Search for double electron capture on 124 Xe with the XMASS-I detector

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Search for double electron capture on 124 Xe with the XMASS-I detector KATSUKI HIRAIDE (ICRR, THE UNIVERSITY OF TOKYO) SEPTEMBER 7 TH, 2015 TAUP2015 1

124 Xe 2n double electron capture Natural xenon contains double electron capture nuclei as well as double beta decay nuclei Isotope Natural abundance 124 Xe 0.095% 126 Xe 0.089% 128 Xe 1.9% 129 Xe 26.4% 130 Xe 4.1% 131 Xe 21.2% 132 Xe 26.9% 134 Xe 10.4% 136 Xe 8.9% 124 Xe 2n double electron capture (ECEC) 124 Xe (g.s., 0 + ) + 2e - 124 Te (g.s., 0 + ) + 2n e + 2864keV In the case of 2K-capture, signal is total energy deposition of 63.6keV from atomic X-rays and Auger electrons. 126 Xe can also undergo 2n ECEC, but this reaction is much slower. (Q=896keV) 0 + 124 52Te 2-124 53I 4.2d 0 + 124 54Xe Q ECEC =2864keV 2

124 Xe 2n double electron capture (cont d) Predictions for 124 Xe 2n ECEC half-life Wide spread between 10 20 and 10 24 years Experimental result on 124 Xe 2n ECEC Y.M.Gavrilyuk et al., arxiv:1507.04520 Enriched 58.6g of 124 Xe; proportional counter T 1/2 (2n2K)>2.0x10 21 years (90% CL) Model T 1/2 (2nECEC) (yr) Reference QRPA (0.4-8.8)x10 21 Suhonen (2013) QRPA (2.9-7.3)x10 21 Hirsch et al. (1994) SU(4) st (7-17.7)x10 21 Rumyantsev et al. (1998) PHFB (7.1-18.0)x10 21 Singh et al. (2007) PHFB (61.4-155.1)x10 21 Shukla et al. (2007) MCM (390-986.1)x10 21 Aunola et al. (1996) Large volume dark matter detectors have potential to measure 124 Xe 2n ECEC D.-M.Mei et al. (2014): sensitivity test using XENON100 data T 1/2 (2n2K)>1.66x10 21 years N.Barros et al. (2014): sensitivity study for future detectors 3

The XMASS experiment Proposed as a multi purpose experiment with liquid Xenon Xenon detector for Weakly Interacting MASSive Particles (dark matter) Xenon MASSive detector for solar neutrino (pp/ 7 Be solar neutrino) Xenon neutrino MASS detector (neutrinoless double beta decay) Low energy threshold Sensitive to e/g events as well as nuclear recoil WIMPs (by elastic and 129 Xe inelastic scattering), Solar axions, Bosonic super-wimps, Supernova neutrino burst, double electron capture, XMASS-1 (total ~1ton) XMASS-1.5 (total ~5tons) XMASS-2 (total ~24tons) Large target mass and its scalability 4

11m The XMASS-1 detector Located in the Kamioka mine in Japan (~2,700m water equivalent) A single-phase detector employing ~830kg of liquid xenon Equipped with 642 PMTs Active water shield 10m 5

Detector calibration Various calibration sources: 55 Fe, 109 Cd, 241 Am, 57 Co, 137 Cs Light yield, optical parameters, position reconstruction Reconstructed vertex distribution Data Simulation(MC) Total photoelectron distribution 57 Co W X-ray 60keV 122keV 4%rms 6

History of XMASS-1 2010 2011 2012 2013 2014 2015 Dec. May Nov. Today Construction Commissioning data taking Detector refurbishment Data taking (ongoing) Low mass WIMP search [PLB 719 (2013) 78] Solar axion search [PLB 724 (2013) 46] WIMP- 129 Xe inelastic scattering search [PTEP (2014) 063C01] Bosonic super-wimp search [PRL 113 (2014) 121301] 124 Xe double electron capture search: This talk (New result) Dark matter search by seasonal modulation [Talk by K. Kobayashi in Dark Matter A session on Sep. 8] (New result) 7

Data set and event selection (1/2) Data set Dec 24, 2010 ~ May 10, 2012 (Total livetime of 165.9 days) Pre-selection No outer detector trigger is associated with the event. The event is separated from the nearest event by at least 10 msec. RMS spread of hit timings of the event is less than 100 nsec. Dead time due to pre-selection reduces the total effective livetime to 132.0 days. Fiducial volume cut (Radius cut) Event vertex is reconstructed based on the observed light distribution in the detector. Select events with the reconstructed position is within 15 cm from the center. Fiducial mass of natural xenon is 41kg (It contains 39g of 124 Xe) 8

Hit timing [ns] Data set and event selection (2/2) Timing cut Hits timing is used to reject events from the detector inner surface that are wrongly reconstructed. d Events with smaller dtm are less likely to be surface BG and selected. Band-like pattern cut BG events occurred in groves in the inner detector surface make band-like pattern. F B T m t mean t of 2nd half hits 1st hit Max. PE in a band of width 15cm Total PE in the event of Real data (Cd-109) Gap MC PMT position z [mm] z=-40cm z=0cm Events with larger F B are likely to be those BG and rejected. 9

Expected 124 Xe 2n 2K-capture signal -- Fiducial volume cut -- Timing cut -- Band-like pattern cut X-rays and Auger electrons after 2n 2K-capture are simulated. The energy window (56-72keV) is determined so that it contains 90% of the simulated signal. Efficiency for signal is 59.7%. 10

Observed data -- Fiducial volume cut -- Timing cut -- Band-like pattern cut Effective live time of 132.0 days Fiducial mass of natural xenon is 41kg (It contains 39g of 124 Xe) 5 events remained in the signal region 11

Comparison with background prediction + Data -- Pb-214 background MC (w/ sys. error) Main background in this energy region is 214 Pb (daughter of 222 Rn) in the detector. The amount of 222 Rn was estimated from the observed rate of 214 Bi- 214 Po decay. Expected number of 214 Pb BG events in the signal region: 5.3+/-0.5 events No significant excess in the signal region 12

Systematic uncertainty in signal prediction Item Fractional uncertainty Abundance of 124 Xe +/-8.5% Liquid xenon density +/-0.5% Energy scale +0%, -8.6% Energy resolution +0%, -5.3% Scintillation decay time +0%, -7.1% Radius cut (R<15cm) +0%, -6.7% Timing cut (T<12.54ns) +3%, -0% Band cut (B<0.248) +/-5% Total +10.3%, -17.2% A sample was taken from our detector and its isotope composition was measured. Systematic uncertainty in signal efficiency was estimated from comparisons between data and MC simulation for 241 Am (60keV g) calibration data at various positions. 13

Limit on 124 Xe 2n 2K-capture half-life We derive a lower limit using a Bayesian method Conditional probability density function for the decay rate G P(Γ n obs ) = where 90% confidence level limit e μ μ n obs n obs! μ = (Γλε + b)ε corr Γ limit P(Γ n 0 obs )dγ P(Γ nobs ) dγ = 0.9 0 P Γ P λ P ε P(ε corr )P b dλdεdε corr db l: exposure e: signal efficiency (uncorrelated with BG) e corr : correlated efficiency be corr : number of BG events in the signal region T 1/2 2ν2K > ln 2 Γ limit = 4.7 10 21 years (90%CL) 14

Limit on 124 Xe 2n 2K-capture half-life T 1/2 >4.7x10 21 years (90%CL) Cf. Other experimental result T 1/2 (2n2K)>2.0x10 21 years (90% CL) by Y.M.Gavrilyuk et al., arxiv:1507.04520 Expected 124 Xe 2n 2K-capture signal with T 1/2 (2n2K)=4.7x10 21 years 214 Pb background 15

Conclusions XMASS is a multi-purpose experiment using liquid xenon at Kamioka in Japan. Direct detection of dark matter Neutrino-less double beta decay 7 Be/pp solar neutrinos We performed a search for 2n double electron capture on 124 Xe using data collected with the XMASS-I detector. Effective livetime of 132.0 days, 39g of 124 Xe in fiducial volume. No significant excess above background was observed. We set a lower limit T 1/2 (2n2K)>4.7x10 21 years (90% CL) 16

Backup slides 17

Data/MC comparison for 241Am calibration data Reconstructed radial position Timing parameter Band pattern parameter (Solid) Data (Dashed) MC 18