Granular materials (Assemblies of particles with dissipation )
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2 Granular materials (Assemblies of particles with dissipation ) Saturn ring Sand mustard seed Ginkaku-ji temple
3 Sheared granular materials packing fraction : Φ Inhomogeneous flow Gas (Φ = 012) Homogeneous flow (Shear rate γ) Dense liquid (Φ = 08) No flow Amorphous solid (Φ = 085)
4 Jamming transition Below ΦJ Above ΦJ Homogeneous flow (Shear rate γ) Dense liquid (Φ = 08) Transition point ΦJ Onset of rigidity No flow Amorphous solid (Φ = 085)
5 Rheology under steady shear frictionless case Shear stress σ T Hatano, M Otsuki, S Sasa, J Phys Soc Jpn, 76, (2007) non-linear rheological property For Φ < ΦJ, σ γ 2 (liquid) For Φ > ΦJ, σ const (solid) For Φ ΦJ, σ γ y γ Shear rate γ
6 Rheology under steady shear Shear stress σ T Hatano, M Otsuki, S Sasa, J Phys Soc Jpn, 76, (2007) σ / Φ - ΦJ β frictionless case T Hatano, J Phys Soc Jpn, 77, , (2008) Shear rate γ non-linear rheological property For Φ < ΦJ, σ γ 2 (liquid) For Φ > ΦJ, σ const (solid) For Φ ΦJ, σ γ y γ scaling plot Critical scaling law γ Φ-ΦJ -α σ(γ, Φ) = Φ - ΦJ y Φ S±(γ Φ-ΦJ -α )
7 Theory for exponents M Otsuki and H Hayakawa, PRE, 80, , (2009) Three Critical scaling laws T(γ, Φ) = Φ - ΦJ x Φ τ±(γ Φ-ΦJ -α ) σ(γ, Φ) = Φ - ΦJ y Φ S±(γ Φ-ΦJ -α ) P(γ, Φ) = Φ - ΦJ y Φ p±(γ Φ-ΦJ -α ) Four Assumptions S / P is constant P in high density region : P ~ Φ Characteristic time : P-1/2 Low density region : collision frequency T 1/2 Theoretical prediction for critical exponents Coulomb s friction : Hatano (2007) O Hern, et al, (2003) Wyart, et al (2005) Kinetic theory xφ = 3, yφ = 1, yφ = 1, α = 5/2 (for disks) Linear repulsive force
8 Rheology under steady shear frictionless case σ / ΔΦ T Hatano, J Phys Soc Jpn, 77, , (2008) M Otsuki and H Hayakawa, PRE, 80, , (2009) σ(γ, Φ) = Φ - ΦJ y Φ S±(γ Φ-ΦJ -α ) Theoretical prediction : α = 1, yφ = 2/5 (for disk) linear repulsive force γ ΔΦ -α σ(γ, Φ) = ΔΦ S±(γ / ΔΦ 5/2 ) ΔΦ = Φ - ΦJ
9 Problem The system under steady shear is not suitable to study the rigidity near the jamming transition In experiments, the steady shear is hard to realize We numerically investigate the rheological properties under oscillatory shear (OS)
10 Previous study on the system under OS B Tighe, PRL 107, (2011) Complex shear modulus G* G : real part close to the critical point close to the critical point G : imaginary part frequency ω System no mass, fixed contact networks, tangential friction Complex shear modulus exhibits critical scalings
11 Purpose of this work In the previous work, the attention is restricted to the small shear limit and the change of the contact network is not considered However, the change of the network dominates the rheological property near the jamming transition point We investigate the rheological properties under OS in a wide range of shear amplitude
12 Fn Fn Fn = k δ - η δ Elastic part Dissipative part
13 Shear strain : γ(t) = γ0 cos (ωt) Amplitude : γ0, Frequency : ω Shear stress : σ(t) Volume fraction : Φ Shear modulus : G* = G + i G G dt σ(t) cos (ωt) / γ0 Real part Storage modulus G - dt σ(t) sin (ωt) / γ0 Imaginary part Loss modulus G * (γ0, ω, Φ)
14 Shear strain : γ(t) = γ0 cos (ωt) Amplitude : γ0, Frequency : ω Shear stress : σ(t) Volume fraction : Φ Shear modulus : G* = G + i G G dt σ(t) cos (ωt) / γ0 Real part Storage modulus G - dt σ(t) sin (ωt) / γ0 Imaginary part Loss modulus G * (γ0, ω, Φ)
15 σ = σe + σk, σe = E γ, σk = η γ G = E, G = η ω Shear stress σ(t) red ω = 10-4 green ω = 10-3 blue ω = 10-2 ω 0 slope G width G Shear strain γ(t) Complex shear modulus G* G storage modulus G loss modulus G ω frequency ω
16 G * (γ0, ω, Φ) γ0 1 G * (γ0, ω, Φ) γ0 < 1 G * (γ0, ω, Φ) ω 0
17 G*(γ0, ω, Φ) γ0 1 Complex shear modulus G* Φ= 067, γ0=1 G loss modulus G storage modulus frequency ω Shear stress σ(t) ω 0 Φ= 067, γ0=1 Shear strain γ(t)
18 G*(γ0, ω, Φ) γ0 1 Complex shear modulus G* Φ= 067, γ0=1 G loss modulus G storage modulus frequency ω ω 0 elastic plastic plastic elastic σ = { E γ, (γ < γc) σy, (γc < γ)
19 G*(γ0, ω, Φ) γ0 1 Storage modulus G close to ΦJ red Φ = 067 green Φ = 066 blue Φ = 065 magenta Φ = 0648 γ0=1 γ0=1 Loss modulus G close to ΦJ red Φ = 067 green Φ = 066 blue Φ = 065 magenta Φ = 0648 frequency ω frequency ω
20 G*(γ0, ω, Φ) γ0 1 G*(ω, Φ) = ΔΦ g(ω / ΔΦ 5/2 ) ΔΦ = Φ - ΦJ γ0=1 γ0=1 G / Δφ red Φ = 067 green Φ = 066 blue Φ = 065 magenta Φ = 0648 G / Δφ red Φ = 067 green Φ = 066 blue Φ = 065 magenta Φ = 0648 ω / Δφ 5 / 2 ω / Δφ 5 / 2 γ0 σ(γ, Φ) = ΔΦ F±(γ / ΔΦ 5/2 )
21 G * (γ0, ω, Φ) γ0 > 1 G * (γ0, ω, Φ) γ0 < 1 G * (γ0, ω, Φ) ω 0
22 G*(γ0, ω, Φ) γ0 1 Complex shear modulus G* 006 γ0=10-3 γ0=10-3, ω=10-4 G : storage modulus close to ΦJ red Φ = 067 green Φ = 066 blue Φ = 065 G loss modulus frequency ω G G ~ ΔΦ 1/ Volume fraction Φ C O Hern, et al, Phys Rev Lett 88, (2002)
23 G * (γ0, ω, Φ) γ0 > 1 G * (γ0, ω, Φ) γ0 < 1 G * (γ0, ω, Φ) ω 0
24 G*(γ0, ω, Φ) ω 0 G0 (γ0, Φ) lim G (γ0, ω, Φ) ω 0 γc(φ) G0 G 0 = const γ0 < γc(φ) close to ΦJ red Φ = 0650, green Φ = 0652 blue Φ = 0655, magenta Φ = 0660 cyan : Φ = 0670 Shear amplitude : γ0 G 0 decreases as γ0 increases for γ0 > γc(φ) G 0 decreases as Φ approaches ΦJ
25 G*(γ0, ω, Φ) ω 0 G0 (γ0, Φ) = ΔΦ 1/2 h(γ0 / ΔΦ) lim h(x) x -1/2 x G ~ γ0-1/2 G ~ ΔΦ 1/2, for γ0 0 C O Hern, et al, Phys Rev Lett 88, (2002) G0 /ΔΦ 1/2 red Φ = 0650, green Φ = 0652 blue Φ = 0655, magenta Φ = 0660 cyan : Φ = 0670 γ0 / ΔΦ The yield strain γc is proportional to the contact length γc(φ) ~ ΔΦ B Tighe, et al, Phys Rev Lett 105, (2010) G0 is independent of Φ for ΔΦ 0
26 G*(γ0, ω, Φ) ω 0 G0 (γ0, Φ) = ΔΦ 1/2 h(γ0 / ΔΦ), lim h(x) x -1/2 x lim lim G0 (γ0, Φ) ΔΦ 1/2 ΔΦ γ0 0 γ0=10-4 C O Hern, et al, Phys Rev Lett 88, (2002) G ~ ΔΦ 1/2 lim G0 (γ0, Φ) ΔΦ ΔΦ cf TG Mason et al PRE (1997), experiments of emulsions H Yoshino, analysis of the replica method γ0=10-2 G ~ ΔΦ G0 G Volume fraction Φ Volume fraction Φ
27 G*(γ0, ω, Φ) ω 0 G0 (γ0, Φ) = ΔΦ 1/2 h(γ0 / ΔΦ), lim h(x) x -1/2 x log G 0 C ( ) = 10-1 = 10-2 = 10-3 = 10-4 = 10-5 lim lim G0 (γ0, Φ) ΔΦ 1/2 γ0 0 ΔΦ 0 log 0 lim G0 (γ0, Φ) ΔΦ ΔΦ 0
28 G*(γ0, ω, Φ) ω 0 G0 (γ0, Φ) = ΔΦ 1/2 h(γ0 / ΔΦ), lim h(x) x -1/2 x lim lim G0 (γ0, Φ) ΔΦ 1/2 ΔΦ γ0 0 γ0=10-4 C O Hern, et al, Phys Rev Lett 88, (2002) G ~ ΔΦ 1/2 lim G0 (γ0, Φ) ΔΦ ΔΦ cf TG Mason et al PRE (1997), experiments of emulsions H Yoshino, analysis of the replica method γ0=10-2 G ~ ΔΦ G G Volume fraction Φ Volume fraction Φ
29 G*(ω, Φ) = ΔΦ g(ω / ΔΦ 5/2 ) G (Φ - ΦJ) 1/2, G ω G0 (γ0, Φ) = ΔΦ 1/2 h(γ0 / ΔΦ)
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31 Model of granular materials Fn Ft Φ < ΦJ Φ > ΦJ Ft Normal force Fn Tangential force Friction coefficient : μ Fn = k δ Δ - η vn Ft < μ Fn (Coulomb s friction) Elastic part Dissipative part Δ = 1 (Disk) Frictionless : μ = 0 Δ = 3 / 2 (Sphere) Frictional : μ > 0 Important parameters : Δ, μ
32 Critical property (without shear) Frictionless case, Δ = 1 Φ < ΦJ Φ > ΦJ Shear modulus G ~ (Φ- ΦJ) 1/2 Pressure P ΦJ Viscosity η η ~ (ΦJ- Φ) -3 P ~ (Φ- ΦJ) ΦJ Φ - ΦJ
33 Critical scalings Shear stress σ Frictionless case, Δ = 1 σ(γ, Φ) / Φ - ΦJ β scaling plot Shear rate γ non-linear transport property For Φ < ΦJ, σ γ 2 (liquid) For Φ > ΦJ, σ const (solid) For Φ ΦJ, σ γ y γ γ Φ-ΦJ -α Hatano, 2008 σ(γ, Φ) = Φ - ΦJ β S±(γ Φ-ΦJ -α ) second order transition
34 Characteristic features Mean field theory Dimension D = 2, 3, 4 with the same exponents obtained from the theory The critical exponents depend on the type of the contact force Fn = k δ Δ The critical exponents are independent of the dimension M Otsuki and H Hayakawa, Phys Rev E, 80, , (2009)
35 Effect of Friction σ σ Frictionless (μ = 00) Frictional (μ = 20) Hysteresis loop for frictional case M Otsuki and H Hayakawa, Phys Rev E 83, (2011)
36 Effect of friction (pressure in the zero shear limit) Pressure P Pressure P ΔP Frictionless (μ = 00) Continuous transition Frictional (μ = 20) Discontinuous transition
37 Effect of friction (type of the transition) 0005 ΔP ΔP Continuous transition Discontinuous transition Friction coefficient μ
38 Phase diagram P ~ (Φ- ΦS) Area of the hysteresis loop ΔP ΦC ΦS ΦS ΦC Many critical densities
39 An amount of the hysteresis loop phase diagram
40 Scaling relations Solid branch P ~ ( ) Δ, S ~ ( ) Δ,
41 Scaling relations liquid branch P ~ γ 2 ( ) -4, S ~ γ 2 ( ) -4
42 Granular rheology Shear stress : S low density critical density high density 0 70 Shear rate γ2 Yield stress : SY low density S γ 2 critical density S γ y γ high density S SY Yield stress : SY (Φ - ΦJ) y Φ Bagnold law
43 Theory for exponents Assumption S / P is constant P in high density region : P ~ Φ Δ Δ-dependent critical exponents PTP, PRE (2009) Coulomb s friction : Hatano (2007) O Hern, et al, (2003) Characteristic time : P-1/2 Wyart, et al (2005) Low density region : collision frequency T 1/2 Kinetic theory normal force cf Hatano 2010, Teigh 2010 (yφ = Δ + 05)
44 Derivation of exponents γ 0, Φ > 0 Δ average force : Fc(Φ) k δ(φ) compression length δ(φ) Φ Fn=kδ Δ δ C S O Hern, et al (2003) Assumption : S/P is constant Coulomb s law
45 Two branches Solid branch Liquid branch different contact number contact number > 3 contact number < 2
46 Exponents in other works Author yφ yγ = α / yφ yφ xφ α system critical point shear rate Number of particles Olsson & Titel 2007 Hatano 2008 Otsuki, Hayakawa, 2009 Tighe et al 2010 Hatano 2010 Nordstrom et al 2010 Olsson & Titel = Δ+02 (Δ=1) 12 = Δ+02 (Δ=1) foam 063 (Δ=1) 12 = Δ+02 (Δ=1) 25 (Δ=1) 19 (Δ=1) granular Δ 2Δ / (Δ+4) Δ Δ+2 (Δ+4) / 2 granular Δ+05 1/2 foam 15 = Δ+05 (Δ=1) 21 = Δ+06 (Δ=15) 108 = Δ +008 (Δ=1) 06 (Δ=1) 048 (Δ=15) 028 (Δ=1) 15 = Δ+05 (Δ=1) 108 = Δ +008 (Δ=1) 33 (Δ=1) 25 (Δ=1) 41 (Δ=15) 385 (Δ=1) granular (diameters 1:14) 0646 (diameters 1:14) 0648 (diameters 1:14) (diameters 1:14) (diameters 1:14) foam 0635 foam (diameters 1:14) ~ x 10-7 ~ 5 x ~ ~ ~ 10-6
47 Correlation length ξ μ
48 Correlation function Cp(r) r
49 glass spheres in oil Sheared granular material Eric Brown, et al (2010) Hysteresis loop appears in this system [private communication] Related experiment
50 Granular rheology Shear stress : S low density critical density high density 0 70 Shear rate γ2 Yield stress : SY low density S γ 2 critical density S γ y γ high density S SY Yield stress : SY (Φ - ΦJ) y Φ Bagnold law
51 Critical scaling γ : scaling plot Hatano, 2008
52 Theory for exponents Assumption S / P is constant P in high density region : P ~ Φ Δ Δ-dependent critical exponents PTP, PRE (2009) Coulomb s friction : Hatano (2007) O Hern, et al, (2003) Characteristic time : P-1/2 Wyart, et al (2005) Low density region : collision frequency T 1/2 Kinetic theory normal force cf Hatano 2010, Teigh 2010 (yφ = Δ + 05)
53 Derivation of exponents γ 0, Φ > 0 Δ average force : Fc(Φ) k δ(φ) compression length δ(φ) Φ Fn=kδ Δ δ C S O Hern, et al (2003) Assumption : S/P is constant Coulomb s law
54 Validity of the theory normal force yφ / α
55 Scaling law high density region( ) + low shear limit(γ 0) P ~ ( ) Δ, S ~ ( ) Δ low density region( ) + low shear limit(γ 0) P ~ γ 2 ( ) -4, S ~ γ 2 ( ) -4 ( ) -4 ( ) -4 P / γ 2 S / γ 2 low shear limit low shear limit
56 Protocol We sequentially change shear rate Shear rate Shear rate time time
57 Shear stress μ=00 μ=20 Similar behavior to the frictionless case γ critical density γ Hysteresis loop appears around the critical point
58 Scaling law frictionless high density region( ) + low shear limit(γ 0) P ~ ( ) Δ, S ~ ( ) Δ, low density region( ) + low shear limit(γ 0) P ~ γ 2 ( ) -4, S ~ γ 2 ( ) -4
59 Scaling laws frictional Solid branch liquid branch P ~ ( ) Δ, S ~ ( ) Δ, critical densities P ~ γ 2 ( ) -4, S ~ γ 2 ( ) -4 cf Somfai, et al (2007), Silbert (2010) [unsheared case]
60 Finite-size effect μ=12 μ=20 solid to liquid :N=8000 :N=16000 :N=32000 :N=8000 :N=16000 :N=32000 solid to liquid
61 Scaling in the liquid branch S ~ γ 2 ( ) -4 P ~ γ 2 ( ) -4, S / (A γ 2 ) P / (A γ 2 )
62 Scaling in the liquid branch S ~ γ 2 ( ) -4 P ~ γ 2 ( ) -4, S / (A γ 2 ) P / (A γ 2 )
63 Critical exponents
64 Model (frictionless grains) δ Δ=1(Linear model) Δ=3/2(Hertz model) Δ Interaction Force F=kδ Compressed Length δ The exponent for the interaction Δ Dissipative force between the contacting particles
65 Scaling function Scaling properties of S, T, P, ω jammed 1st eq
66 Pressure & shear stress For γ 0, Φ > 0 jammed phase Δ average force : Fc(Φ) k δ(φ) compressed length δ(φ) (σ/dφj)φ C S O Hern, et al (2003) Assumption S/P is independent of Φ Coulomb friction T Hatano (2007) 2nd eq 3rd eq
67 Characteristic frequency For γ 0, Φ > 0 jammed phase fc D(f) D(f) : Density of state f : frequency, fc : cut-off frequency,, Wyart et al (2005) f Assumption ω is scaled by fc For γ 0, Φ < 0 unjammed phase vc : characteristic velocity l (Φ) : mean free path 4th eq final eq 2 vc T/m l (Φ) (σ/dφj) Φ
68 Critical exponents The exponents depend on Δ
69 Previous works Our theory : The results are consistent with Previous works : our prediction 2-dimensional elastic particles R Garcia-Rojo, et al, PRE (2006) 3-dimensional elastic particles Singular behavior around Φ = ΦG < ΦJ L Berthier and T A Witten, EPL (2009)
70 Pair correlation functions Structure factor Pair correlations The first peak exceeds the maximum value of this graph D=3, mono-disperse, Δ=1 S(k) does not show any critical behaviors The first peak of g(r) changes drastically near ΦJ
71 Divergence of the first peak small shear magnification σ0 The first peak diverges as the shear rate gets smaller
72 Scaling of the first peak coordination number : Z Pressure : P The results are consistent with our predictions dilute g(r) have peak g0 around r=σ0 dense D=3, mono-disperse,δ=1
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76 There is no singularity other than point J
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81 ΦJ for static granular packing Stress control simulation φj1 is related with φj Silbert, et al (2001) Ciamarra, et al (2010) φj2 is related with φl Discussion : previous works
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