New half-live results on very long-living nuclei

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Fakultät Mathematik und Naturwissenschaften, Institut für Kern- und Teilchenphysik New half-live results on very long-living nuclei 29.9. 2016, NNR 2016 Osaka Institut für Kern- und Teilchenphysik

Contents A look on alpha decays Highly forbidden beta decays Double EC captures Double beta decays Nuclear astrophysics Summary

Alpha-decays Long living = Half-life longer than the age of the Universe Low background Frisch grid ionisation chamber (< 10 per day between 1-9 MeV, in region 1-3 MeV only 1 event per 2 days) 0.35 Normilised Amplitude [.arb] 0.3 0.25 0.2 0.15 0.1 147 Sm Calibration 239 Pu 241 Am 244 Cm 0.05 0 2 2.5 3 3.5 4 4.5 5 5.5 6 Energy [MeV] 30.8 days background A. Hartmann, J. Hutsch, F. Krüger, M. Sobiella,H. Wilsenach, K. Zuber, NIM A 814, 12 (2016)

Alpha-decays Sm147 Abundance : 14.99% Our ICP-MS: 14.77% Ex: 19 days of data taking First test: Calibration source [years] T 1/2 130 125 9 10 (1958Be01) (1954Be01) (1992Mar01) Data Point Weighted mean 120 115 (1961Ma01) (1960Ka01) (2003Ki01) 110 105 (1965Va01) (1970Gu01)(1978Lu01) (1961Wr01) (1987Al01) (1964Do01) (2009Ko01) (2001Beg01)(2010Su30) 1 st excited state search 100 1960 1970 1980 1990 2000 2010 Year In total about 60000 Sm-147 events Results: Ground state: T 1/2 = 1.097(35) x 10 11 years 1st excit. state: T 1/2 > 3.1 10^18 years (90% CL) R. Heller, V. Neu, H. Wilsenach, K. Zuber, in preparation

Alpha-decays Pt-190 Abundance : 0.014% Can we use Pt-190 as cosmochronometer? Laboratory: 3.9 +- 0.2 [10^11 years] Geochemical : 4.78 +- 0.05 Semi-empirical calculations : 3.5+- 0.3 O,Tavares et al., NIM B 243, 256 (2006) cnt/(40 kev) 300 250 200 150 100 About 3500 events Latest theory: 2.78 Y. Qian, Z. Ren, PLB 738, 87 (2014) Y. Georgiev, H. Wilsenach, K. Zuber, in preparation 50 0 1 2 3 4 5 6 7 8 9 Energy [MeV]

Highly forbidden beta decays Highly forbidden decays have different energy spectra, a lot of operators 3-fold forbidden: 180m Ta,... 4-fold forbidden non-unique : 50 V, 113 Cd, 115 In 5-fold forbidden: 96 Zr, 48 Ca (in the range of double beta decay)

Ta-180m Natures rarest stable isotope, only nucleus present in nature in an isomeric state M. Hult et al., Appl. Rad. Isot. 67, 918921 (2009) New measurement : - Sandwich Ge-detector at HADES - Almost twice as much statistics - Lower intrinsic background - Improved statistical analysis - Combining all data sets Example: > 2 x10 17 yrs > 5.8 x10 16 yrs B. Lehnert, M. Hult, G. Lutter, K. Zuber, arxiv:1609.03725

The case of V-50 The search for V-50 has a long history...started 1955 Half-Life [years] 18 10 10 17 V50 Half-Life Measurement Half-Life Value Half-Life Upperbound (this work) 16 10 T 1/2 > 1.7 x 10 18 yrs 15 10 T 1/ 2 = 2.29 ± 0.25 10 17 years 1960 1970 1980 1990 2000 2010 Year Measurement at PTB Braunschweig (ASSE)

The case of V-50 H. Dombrowski, S. Neumaier, K. Zuber, PRC 83, 054322 (2011) What about beta- branch? Theoretical prediction (shell model) for beta- branch: T 1/ 2 2 10 19 yrs M. Haaranen, P. Srivastava, J. Suhonen, K. Zuber, PRC 90, 044314 (2014) New measurement ongoing at LNGS: M. Laubenstein, S. Nagorny, K. Zuber in preparation

The case of 113 Cd 4-fold forbidden non-unique beta decay (1/2 + 9/2 + ) COBRA experiment (CdZnTe detectors) 113Cd Preliminary Q-value: J. V. Dawson et al., Nucl. Phys. A 818,264 (2009) AME 2012 value: 322.6 0.8 kev Penning trap value: 323.89 (27) kev N. D. Gamage et al., Phys. Rev. C 94,025505 (2016) Shape depends on g A Half-life: M. T. Mustonen, M. Aunola, J. Suhonen, PRC 73,054301 (2006) M. T. Mustonen, J. Suhonen,, PLB 657,38 (2007) 64 independent measurements of the half-life!

Beta decay spectra There is a general demand to measure beta spectrafor various reasons High resolution, low background beta spectroscopy

Double EC and DBD Mass parabola (isobar) There are 35 double beta (and ECEC) emitters out of which are 6 double positron emitters Depending on Q-value competing with double positron and EC/positron decay Both modes can occur with/without neutrinos Also transitions into excited states possible

Excited state transitions Only first excited 0 + state has been seen in Mo-100 and Nd-150 GERDA phase I : First (and only) multi-detector analysis in GERDA M. Agostini et al., J. Phys. G 42. 115201 (2015)

Excited state transitions More measurements : Our measurements More half-life limits exist but almost always below 10 20 years

Double EC and DPD Theory prediction lacking for neutrinoless double EC: - Internal bremsstrahlungs gamma (monoenergetic) - Pair production in nuclear field - Internal conversion M. Doi, T. Kotani, Prog. Theo. Phys. 89,130 (1993) (GERDA and our measurements) Again more measurements exist

Resonances? (A,Z) (A,Z-2) + 2 e + (+2ν e ) β+β+ e - + (A,Z) (A,Z-2) + e + (+2ν e ) β+/ec 2 e - + (A,Z) (A,Z-2) (+2ν e ) EC/EC Resonant enhancement (*10 6 ) of 0nu ECEC if excited state in daughter is degenerate (within 200 ev) with initial ground state (-> Q-values) Q-4m e c 2 Q-2m e c 2 Q Enhanced if V+A is at work M. Hirsch et al, Z. Phys. A 347,151 (1994) Best candidate : 152Gd measured with SHIPTRAP at GSI J. Bernabeu, A. derujula, C. Jarlskog, Nucl. Phys. B 221,15 (1983) S. Zujkoswski, S. Wycech, PRC 70, 052501 (2004) Still not good enough to compete with neutrino mass bounds from double beta decay S. Eliseev et al., Phys. Rev. Lett. 106,052504 (2011)

Solar neutrinos Assumption: The Sun is producing energy via nuclear fusion 60 billion solar neutrinos penetrate us per cm 2 every second Not measured yet: CNO-neutrinos, hep-neutrinos

Fusion reactions Charged particle reactions -> Coulomb barrier Compromise between Maxwell Boltzmann distribution and tunneling probability

Solar neutrinos - Felsenkeller SNO for the first time neutrino flux measurements more precise than solar model predictions

Uncertainties

3 He( 3 He,2p) 4 He 2H(p,γ)3He C. Broggini et al., Ann. Rev. Nucl. Part. Sci. 60,53 (2010)

3 He( 4 He,γ) 7 Be

Felsenkeller Laboratory Dresden T. Szücs et al., Eur. Phys. J. A 48,8 (2012) We have the accelerator We have the underground lab 8 existing, ultralow background HPGe detectors Tunnel for accelerator

Felsenkeller -accelerator

Felsenkeller - Status - Accelerator will provide p, alpha and C beams - Construction work on site has started one month ago - Accelerator planned to go underground spring 2017 - First light autumn 2017 Remember: it will be a user facility, i.e. there will be a Scientific Advisory Committee and everybody can send proposals

Summary Measurement of half-lives of long living nuclides is still interesting as some values are not as good as they look at first glance A new half-live measurement of Pt-190 has been obtained The EC-branch half-life of V-50 has been measured A new value for Ta-180m half-live is given Spectral shape searches in highly forbidden beta decay sounds interesting for learning about quenching of g A Various new limits on excited states searches in double beta decay and in radiative double EC have been obtained Resonance enhancement for double EC into excited state seems to be realised in Gd-152, but still worse than neutrino mass searches in double beta decay New facilities built to study long-living alpha decays, spectral shapes of beta decays and (soon) cross sections measurements using p, alpha, C - beams