Spin excitations of a ferromagnetic wire with a magnetic domain wall
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1 26 February 2001 Physics etters A 280 (2001) pin excitations of a ferromagnetic wire with a magnetic domain wall Atsunobu Nakamura a,, hinji Nonoyama b a Department of Physics, Anan College of Technology, Anan, Tokushima , Japan b Faculty of Education, Yamagata University, Yamagata , Japan Received 3 November 2000; accepted 15 January 2001 Communicated by.j. ham Abstract The spin excitation for a ferromagnetic wire with a domain wall (D) is studied in a framework of the random phase approximation. e show that the excitation energy due to the D is much smaller than that for the spin wave. In the spin-wave spectrum, there are lots of peaks or shoulders, which is related to the existence of the D and the dimension of the leads. Using the results, the energy dissipation of conduction electrons is also discussed Elsevier cience B.V. All rights reserved. PAC: r; Fk; Ds; d Keywords: Ferromagnetic wire; Mesoscopic system; Domain wall; Elementary excitations Recent advances in the microprocessing technology enable us to fabricate ferromagnetic metals with various sample structures on nanometer scale. In these mesoscopic metals, the interplay between the electron transport and the magnetic object including domain walls (Ds) has become one of the subjects of current interest. In particular, a D nucleation and dynamics are examined experimentally using a magnetoresistance (MR) in thin films and nanowires [1 6]. Ever since the first experiment on the electrical resistivity due to the D in ferromagnetic Ni and Fe wires [1], the negative MR effect has been reported by many researchers [3 5]. Opposed to those findings, a positive contribution of the D scattering to the resistance are reported for an experiment in Co thin films [6]. In order to explain such features, theoretical approaches * Corresponding author. address: anakamur@anan-nct.ac.jp (A. Nakamura). have been done actively by many authors [4,7 11]. Furthermore, over the past years, the conductance in atomic-scale contacts has also been studied in the experiments [12 14] and simulations [15 19]. hen magnetic metals are used [13], the spin fluctuation at the very narrow constriction is expected to affect the quantied conductivity. o that it is considered to be important for us to examine the behavior of spins of the mesoscopic or atomic sie in the vicinity of ad. Many theoretical works on the spin excitations around a D have been performed for Heisenbergtype models without taking sample structures into consideration [20 25]. In this etter, to understand basic features of a magnetic wire of sample structures used in measurements, we calculate the excitation spectrum for the spin fluctuation laying stress on the presence of a D. e present the method to obtain the Green function for the magnetic wire in a framework of the random phase approximation (RPA) /01/$ see front matter 2001 Elsevier cience B.V. All rights reserved. PII: (01)
2 228 A. Nakamura,. Nonoyama / Physics etters A 280 (2001) Fig. 1. chematic illustration of the system. The wire in the region II (1 n N)connects to the left (region I, n 0) and the right (region III, N + 1 n) leads. pins of the left (right) side are up (down) and a magnetic D exists at the center of the wire. e consider a ferromagnetic spin system as illustrated in Fig. 1, where a magnetic wire described by an one-dimensional (1D) Heisenberg model (region II) connects to left and right leads described by two-dimensional (2D) Heisenberg models (regions I and III). The Hamiltonian is given by H spin = H 2J 0,0 1 + H 2J R N N+1,0 + H R, (1) N 1 H = 2J n n A H = 2J 2J 1 2 A n=1 n 1,m n 0,m n 0,m n,m n+1,m n,m n,m+1 ( n,m ) 2, N ( ) 2, n n=1 (2) (3) where H and H are the Hamiltonians for the wire and the left lead, respectively. The Hamiltonian for the right lead H R is written down in the same manner of H. The spin sites in the 1D wire are labeled with the coordinate 1 n N. Those in the 2D left (right) lead are labeled with the coordinate n 0 (N + 1 n) and <m<+ (see Fig. 1). n ( n,m ) is the spin operator at the nth site of the wire ((n, m) of the leads). The quantities J and A (J and A ) are the exchange integral and the anisotropy energy for the wire (left lead), respectively. The exchange integrals between the spins at the junctions are J and J R. e choose the -direction as the uniaxial magnetocrystalline easy axis, which is parallel to the wire. For simplicity, the exchange integral, the anisotropy energy and the easy axis do not vary for whole region, i.e., J = J = J = J R = J and A = A = A. The present method can be extended easily to other parameter regions. In order to discuss the spin fluctuation of the system, we calculate the retarded Green function χ (l) (t) = iθ(t) [ + (t), ( ) l ], with being a thermal average and θ(t) being a step function. ince the wire interacts with each lead only through the junction sites (0, 0) and (N + 1, 0), the matrix χ (l) (t) should be treated by dividing into three sub-matrices, i.e., a submatrix for the left lead χ (l), that for the right lead, and that for the wire and those junction sites χ (l) R χ (l). e solve these matrices of Green functions selfconsistently so as to continue at the junction sites. Using the RPA method, χ (l) can be expressed as a
3 A. Nakamura,. Nonoyama / Physics etters A 280 (2001) Dyson-type equation: n χ (l) (ω) n = g n (l) (ω)δ nn + N+1 n =0 g n (l) (ω)v nn n (l) χ (ω) n. (4) Here χ (l) (l) (ω) is a Fourier transform of χ (t) and we use a simplified suffix; n = 0, 1 mean the junction sites (0, 0) and (N + 1, 0), respectively. The non-ero elements of g (l) (ω) and V are as follows: 0, 0 χ (l) (ω) 0, 0, n= 0, g n (l) (ω) = α n (l) /(ω A n ), 1 n N, (5) N + 1, 0 χ (l) R (ω) N + 1, 0 n = N + 1, J, n = n ± 1, J 1 / 0,0, n= n = 0, V nn = J j=±1 n+j / n, n = n, 1 n N, J N / N+1,0, n= n = N + 1, (6) where α n (l) = [ n +,( n )l n ]. The Green function matrix for the left lead χ (l) (ω) is calculated as χ (l) (ω) = g(l) (ω) + g(l) (ω)v χ (l) (ω), (7) n, m g (l) (ω) ) n, m = α (l) n,m/( ω A n,m, (8) n, m V n, m = J / n,m n,m, (9) where means a summation of (n,m ) over the neighboring sites of (n, m) inside the left lead. The off-diagonal matrix elements n, m V n,m = J when (n,m )-site is a neighbor of (n, m). The Green function of the right lead χ (l) R (ω) is evaluated in the same manner. The Green functions for the whole system are calculated self-consistently these equations and the spectrum theorem + ( ) l n n n + = ( 1/π) Im n (l) χ (ω) n f B (ω) dω, (10) where f B (ω) = 1/[exp(ω/T) 1] with T being a temperature. The spectrum theorem for the leads can also be written in the same form. Here, we describe the calculation briefly. e are interested in the spin fluctuation in the vicinity of a magnetic D in the wire, which comes out of the boundary condition that spins in the left lead are up and those in the right lead are down ( n,m for n ± ; see Fig. 1). To solve the equations, we use an approximation that the thermal average of all spins in each lead is the same as that of the bulk. For the left lead, averaged values in the bulk are obtained by π π ( ) l B B + α (l) [ B = B π 2 dk x dk y f B εb (k x,k y ) ], 0 0 (11) where ε B (k x,k y ) = 4J B [2 cos k x cos k y ]+ A B. This simplicity is not essential in the following calculation and discussion for the wire when the width of the D (λ D ) is less than the length of the wire. By solving Eqs. (4) (10) self-consistently, we can obtain the Green function of the wire χ (l) (),whichis an analytic continuation of χ (l) (ω). Then the Green function has two poles and two cuts on the real axis [20], which can be expressed in a form n χ (l) (ω) n = r(l) nn + + E D + D r(l)+ nn E D ρ (l) nn (ω) ω dω. (12) The domain of integration D is E 1 < ω <E 2,where E 1 = A B and E 2 = E J B.Thenρ(l) nn (ω) is an excitation spectrum of the spin wave in the wire with a D. On the other hand, the poles = ±E D, which lie in the gap of the spin-wave spectrum (E D <E 1 ), correspond to the excitation energy based on the local spin fluctuation around the D. Because the poles do not come out in the case where a D does not exist in the wire. It is considered that the spins in the D can flip with a small energy ( E D ) compared to that in the ferromagnetic ordered state ( E 1 ),since n reduces effectively around the D. In the following, we consider the case of = 1. Then it is adequate to evaluate above equations for l = 0, 1. In Fig. 2, we show the spin distribution n and (n )2 of the wire. The site number of the wire
4 230 A. Nakamura,. Nonoyama / Physics etters A 280 (2001) Fig. 2. Calculated spin distribution (a) n and (b) ( n) 2 of the wire for N = 50 at T = 0. The anisotropy energy A/J equals 0.2 (solid line) and 0.4 (dashed). The vertical line is the center of the wire (N/ ). Fig. 3. Calculated residues (a) r nn (0)± and (b) r nn (1)± ±E D of the Green functions. at the poles N equals 50 throughout this etter. The center of the wire is expressed as a vertical line, where n =0and (n )2 =1/3. From these figures it is seen that λ D is sufficiently small compared to the length of the wire for these parameters. Fig. 3 shows the residues r nn (l)± ineq.(12).itis seen that the quantities r nn (l)± do not have any symmetry around the center (vertical line). The excitation spectrum of the spin wave ρ nn (0) (ω) in the vicinity of the D is shown in Fig. 4. The spectrum for just left site of the D (n = 25) concentrates around ω 0(but ω E 1 ). As the distance between the site and the center of the D increases, the spectrum in ω< E 1 disappears while that in ω>e 1 grows. This corresponds to that the spin fluctuation of up down up becomes dominant as the site index n decreased in the left side of the wire. As a remarkable feature in Fig. 4, we can see a lot of peaks, the number of which is (N 2)/2 inω>e 1. Moreover, we can see (n 25) humps in the envelope of peaks (dotted lines), except for n = 25. Note that, when leads are 1D spin systems, the spectrum curve at each site is similar to the envelope of peaks in Fig. 4. Fig. 5(a) shows the ex- citation spectrum of n = 10. Around the site, the spins are up (see Fig. 2). The dotted line denotes the spectrum for the ferromagnetically ordered 1D spin chain. The difference of the spectra is caused by the existence of the D and the difference of the dimension of the leads. The spectra at the junction sites n = 1, 0 are shown in Figs. 5(b) and (c). For n = 0 the spectrum spread over E 1 <ω<e 2, since the n = 0 site is inside the left 2D lead. The feature can be seen slightly in Fig. 5(b) for n = 1. The dashed line in Fig. 5(c) denotes the spectrum at the surface site of the 2D lead when the wire does not connect with the 2D lead. This spectrum has no symmetry, because the lead is a half-plane. In Figs. 4 and 5, the energies at peaks and shoulders are the same values. From these results, it is considered that the discrete excitation energies for the isolated wire consisting of finite number of sites are smeared due to the resonance with the 2D leads consisting of infinite number of sites through the junction sites. These features can be also seen in the spectrum of ρ nn (1) (ω). Next, we discuss the energy E D in Eq. (12), which can be regarded as a characteristic energy of the spin fluctuation due to the D. Fig. 6 shows the tempera-
5 A. Nakamura,. Nonoyama / Physics etters A 280 (2001) Fig. 4. Excitation spectra for the spin wave at the sites (a) n = 25 ( just left of D), (b) n = 23, and (c) n = 21 for A/J = 0.2 and N = 50 at T = 0. The dotted lines in (b) and (c) are the envelopes of peaks. ture dependence of E D. It is seen that E D is much smaller than the excitation energy of the spin wave (E D E 1 /20 for A/J = 0.2 att = 0). Though E D increases monotonically as the temperature increases, E D E 1 /10 even at T/J = Using these results, we discuss the spin-flip scattering of conduction electrons by introducing an interaction term such as H int = J int (c n c n n + h.c.), wherec nσ is an annihilation operator of the conduction electron with spin σ on nth site. According to the fluctuation dissipation theorem, the local spin fluctuation with energy E D plays a crucial role for the energy dissipation of the conduction electron. Moreover, the results of Fig. 3 indicates that the maximum position of the energy dissipation due to the D shifts slightly from the center of the D. Note that the D contribution to the resistivity is positive for the present model. To elucidate the negative MR, we must take other mechanisms into consideration, such as an interaction between a D and impurities [7,8]. Fig. 5. Excitation spectra for the spin wave at the sites (a) n = 10 (up spin regime), (b) n = 1, and (c) n = 0forA/J = 0.2 andn = 50 at T = 0. The dotted line in (a) is the well-known spectrum for a ferromagnetically ordered 1D spin chain. The dashed line in (c) denote the spectrum at the surface site of the 2D lead without a connection with the wire. Fig. 6. Temperature dependence of E D for A/J =0.2 (solid line) and 0.4 (dotted) for N = 50. In summary, we have presented the method to calculate the Green function for the spin system with a D in a framework of RPA and discussed the elementary excitations. e have shown that the spinwave spectrum of the wire has lots of peaks and
6 232 A. Nakamura,. Nonoyama / Physics etters A 280 (2001) shoulders, which is related to the existence of the D and the dimension of leads. It is also shown that the excitation energy due to the D is much smaller than that for the spin-wave excitation. The effects of the spin system on the conductance can be evaluated with the use of obtained spectrum, the results of which will be published elsewhere. The results are regarded as a base for more improved calculations and the method presented here can be easily extended to other spin systems. Acknowledgements The authors thank the Computation Center of Nagoya University, Institute for olid tate Physics of University of Tokyo, Institute for Molecular cience, and Yukawa Institute for the facilities and the use of supercomputers. e thank T. Koma and M. Yamanaka for useful discussions. References [1] K. Hong, N. Giordano, Phys. Rev. B 51 (1995) 9855; K. Hong, N. Giordano, J. Magn. Magn. Mater. 151 (1995) 396. [2] M. Viret, D. Vignoles, D. Cole, J.M.D. Coey,. Allen, D.. Daniel, J.F. Gregg, Phys. Rev. B 53 (1996) [3] Y. Otani, K. Fukamichi, O. Kitakami, Y. himada, B. Pannetier, J.P. Noieres, T. Matsuda, A. Tonomura, in: Proc. MR pring Meeting, an Francisco, Vol. 475, 1997, p. 215; Y. Otani, K. Fukamichi, O. Kitakami, Y. himada, B. Pannetier, J.P. Noieres, T. Matsuda, A. Tonomura, IEEE Trans. Magn. 34 (1998) [4] U. Rüdiger, J. Yu,. Zhang, A.D. Kent,..P. Parkin, Phys. Rev. ett. 80 (1998) 5639; U. Rüdiger, J. Yu,. Zhang, A.D. Kent,..P. Parkin, J. Magn. Magn. Mater (1999) 261. [5] T. Taniyama, I. Nakatani, T. Namikawa, Y. Yamaaki, Phys. Rev. ett. 82 (1999) 2780; T. Taniyama, I. Nakatani, T. Namikawa, Y. Yamaaki, J. Magn. Magn. Mater (1999) 77. [6] J.F. Gregg,. Allen, K. Ounadjela, M. Viret, M. Hehn,.M. Thompson, J.M.D. Coey, Phys. Rev. ett. 77 (1996) [7] G. Tatara, H. Fukuyama, Phys. Rev. ett. 78 (1997) [8] Y. yanda-geller, I.. Aleiner, P.M. Goldbart, Phys. Rev. ett. 81 (1997) [9] P.M. evy,. Zhang, Phys. Rev. ett. 79 (1997) [10] M. Yamanaka, T. Koma, J. Magn. oc. Jpn. 23 (1999) 141. [11] G.G. Cabrera,.M. Falicov, Phys. tatus olidi B 61 (1974) 539; G.G. Cabrera,.M. Falicov, Phys. tatus olidi B 62 (1974) 217. [12] J.M. Krans, C.J. Muller, I.K. Yanson, Th.C.M. Govaert, R. Hesper, J.M. van Ruitenbeek, Phys. Rev. B 48 (1993) [13]. Olesen, E. ægsgaard, I. tensgaard, F. Besenbacher, J. chiøt, P. tolte, K.. Jacobsen, J.K. Nørskov, Phys. Rev. ett. 72 (1994) [14] G. Rubio, N. Agraït,. Vieira, Phys. Rev. ett. 76 (1996) [15] T.N. Todorov, A.P. utton, Phys. Rev. ett. 70 (1993) [16] J.A. Torres, J.J. áen, Phys. Rev. ett. 77 (1996) [17] R.N. Barnett, U. andman, Nature (ondon) 387 (1997) 788. [18] M. Brandbyge, M.R. ørensen, K.. Jacobsen, Phys. Rev. B 56 (1997) [19] A. Nakamura, M. Brandbyge,.B. Hansen, K.. Jacobsen, Phys. Rev. ett. 82 (1999) [20] J.M. inter, Phys. Rev. 124 (1961) 452. [21] A. Pawlikowski, Acta Phys. Polon. 27 (1965) 545. [22] A. Antoulas, R. chilling,. Baltensperger, olid tate Commun. 18 (1976) [23] R. chilling, Phys. Rev. B 15 (1977) [24] G.T. Cantieni, R. chilling, J. Phys. C 13 (1980) [25] Y. Takane, Y. Isawa, J. Phys. oc. Jpn. 69 (2000) 3170.
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