MISR remote sensing of tropospheric aerosols

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MISR remote sensing of tropospheric aerosols David J. Diner, John V. Martonchik, Ralph A. Kahn Jet Propulsion Laboratory, California Institute of Technology Michel M. Verstraete Institute for Environment and Sustainability, Joint Research Centre International course on Remote Sensing of the Earth s Environment from Terra Scuola Superiore Reiss Romoli, L Aquila, Italy August 29, 2002

Aerosols are tiny particles suspended in the air What are aerosols? Natural sources: Volcanoes Dust storms Forest and grassland fires Living land and ocean vegetation Sea spray January Anthropogenic sources: Burning of fossil fuels through industrial activities, transportation systems, and urban heating Land cover and land use changes, e.g., biomass burning, deforestation, desertification July From Kahn et al. (2001), Showing aggregate of five aerosol transport models Carbonaceous + Dusty Maritime Dusty Maritime + Coarse Dust Carbonaceous + Black Carbon Maritime Carbonaceous + Dusty Continental Carbonaceous + Black Carbon Continental

Why are aerosols important? Aerosols scatter and absorb sunlight, and thus can cool or warm the surface and atmosphere As nucleation centers, aerosols can change the drop size distribution within clouds, affecting cloud reflectance and lifetime Fine particles penetrate lung tissue and affect respiratory function High altitude aerosol plumes present hazards to aircraft Aerosols affect the appearance of scenic vistas Remote sensing studies of the surface must account for radiation transfer through the intervening atmosphere

Key aerosol microphysical parameters Particle size and size distribution Aerosol particles > 1 mm in size are produced by windblown dust and sea salt from sea spray and bursting bubbles. Aerosols smaller than 1 mm are mostly formed by condensation processes such as conversion of sulfur dioxide (SO 2 ) gas to sulfate particles and by formation of soot and smoke during burning processes Effective radius Moment of size distribution weighted by particle area and number density distribution Complex refractive index The real part mainly affects scattering and the imaginary part mainly affects absorption Particle shape Aerosol particles can be liquid or solid, and therefore spherical or nonspherical. The most common nonspherical particles are dust and cirrus

Key aerosol optical parameters Optical depth negative logarithm of the direct-beam transmittance column integrated measure of the amount of extinction (absorption + scattering) Single-scattering albedo v 0 given an interaction between a photon and a particle, the probability that the photon is scattered in some direction, rather than absorbed Scattering phase function probability per unit solid angle that a photon is scattered into a particular direction relative to the direction of the incident beam Angstrom exponent a exponent of power law representation of extinction vs. wavelength

Microphysical properties Remote sensing of aerosols requires inferring particle properties from observed top-of-atmosphere radiances Optical properties Challenges: - nonuniqueness - surface reflection Atmospheric radiative transfer Observed multi-spectral, multi-angular radiances

Path radiance (no surface interaction) singly-scattered Top-of-atmosphere radiation consists of singly- and multiplyscattered components that may or may not have interacted with the surface Path radiance (no surface interaction) multiply-scattered Directly transmitted radiance

How do multi-angle observations from MISR facilitate aerosol remote sensing? 1. CONDITIONING THE SIGNAL a. Avoiding sunglint Over water, sunglint invalidates the assumption of a nearly black surface, and multiple cameras enable using non-glint contaminated views b. Identifying clouds Multi-angle observations offer several powerful approaches c. Enhancing sensitivity to thin aerosols Off-nadir observations look through a longer atmospheric path, thus providing greater sensitivity to aerosols, particularly over land

How do multi-angle observations from MISR facilitate aerosol remote sensing? 2. INTERPRETING THE OBSERVATIONS a. Accounting for the surface contribution to the top-of-atmosphere (TOA) radiances Different methodologies are used depending on whether the underlying surface is land or water, and new methodologies over land are made possible b. Constraining the non-uniqueness of the solutions Multi-angle information complements multi-spectral constraints on particle properties

How do multi-angle observations from MISR facilitate aerosol remote sensing? 3. APPLYING THE RESULTS a. Radiative effects In addition to the aerosol product, the multi-angle data provide simultaneous estimates of top-of-atmosphere albedo b. Volcano and smoke plume propagation Besides the aerosol product, stereoscopic retrievals provide simultaneous information about plume altitudes c. Air quality Multi-angle algorithms enable retrievals over non-vegetated areas, such as arid and urban regions

1a. Avoiding sunglint glint Sunglint over water invalidates the assumption of a dark surface, and multiple cameras provide the flexibility to avoid this smoke cloud glint Southern Mexico 2 May 2002 nadir 70º backward

49ºN Example of glitter geometry July 3 specular reflection of solar beam equator x 100º 80º 49ºS An Aa Ba Ca Da 60º 40º 20º 0º Glitter angle x MISR aerosol retrievals require glitter avoidance of at least 40º

1b. Identifying clouds Cloud clearing is essential for aerosol retrievals Global radiance map, nadir camera March 2002

MISR uses multiple scene classification methodologies to screen for clouds Smoothness of radiance variation with angle Correlation of spatial radiance pattern with angle Use of darkest 1.1-km subregion within 17.6-km aerosol retrieval region (over water) Radiance thresholding cloud mask (RCCM) Stereoscopic cloud mask (SDCM)

Multiple classification methods Poor quality data Topographically obscured Cloudy Not smooth with angle Not correlated with angle Region not suitable 70º backward image RCCM SDCM Retrieval ClearHC CloudLC ClearLC CloudHC applicability mask Southern Mexico 2 May 2002

1c. Enhancing sensitivity to thin aerosols Thin haze over land is difficult to detect in the nadir view due to the brightness of the land surface The longer atmospheric path length enhances the haze path radiance nadir 70º Appalachians, 6 March 2000 nadir 70º 558-nm aerosol optical depth

Southern California 9 February 2002

2a. Accounting for the surface contribution to TOA radiances Despite the different ways of treating the surface, and the vast difference in water and land reflectance, good continuity is obtained across the land-water boundary Southern California and western Nevada 3 January 2001 70º forward nadir 70º backward 558-nm optical depth

Aerosol retrieval methodology over water MISR multi-angle imagery Compositional models consisting of mixtures of prescribed particles Surface glitter and whitecap model Calculate model path radiance as function of optical depth Minimize residuals between observations and modeled radiation field Accept models and associated optical depths with residuals below a specified threshold

Multiple goodness of fit metrics 2 = N -1 S S [L MISR - L path - L surface ] 2 / [0.05L MISR ] 2 abs channels angle band where L surface is modeled as a prescribed contribution from sunglint and whitecaps 2 geom : Similarly defined except measured and modeled radiances are normalized to the camera-average values 2 spec : Similarly defined except measured and modeled radiances are normalized to the red-band values 2 : Largest term in the 2 summation maxdev abs

Aerosol retrieval methodology over land MISR multi-angle imagery Compositional models consisting of mixtures of prescribed particles Subtract minimum reflectance to remove path radiance Calculate model path radiance as function of optical depth Calculate surface-leaving angular shape eigenvectors Minimize residuals between observations and synthesized radiation field Accept models and associated optical depths with residuals below a specified threshold

Goodness of fit metric 2 = N -1 S S [L MISR - L path - L surface ] 2 / [0.05L MISR ] 2 het channels angle band where L surface is modeled as a dynamically derived sum of empirical orthogonal functions that are least-square fitted to L MISR - L path Simplified concept: The technique requires surface contrast to be visible through the atmosphere Imagine two pixels with different albedos but the same variation in reflectance as a function of angle L MISR,TOA(1) = L path + L surface(1) ; L MISR,TOA(2) = L path + L surface(2) DL MISR,TOA = DL surface (path radiance subtracts out) The angular variation of L surface is then given by DL MISR,TOA. To within a constant of proportionality, this is used to constrain L MISR - L path by summing over all angles The EOF approach is invoked to account for multiple surface angular reflectance shapes within the scene

The Red Sea, 25 March and 29 June 2001 nadir images 558-nm aerosol optical depth

The Red Sea, 25 March and 29 June 2001 70º-forward images 558-nm aerosol optical depth

2b. Constraining the non-uniqueness of the solutions A set of component particles of prescribed microphysical/optical properties is established spherical nonabsorbing (e.g., sulfates, sea spray) small absorbing (admixtures with black carbon) nonspherical nonabsorbing (cirrus) nonspherical absorbing (dust) Mixtures of these component particles in predetermined ratios are also established and various radiative transfer quantities (e.g., path radiance) are precalculated and stored in a look-up table

Spectral extinction of component aerosols relative to 558 nm 2.5 2.0 1.5 Component particle type and effective radius of distribution (mm) spherical_nonabsorbing_0.06 spherical_nonabsorbing_0.12 spherical_nonabsorbing_0.26 spherical_nonabsorbing_0.57 spherical_nonabsorbing_1.28 small_absorbing_0.04 nonspherical_absorbing_1.18 nonspherical_absorbing_7.48 1.0 0.5 0.0 400 500 600 700 800 900 Wavelength (nm)

Phase function Scattering phase functions of component aerosols 10000.00 1000.00 100.00 10.00 Component particle type and effective radius of distribution (mm) spherical_nonabsorbing_0.06 spherical_nonabsorbing_0.12 spherical_nonabsorbing_0.26 spherical_nonabsorbing_0.57 spherical_nonabsorbing_1.28 small_absorbing_0.04 nonspherical_absorbing_1.18 nonspherical_absorbing_7.48 1.00 0.10 0.01 0 20 40 60 80 100 120 140 160 180 Scattering angle (degrees)

Example MISR scattering angle coverage (March 21)

24 mixtures used in retrievals r eff (components) a v 0 1 Spherical Small Clean 0.06 3.22 1.00 2 Spherical Small Clean 0.06, 0.12 2.71 1.00 3 Spherical Small Clean 0.12 2.24 1.00 4 Spherical Small Clean 0.12, 0.26 1.63 1.00 5 Spherical Medium Clean 0.26 1.09 1.00 6 Spherical Medium Clean 0.26, 0.57 0.56 1.00 7 Spherical Medium Clean 0.57 0.10 1.00 8 Spherical Medium Clean 0.57, 1.28-0.05 1.00 9 Spherical Bimodal Clean 0.12, 1.28 0.82 1.00 10 Spherical Bimodal Clean 0.06, 1.28 1.19 1.00 11 Spherical Small Absorbing 0.06. 0.04 2.87 0.88 12 Spherical Small Absorbing 0.06, 0.12, 0.04 2.50 0.88 13 Spherical Small Absorbing 0.12, 0.04 2.09 0.88 14 Spherical Small Absorbing 0.12, 0.26, 0.04 1.62 0.88 15 Spherical Medium Absorbing 0.26, 0.04 1.13 0.88 16 Spherical Medium Absorbing 0.26, 0.57, 0.04 0.71 0.88 17 Spherical Medium Absorbing 0.57, 0.04 0.29 0.88 18 Dusty Low 0.26, 1.18 1.46 0.97 19 Dusty Low 0.26, 1.18 0.85 0.94 20 Dusty Low 0.26, 1.18 0.33 0.91 21 Dusty Low 1.18-0.11 0.88 22 Dusty Low 1.18, 7.48-0.08 0.83 23 Dusty Low 1.18, 7.48-0.06 0.79 24 Dusty High 1.18-0.11 0.88

Retrieval case study Southern Mexico 2 May 2002 558-nm optical depth

Retrieval case study Orbit 12616, smoke 1.2 Optical depth upper bound Mixture optical depth 1 0.8 0.6 0.4 0.2 0 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 Mixture Optical depth is a function of aerosol type, so multi-angle and multi-spectral information is used to narrow the range of candidate solutions Step 1: All 36 channels of MISR are used to establish an optical depth upper bound, and mixtures for which the best-fitting optical exceeds this limit are eliminated

Retrieval case study Orbit 12616, smoke 50 45 40 35 Mixtures in lighter orange were eliminated in step 1 30 25 20 15 10 5 0 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 Mixture Step 2: Mixtures for which the 2 abs are eliminated residual exceeds a specified threshold Ideally the threshold is ~1, but with quantized proportions of component particles in the mixtures, this is relaxed so as not to sacrifice coverage

Retrieval case study Orbit 12616, smoke 14 Chisquare_geom Chisquare_spec Chisquare_maxdev 12 10 8 6 4 2 0 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 Mixture Step 3: Mixtures for which the other 2 are eliminated residuals exceed specified thresholds For this case the best mixture is: (13) Spherical Small Absorbing

3a. Radiative effects 0.18 0.16 0.14 0.12 0.1 0.08 0.06 wavelength = 558 nm solar zenith angle = 18º 0.04 0 0.2 0.4 0.6 0.8 1 1.2 Aerosol optical depth 70º backward TOA local albedo Southern Mexico 2 May 2002

3b. Smoke and volcanic plume propagation multi-angle fly-over Hayman Fire, southwest of Denver, Colorado 9 June 2002

Optical depth / stereo height retrievals Hayman Fire 9 June 2002

Automated stereoscopic retrieval of plume height Eruption of Mt. Etna, Sicily 22 July 2001 70º image height (kilometers) 0 5 10

3c. Air quality India and the Tibetan Plateau 15 October 2001 558-nm optical depth

MISR optical depth over 3x3 region area MISR / Aeronet optical depth comparisons (558 nm) Retrievals over water Retrievals over land Aeronet optical depth (cloud screened) September - November 2001

Global distribution of Aeronet sites used in Sept. - Nov. 2001 matchups

Summary MISR aerosol products are based upon new algorithms -- novel cloud screening approaches -- unprecedented aerosol retrieval approach over land, enabling monitoring of vegetated and non-vegetated areas Products are improving with time as we gain more experience -- quality assessment and validation are underway Much work is in progress or planned -- refinement of instrument radiometric and geometric calibration -- improved cloud screening, including implementation of multiangular cirrus mask -- improvement in retrievals over bright, homogeneous areas -- formal validation of retrieval uncertainties and particle property characterizations -- improved dust models -- comparisons with other satellite instruments

MISR aerosol data products are available through the Langley Atmospheric Sciences Data Center DAAC http://eosweb.larc.nasa.gov More information about MISR http://www-misr.jpl.nasa.gov