Energy Resolution of LaBr 3 (Ce) Gamma-Ray spectrometer for Fusion Plasma Studies on JET

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EFDA JET CP(10)03/19 M. Nocente, M. Tardocchi, I. Chugunov, R.C. Pereira, T. Edlington, A.M. Fernandes, D. Gin, G. Grosso, V. Kiptily, A. Murari, A. Neto, E. Perelli Cippo, A. Pietropaolo, I. Proverbio, A. Shevelev, J. Sousa, B. Syme, G.Gorini and JET EFDA contributors Energy Resolution of LaBr 3 (Ce) Gamma-Ray spectrometer for Fusion Plasma Studies on JET

This document is intended for publication in the open literature. It is made available on the understanding that it may not be further circulated and extracts or references may not be published prior to publication of the original when applicable, or without the consent of the Publications Officer, EFDA, Culham Science Centre, Abingdon, Oxon, OX14 3DB, UK. Enquiries about Copyright and reproduction should be addressed to the Publications Officer, EFDA, Culham Science Centre, Abingdon, Oxon, OX14 3DB, UK. The contents of this preprint and all other JET EFDA Preprints and Conference Papers are available to view online free at www.iop.org/jet. This site has full search facilities and e-mail alert options. The diagrams contained within the PDFs on this site are hyperlinked from the year 1996 onwards.

Energy Resolution of LaBr 3 (Ce) Gamma-Ray spectrometer for Fusion Plasma Studies on JET M. Nocente 1, M. Tardocchi 1, I. Chugunov 2, R.C. Pereira 3, T. Edlington 4, A.M. Fernandes 3, D. Gin 2, G. Grosso 1, V. Kiptily 4, A. Murari 5, A. Neto 3, E. Perelli Cippo 1, A. Pietropaolo 1, I. Proverbio 1, A. Shevelev 2, J. Sousa 3, B. Syme 4, G.Gorini 1 and JET EFDA contributors* JET-EFDA, Culham Science Centre, OX14 3DB, Abingdon, UK 1 Dipartimento di Fisica, Università degli Studi di Milano-Bicocca and Istituto di Fisica del Plasma, Associazione EURATOM-ENEA-CNR, 20125 Milano, Italy 2 A. F. Ioffe Physico-Technical Institute, St. Petersburg 194021, Russian Federation 3 Associação EURATOM/IST Centro de Fusão Nuclear, Instituto Superior Técnico, 1049-001 Lisboa, Portugal 4 EURATOM-CCFE Fusion Association, Culham Science Centre, OX14 3DB, Abingdon, OXON, UK 5 Associazione EURATOM-ENEA sulla Fusione, Consorzio RFX Padova, Italy * See annex of F. Romanelli et al, Overview of JET Results, (Proc. 22 nd IAEA Fusion Energy Conference, Geneva, Switzerland (2008)). Preprint of Paper to be submitted for publication in Proceedings of the 18th High Temperature Plasma Diagnostics, Wildwood, New Jersey, USA. (16th May 2010-20th May 2010)

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ABSTRACT. A new high efficiency, high resolution, fast γ-ray spectrometer was recently installed at the JET tokamak. The spectrometer is based on a LaBr 3 (Ce) scintillator coupled to a photo multiplier tube. A digital data acquisition system is used to allow spectrometry with event rates in excess of 1MHz expected in future JET DT plasmas. However at the lower rates typical of present day experiments digitization can degrade the energy resolution of the system depending on the algorithms used for extracting pulse height information from the digitized pulses. In this paper the digital and analog spectrometry methods were compared for different experimental conditions. An algorithm based on pulse shape fitting was developed providing energy resolution equivalent to the traditional analog spectrometry method. 1. INTRODUCTION Gamma Ray Spectrometry (GRS) is used on the JET fusion device for observation of reactions between energetic ions and plasma impurities [1,2,3]. Different γ-ray spectrometers are available since 2009: i) A High purity Germanium (HpGe) was installed because of its very high energy resolution [4]. The crystal is sensitive to neutron damage, which limits the use of this detector in a fusion environment. When used, it provides data of excellent quality in the γ-ray energy range up to 5MeV. ii) Bismuth Germanate (BGO) and Sodium Iodide (NaI) detectors. These detectors were used at JET for a number of years [3] because of their high efficiency and reasonably good energy resolution over a broad range of γ-ray energies. iii) The latest addition to the GRS instrument suite is a Lanthanum Bromide (Brillance) detector. LaBr3(Ce) is a new scintillating material [5] delivering a very high light yield and hence energy resolution. It is also fast (see pulse shape in Fig.1) and insensitive to neutrons. Our 3 6 LaBr 3 (Ce) crystal is coupled to a Hamamatsu Photo Multiplier Tube (PMT) designed to allow operations at rates up to 2MHz [6]. The PMT signal is fed into a fast pre-amplifier with 5 gain before being digitized. High rate capability is enabled by a dedicated pulse digitization data acquisition system [7] based on the ATCA platform with a sampling frequency up to 400MSPS and a nominal 14-bit resolution. The acquisition board has channels with AC or DC coupling. A threshold on the signal coming from the PMT is set to avoid noise peak-up. When the signal exceeds the threshold a trigger is set and a data segment is stored consisting of 128 samples. The first 30 sample points are taken immediately before the trigger. This provides the baseline level for each event. The remaining points contain the actual digitized pulse. Each digitized event has an associated time-stamp to allow for time resolved data analysis. The digital data acquisition system is used to allow for spectrometry measurements with event rates in excess of 1MHz, expected in future JET DT plasmas. However at the lower rates typical of 1

present day experiments digitization can degrade the energy resolution of the system depending on the algorithms used for extracting pulse height information from the digitized pulses. The effect of digitization and different processing algorithms are studied here by comparing the results of digital and analog spectrometry for different experimental conditions. 2. SPECTRUM RECONSTRUCTION ALGORITHMS Dedicated algorithms were developed to build the event pulse height spectrum. A first algorithm named MAIA (Maximum Algorithm for Intershot Analysis) was written with the aim of providing a spectrum immediately after a JET discharge. The code is written in C and takes about 15 seconds to reconstruct a spectrum made of 10 5 events when running on a computer of the JET Analysis Cluster (JAC). The event pulse height is extracted from the corresponding data segment by taking the difference between the sample with maximum height inside the segment and the baseline. The latter is evaluated as an average of the first 20 points of the segment. A second algorithm named ORSA (Offline Reconstruction Simple Algorithm) was developed to better cope with noisy data. The absence of an hardware noise filtering stage between the PMT and the ATCA implies that baseline noise is reflected into the sampled pulse. Moreover, amplitude walks can introduce an uncertainty on the baseline value determined as average of the first 20 points of each segment. Noise filtering is achieved in ORSA by pulse fitting. The shape S(t) of each digitized event is described as y 0 if t < t 0 S (t) = y 0 + N (1- exp (-(t-t 0 ) / τ 1 )) p. exp (-(t-t 0 ) / τ 2 ) if t > t 0 (1) where y 0, N, t 0, are fit parameters. τ 1, τ 2 and P are instead determined by a pre-fit and kept constant for all the pulses; i.e. the pulse shape is assumed not to depend on γ-ray energy. Best values for these parameters were found to be τ 1 = 31.6ns, τ 2 = 23.8ns and P = 3.5 when the accelerating voltage VHV between the anode and the photocathode of the PMT was 800 V. τ 1 was found to have a slight dependence on VHV, while τ 2 and P were independent of VHV. An example of the fit accuracy is shown in Figure 1. Like MAIA, the pulse height of each event is determined from the difference between the maximum and the baseline, but now the fitted pulse shape is used instead of the raw data. ORSA is slow compared to MAIA but provides better results. 3. RESULTS The pulse height resolution of the system was investigated in laboratory tests and compared to that of an analog spectrometry chain consisting of a preamplifier+shaping amplifier and an ADC unit. The PMT was operated with V HV = 800V. Gamma rays from 137 Cs and 60 Co radioactive sources were detected and the pulse height spectrum reconstructed using both ORSA and MAIA algorithms. 2

The reconstructed 137 Cs peak at 661.66 kev is shown in Fig.2 as resulting from the three approaches in the case of measurements performed in low noise laboratory conditions. Pulse height resolution (FWHM) values at the three calibration peaks can be compared in Table 1. One can see that the values obtained with the ORSA algorithm are close to the analog spectrometry values. This is an important result since it shows that digitization in itself does not degrade the resolution of the measurement. On the other hand it is essential for enabling spectrometry at high rates. The results obtained with MAIA, although not optimal, are still better than the NaI and BGO detectors previously used at JET: they feature a resolution of about 7% at the same energy. Figure 3 shows the achieved resolution (FWHM in kev and in %) of the 137 Cs line at 661.66keV during experiments at a Tandem accelerator for different photo multiplier voltage. For comparison the best resolution obtained with an analog chain in low noise laboratory conditions is also shown. Again the analog spectrometry chain and the ORSA algorithm are found to provide similar results. Optimal resolution is achieved when V HV 800V, with no significant improvement in resolution at higher PMT operating voltages. Resolution with the MAIA algorithm is instead improved by choosing a higher voltage value. This suggests that cable noise is the main cause for resolution deterioration and is partly compensated for by increasing the signal amplitude. The LaBr 3 spectrometer was successfully used at JET to measure γ-ray spectra in recent experiments where fast ions were produced by Ion Cyclotron Resonance Heating (ICRH). The digital data acquisition proved to be high reliable with practically no loss of data due to malfunction. Figure 4 shows a pulse height spectrum measured during an experiment in a ( 3 He)H plasma meant to study minority and mode conversion heating in inverted ( 3 He)H scenarios [8, 9] of relevance for the non-active phase of ITER [10]. First harmonic ICRH was tuned to fundamental 3 He frequency. When the 3 He concentration was sufficiently low, high energy tails in the 3 He distribution function were created as a result of ICRH heating. These fast ions in turn induced γ-ray emission when interacting with impurities inside the machine (typically 12 C and 9 Be at JET)[3]. In ( 3 He)H plasmas γ-rays from the reaction 9 Be( 3 He, pγ) 11 B were expected to be observed. These are represented by the peak at 4.44 MeV in Figure 4, due to a transition from the second to ground state of 11B. However, γ-ray emission from the reaction 12 C(d, p) 13 C was also observed, which implied production of deuterons with energy greater than 0.5MeV [3]. This unexpected event is represented by the peak at 3.09MeV in figure 4 due to transition from the first to ground state of 13 C. The two peaks at lower energies are instead due to calibration sources (the peak at 661.66keV is due to 137 Cs) or to the detector intrinsic radioactivity (peak at 1473keV due to excited 138 Ba, produced after electron capture on 138 La). Figure 5 shows the temporal evolution of signal proportional to the γ-ray emission due to the reactions 9 Be( 3 He, pγ) 11 B and 12 C(d, p) 13 C. The coherent trend shows that 3 He and d ions were both accelerated by the applied ICRH and illustrates the time resolution achieved with the new LaBr 3 spectrometry system. Much higher rates and better time resolutions are expected from this system when plasmas with alpha particles and 9 Be impurities are available e.g. in DT fusion experiments in JET and ITER. 3

CONCLUSIONS A LaBr 3 (Ce) scintillator with fully digital data acquisition designed for high rate operation was installed at JET. Dedicated spectrum reconstruction algorithms were written to allow for immediate visualization of the measured γ-ray spectrum or to provide pulse height resolution matching the best resolution available from conventional analog spectrometry chains. The system was successfully used during recent JET experiments where it provided data at relatively low rates. Much higher rates are envisaged in future DT plasmas due to the presence of energetic alpha particles. REFERENCES [1]. F.E. Cecil et al., Nucl. Instrum. Methods 221, 449 (1984) [2]. V. G. Kiptily et al., Rev. Sci. Instrum. 74, 1753 (2003) [3]. V.G. Kiptily et al., Nucl Fus. 42, 999 (2002) [4]. A.Murari et al., New Developments in the Diagnostics for the Fusion Products on JET in preparation for ITER, these Proceedings [5]. E.V.D. Van Loef et al., Nucl. Instr. Meth. A 486, 254 (2002) [6]. M. Tardocchi et al., Rev. Sci. Instrum. 79, 10E524 (2008) [7]. R.C. Pereira et al., Fusion Eng. Des. 83, 341 (2008). [8]. M.-L. Mayoral et al., Nucl. Fus. 46, S550-S563 (2006) [9]. E. Lerche et al., Experimental investigation of ICRF heating scenarios for ITER s half-field phase performed in JET, in Proc. 37th EPS Conference on Plasma Phys. and Contr. Fusion Dublin, Ireland, 21-25 June 2010, to be published [11]. ITER Physics Basis Editors, ITER Physics Expert Group Chairs and Co-Chairs and ITER Joint Central Team and Physics Integration Unit Nucl. Fusion 39 12 (1999) Gamma ray peak MAIA ORSA Analog Chain 662 kev ( 137 Cs) 4.4% 3.3% 3.2% 1173 kev ( 60 Co) 3.2% 2.5% 2.4% 1333 kev ( 60 Co) 3.0% 2.4% 2.3% Table 1: Comparison of pulse height resolution values obtained with the digital spectrometry system and the ORSA and MAIA algorithms described in the text for characteristic calibration γ-ray peaks. Results from an analog spectrometry chain are also shown for comparison. 4

Amplitude (a.u.) 800 400 Data Fit Counts (a.u.) 1.0 MAIA ORSA Analog chain 0.6 0 0 80 160 240 Time (ns) JG10-50-1c 320 0.2 630 650 670 690 710 Energy (kev) JG10.50-2c Figure 1: Example of LaBr 3 (Ce) digitized pulse from a 1.5 MeV γ- ray. The solid line is the best fit to the data using Eq. 1. Figure 2: Comparison of a reconstructed 137 Cs peak at 661.66keV using the digitized data processed with the MAIA (dashed) and ORSA (dash-dotted) algorithms. Results from an analog spectrometry chain are also shown for comparison (full line). Measurements performed in low noise laboratory conditions. JG10.50-3c 40 MAIA ORSA Analog chain 6.5 137 Cs 138 Ba 12 C(d, pγ) 13 C Resolution (kev) 30 5.5 4.5 Resolution (%) Intensity (counts/kev) 1 9 Be( 3 He, pγ) 11 B 20 700 800 900 1000 V HV (V) 3.5 0.1 1000 2000 3000 4000 5000 Energy (kev) JG10.50-4c Figure 3: Resolution (FWHM in kev and in %) of the 137Cs line at 661.66keV during experiments at a Tandem accelerator for different photo multiplier voltage. The analog spectrometry chain (triangles) and the ORSA algorithm (circles) provide similar results. The MAIA algorithm (squares) is somewhat worse. The dashed line represents the best resolution obtained with an analog chain in low noise laboratory conditions. Figure 4: Gamma ray spectrum from JET Pulse No: 79352 obtained with the digital spectrometry system and the ORSA algorithm described in the text. Gamma ray peaks due to the 12 C(d, pγ) 13 C and 9 Be( 3 He, pγ) 11 B reactions are marked. Other peaks due to calibration sources or intrinsic detector radioactivity can also be identified. 5

400 12 C(d, pγ) 13 C 9 Be( 3 He, pγ) 11 B Rate (Hz) 200 0 ICRH Power (MW) 3 2 1 0 0 5 10 20 Time (s) JG10.50-5c Figure 5: Time traces of measured rates in the pulse height energy regions E=3.0-3.2MeV and E=4.3-4.6MeV corresponding to g-ray peaks from the reactions 12 C(d, pγ) 13 C and 9 Be( 3 He, pγ) 11 B observed in JET Pulse No: 79352. The corresponding ICRH power time trace is also shown for comparison. 6