Time-modulation of electron-capture decay factor detected at GSI, Darmstadt

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Time-modulation of electron-capture decay factor detected at GSI, Darmstadt Byung Kyu Park Department of Physics University of California, Berkeley Physics 250 March 20, 2008 Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 1 / 19

Outline 1 The Experiment 2 Hypotheses 3 Neutrino Oscillation 4 Prospects Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 2 / 19

The Facility Gesellschaft für Schwerionenforschung, Darmstadt 1 1 http://www.gsi.de/ Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 3 / 19

What they study Decay schemes for neutral Pr-140 and Pm-142 Atomic charge state affects decay rates and branching ratio. Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 4 / 19

Heavy-ion production and storage For runs 1 and 2 Schematic layout of the facility with heavy-ion synchrotron SIS, the fragment separator FRS, and the storage-cooler ring ESR highlighted. 2 2 Yu. A. Litvinov et al., arxiv:nucl-ex/0509019 Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 5 / 19

Heavy-ion production and storage For runs 3 and 4 Revolution frequency of ions in storage is measured by Schottky mass spectroscopy. This experiment is described in detail by Litvinov. 3 3 Yu. A. Litvinov et al., arxiv:0801.2079v1 Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 6 / 19

Heavy-ion production and storage Tabulated experimental parameters for all runs run ion E( 152 Sm) L( 9 Be) # inj [MeV/u] [mg/cm 2 ] 1 140 Pr 58+ 507.8 1032 453 2 140 Pr 58+ 507.8 1032 842 3 140 Pr 58+ 601.1 2513 5807 4 142 Pm 60+ 607.4 2513 7011 Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 7 / 19

Weak decay Example signal electron-capture: 140 Pr 58+ 140 Ce 58+ + ν e + KE, f 300 Hz β + decay: 142 Pm 60+ 142 Nd 59+ + e + + ν e + KE, f 150 khz Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 8 / 19

Weak decay Example signal electron-capture: 140 Pr 58+ 140 Ce 58+ + ν e + KE, f 300 Hz β + decay: 142 Pm 60+ 142 Nd 59+ + e + + ν e + KE, f 150 khz Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 8 / 19

Experimental result with 140 Pr 58+ Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 9 / 19

Experimental result with 140 Pr 58+ Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 9 / 19

Experimental result with 140 Pr 58+ Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 9 / 19

Experimental result with 140 Pr 58+ Exponential decay with a modulation at a period of 7 s. Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 9 / 19

Experimental result with 142 Pm 60+ Inset shows Fourier transform of the data showing a peak at f = 0.14 Hz again. Data with the sinusoidal fit for first 36 seconds Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 10 / 19

Experimental result Fit parameters Fit parameters of 140 Pr data Eq. N 0 λ EC λ a ω χ 2 /DoF 1 34.9(18) 0.00138(10) - - 107.2/73 2 35.4(18) 0.00147(10) 0.18(3) 0.89(1) 67.18/70 Fit parameters of 142 Pm data Eq. N 0 λ EC λ a ω χ 2 /DoF 1 46.8(40) 0.0240(42) - - 63.77/38 2 46.0(39) 0.0224(41) 0.23(4) 0.89(3) 31.82/35 Null hypothesis of pure exponential decay is excluded to 99% confidence level based on χ 2 tests. Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 11 / 19

Hypotheses: (1) technical artifact? Pro common period of 7 s for 140 Pr 58+ and 142 Pm 60+. Con apparatus sensitive to single ion Pr and Pm ions coast on different orbits in ESR uncertainty of decay time ( 1 s) less than observed period. Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 12 / 19

Hypotheses: (1) technical artifact? Pro common period of 7 s for 140 Pr 58+ and 142 Pm 60+. Con apparatus sensitive to single ion Pr and Pm ions coast on different orbits in ESR uncertainty of decay time ( 1 s) less than observed period. Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 12 / 19

Hypotheses: (2) quantum beat of hyperfine states Pro 140 Pr and 142 Pm have nuclear spin I = 1. H-like ions probably produced in coherent superposition of two 1s hyperfine states with F = 1/2 and F = 3/2. Final state (daughter ion plus ν e ) has F = 1/2. EC-decay from F = 3/2 state is not allowed. Con The well-known hyperfine splitting in hydrogen is in microwave range (ν = E/h = 1420 MHz), with period of, T = h/ E = 0.7 ns, and T for 140 Pr 58+ is even smaller by a factor of 10 5. Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 13 / 19

Hypotheses: (2) quantum beat of hyperfine states Pro 140 Pr and 142 Pm have nuclear spin I = 1. H-like ions probably produced in coherent superposition of two 1s hyperfine states with F = 1/2 and F = 3/2. Final state (daughter ion plus ν e ) has F = 1/2. EC-decay from F = 3/2 state is not allowed. Con The well-known hyperfine splitting in hydrogen is in microwave range (ν = E/h = 1420 MHz), with period of, T = h/ E = 0.7 ns, and T for 140 Pr 58+ is even smaller by a factor of 10 5. Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 13 / 19

Hypotheses: (3) neutrino oscillation Suggestive kinematic consideration For two mass eigenstates, m 1 and m 2, { E1 + p 2 1 /2M = Q EC E 2 + p 2 2 /2M = Q EC In approximation (E 1 + E 2 )/2M 1 E = E 2 E 1 = (m 2 2 m2 1 )/2M From KamLAND data 4, with M = 140 amu, E 6 10 16 ev, andt = h/e 7 s 4 Phys. Rev. Lett. 94, 081801 (2005), m 2 8 10 5 ev 2 Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 14 / 19

Hypotheses: (3) neutrino oscillation Suggestive kinematic consideration For two mass eigenstates, m 1 and m 2, { E1 + p 2 1 /2M = Q EC E 2 + p 2 2 /2M = Q EC In approximation (E 1 + E 2 )/2M 1 E = E 2 E 1 = (m 2 2 m2 1 )/2M From KamLAND data 4, with M = 140 amu, E 6 10 16 ev, andt = h/e 7 s 4 Phys. Rev. Lett. 94, 081801 (2005), m 2 8 10 5 ev 2 Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 14 / 19

Hypotheses: (3) neutrino oscillation Suggestive kinematic consideration For two mass eigenstates, m 1 and m 2, { E1 + p 2 1 /2M = Q EC E 2 + p 2 2 /2M = Q EC In approximation (E 1 + E 2 )/2M 1 E = E 2 E 1 = (m 2 2 m2 1 )/2M From KamLAND data 4, with M = 140 amu, E 6 10 16 ev, andt = h/e 7 s 4 Phys. Rev. Lett. 94, 081801 (2005), m 2 8 10 5 ev 2 Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 14 / 19

Hypotheses: (3) neutrino oscillation Suggestive kinematic consideration For two mass eigenstates, m 1 and m 2, { E1 + p 2 1 /2M = Q EC E 2 + p 2 2 /2M = Q EC In approximation (E 1 + E 2 )/2M 1 E = E 2 E 1 = (m 2 2 m2 1 )/2M From KamLAND data 4, with M = 140 amu, E 6 10 16 ev, andt = h/e 7 s 4 Phys. Rev. Lett. 94, 081801 (2005), m 2 8 10 5 ev 2 Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 14 / 19

Hypotheses: (3) neutrino oscillation Suggestive kinematic consideration For two mass eigenstates, m 1 and m 2, { E1 + p 2 1 /2M = Q EC E 2 + p 2 2 /2M = Q EC In approximation (E 1 + E 2 )/2M 1 E = E 2 E 1 = (m 2 2 m2 1 )/2M From KamLAND data 4, with M = 140 amu, E 6 10 16 ev, andt = h/e 7 s 4 Phys. Rev. Lett. 94, 081801 (2005), m 2 8 10 5 ev 2 Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 14 / 19

Neutrino oscillation, a brief introduction Predicted in 1950s and 1960s by Bruno Pontecorvo, in analogy with a similar phenomenon in neutral kaons. 5 flavor (e, µ, τ) eigenstates: ν α = i U αi ν i mass (1, 2, 3) eigenstates: ν i = α( U αi ν α ) cos θ sin θ mixing matrix for two neutrinos: U = sin θ cos θ 5 http://en.wikipedia.org/wiki/neutrino_oscillation Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 15 / 19

Neutrino oscillation, a brief introduction Predicted in 1950s and 1960s by Bruno Pontecorvo, in analogy with a similar phenomenon in neutral kaons. 5 flavor (e, µ, τ) eigenstates: ν α = i U αi ν i mass (1, 2, 3) eigenstates: ν i = α( U αi ν α ) cos θ sin θ mixing matrix for two neutrinos: U = sin θ cos θ 5 http://en.wikipedia.org/wiki/neutrino_oscillation Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 15 / 19

Neutrino oscillation, a brief introduction Predicted in 1950s and 1960s by Bruno Pontecorvo, in analogy with a similar phenomenon in neutral kaons. 5 flavor (e, µ, τ) eigenstates: ν α = i U αi ν i mass (1, 2, 3) eigenstates: ν i = α( U αi ν α ) cos θ sin θ mixing matrix for two neutrinos: U = sin θ cos θ 5 http://en.wikipedia.org/wiki/neutrino_oscillation Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 15 / 19

Neutrino oscillation, a brief introduction Predicted in 1950s and 1960s by Bruno Pontecorvo, in analogy with a similar phenomenon in neutral kaons. 5 flavor (e, µ, τ) eigenstates: ν α = i U αi ν i mass (1, 2, 3) eigenstates: ν i = α( U αi ν α ) cos θ sin θ mixing matrix for two neutrinos: U = sin θ cos θ 5 http://en.wikipedia.org/wiki/neutrino_oscillation Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 15 / 19

Neutrino oscillation, a brief introduction Predicted in 1950s and 1960s by Bruno Pontecorvo, in analogy with a similar phenomenon in neutral kaons. 5 flavor (e, µ, τ) eigenstates: ν α = i U αi ν i mass (1, 2, 3) eigenstates: ν i = α( U αi ν α ) cos θ sin θ mixing matrix for two neutrinos: U = sin θ cos θ 5 http://en.wikipedia.org/wiki/neutrino_oscillation Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 15 / 19

Decay amplitude, coherent or incoherent sum? According to Ivanov et al., 6 decay amplitude is given by, A(t) = k=1,2,3 A k (t) = k t 0 dτ I f, ν k H W (τ) I i. Giunti 7 argues that A(t) is an incoherent sum over different channels, because, ν e = Uek ν k, k and in the time-dependent perturbation theory, ν e (t) = j A j (t) 2 1/2 6 Ivanov et al. arxiv:0801.2121v1, Eq. 3, simplified 7 Giunti, arxiv:0801.4639v2 k A k (t) ν k. Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 16 / 19

Decay amplitude, coherent or incoherent sum? According to Ivanov et al., 6 decay amplitude is given by, A(t) = k=1,2,3 A k (t) = k t 0 dτ I f, ν k H W (τ) I i. Giunti 7 argues that A(t) is an incoherent sum over different channels, because, ν e = Uek ν k, k and in the time-dependent perturbation theory, ν e (t) = j A j (t) 2 1/2 6 Ivanov et al. arxiv:0801.2121v1, Eq. 3, simplified 7 Giunti, arxiv:0801.4639v2 k A k (t) ν k. Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 16 / 19

Decay amplitude, coherent or incoherent sum? According to Ivanov et al., 6 decay amplitude is given by, A(t) = k=1,2,3 A k (t) = k t 0 dτ I f, ν k H W (τ) I i. Giunti 7 argues that A(t) is an incoherent sum over different channels, because, ν e = Uek ν k, k and in the time-dependent perturbation theory, ν e (t) = j A j (t) 2 1/2 6 Ivanov et al. arxiv:0801.2121v1, Eq. 3, simplified 7 Giunti, arxiv:0801.4639v2 k A k (t) ν k. Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 16 / 19

Analogy: double-slit interference Lipkin 8 asserts that coherence results from uncertainty relationship (localized ion, finite momentum uncertainty). 8 Lipkin, arxiv:0801.1465v2 Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 17 / 19

Analogy: double-slit interference Lipkin 8 asserts that coherence results from uncertainty relationship (localized ion, finite momentum uncertainty). 8 Lipkin, arxiv:0801.1465v2 Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 17 / 19

Analogy: double-slit interference Lipkin 8 asserts that coherence results from uncertainty relationship (localized ion, finite momentum uncertainty). 8 Lipkin, arxiv:0801.1465v2 Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 17 / 19

Analogy: double-slit interference Lipkin 8 asserts that coherence results from uncertainty relationship (localized ion, finite momentum uncertainty). 8 Lipkin, arxiv:0801.1465v2 Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 17 / 19

Prospects Experimental verification It is obvious that our findings must be corroborated by the study of other two-body beta decays (EC and β b ). 9 A similar analysis can be applied to a K-capture experiment... Here there are a number of initial states having different degrees of ionization. Interference can only occur between initial states having the same degree of ionization. Otherwise the analysis is the same. 10 New method for studying neutrino mixing If the effect is real and realistic theoretical model can be set up, this is a new method to study neutrino oscillation without the need to directly detect neutrinos. 9 Yu. A. Litvinov et al., arxiv:0801.2079v1 10 Lipkin, arxiv:0801.1465v2 Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 18 / 19

References Litvinov, et al., Observation of non-exponential orbital electron capture decays of hydrogen-like 140 Pr and 142 Pm ions, http://arxiv.org/abs/0801.2079v1 Ivanov, et al., On the time-modulation of the K-shell electron capture decay of H-like 140 Pr 58+ ions produced by neutrino-flavour mixing, http://arxiv.org/abs/0801.2121v1 Giunti, C., Comment on the neutrino-mixing interpretation of the GSI time anomaly, http://arxiv.org/abs/0801.4639v2 (Note: this comment refers to arxiv:0801.1465v1.) Lipkin, H. J., New method for studying neutrino mixing and mass differences, http://arxiv.org/abs/0801.1465v2 Byung Kyu Park (UC Berkeley) Time-modulation of EC decay Physics 250 March 20, 2008 19 / 19