Volcanic Ash Cloud Observations with the DLR- Falcon over Europe during Air Space Closure

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Volcanic Ash Cloud Observations with the DLR- Falcon over Europe during Air Space Closure Ulrich Schumann, Bernadett Weinzierl, Oliver Reitebuch, Andreas Minikin, Hans Schlager, Stephan Rahm, Monika Scheibe, Michael Lichtenstern, Caroline Forster, Robert Baumann, Martin Wirth, Thomas Sailer, Kaspar Graf, Hermann Mannstein, DLR, IPA + many partners (IPA, FB, CNRS-LaMP, TU Darmstadt, IfT Leipzig, LMU München, NILU, Uni. Iceland, DWD, VAAC, DFS, LBA, KNMI, etc.) in cooperation with Ludwig-Maximilians University Munich

April 14 - April 17, 2010: EUMETSAT-DWD-DLR_IPA processing and animation by K. Graf, DLR-IPA 2

19 April, 13:00 UTC - Mid-European airspace closed DLR-Falcon started at 14:11 UTC http://www.radarvirtuel.com/ taken from BBC: Iceland volcano in maps 4

Objectives: Operational & scientific, until May 3 Closure of airspace justified or exaggerated? Quality of forecasts? Comparable to Saharan dust? What do the lidar instruments see? How to convert particle number concentrations to mass concentration? Aviation conditions near Iceland Volcanic source (mass, particle sizes, chemistry) Chemical composition Volcanic dynamics 5

Falcon 20E D-CMET, DLR Oberpfaffenhofen, since 1976 meteorological measurements DLR Falcon 20-E5 max. altitude: 42.000 ft max. endurance: 4 h aerosol & trace gas inlet total & non-vol. aerosol, 3-λ B ap, particle comp. & shape (4 nm - 2.5 µm) CO (UV fluoresc.), O 3 (UV photom.), SO 2 (fluoresc.), H 2 O (τ-point, Ly-α) GPaC (particle collector) TU Darmstadt 2- μm-wind-lidar (heterodyne) PCASP-100X (dry accumulation mode concentration) FSSP-300 & 2-DC (0.3-800 µm) DLR & CNRS 6

Nine DLR Falcon flights, April 19 - May 2: OP - Iceland Eyjafjöll N Keflavik Stornoway Oslo Koszalin De Bilt Leipzig range-corrected backscatter signal @ 2 µm Oberpfaffenhofen OP Keflavik: 2700 km 7

Vulcanic ash layer over Leipzig, April 19, 2010, 15:00 UTC 9

19 April 2010: Vertical profile measurements over Leipzig Leipzig lidar DLR-Falcon, 14:50-15:30 UTC 10 9 coarse mode (> 3 µm) altitude (km) Falcon profile pressure altitude (km) 8 7 6 5 4 3 2 60 µg/m 3 (20-200) 1 0 10-2 10-1 10 0 number conc. (cm -3 stp) (Ift Leipzig: A. Ansmann, M. Tesche, P. Seifert et al.) 10

Lagrangian: Iceland - North Atlantic - Ireland - Scotland (29/04/2010: 50 km distance, arriving in Iceland) 01/05/2010: (8-)200 km distance, 62.5 N, 16.5 W, 11:44 UTC, 1-5 km altitude (age < 3.7 h) 02/05/2010: 450 km distance, 15 W, 60 N, 15:00 UTC, May 2, 2010, age 7 h 04/05/2010: Mace Head, W, N,? UTC, May 4, 2010, age about 60 h 05/05/2010: ARSF and FAAM (U Manchester), Scotland airborne, age about 80 h 1800 UTC 29/4 18001200 UTC 01/05 0600 URC 04/05/2010 11

Eyjafjallajökull volcano plume, 29 April, late afternoon time Eyjafjallajökull Bernadett Weinzierl 12

Eyjafjallajökull volcano plume, May 1, noon time 13

Eyjafjallajökull volcano plume, May 1, noon time 14

Plume and Keflavik (Iceland) soundings, May 1 plume sounded 1st time range-corrected backscatter signal @ 2 µm N Ci clouds Volcanic ash plume Eyjafjallajökull 7.4 km St Cu clouds 60 km 16

Simulated (HYSPLIT) cross-section of the plume HYSPLIT model, GDAS 1x1, 7 particle size classes, line-source from 1.7 km to 4.5 km height a.s.l., mass flux 5000 t/h in 0-50 µm size-range high cloud column mass concentration, all particles ash plume pos. of cross section 1-3 µm 20-30 µm 30-50 µm (R. Baumann, DLR) 17

From Keflavik to Stornoway, May 2 Plume sounded and sampled, 2nd time Outer Hebrides 570 km range-corrected backscatter signal @ 2 µm N Iceland Eyjafjallajökull 18

North Atlantic (60 N): 15 minutes before flying into the plume 19

Mass concentrations in the plume over the North Atlantic dn / dlog D p (cm -3 ) 10 4 May 2, 2010-60 N 10 3 PCASP-100X FSSP-300, m = 1.54 + 0.0i FSSP-300, m = 1.50 + 0.0008 i 10 2 10 1 10 0 10-1 10-2 no signal in the 2-DC probe (D p > 30 µm)! 0.1 1 10 100 particle diameter (µm) distance settled within 7 h (km) 0.0 0.5 1.0 1.5 2.0 2.5 3.0 3.5 ( 273 K, 1013 hpa, no turbulence) =1.36, = 1 g/cm 3 =1.36, = 2.45 g/cm 3 10 100 D p (µm) m = 1.54 + 0i PM2.5 FSSP-300 "total" D eff 7 µm 10 µg/m³ 400 µg/m³ m = 1.50 + 0.008i PM2.5 FSSP-300 "total" D eff 26 µm 10 µg/m³ 3400 µg/m³...assuming a particle density of 1 g/cm -3 20

In-situ chemistry in the plume over the North Atlantic 450 km dist., 15 W, 60 N, 15:00 UTC, 02/05/2010, age 7 h 3 min in volcanic ash plume, 3400 3700 m altitude (FL 110 und 120): O 3 mixing ratio decrease CO increase CO correlates with O 3 SO 2 >150 nmol/mol (outside 0.1 nmol/mol) H 2 O-RH: reduced to 45 % (outside: 70 %) adiabatic warming? CO mixing ratio/(nmolmol) O 3 mixing ratio/(nmolmol) 21

Conclusions (science & operations) Falcon measurements between April 19 and May 3, 2010: 2- m-lidar, in-situ aerosols, CO, O 3, SO 2, H 2 O Particles sizes 10 nm - 30 µm age dependent (mainly silicate, ammonia sulfate, more Na, K than in Saharan dust), Mass loading (60 µg/m 3, Leipzig, 5 days) comparable to Saharan dust (< 0.2 mg/m 3 ) 200 km distance, 3-4 h age: 40 km wide, 2 km thick, 15 m/s, sharply edged, strong wet convective turbulence, well mixed? 450 km distance (same plume), 7 h age: at upper plume edge: 400-3400 µg/m 3, no 2-DC probe particles, mass flux > 3000 kg/s, strong chemistry Lidar signal and FSSP-300 signal strongly dependent on refractive index, ash density, particle size spectrum 1-50 µm Mid-European airspace closure justified until Sat. April 17; then ageing of ash load Keflavik/Iceland free of ash as predicted on April 19 - May 2 Quality of forecasts reliable enough for aviation Future: Combination of models + lidar + satellite + in-situ Improved linking between operations and academia Continue operations of the Institut DLR für Falcon Physik der as Atmosphäre Emergency Aircraft 23

Further Falcon Flights May 9: Southern Germany: < 10 g/m3; questionable air space closure May 13: English Channel: MSG detected thin ash cloud < 30 g/m3, without VAAC warning May 16: England and North Sea: thick volcanic ash plume > 2000 g/m3 May 17: North Sea VA 450 g/m3, observed also by MSG and Lidar Cabauw May 18: Thin ash cloud over Germany (Lidar Stuttgart) 24

DLR-Falcon flight over Southern Germany, May 9, 2010 17:53 UTC: profile measurements at Munich airport and over Maisach lidar mass loading below 10 g/m3 <- Measurements performed by the Met. Institute of the LMU Munich 25

England, May 16, 2010 0 UTC 26

England, May 16, 2010 6 UTC 27

England, May 16, 2010 12 UTC Guided by MSG ash product: Falcon observes heavy VA plume 28

Satellite image with Falcon track, volcaon ash plume reaching Amsterdam at about 19:00 UTC colours to compare approximately with VAAC predictions 29

Vertical profiles SO2, CO, O3 Particle size distribution; 0.1 to 25 m diameter: derived mass concentration assuming refractive index 1.54+0i and density 3 g/cm³: 450 µg/m³ ± 50 % 30

UV LIDAR CABAUW: Falcon-traced ash plume arrived at Cabauw, NL, 16:30 UTC in cooperation with Ludwig-Maximilians University Munich http://www.knmi.nl/~savenije/uvlidar/

Further Conclusions, after 5 weeks with 51.5 Falcon flight hours Falcon measurements between April 19 and May 18, 2010: 2- m-lidar, in-situ aerosols, CO, O 3, SO 2, H 2 O Falcon confirms MSG ash product at least qualitatively Further in-situ data for comparison to Lidar observations The set of flight paths data (waypoints versus time) are available on the internet with permit of BMVBS/DWD DLR offers comparison of Falcon in-situ (CO,O3, SO2, H2O, particles, mass concentration) and 2-um-Lidar data with any other available data. Contact via Ulrich Schuman Southern German airspace closure Sun. May 9, 6 days aged VA: questionable Closure over UK, May 16, 1-2 days aged plume: fully justified Fresh and heavy VA is well predictable - >3 days aged VA: far more difficult 1 hour of flight in VA ash of 450 um/m3: no Falcon engine problem detected Next: HSRL on HALO 32