UPPER TROPOSPHERIC WATER VAPOUR AND ITS INTERACTION WITH CIRRUS CLOUDS

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UPPER TROPOSPHERIC WATER VAPOUR AND ITS INTERACTION WITH CIRRUS CLOUDS INSIGHTS FROM TWO DECADES OF IAGOS IN-SITU OBSERVATIONS ANDREAS PETZOLD FORSCHUNGSZENTRUM JÜLICH AND THE IAGOS TEAM Contact: a.petzold@fz-juelich.de or GEWEX UTCC-PROES Workshop UPMC Sorbonne University Paris 22-23 Oct 2018

IN-SERVICE AIRCRAFT FOR A GLOBAL OBSERVING SYSTEM Association Internationale sans but lucratif European Research Infrastructure for Earth observation by passenger aircraft since 2014 Regular in situ global-scale monitoring of essential climate variables H 2 O, O 3, CO, NO x, CO 2, CH 4, aerosols, clouds Long-term deployment envisaged (> 20yrs) Today, 8 long-haul aircraft (IAGOS-CORE) and one flying laboratory (IAGOS-CARIBIC) Open data policy; visit Provision of data in near real time for Copernicus and other services Long time series from available for - tropopause temperature (> 20 yrs) - O 3, H 2 O, RH ice (> 20 yrs) - CO (> 15 yrs) - NO x (2 yrs)

THE IAGOS CORE SYSTEM H 2 O Cloud Det. Pump O 3 CO DAS/Modem Instrument: NO x or NO y CO 2, CH 4 or Aerosol O 2 Synth. Air Ventilation Smoke Det. Safety Panel Breaker

THE IAGOS CORE SYSTEM H 2 O Cloud Det. Pump O 3 CO DAS/Modem Instrument: NO x or NO y CO 2, CH 4 or Aerosol O 2 Synth. Air Ventilation Smoke Det. Safety Panel Breaker

IAGOS CAPACITIVE HYGROMETER (ICH) Hydroactive Polymer Film which adsorbes H 2 O molecules Capacitance depends on relative humidity (RH); C= 180-220 pf Strong temperature dependence Measured Signal = RH LIQUID In operation since 1995 Established technique for balloon soundings Low maintenance requirements Calibrations traceable to frost point mirror In-flight blind intercomparison: 5% RH liquid uncertainty, LOD approx. 20 ppmv Helten et al., JGR 1998; Neis et al., Tellus B 2015

BACKSCATTER CLOUD PROBE (BC) Particles pass through open laser beam and backscattered light is collected by a photodiode Size range: d p = 5 75 µm N ice, min = 0.015 cm -3 with 50% uncertainty No size distribution information provided In operation since 2011 Beswick et al., AMT 2014

THE IAGOS DATA SET - COVERAGE IAGOS - MOZAIC UTH / RH ice data IAGOS Cirrus RH ice - N ice data Data available since 1995 > 20 years of UTH data > 57000 flights, 500 flights/year/aircraft Data available since 2011 360 hours of in-cloud RH ice N ice data from 2014 to 2015 analysed Data selection criteria Altitude > 8 km, p < 350 hpa T amb < 233 K to exclude super-cooled water droplets

UTH VERTICAL VARIABILITY North Atlantic Central Europe Seasonal variation of 15 yrs. mean monthly median H 2 O VMR [ppmv] Distribution relative to the thermal tropopause height z TPH clearly visible moistening of the LMS in summer

UTH VERTICAL VARIABILITY North Atlantic Central Europe Seasonal variation of 15 yrs. mean monthly median H 2 O VMR [ppmv] Distribution relative to the thermal tropopause height z TPH clearly visible moistening of the LMS in summer Vertical distribution of RH ice in the vicinity of the thermal tropopause Vertical spacing of layers at z TPH is 30 hpa PDFs of occurrence indicate frequent supersaturation of UT Neis et al., in preparation

RH ICE TIME SERIES Average RH ice values LMS: approx. 10%, close to the LOD of ICH UT: > 80% Ice-supersaturation occurs regularly in the UT close to the tropopause No significant trends of the deviation of monthly RH ice from long-time average ( RH ice ) are observed Neis et al., in preparation

CIRRUS CLOUD PROPERTIES modal RH ice 100% > 100% > 110%? Dynamical equilibrium RH ice in clouds > 100% is driven by vertical velocity cooling during air mass updraft decrease of e sat,ice ice RH ice deposition of excess water vapour on existing ice crystals RH ice RH ice N ice correlations indicate: dynamic equilibrium RH ice N ice Petzold et al., Faraday Discuss. doi: 10.1039/c7fd00006e, 2017

CIRRUS CLOUD PROPERTIES Cirrus type: Equilibrium higher updraft convectively induced RH ice, mod 100% RH ice, mod > 100% RH ice, mod > 110% Petzold et al., Faraday Discuss. doi: 10.1039/c7fd00006e, 2017

OCCURRENCE OF ICE SUPERSATURATION North Atlantic Central Europe Neis et al., in preparation

OCCURRENCE OF ICE SUPERSATURATION January 2003 2008 AIRS High Cloud Amount July 2003-2008 Stubenrauch et al., ACP 2010

OCCURRENCE OF ICE SUPERSATURATION January 2003 2008 AIRS High Cloud Amount July 2003-2008 Stubenrauch et al., ACP 2010 IAGOS Occurrence of RH ice 100% 35% 30% 28% 21% 0 10 20 30 40 50 0 10 20 30 40 50

SUMMARY & NEXT STEPS Regular global-scale in situ data from MOZAIC / IAGOS are available for open access RH ice data since 1995 and RH ice N ice data since 2011 provide a highly valuable basis for research on upper tropospheric humidity and cirrus clouds IAGOS water vapour data will be used for SPARC OCTAV-UTLS (Observed Composition Trends and Variability in the UTLS) IAGOS water vapour cirrus data may be of value for GEWEX UTCC-PROES purposes Investigate long-term evolution of cirrus coverage over regions sampled by IAGOS Link IAGOS RH ice - cirrus observations to satellite observations of cirrus coverage

IN-SERVICE AIRCRAFT FOR A GLOBAL OBSERVING SYSTEM Association Internationale sans but lucratif IAGOS Data Services Available: O 3, CO, H 2 O (CORE NRT) O 3, CO (CARIBIC L1) In preparation: Cloud Index (CORE NRT) NO x /NO 2 (CORE L1) Calibration Centres calibration maintenance calibration data meta data IAGOS data products IAGOS Data Centre hosted by AERIS (CNES- CNRS/INSU) in Toulouse data near real time data for Copernicus model validation

IN-SERVICE AIRCRAFT FOR A GLOBAL OBSERVING SYSTEM Association Internationale sans but lucratif

THE IAGOS DATA SET VERTICAL COORDINATES Seasonal and regional variation of the tropopause height requires relative altitude coordinates. Data are grouped relative to the dynamical or thermal tropopause height (p dyn.tph ; p therm.tph ) according to Thouret et al. (JGR 2006).