A.BIDAUD, I. KODELI, V.MASTRANGELO, E.SARTORI

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1 SENSITIVITY TO NUCLEAR DATA AND UNCERTAINTY ANALYSIS: THE EXPERIENCE OF VENUS2 OECD/NEA BENCHMARKS. A.BIDAUD, I. KODELI, V.MASTRANGELO, E.SARTORI IPN Orsay CNAM PARIS OECD/NEA Data Bank, Issy les moulineaux

2 One certainty about nuclear data : they are not the «good» one ----JEFF-30 MATERIAL INCIDENT NEUTRON DATA ENDF-6 FORMAT ***************************** JEFF-3.0 ************************* DATA TAKEN FROM :- ENDF/B-VI.3 (DIST-SEP91 REV1-JUL91)

3 Geometry Mesh size Nuclear Data Geometry Temperatures Sensitivity and Uncertainty Code System Mesh + input generation BOT3P Adjoint and direct calculation DORT Nuclear Data Geometry, densities Temperatures Energy group structure multigroup cross-section set production Partial Cross Section Covariance matrices production NJOY Sensitivity and uncertainty calculation SUSD3D

4 VENUS 2 Benchmark Zero power Thermal Water reactor in SCK*CEN (Belgium) Partial MOX fuelled Axial and radial pin power distribution measurements are available Deterministic and Monte-Carlo calculations are compared Most recent data libraries were used

5 Cross section preparation 199 group library based on VITAMIN-B6 fine group library processed with SCALE group library processed by RESMOD code, provided by W. Zwermann(GRS) 2D and 3D calculations with both library Impact of Buckling factor on 2D results

6 Calculation Kinf or keff Participant's average UO2 3,3% Cell 1, ,40646 UO2 4,0% Cell 1, ,33769 MOX Cell 1, , D 199g core 0, D 18g Core 1,0052 1, ,15 1,1 1,05 C/E 1 0,95 0,9 0,85 UO2 3/0 UO2 4/0 MOX 2/2,7 SCALE199g ZWERMAN 18g C/E=1

7 material H1 B10 O16 (n,gamma) (n,alpha) (n,gamma) 2D zwermann -3,86E-02-4,35E-02-2,05E-05 3D zwermann -4,63E-02-4,27E-02-2,21E-05 2D 199g -3,98E-02-3,18E-02-2,10E-05 3D 199g -5,41E-02-3,28E-02-2,49E-05 material U235 U238 Pu239 reaction (n,gamma) fission Nu total (n,gamma) fission Nu total (n,gamma) fission Nu total 2D zwermann -1,05E-01 3,21E-01 8,06E-01-1,75E+00 5,74E-02 7,97E-02-3,25E-02 5,39E-02 1,15E-01 3D zwermann -1,04E-01 3,23E-01 8,06E-01-1,70E+00 5,73E-02 7,91E-02-3,25E-02 5,41E-02 1,15E-01 2D 199g -1,09E-01 3,45E-01 8,38E-01-1,66E+00 4,00E-02 6,12E-02-2,79E-02 4,87E-02 1,00E-01 3D 199g -1,16E-01 3,10E-01 8,36E-01-1,73E+00 4,13E-02 6,21E-02-3,03E-02 4,57E-02 1,02E-01

8 2D-3D Comparison 3D allows axial reflector explicit model =>more H2O atoms in the 3D model! Mat. Reaction 2D 3D(Volume corrected) H-1 Elastic 3.37E E-1 (3.55E-1) (n,γ) -3.86E E-2 (-3.84E-2) O-16 Elastic 3.59E E-2 (4.69E-2) (n,γ) -6.54E3-6.45E-3 (-6.40E-3)

9 Buckling Effect Material reaction 2D 199g critical B2 H1 (n,gamma) -3,98E-02-3,93E-02 B10 (n,alpha) -3,18E-02-3,59E-02 O16 (n,gamma) -2,10E-05-2,08E-05 (n,gamma) -1,09E-01-1,09E-01 U235 fission 3,45E-01 3,47E-01 Nu total 8,38E-01 8,40E-01 (n,gamma) -1,66E+00-1,67E+00 U238 fission 4,00E-02 4,09E-02 Nu total 6,12E-02 6,26E-02 (n,gamma) -2,79E-02-2,69E-02 Pu239 fission 4,87E-02 4,79E-02 Nu total 1,00E-01 9,78E-02 No real impact but for boron =>Strong impact of self shielding effect

10 Sensitivity profile 5,00E-01 Sensitivity per Unit Lethargy 0,00E+00-5,00E-01-1,00E+00-1,50E+00-2,00E+00 U238 capture 18g U238 capture 199g -10*(H1 elas) -2,50E+00 1,E-05 1,E-03 1,E-01 1,E+01 1,E+03 1,E+05 1,E+07 1,E+09 Energy

11 5% underestimation on fission rates == 15% underestimation in sensitivity 3,50E-02 3,00E-02 Sensitivity per Unit Lethargy 2,50E-02 2,00E-02 1,50E-02 1,00E-02 5,00E-03 Pu 239 fission 18g Pu 239 fission 199g 0,00E+00 1,E-05 1,E-03 1,E-01 1,E+01 1,E+03 1,E+05 1,E+07 1,E+09 Energy

12 Impact of Boron macrocell calculation 7,0E+03 6,0E+03 5,0E+03 4,0E+03 3,0E+03 2,0E+03 1,0E+03 without self shielding with selfshielding 0,0E+00 1,0E-05 1,0E-04 1,0E-03 1,0E-02 1,0E-01 1,0E+00 0,00E+00-2,00E-03-4,00E-03-6,00E-03-8,00E-03-1,00E-02-1,20E-02-1,40E-02 2D 18g 2D 199g 2D 18g corrected -1,60E-02 1,E-05 1,E-03 1,E-01 1,E+01 1,E+03 1,E+05

13 Covariances matrices : U238 capture σ/σ vs. E for 238 U(n,γ) Correlation Matrix Linear Axes: Rel. Standard Dev. (%) Logarithmic Axes: Energy (ev) σ/σ vs. E for 238 U(n,γ) σ/σ vs. E for 238 U(n,γ) Correlation Matrix Linear Axes: Rel. Standard Dev. (%) Logarithmic Axes: Energy (ev) σ/σ vs. E for 238 U(n,γ)

14 Uncertainties based on various covariance data Uncertainty Uncertainty Material reaction Sensitivity (%/%) JENDL 3.2 (pcm) IRDF-90 (pcm) B10 (n,alpha) -4,35E (n,gamma) -1,05E _ U235 fission 3,21E Nu total 8,06E _ (n,gamma) -1,75E U238 fission 5,74E Nu total 7,97E _ (n,gamma) -3,25E _ Pu239 fission 5,39E Nu total 1,15E-01 6 _ Total (pcm)

15 Conclusions (1) Our multidimentional tests shows that : Sensitivities to fuel isotopes are not much sensitive to geometrical modelisation Errors on reaction rates due to cross section preparation impacts the sensitivities For some isotopes with strong self-shielding, the partial cross sections needed for sensitivity analysis done with NJOY bodarenko s method can be inacurrate.

16 Conclusions (2) Total uncertainty is about 1% which is larger than participant results spread. U238 first resonances are responsible for a very large part of it. Neutron yelds are the second source of uncertainties. Analysis results are limited by poor nuclear data uncertainty information (lack of covariance matrices in evaluated files).

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