analysis of multi wavelength lidar and chemical transport model PI: Itsushi Uno (Kyushu University, Research Institute for Applied Mechanics) Toyama Okinawa Fukuoka 2α+3β+2δ (Raman)

18 Observation operator for data assimilation K. Yumimoto, T. Nishizawa Particle extinction coefficient (355, 532 nm) Model result Observation operator Backscatter coefficient (355, 532, 1064 nm) Particle depolarization ratio (355, 532, 1064 nm) Attenuated backscat. coeffi. (355, 532, 1064 nm) Aerosol optical thickness (355, 532, 1064 nm) Example Attenuated backscatter coefficient (532 nm) Matsue, April 2007 Model Matsue, April 2007 Observation

19 On going studies Data assimilation of multi parameter lidars To develop data assimilation method for aerosol components and to construct aerosol reanalysis data set in East Asia Development of aerosol retrieval algorithms and validation methods for EarthCARE ATLID(355nm HSRL:1α+1β+1δ) (scheduled for launch in 2016) Our target includes establishing compatibility of different lidar (+radiometer) observations based on the aerosol component analysis method (+data assimilation).

20 Validation of the ATLID aerosol component product ATLID (α, β, δ at 355 nm) + supplementary data Concentrations of 4 aerosol components (Mineral dust, Sea salt, Black carbon, Sulfate+Nitrate+OC) Validation with ground-based multi-wavelength HSRLs and Raman lidars + aerosol component analysis method. (1) Multi-wavelength HSRL or Raman lidar α at 355 nm, 532nm β at 355 nm, 532nm, 1064 nm δ at 355 nm, 532 nm, (1064 nm) (2) AD-Net lidar with Raman β at 532 nm, 1064 nm, α, δ at 532 nm The results should (3) Raman lidar α, β, δ at 355 nm (4) Standard AD-Net lidar + radiometer Aerosol component retrievals be consistent if the aerosol optical model is reasonable

21 AD Net Ulaanbaatar Sainshand Zamynuud Takikawa Lanzhou + Hefei + Beijing* + Niigata Seoul* Sendai Toyama** Daejeon Matsue* Tsukuba* Fukuoka** Jeju Osaka Tokyo Chiba Nagasaki Fukue* Shenzhen + Hedo** Phimai* Lidar specification (532,1064)+ (532) * (532 Raman)+ (532,1064)+ (532) ** (355,532 Raman)+ (355,532,1064)+ (355,532) (355,532 HSRL)+ (355,532,1064)+ (532,1064) +Cooperative stations without realtime data sharing

22 Thank you

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