Fundamental Neutron Physics II. Fundamental Neutron Physics III

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Fundamental Neutron Physics II Neutron Sources and Neutron Beams Fundamental Neutron Physics III Neutron Beta Decay Geoffrey Greene University of Tennessee / Oak Ridge National Laboratory 1

Introduction to Neutron Sources Early neutron sources were based on simple nuclear processes: α+ 9 12 Be C + n Such sources are still used ( Pu-Be ) but are limited in intensity. Modern neutron research is based at sources of two types: 1. High Flux Fission Reactor 2. Accelerator Spallation Sources 2

The Fission Reactor 3

Enrico Fermi Leo Szilard 4

Each Fission Event Produces ~200Mev and ~1.5 Useful Neutrons 5

Some Essential Features of a High Flux Reactor Figure of Merit is the Peak Neutron Flux at the Core n/cm 2 /s Key Design Features: 1. High Power Density 2. Compact Core 3. Highly Enriched Fuel 4. D 2 0 Moderation and Cooling 5. Cryogenic Cold Source(s) 6 Ultimate engineering limitation is ability to remove heat from the compact core at ~100MW

The Institute Laue Langevin, Grenoble 57 MW High Flux Reactor 7

8

Most Neutron Sources Have Multiple Moderators 9 The High Flux neutron Source at the ILL

A Neutron Source Can Serve Many Neutron Instruments 10 Instrument Layout at the Institut Laue Langevin

The Guide Hall at the ILL Houses ~30 Neutron Spectrometers 11

The NIST High Flux Reactor 12

The NIST Cold Neutron research Center 13

The NIST Cold Neutron research Center NEW EXPT. HALL 14

Spallation Sources 15

At ~1.4 GeV, Each Incident Proton Produce ~40 Useful Neutrons

Neutron Production is Roughly Proportional to Power 100 LOW-ENERGY (< 20 MeV) NEUTRONS PER INCIDENT PROTON 80 60 40 20 total spallation/high-energy fission (n,xn) 0 0 500 1000 1500 2000 2500 PROTON ENERGY (MeV) NOTE: Spallation gives ~x10 more neutrons per MW 17 (Courtesy,Gary Russell)

The Spallation Neutron Spectrum is Broad (Courtesy,Gary Russell)

Moderators are Engineered for Specific Neutronic Performance WING P P SLAB TRANSMISSION/TRANSMISSION P FLUX-TRAP/SOLID TARGET TRANSMISSION/TRANSMISSION P FLUX-TRAP/SPLIT TARGET TRANSMISSION/TRANSMISSION P FLUX-TRAP/SOLID TARGET TRANSMISSION/BACKSCATTERING P FLUX-TRAP/SPLIT TARGET TRANSMISSION//BACKSCATTERING (Courtesy,Gary Russell)

Neutron Source Intensities Have Increased by Nearly 18 Orders of Magnitude* Since Chadwick 20

The Spallation Neutron Source

Target, Reflectors, and Moderators Cryogenic H 2 moderators Be reflector Proton Beam Ambient H 2 0 moderator Mercury target Steel reflector

Target-Moderator System

Beamline 13 Has Been Allocated for Nuclear Physics 11A - Powder Diffractometer Commission 2007 9 VISION 7 - Engineering Diffractometer IDT CFI Funded Commission 2008 12 - Single Crystal Diffractometer Commission 2009 6 - SANS Commission 2007 13 - Fundamental Physics Beamline Commission 2007 14B - Hybrid Spectrometer Commission 2011 15 Spin Echo 5 - Cold Neutron Chopper Spectrometer Commission 2007 4B - Liquids Reflectometer Commission 2006 4A - Magnetism Reflectometer Commission 2006 17 - High Resolution Chopper Spectrometer Commission 2008 18 - Wide Angle Chopper Spectrometer Commission 2007 1B - Disordered Mat ls Commission 2010 2 - Backscattering Spectrometer Commission 2006 3 - High Pressure Diffractometer Commission 2008

Beamline 13 Has Been Allocated for Nuclear Physics 11A - Powder Diffractometer Commission 2007 9 VISION 7 - Engineering Diffractometer IDT CFI Funded Commission 2008 12 - Single Crystal Diffractometer Commission 2009 6 - SANS Commission 2007 13 - Fundamental Physics Beamline Commission 2007 5 - Cold Neutron Chopper Spectrometer Commission 2007 14B - Hybrid Spectrometer Commission 2011 15 Spin Echo 4B - Liquids Reflectometer Commission 2006 4A - Magnetism Reflectometer Commission 2006 Neutrino Detector Here 17 - High Resolution Chopper Spectrometer Commission 2008 18 - Wide Angle Chopper Spectrometer Commission 2007 1B - Disordered Mat ls Commission 2010 2 - Backscattering Spectrometer Commission 2006 3 - High Pressure Diffractometer Commission 2008

Neutron Guides 30

At low energies S-wave scattering dominates, phase shift is given by cot( δ ) b coh b coh critical range for b coh <0 = 1 kb coh For most nuclear well depths and well sizes, it is unlikely to obtain a positive coherent scattering length: n = 1 N λ coh 2 b π Index of refraction is therefore <1 for most nuclei * *In the vicinity of A~50 (V,Ti,Mn) nuclear sizes are such that b coh <1 and thus n>1 31

n 2 Neutron Reflection from Matter 2 λ Nbcoh = 1 cosθ crit = n 2π Neutrons will undergo complete external reflection from a polished surface for most materials Ni or 58 Ni are particularly useful as a neutron mirror material 3 θ ( ) 1.7x10 crit Ni λ( Angstrom) For most neutron beams this means θ crit 10 2 32

Guide Section from SNS

Neutron Guides can be used to Focus Neutron Beams 34 Photo: Swiss Neutronics

Large Cross Section Guides are Commercially Available Prototype Guide for SNS Ultracold Beam

Neutron Guide Installation at LANSCE 36 Photo: LANSCE

A Single Moderator can Feed Multiple Neutron Guides 37 Photo: Institut Laue Langevin

Reflectivity of Neutron Mirror A Simple Neutron Mirror has Nearly Unit Reflectivity Up to a Maximum Critical Angle 1 Reflectivity n θ θ critical Angle Θ critical 2 mr/å for 58 Ni 38

The Supermirror Extends the Effective θ critical Commercial Supermirror Neutron Guides are Available With m 3-4 1 ~ 1000 layers Reflectivity θ critical mθ critical Angle NOTE: Flux scales as Square of Critical Angle 39

Commercial Supermirrors are available with m~4 Note that the number of layers scales as ~m 4 100 80 070223-A/7 m35.min Reflectivity (%) 60 40 20 0 0 1 2 3 4 m 40 Data: Mirrotron

Neutron Polarization 41

Neutron Polarization by Mirror Reflection For a magnetic material, the index of refraction includes an additional spin dependent term: n = Nb π µ B 2π h coh 2 1 ± λ 2 2 For a judicious selection of material (~60% Fe-40% Co at saturation works quite well) it is possible to have n=1 for one state and n<1 for the other. The reflected (or transmitted beam from such a mirror will be polarized) 42

Mirror Polarizers are Usually Configured as Multi-Channel Benders Photo: Swiss Neutronics 43

Some Advantages of Magnetic Supermirror Reflection Polarizers: High Polarization ~99% Simple to Use Commercially Available Highly Reliable Some Disadvantages of Magnetic Supermirror Reflection Polarizers: Challenging to Accurately Determine Polarization Limited Range of Neutron Energies Beam is Deflected Photo: Swiss Neutronics 44

Spin Polarized 3 He Works as a Neutron Spin Filter n + 3 He 3 H + p σ J=0 = 5300 barn at v 0 =2200 m/s σ J=1 0 For low energy neutron there is essentially NO capture in the triplet state An un-polarized neutron beam incident on a Polarized 3 He Target yields a polarized neutron beam. 45

Accurate Absolute Determination of Polarization Neutron polarization depends upon thickness of cell, pressure in cell, 3He polarization, etc. which are hard to measure to high accuracy P n = σ tanh ρ He dp He 2 However, the neutron transmission depends on the same parameters: T n σ = cosh ρ He dp He 2 The application of a few hyperbolic trigonometric identities provides a greatly simplified relation for the neutron polarization that is based only on (relatively) easy to measure neutron transmission: P n = T 1 2 0 T 2 Where T 0 is the transmission through the cell when unpolarized and T is the transmission when the cell is polarized. 46 Greene, Thompson, Dewey, NIM 356, 177, (1995)

3 He Neutron Polarizer for n+p d + γ Experiment 3He Optical Pumping Cell 3He Cell in Oven 47 Polarizer System on Beamline at LANSCE

Ultra Cold Neutrons *see Golub, Richardson, Lamoreaux, Ultracold Neutrons 48

Neutron Index of Refraction n 2 2 λ Nbcoh = 1 cosϕ crit = n 2π For sufficiently large neutron wavelength, λ, n=0 and cosφ crit =90 This implies that neutrons will be reflected at all angles and can be confined in a bottle 49 These are known as Ultracold Neutrons.

Ultracold Neutron Energies are Very Low The Fermi Pseudo-Potential the most advantageous materials is ~ 100 nev This corresponds to a: Neutron Velocity Neutron Wavelength Magnetic Moment Interaction Gravitational Interaction 500 m/s 500 Å µ n B 100 nev for B~1Tesla m n gh 100 nev for h~1 m Ultracold Neutron can be trapped in material, magnetic, or gravitational bottles 50

A Thermal Source of UCN* 2 2 In thermal equilibrium: ρ 2Φ v v () v dv e dv 0 α 2 = 2 α α α 2k T α B n 0 m Φ is total thermal flux For a maximum UCN energy V: ρ UCN = 2 3 Φ 0 α V k B T n 3 2 For T~300k, α~2.2x10 5 cm/s, and V~ 250 nev: ρ UCN = 13 10 Φ0cm 3 The most intense neutron sources in the world (HFIR at ORNL or ILL) have Φ 0 ~10 15 n/cm 2 /s So: ρ UCN 100cm 3 51 *see Golub, Richardson, Lamoreaux, Ultracold Neutrons

Limits to Thermal UCN Production In thermal equilibrium: ρ UCN = 2 3 Φ 0 α V k B T n 3 2 Increase the Flux Φ 0 : Reactors are at the practical limit of heat transfer. Only practical hope would be a 10-20 MW Spallation Source. Lower the temperature T n (also reduces α): Practical limit for true moderator is about 20k which gives a density increase of ~x20 Practical Thermal Source Limit for UCN production: 52 ρ UCN 2 10 3 cm 3

Limits to Thermal UCN Production In thermal equilibrium: = 2 3 Φ 0 α Increase the Flux Φ 0 : Reactors are at the practical limit of heat transfer. Only practical hope would be a 10-20 MW Spallation Source. Lower the temperature T n (also reduces α): ρ UCN V k B T n 3 2 Practical limit for true moderator is about 20k which gives a density increase of ~x20 Practical Thermal Source Limit for UCN production: ρ UCN 2 10 3 cm 3 53

Super Thermal Source of UCN Neutrons of energy E 0.95 mev (11 k or 0.89 nm) can scatter in liquid helium to near rest by emission of a single phonon. Upscattering by absorption of an 11 k phonon is a UCN loss mechanism. But population of 11 K phonons is suppressed by a large Boltzman Factor: ~ e 11/T 54 where T~200 mk Golub and Pendlebury (1977)

Fundamental Neutron Physics III Neutron Beta Decay Geoffrey Greene University of Tennessee / Oak Ridge National Laboratory 55

Neutron Beta Decay 56

Historical Digression 1934 Chadwick and Goldhaber make the first precision measurement of the neutron mass by looking at the photo-disassociation of the deuteron h ν + + 2 2 0 1D 1H 1n Using 2.62MeV gammas from Thorium and determining the recoil energy of the protons they we re able to determine*: M n = 1.0080 ± 0.0005 M n > M p + M e It is energetically possible for a neutron to decay to e + p *Chadwick and Goldhaber, Nature, 134 237 (1934) 57

1930 Pauli proposes the neutrino to explain apparent energy and angular momentum non-conservation in beta decay Wolfgang Pauli 1934 Fermi takes the neutrino idea seriously and develops his theory of beta decay Enrico Fermi 1935 The β decay of the neutron is predicted by Chadwick and Goldhaber based on their observation that M n >M p +M e. Based on this M, the neutron lifetime is estimated at ~½ hr. 1948 Snell and Miller observe neutron decay at Oak Ridge 1951 Robson makes the first measurement of the neutron lifetime 58

Fermi s View of Neutron Decay: Modern View of Neutron Decay: 59

Processes with the same Feynman Diagram as Neutron Decay After 60 D. Dubbers

Introduction to Big-Bang Nucleosynthesis 61

The Later Big Bang Time Since Big Bang Temp 0.01s 10 11 K Era of Nuclear Physics At this temperature, only familiar nuclear physics particles are present, the density is well below nuclear densities, and only well understood processes are relevant. Neutrons and Protons are in thermal equilibrium through the processes: ν e + n p + + e - e + + n p + + ν e 62 N ( mn mp ) n kt N p = e

The Later Big Bang Time Since Big Bang Temp 1s 10 10 K Neutrinos decouple Neutrino cross-sections are highly energy dependent and at this energy they become so small that neutrino scattering is insignificant. Thermal equilibrium between neutron and protons is no longer maintained. N N If nothing else happened ALL the neutrons would decay via n p 1 3 n p + + e +ν 63 and the universe would be end up with only protons (Hydrogen)

Big Bang Nucleosynthesis Time Since Big Bang Temp 3 min 10 9 K Nucleosynthesis Begins Nuclei are now stable against photo disassociation e.g. n + p d + γ and nuclei are quickly formed. The Universe is now ~87% protons & 13% neutrons 3½ min 10 8 K Nucleosynthesis Ends Neutrons are all used up making 4 He and the Universe is now has ~80% H and ~20% He. 64

Some of the Reactions in Big Bang Nucleosynthesis 65 n p + e + ν p + n d + γ 3 p + D He + γ 3 D + D He + n D + D T + p D + T 4 He + n 3 D+ He He + p 3 3 4 He+ He He + 2 p..... N n = N 0 e t /τ n Disassociation Energy 2.2MeV

Some of the Reactions in Big Bang Nucleosynthesis 66

67 Burles et al. 1999

The Cosmic He/H Ratio Depends upon three quantities: 1) The Cooling rate of the Universe Given by the heat capacity of the Universe Determined mainly by the number of light particles (m 1 MeV ) Includes photons, electrons (positrons), neutrinos (x3) 2) The Rate at which Neutrons are decaying The neutron lifetime 3) The rate at which nuclear interactions occur Determined by the the logarithm of the density of nucleons (baryons)* *Because of expansion, the absolute baryon density is decreasing with time so the density is scaled as the ratio of matter to photons. 68

69 The Parameters of Big Bang Nucleosynthesis Y 0.264 + 0.023log η 10 + 0.018( τ p = n 10.28) Cosmic Helium Abundance Neutron Lifetime in Minutes Cosmic Baryon Density

We can invert this line of reasoning. If we measure the Helium Abundance and the Neutron Lifetime, we can determine the density of ordinary matter in the universe. log [ 0.264 Y + 0.018( 10.28 )]/ 0. 023 η Cosmic Baryon Density 10 = P τ n Cosmic Helium Abundance Neutron Lifetime in Minutes 70

A Brief Digression on the Mass of the Universe From Big Bang Nucleosynthesis, we conclude that, averaged over the entire universe today, after expansion, there are a few protons per cubic meter. 71

A Brief Digression on the Mass of the Universe From Big Bang Nucleosynthesis, we conclude that, averaged over the entire universe today, after expansion, there are a few protons per cubic meter. Is this a lot, or this it a little? 72

A Brief Digression on the Mass of the Universe From Big Bang Nucleosynthesis, we conclude that, averaged over the entire universe today, after expansion, there are a few protons per cubic meter. Is this a lot, or this it a little? Compared to What? 73

A Scale for the Density of the Universe From red-shift observations we know that the Universe is in a state of (nearly) uniform expansion. If the density of the Universe is sufficiently high, this expansion will come to a stop and a universal collapse will ensue. If the density of the Universe is sufficiently low, it will expand forever. The critical density of the universe is given by the Hubble constant H, and the Gravitational constant G ρ = critical We define: 8π G 3 H Ω = ρ / ρ critical 2 74

A Lower Limit for Ω By simply counting the number of visible stars and galaxies we find 0.005 Ω total From extremely simple reasoning we have: 0.005 Ω total 2.5 75

Ω is NOT necessarily constant over time If Ω >1 at any time, Then Ω will continue to grow larger with time. If Ω <1 at any time, Then Ω will tend toward zero with time. Only if Ω = 1 EXACTLY, will it stay constant for all time We observe that Ω is NOW not too far from 1 (0.01 < Ω < 2.5). Thus: Ω was EXTREMELY close to 1 early in the big bang ( Ω-1 10-16 ) This raises the Fine Tuning question: If Ω is very nearly equal to 1, is it exactly 1? For a many compelling reasons ( fine tuning, inflation, microwave background, ),We strongly believe that 76 Ω Total = 1

Big Bang Nucleosynthesis provides a determination of the Cosmic Baryon Density: ρ ΩB ρ Baryon critical Ω B = ( 3.3 ± 0.7)% BBN This can be compared with the determination from the Cosmic Microwave Background: Ω B = ( 2.3 ± 0.1)% CMB The largest uncertainty to the nuclear theory of Big Bang nucleosynthesis is the experimental value of the neutron lifetime. 77