Airborne and satellite observations of volcanic ash from the Eyjafjallajökull eruption

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Airborne and satellite observations of volcanic ash from the Eyjafjallajökull eruption

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Airborne and satellite observations of volcanic ash from the Eyjafjallajökull eruption Stuart Newman and co-authors ITSC-18, Toulouse, France, 21-27 March 2012 Photo credit: Arnar Thorisson 17.4.10

Acknowledgements This talk is based on a paper published recently for a JGR special issue From the Met Office: Stuart Newman Franco Marenco Ben Johnson Kate Turnbull Stephan Havemann Anthony Baran Debbie O Sullivan Jim Haywood From the Université Libre de Bruxelles: Lieven Clarisse Daniel Hurtmans With thanks to Deutsches Zentrum für Luft- und Raumfahrt (DLR)

Talk contents FAAM aircraft and instrumentation Case study from 17 May 2010 Radiative transfer modelling of infrared spectra IASI retrievals of ash mass concentration (ULB) Choice of ash refractive index

FAAM aircraft and instrumentation

FAAM BAe146-301 ARA Instrumentation ARIES interferometer (Bomem MR200) Radiances: spectral range 550-3000 cm -1 HgCdTe and InSb detectors ADA on other side Max. resolution 1 cm -1 (0.5 cm -1 sampling) FAGE Inlet Multiple viewing geometries (up and down) CVI on other side Air sample inlets Field of view 44 mrad (full angle) BBRs SHIMS SWS on other side Upward and Forward Video Cameras Alan Vance 5 port turbulence probe Total water probe JW Liq water Nevzerov total/liq water probe Rosemount temp probes Deimos or IR Camera TAFTS ARIES BBRs SHIMS Lidar MARSS Cloud Physics Probes Dropsonde on other side Rearward and Downward Video Cameras Cloud Physics Probes ARIES with starboard side removed showing electronics modules (top), detector/cooler unit (bottom right), heater controller (mid left) and folding/focusing optics (bottom left).

Lidar Observations of Volcanic Ash Franco Marenco

Particle measuring instrumentation on FAAM BAe 146 Particle counter name Effective size range Aircraft flown on CAPS/CAS 0.5 50 µm FAAM BAe146-301 PCASP 0.1-3 µm FAAM all Dornier 18 19 & 20 April CAPS probe was essential to capture the larger particles

Case study from 17 May 2010

Case study North Sea event on 17 May 2011 TERRA MODIS imagery (thanks to Jim Haywood)

SEVIRI dust RGB imagery

Flight tracks FAAM and DLR aircraft sampled the same event

Thanks to University of Manchester for provision of CAS data Around 98% particles by mass were found in the coarse mode, around 2% in the fine mode DLR size distribution has mean diameter of approx. 9.6 µm, larger than estimated by CAS on FAAM BAe 146 (3.6-4.5 µm) Some support for CAS size distribution from ground-based AERONET retrievals Number Mass DLR Turnbull, Kate; Johnson, Ben; Marenco, Franco; Haywood, Jim; Minikin, Andreas; Weinzierl, Bernadett; Schlager, Hans; Schumann, Ulrich; Leadbetter, Susan; Woolley, Alan A case study of observations of volcanic ash from the Eyjafjallajökull eruption: 1. In situ airborne observations J. Geophys. Res., Vol. 117, No. null, D00U12

1. 2. 3. 2. 3. 1. 1. 2. 3. 12 µm 8 µm Lidar: Franco Marenco

Radiative transfer modelling of infrared spectra

Radiative transfer modelling Infrared airborne radiances: use Havemann-Taylor Fast Radiative Transfer Code (HTFRTC). Based on singular value decomposition of spectral information to speed up calculations. Ability to treat scattering by clouds and aerosol particles. IASI mass retrievals: code developed at ULB. Optimal estimation for simultaneous retrieval of trace gases, aerosol size and concentration. Treats multiple scattering in spherical geometry.

Can we model the infrared ash signature? Lidar extinction profile has been used as input to forward calculation along with representative temperature and humidity profiles. Aerosol properties are based on measured size distribution and dust refractive index due to Balkanski et al. (2007) Agreement is (surprisingly) good Increasing ash concentration

IASI: mineral dust refractive index is a good match here too Name Mineral Dust RMS of residual (in W m -2 m sr -1 ) Mass (in % of first ) Reference 5.5 10-6 100 Balkanski et al., 2007 ARIES: mineral dust refractive index is a better match than andesite or obsidian for 17 May 2010 Obsidian 7.2 10-6 79 Pollack et al., 1973 Basalt 1.6 10-5 65 Pollack et al., 1973 Spectral residual of fit to IASI observations Andesite 1.5 10-5 63 Pollack et al., 1973 Pumice 1.4 10-5 73 Volz, 1973 Rained out dust 1.5 10-5 159 Volz, 1973

IASI retrievals of ash mass concentration

IASI ash retrievals AM PM ULB IASI ash mass loadings (g/m 2 ) for 17 May am and pm overpasses Lidar and IASI distribution of column loadings over same advected part of ash plume area

Choice of ash refractive index

Why does mineral dust refractive index match ash cloud spectra? 2 May 2010 17 May 2010 This case study Citation: Schumann, U., Weinzierl, B., Reitebuch, O., Schlager, H., Minikin, A., Forster, C., Baumann, R., Sailer, T., Graf, K., Mannstein, H., Voigt, C., Rahm, S., Simmet, R., Scheibe, M., Lichtenstern, M., Stock, P., Rüba, H., Schäuble, D., Tafferner, A., Rautenhaus, M., Gerz, T., Ziereis, H., Krautstrunk, M., Mallaun, C., Gayet, J.-F., Lieke, K., Kandler, K., Ebert, M., Weinbruch, S., Stohl, A., Gasteiger, J., Groß, S., Freudenthaler, V., Wiegner, M., Ansmann, A., Tesche, M., Olafsson, H., and Sturm, K.: Airborne observations of the Eyjafjalla volcano ash cloud over Europe during air space closure in April and May 2010, Atmos. Chem. Phys., 11, 2245-2279 Large particles are dominated by silicates on 17 May 2010 This is less evident on 2 May 2010

Summary and conclusions Airborne and satellite infrared radiances can be accurately modelled based on the in situ measured size distribution and a mineral dust refractive index Retrievals of ash mass column loading using IASI observations are in accord with lidar-derived mass estimates, giving a verification for the hyperspectral ash retrieval method Modelling of ARIES and IASI ash-affected spectra demonstrates the importance of accurately specifying the refractive index There is evidence that the composition of airborne ash from the Eyjafjallajökull eruption varied within the same event It was recognised in the UK that there is a requirement for a well instrumented airborne facility to be able to monitor ash concentrations the Met Office now operates a twin piston engine aircraft for civil contingency use

Questions and answers

Other eruptions: Puyehue in Chile and Grímsvötn in Iceland as seen by IASI

But ash particles are NOT spheres! Electron microscope images of ash collected on filters during FAAM flight B526

But ash particles are NOT spheres! SID2h scattering patterns for ash SID2h scattering patterns for hydrated sea-salt aerosol (spherical)

FAAM (A) [irregulars] and FAAM (B) [spheres] give similarly good agreement obs v calc DLR [different size distribution] gives worse agreement Other refractive indices: Balkanski mineral dust gives best agreement Other choices (andesite and obsidian) fail to match observations

ARIES looking up under the ash With scaled extinction profile agreement of simulation with measured brightness temperature is good

Aerosol scattering properties Normalised extinction Single scattering albedo Aerosol refractive index Representative particle size distribution Mie theory Asymmetry parameter Scattering properties at IR wavelengths (calculations Crown copyright Met by Office Ben Johnson)