Overview. 1. What range of ε eff, µ eff parameter space is accessible to simple metamaterial geometries? ``

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MURI-Transformational Electromagnetics Innovative use of Metamaterials in Confining, Controlling, and Radiating Intense Microwave Pulses University of New Mexico August 21, 2012 Engineering Dispersive Properties of Metamaterials Robert Lipton LSU

Overview 1. What range of ε eff, µ eff parameter space is accessible to simple metamaterial geometries? `` 2. A systematic & mathematically rigorous multi-scale ``bottom up methodology for linking subwavelength metamaterial geometry to effective parameters ε eff, µ eff?

Overview & Perspective 3. Goal: optimal beam-wave interaction. Design metallic sub-wavelength structures that mimic the response of a dielectric for generating slow electromagnetic waves. D. Shiffler, J. Luginsland, D.M. French, J. Watrous, IEEE Trans. Plasma Sci. 2010. 4. Objective. Control beam wave interaction frequencies by controlling intrinsic electrostatic resonances of metallic sub-wavelength structure.

Metamaterials & novel effective properties The first double negative materials made from metallic resonators and metallic posts. Smith et. al. Phys Rev. (2000). Operational at microwave frequencies. Several subsequent novel designs operational up to infrared. 1.Dolling, G., Enrich, C., Wegener, M., Soukoulis, C. M., Linden, S.: Opt. Lett. Vol 31, 1800 1802(2006) 2. Huangfu, J., Ran, L., Chen, H., Zhang, X., Chen, K., Grzegorczyk, T. M., Kong, J., A.: Appl. Phys. Lett. Vol 84, 1537(2004) Metamaterials proposed for Higer frequencies 1. Plasmonic nano particles: A. Alù, A. Salandrino, and N. Engheta, Opt. Expr. 14, 1557 (2006). 2. Optically thin metal films: V. Lomakin, Y. Fainman, Y. Urzhumov, & G. Shvets, Opt Expr. 14 11164 (2006) 3. Large permittivity dielectric inclusions K.C. Huang, M.L. Povinelli, & J.D. Joannopoulos, J. D. 2004 Appl. Phys.Lett. 85, 543.

Macroscopic properties µ eff, ε eff from sub-wavelength structure Objectives 1 and 2: recover an explicit multi-scale link between macroscopic properties µ eff, ε eff and geometry of sub-wavelength structures and understand range of properties accessible by simple sub-wavelength geometries. With explicit relation connecting microstructure and properties of an effective medium can systematically design sub-wavelength geometries Map sub-wavelength structure to Dispersion relations involving effective properties µ eff, ε eff

Electromagnetic Waves in Metamaterials Sub-wavelength power series: a bottom up approach Effective properties appear as leading order terms In an explicit sub-wavelength power series for dispersion relation and power series solution to Maxwell Equations Expansion parameter is length scale of structure divided by wavelength. (Sub-wavelength expansion). Higher order terms provide explicit corrections to the effective theory. λ κ k=2π/λ d

Sub-wavelength power series Negative index/ double negative properties from nonmagnetic materials: 1. Y. Chen & R. Lipton, Double Negative Dispersion Relations from Coated Plasmonic Rods. (Multiscale Modeling and Simulation) under revision, arxiv:1202.0602v1 [math.ap] 3 Feb 2012. 2. Y. Chen & R. Lipton, Resonance and double negative behavior in metamaterials. (Submitted) arxiv:1111.3586v1 [math.ap] 15 Nov 2011 3. Y. Chen & R. Lipton Tunable double negative band structure from non-magnetic coated rods. New Journal of Physics Vol. 12 (2010) 083010 Negative magnetic permeability from non magnetic materials: 1. S. Fortes, R. Lipton, S. Shipman ``Power series for high contrast sub wavelength media. Proc. R. Soc. London Series A2010 466: 1993-2022 2. S. Fortes, R. Lipton, S. Shipman``Convergent power series for fields in positive or negative high-contrast periodic media. Communications in PDE 36, 2011, pp.1016--1043

Examples of simple sub-wavelength materials with exotic EM properties Plasma loaded waveguide eff Dielectric loaded µ waveguide Veselago Medium eff Magnetic material loaded waveguide We provide examples of sub-wavelength geometries that capture the behavior in all four quadrants depending upon frequency of operation

Microstructured materials made from metallic and high dielectric rods x 3 d x 1 x 2

Periodic array of metal coated dielectric rods Chen, Lipton, New Journal of Physics Vol. 12 (2010) 083010 x 3 d x 1 x 2

Determine Waves Supported by the Metamaterial λ x 2 κ x 1 k=2π/λ d Sub-wavelength power series solution for the H field H= H 3 (x)e i(kκ x-ωt)

Frequency dependent sub-wavelength local properties To fix ideas consider metal coated rods Magnetic permeability µ=1 in host, rod core & rod coating Crystal period is d. Metallic coating, Drude model: ε P =ε(ω)=(1-(ω p /ω) 2 ) Host permittivity ε H =1. Rod core permittivity ε R =ε r /d 2. The wave number is k=2π/λ. Investigate wave propagation when 2πd/λ=kd=ƞ<1 Find convergent power series solution in kd=η.

Sub-wavelength power series solution Power series for the H field ( " ) exp i(k x #t) j=1 H 3 = u 0 0 (x / d)+ (dk) j i j j (x / d) { } Power series for the dispersion relation = (" (k,#)+ dk " (dk) m " ) 1/2 0 m m=0 Leading order term. Effects of spatial dispersion

The first order term in the dispersion relation Leading order dispersion relation for the metamaterial = " 0 (k, #) ξ 0 is a root of: µ eff ( 0 ) 0 = k 2 " eff ( 0 ) 1 # #

Natural Emergence of Effective Properties The generic effective dielectric constant and magnetic permeability exhibit multiple surface modes These explicit formulas emerge naturally via the power series ``bottom up approach and modes are controlled by the shape of the metallc inclusions and their relative positions µ eff ( 0 ) = " H +" p + " # µ n # n R 2 n=1 (µ n ( 0 ) 1 eff 0 ( ) = " H + p 0 ( ) 0 " r p 2 Formulas emerge from asymptotic analysis, They are not postulated from the top down ( 1/2<% h <1/2 ( 2 0 " r # ) 2 p $ 1 h 2 +2 ( 2 0 " r # p )" r # p2 $ h1 $ 2 h + (" r # 2 p ) 2 $ 2 h 2 " 0 (% h + 1 2 )" 2 $ # r# p % 2 ' & 0 " r # p ( )

A general theory for effective metamaterial properties The surface modes are determined by two distinct spectral problems intrinsic to the geometry & independent of materials Effective magnetic permeability: The poles µ n and weights <ϕ n > are the Dirichlet Eigenvalues µ n and averages of the Dirichlet eigenfunctions ϕ n for associated with the core. Core Effective Dielectric Constant: The numbers λ n and weights α n are the Eigenvalues λ n and averages of the eigenfunctions ψ n for an electrostatic resonance problem: 1 2 # v " $ 1 2 H % ( # v " = "' v * + v " * & ) P # H # P H P Y Generalization of Bergman-Milton Electrostatic resonances to multiple phases

Intervals of double negative and double positive effective properties Plasma loaded waveguide Veselago Medium - - µ eff ++ a Dielectric loaded waveguide eff Magnetic material loaded waveguide - a - b a b µ 1 ++ µ 2 µ 3 ξ 0 Figure: the relation between µ eff and ξ 0 ɛ 1 eff ˆκ ˆκ s 2 a b a b s 1 ɛ r ω 2 p c 2 ξ 0 Figure: the relation between ɛ 1 eff ˆκ ˆκ and ξ 0 YUE CHEN, ROBERT LIPTON

Intervals of single negative and single positive effective properties - + Plasma loaded waveguide Veselago Medium µ eff Dielectric loaded waveguide eff Magnetic material loaded waveguide - + - + +- - +

Example: Electrostatic Resonance Problem for Coated Cylinders The electrostatic resonances λ h are found by solving the following problem for the potential u inside a unit cell, i.e., d = 1: { u = 0 in H, (33) u = 0 in P, with the boundary conditions u = u on P, r u r=a = 0 on R, λ[ r u] + = 1 2 ( r u + r u + ) on P, H u is Y -periodic. (34) P R YUE CHEN, ROBERT LIPTON H

Electrostatic Resonances & Dirichlet Spectra Tools for designing leading order dispersion relation The first 10 electrostatic resonances λ n explicitly control the first 10 surface modes for the metamaterial Electro static resonances 3.508x10-1 1.537x10-2 9.755x10-4 6.103x10-5 3.814x10-6 -2.028x10-3 -5.533x10-3 -1.501x10-2 -4.453x10-2 -4.497x10-2 a b

Electrostatic Resonances (a) (b) Figure: (a) the solution corresponding to the eigenvalue λ = 3.5080 10 1 ; (b) the solution corresponding to the eigenvalue λ = 1.5379 10 2. YUE CHEN, ROBERT LIPTON

Comparison of leading order dispersion relations with direct numerical simulation I The following figures show the exact numerical solutions via COMSOL and how they compare to the leading order dispersion relation. 5 1.2 1 4 1 0.95 3 0.8 0.9 1 " eff #$# 2 1 0 µ eff 0.6 0.4 0.2 / p 0.85 0.8 0 0.75 1 0 0.2 0.4 0.6 0.8 1 1.2 1.4 0 / p 0.2 0 0.5 1 1.5 2 0 / p 0.7 0 0.2 0.4 0.6 0.8 1 dk (a) (b) (c) Figure: the case of a = 0.2d, b = 0.4d and ɛ R = 285. YUE CHEN, ROBERT LIPTON

Comparison of leading order dispersion relations with direct numerical simulation II 5 1.2 1 1 " eff #$# 4 3 2 1 0 1 2 µ eff 1 0.8 0.6 0.4 0.2 0 / p 0.95 0.9 0.85 0.8 0.75 3 0 0.2 0.4 0.6 0.8 1 1.2 1.4 0 / p 0.2 0 0.5 1 1.5 2 0 / p 0.7 0 0.2 0.4 0.6 0.8 1 dk (a) (b) (c) Figure: the case of a = 0.15d, b = 0.4d and ɛ R = 285. YUE CHEN, ROBERT LIPTON

Design of Microstructure for Double Negative Properties via Electrostatic & Dirichlet resnonances a 0.5xb 0.55xb 0.6xb 0.65xb b 0.3 0 0 0 0.8919 0.0332 a b 0.35 0 0.9003 0.02733 0.8315 0.03824 0.7716 0.04425 0.4 0.8707 0.03541 0.7960 0.04204 0.7345 0.04893 0.6830 0.05579 0.45 0.7795 0.04366 0.7141 0.05143 0.6605 0.05944 0.6161 0.06801

To add the additional effects of damping: just change frequency dependence of metallic phase to include damping the geometrically intrinsic electrostatic resonances stay the same ( p ) p =1 ( 0 ) 2 p ( ) 2 p i ( c )( p ) p c p = 0.01

Dispersion curves Complex wave number dk = dk r + idk i

Dielectric behavior from sub-wavelength metallic structure J.B. Pendry, A.J. Holden, W.J.Stewart, & I. Youngs, Phys. Rev. Lett. (76)25 4773 (1996). Use of structural geometry to generate low frequency plasmons. Apply this phenomena to design slow wave structures for amplifiers ``A Cerenkov-like Maser Based on a Metamaterial Structure, D.Shiffler, J. Luginsland, D.M. French, & J. Watrous, IEEE Transactions on Plasma Science (38)6 1462 (2010).

Control beam wave interaction frequencies by tailoring electrostatic resonances of metal structure Custom design of TWT from subwavelength metal dielectric structure in a circular waveguide through: (1) Geometric tailoring of intrinsic electrostatic resonances of the metallic structure. - This controls beam wave interaction frequencies. (2) Provide a capability for systematic design of TWT for maximum gain over maximum band width. (3) Corrections to dispersion relation associated with spatial dispersion can be computed explicitly with no phenomenology. V Beam k c eff "#

Dielectric behavior from sub-wavelength metallic structure Goal: Engineer shape so surface modes far below ω p / 2. Method: engineer electrostatic resonances (" ( ) 0 " p ) 2 = H + p ( 0 p ) 2 1 1 eff " 0 " p " 1/2<# h <1/2 (( 0 p ) 2 1) 2 " 1 h 2 +2 (( 0 p ) 2 1)" h1 " 2 h + " 2 h 2 (( 0 p ) 2 (# h +1/ 2) )(( 0 p ) 2 1) Chen, Lipton (Multiscale Modeling and Simulation) under revision, arxiv:1202.0602v1 [math.ap] 3 Feb 2012. Dielectric resonances or surface modes for 0 = s = p " h + 1 2 1 2 < < 1 h 2 Analysis gives And h " 1 2 Gives lowest surface mode s near zero

Controlling λ h provides control of surface modes and allows for the systematic design of effective dielectric functions for generation slow electromagnetic waves k eff c eff 1 V Beam r d = 200 + i5 c p = 0.01 ( p ( p ) 0 p ) 2 =1 ( p ) 2 i ( c p )( p )

Plans Development of a systematic theory & methodology for design of sub-wavelength metallic structures for dielectric response for generating slow electromagnetic waves. Method will address the control of surface modes through the tuning of sub-wave length geometry for control of electrostatic resonances. Provides a means for engineering dispersion relations for wave guides with slow waves.

Plans The associated analysis of bandwidth for short TWT s loaded with metamaterial will be carried out following the Methods of Schachter, Nation and Kerslick J. Appl. Phys. 68 (11) 1990, 5874. The results will be compared with direct numerical simulation for TWT s loaded with metallic sub-wavelength structures.