Effects of Interactions in Suspended Graphene

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Effects of Interactions in Suspended Graphene Ben Feldman, Andrei Levin, Amir Yacoby, Harvard University Broken and unbroken symmetries in the lowest LL: spin and valley symmetries. FQHE Discussions with Bert Halperin and Dima Abanin In collaboration with Benjamin Krauss, Jurgen Smet, MPI Stuttgart

Degeneracy and Interactions Kinetic energy (Pauli exclusion) vs Interaction energy 2 2 r s E E e e = K = 2 e εr E F E e e E F e = εr 2 k 2m = α F * e ε n = n g ( ) d k F α -Disperssion 1-graphene 2 - bilayer g - Degeneracy: spin, layer, valley r s g m 1 1 α d n 2 d ε * d - Dimensionality (1d,2d,3d) We want: Large degeneracy, large mass, low density, low dielectric.

Bilayers - Band Structure B=0 Quadratic dispersion: α=2 m~0.03m e Near E=0; g =8 - Spin, valley and sublattice Low density Suspended ε~1 r s g m 1 1 α d n 2 d ε * Degenerate bands correspond to B1 and B2 sub-lattices

B=0 Generalization to Multi-layers For N layers: ABCABC stacking Dispersion k N α = N g - Spin, valley and sub-lattice Low density r s g m 1 1 d n 2 N d ε * Screening? Experiments: Lau, Tarucha, Jarillo-Herrero, Kim, Zaliznyak, Geim, Novoselov, Andrei, Heintz, Crommie, Schoenenberger, Ong Theory: Falko, McCann, Levitov, Katsnelson, Castro-Neto, Macdonald, Fogler, Fertig, Shimshoni Das Sarma, Polini, Guinea, Aleiner, Altshuler, Abanin, Sondhi, Kharitonov

QHE - Degeneracy s E n = ω n( n 1) c E n = n 2e v 2 F B Diverging mass McCann, Falko, 06

Quantum Hall Ferromagnetism For - ν=1 N=1 ν=2 N=0 ν=1 Spin φ θ Neglect Zeeman: SU(2) spontaneous symmetry breaking

Quantum Hall Ferromagnetism Isospin Top φ θ Bottom Simple example - ν=1 K. Moon, H. Mori, Kun Yang, S. M. Girvin, A. H. MacDonald, L. Zheng, D. Yoshioka, and Shou-Cheng Zhang, Phys. Rev. B 51, 5138 1995. S. L. Sondhi, 95

Monolayer and Bilayers Interplay between valley and spin: Lowest LL occupied by electrons and holes 4 fold degenerate: Valley and spin Valley/ sub-lattice (pseudospin) spin Along B T Space of symmetries SU(4) ν=0 Partial spin ordering Partial valley ordering Abanin et al 07, Macdonald et al, M. Kharitonov 11, 12 AF CAF F Increasing Zeeman Kekule CDW PLP- Bilayers Determined by lattice scale anisotropy

Experimentally (Kim group): Increasing Zeeman reduces transport gap; suggests absence of strong spin polarization?? CAF?? Monolayers at the Edge Partial spin ordering AF CAF F Increasing Zeeman Analogous to QSH Kharitonov 12 Partial valley ordering F Kekule CDW PLP- Bilayers

Phase diagram for ν=0 in Bilayers CAF Zeeman Electric field PLP R. T. Weitz, AY, et al, Science 2010. Electric field From: Kharitonov, 2011 See also: Macdonald, Levitov

Fractional Quantum Hall Effect - GaAs Fractional QHE IQHE of composite Fermions (Jain) p ν = 2 p ±1 ν = N e N φ 0 Non Abelian phases at 5/2 and 12/5?? (Moore and Read) Edge reconstruction (Barak, AY et al) Neutral edge excitation modes (Heiblum et al, Venkatachalam, AY et al)

arxiv:1111.3640v2 19 May 2012

arxiv:1204.5733v2-5 Jul 2012

Background on FQHE - Suspended Andrei group: Nature 462, 192, (2009) (e/3)= 2meV @12T 1/3 most developed Kim group Phys. Rev. Lett. 106, 046801 (2011)

Background on FQHE - hbn 4/3 most developed 5/3 absent Kim group, Nature Physics 7, 693 (2011)

n µ How to Measure Local Density of States? = Density of states µ n = Inverse (DOS ; Compressibility) Energy Electrochemical V Chemical µ = V - φ Need to measure δµ δµ = -δφ δv=0 Thermodynamic equilibrium V is constant in space Position δµ = -δφ If we can measure the local δφ we will immediately get the local δµ

Using a SET as a Local Electrostatic Probe I e QD e Current flow Coulomb Blockade N N + 1 N U e 2 = > kt c E V G E Use graphene as the gate. By monitoring the current we can extract the local electrostatic potential. N-1 N N+1 # Charge sensitivity: U N N+1 Voltage sensitivity: # 4 ~ 10 e / ~ 1µ V / Hz Hz Single Electron Transistor SET Current Spatial resolution: SiO2 ~ 100nm Electrostatic Potential T=300mK Si H. Hess, T. Fulton, M. Yoo, AY

Local Measurement of DOS Scanning Fixed T=300mK T=50mK Metal-Insulator Transition in 2D S. Ilani, et. al., PRL 84 (2000) Science 292 (2001) S. Ilani et al, Nature 328 (2004) Martin et al, Science (2004) Simultaneous Transport & Local Potential

Inverse compressibility Energy µ (n) Inverse compressibility dµ/dn DOS density density dn: AC voltage on backgate dµ: Single Electron Transistor 1µV, 100nm, B =[0 12 T], UHV, 300mK

Sample Geometry Transport 10µm Red: After first round of current annealing Blue, Green: New

Transport 1/3 2/3 1 R-2T 2 B [T] 2 Vbg [V] Red: After first round of current annealing Blue, Green: New Vbg [V]

Localized states Inverse Compressibility B Parallel to filling factor B. E. Feldman, AY, et al, arxiv: 1201.5128

Lowest Landau Level Localized states N=0 Landau Level 4 fold degeneracy spin and valley Valley ordered / CAF Valley and spin ordering 1/3 down to 1T B. E. Feldman, AY, et al, to appear in Science

Fractions in the Lowest Landau Level 7/5 11/7 5/3 No CF degeneracy s p ν = 2 p ±1

Filling Fraction vs Filling Factor ν=2 N=1 N=0 4-fold degeneracy ff=0 ν=0 ff=2-ν ff=1 ff=0 Filling fraction (ff) is analogous to the filling factor in GaAs

Missing Filling Fractions ff = p 2m = 2 p ± 1 4m ± 1 ν=4/3 ff=2/3 ν=10/7 ff=4/7 ν=14/9 ff=4/9 ν=8/5 ff=2/5 ν=2 ff=0 All fractions present Only even numerators Have CF degeneracy s ff=1+( 2/3, 3/5, 4/7, 5/9,, 4/9, 3/7, 2/5, 1/3 ) ff= 2/3, 4/7,, 4/9, 2/5

Filling Fraction vs Filling Factor ν=2 N=1 N=0 4-fold degeneracy ff=0 ν=0 ff=2-ν ff=1 ff=0 Filling fraction (ff) is analogous to the filling factor in GaAs No degeneracies Symmetries remain See also: Shayegan et al in AlAs Boebinger et al in double wells

Spatial Dependence B Fractions shift with position B = 12 T

Spatial Dependence B Fractions shift with position B = 6 T

Effects of Interactions in Suspended Graphene Ben Feldman, Andrei Levin, Amir Yacoby, Harvard University Broken and unbroken symmetries in the lowest LL: spin and valley symmetries. FQHE Discussions with Bert Halperin and Dima Abanin In collaboration with Benjamin Krauss, Jurgen Smet, MPI Stuttgart