Quantum Control of States of Light (2) Optimization of information extraction from optical measurements

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Quantum Control of States of Light (2) Optimization of information extraction from optical measurements C. Fabre Laboratoire Kastler Brossel Université Pierre et Marie Curie-Paris6, ENS

Two levels in field quantization: - Define a set of modes Optimization of the mode : coherent control - Define a quantum state in each mode Optimization of the quantum state : «pure quantum» control Will not change the mean value of the field, therefore not the mean atomic populations Will change the variance and the correlations Optimization of measurements and extraction of information

Vacuum Coherent state produced by a good laser ΔN = N Intensity noise : shot noise Or «standard quantum limit»

Vacuum squeezed state: less noise than in vacuum for one quadrature Produced by degenerate parametric down-conversion ω P ω 1 Signal=idler ω 1

Two-mode entangled twin-photon state Ψ = c n ω 1 : n, ω2 : n n Produced by degenerate parametric down-conversion ω P ω 1 ω 2 Signal Idler (with intense pump or resonant cavity) Δ ( N N ) 0 1 2 = Strong correlations on one quadrature component Strong anti-correlations on the other quadrature Einstein-Podolsky-Rosen entangled state

Example of change of mode basis Polarization modes y λ / 2 x (1) (2) in the basis of polarization modes x and y: A tensor product of two vacuum squeezed states in the basis of 45, -45 polarization modes An EPR entangled state

OPTIMIZATION OF PARAMETER AND INFORMATION EXTRACTION IN OPTICAL MEASUREMENTS

Light is one of the best carriers of information detector photocurrent - Unavoidable existence of «quantum noise» - Possibility of quantum correlations between measurements Intense beam regime : 1mW=10 16 photons/second

Intensity measurement Phase measurement

Intensity measurement Phase measurement Polarization measurement

Intensity measurement Phase measurement Beam positioning Polarization measurement

Intensity measurement Beam positioning Phase measurement imaging Image processing Polarization measurement

Intensity measurement Beam positioning Phase measurement Temporal variation measurement imaging Image processing Polarization measurement

Intensity measurement Beam positioning Phase measurement imaging Image processing Polarization measurement temporal variation measurement

Intensity measurement Beam positioning Phase measurement Single mode Quantum Optics imaging Image processing Polarization measurement temporal variation measurement

Intensity measurement Beam positioning Phase measurement Polarization measurement imaging temporal variation measurement Image processing Two-mode Quantum Optics

Intensity measurement Beam positioning Phase measurement Highly multi-mode Quantum Optics Polarization measurement imaging temporal variation measurement Image processing

INTENSITY MEASUREMENTS

Weak absorption measurement Tunable laser absorbing medium.............. i = i = i0 1 i 0 light beam ( a) ω abs ω Limit due to the intensity noise of the beam, i.e. shot noise for a coherent beam Shot noise limit of absorption measurement : a SQL = 1 N = 1 Φ T

Absorption measurement using sub-poisonian source F. Marin, A. Bramati, V. Jost, E. Giacobino, Optics Communications 140, 146 (1997) Cesium Saturated absorption experiment shot noise level modulated absorption signal minimum detected absorption: 10-8 for 10 Hz bandwidth 0.8 db improvement (20%) RBW : 1MHz, VBW 3 khz

Absorption measurement using twin beams P. Souto-Ribeiro, C. Schwob, A. Maître, C. Fabre Opt. Letters 22, 1893 (1997) Twin beam generator (non degenerate OPO above threshold) absorbing medium.............. i = i 1 i 1 = i 0 i 2 = i 0 light beam 1 0 ( a) + - i1 i 2 ω abs ω Improvement of signal to noise ratio : 1.9 db (35%) minimum detectable absorption 5.10-8 for 3Hz bandwidth Gao JR, Cui F, Xue C, Xie C, Peng K Opt. Letters 23, 870 (1998) 7dB improvement using dilute dye molecules

INTERFEROMETRIC MEASUREMENTS

phase measurement using squeezed vacuum E 2ˆ i 2 (t) out Φ out E 1ˆ i 1 (t) - + i 1 (t)-i 2 (t) LASER in E 1ˆ in E 2ˆ SQUEEZED VACUUM SOURCE

Interferometric detectors of gravitational waves LIGO VIRGO

MEASUREMENT OF THE TRANSVERSE DISPLACEMENT OF A LIGHT BEAM (NANOPOSITIONING)

d Optical tweezers Atomic Force Microscope

Nano-positioning using a coherent TEM 00 beam w 0 light beam O i 1 (t) i 2 (t) + - i 1 (t)- i 2 (t)=e(p) Uncorrelated shot noise on the two detectors i 1 (t)- i 2 (t) x ( Δ ) = 8 π w 0 x Split Standard Can be very small (sub-nanometer range) Is it possible to go beyond such a limit? N

Use of non-classical state in transverse nano-positioning The noise comes from a single «noise mode»: the «flipped mode» + i 1 (t) O i 2 (t) + - D D C. Fabre, J.-B. Fouet, A. Maître, Optics Letters 25, 76 (2000)

to go beyond the standard quantum limit one must use a two-mode state : D illumination mode Gaussian mode TEM 00 D noise mode intense coherent state In illumination mode squeezed vacuum in noise mode

The superposition of the two modes, one coherent, the other squeezed, gives rise to quantum correlations when one uses another mode basis Photons detected in the two halves of the split detector are correlated light beam spatial ordering of photons N. Treps, U. Andersen, B. Buchler, P.K. Lam, A. Maître, H. Bachor, C. Fabre, Phys. Rev. Letters 88 203601 (2002)

2 D nano-positioning y Laser beam x x flipped mode TEM 00 y flipped mode amplitude y u 1 ( r ) u 0 ( r ) u ( r 2 ) x squeezed vacuum coherent state squeezed vacuum

quadrant detector Spatially squeezed laser beam S+ = SNL S-horizontal = squeeze S-vertical = squeeze non-classical state in which photons are "ordered 4 by 4"

Experimental implementation (collaboration with H. Bachor, Australia) very small oscillation at 5 MHz Intensity difference 1 A Coherent laser beam Three-mode beam quantum laser pointer improvement to with respect to Standard Quantum Limit : displacement (oscillation amplitude) N. Treps, N. Grosse, W. Bowen, C. Fabre, H. Bachor, P.K. Lam, Science, 301, 940 (2003) 70% horizontal, 60% vertical

EXTRACTION OF INFORMATION THROUGH IMAGE PROCESSING

Extraction of a single parameter p by image processing optical image i mm=0, n Image processor E(p) Multi-pixel detector

localisation of a very small scattering object y x 1 2 3 4 C. Tischer et al, Appl. Physics Letters, 79, 3878 (2001) S( x) = i + i i i 1 3 2 4 S ( y) = i + i i i 1 2 3 4

Super-resolution techniques based on image processing Image of fluorescent proteins by conventional high resolution microscopy Super-resolution image Imaging Intracellular Fluorescent Proteins at Nanometer Resolution E. Betzig et al Science 313 1642 (2006)

How is superresolution obtained? laser Fluorescent molecule localized at x 0 Microscope Point Spread Function centered on x 0 CCD camera i 1 (t) i 2 (t) Image processing i 3 (t) i 4 (t) x 0 Resolution: about 2 nm What is the ultimate limit on the accuracy of determination of x 0? Related to the quantum fluctuations of the signals recorded by the pixels of the CCD camera

General case p determined from the value of an estimator E(p) obtained by image processing Information on p is extracted from the local field amplitude normalized field amplitude distribution in the image plane u0 ( x, y, p) y x E( p) = dxdyf( x, y, u0( x, y, p)) Often : E( p) = dxdyg( x, y) u p 0 ( x, y, ) 2 The quantum noise on the local field is the ultimate limit for the accuracy of the determination of p

What is the higher limit imposed by quantum noise to the Signal to Noise ratio S/N on the determination of parameter p? -Maximum signal S : optimize the image processing protocol -Minimum noise N : reduce quantum fluctuations on the estimator E(p)

Answer given by information theory (collaboration with P. Réfrégier, Marseille) The minimum variance of any (unbiased) estimator of p is given by the Cramer-Rao bound ( Δp) CRb -Itisvalidindependently of the precise strategy used in the extraction - It depends only on the statistical distribution of the noise affecting the measured quantities

1) Intensity measurement: V. Delaubert, N. Treps, C. Fabre, H. Bachor, P. Réfrégier, Europhys. Letters 81 44001 (2008) Poisson noise on each pixel ( Δp) S CRb = p 0 2 N N : total number of photons measured p 0 : characteristic parameter value u0 ( x, y, p) 1 p 2 0 = u dxdy p 0 normalized field amplitude distribution in the image plane 2

2) Amplitude measurement: local oscillator of arbitrary shape homogeneous Gaussian noise on each pixel ( Δp) S CRb = p 0 2 N Same expression as for intensity measurement

( Δp) S CRb = p 0 2 N is an «absolute limit»: No measurement can do better on a shot noise limited image

is there a way to reach the Standard Cramer Rao bound? V. Delaubert, N. Treps, C. Fabre, H. Bachor, P. Réfrégier Europhys. Letters 81 44001 (2008)

1) Intensity measurement: i mm=0, n Image processor E(p) Linear processing of intensities: E ( p) = im ( p) gm = dxdy i( x, y, p) g( x, y) pixel m Optimum value of for maximum signal to noise ratio: g optimum = u 0 1 ( x, y, g( x, y) p) p u 0 ( x, y, p)

1) Intensity measurement: i mm=0, n Image processor E(p) Minimum measurable value of p using linear processing (S=N) : p min = Standard Cramer Rao bound reached! 2 p 0 N

1) Amplitude measurement: i 1 (t) i 2 (t) + - i 1 (t)- i 2 (t)=e(p) local oscillator u LO ( x, y) E detectors measure total intensity ( ) ( ) * p dxdyu x, y, p u ( x, ) = 0 LO y Linear processing of amplitudes

1) Amplitude measurement: i 1 (t) i 2 (t) + - i 1 (t)- i 2 (t)=e(p) local oscillator u LO ( x, y) Optimum choice of the local oscillator amplitude: u optimum ( x, y) = p u 0 ( x, y, p) p= 0 Minimum measurable value of p (S=N) : 2 p Standard Cramer 0 pmin = Rao bound reached again! N

Example Laser beam nano-positioning (two-pixel processing)

1) The standard technique : split detector i 1 (t)- i 2 (t)=e(p) light beam TEM 00 beam O i 1 (t) i 2 (t) + - i 1 (t)- i 2 (t) x With coherent beam : ( Δp) ( p) Split Standard = 1. 2 Δ S CRb π w 8 0 Split detector technique is not the best detection technique! N

2) Optimized technique on intensity measurement: E ( p) = dxdyi( x, y, p) g( x, y) optimized choice of g( x, y) for a TEM 00 beam: g ( x, y) = x g( x, y) instead of g( x, y) +1 x x -1

3) Optimized technique on homodyne measurement: light beam E(p) u OL ( x, y) (Detectors measure total intensity) Local Oscillator shape u OL ( x, y) to be found optimized choice of u OL (x,y) for a TEM 00 beam: u OL ( x, y) V. Delaubert et al Phys. Rev A 74 053823 (2006) = TEM 10 Standard Cramer Rao bound reached again!

How to go beyond? 1) Squeeze the total image? Use amplitude squeezed state, or even number state in mode u ( x, )? 0 y does not improve measurements of parameters which do not change the total intensity

2) Squeeze each partial beam? Amplitude squeezed beam Amplitude squeezed beam Amplitude squeezed beam Amplitude squeezed beam New Cramer-Rao bound: p min = S q 2 p 0 N Common squeezing factor of all beams Possible but difficult!

3) Squeeze the right mode The quantum noise on the estimator E(p) comes from a single «noise mode» u 1 (x,y) N. Treps et al Phys. Rev A71 013820 (2005) One can build a basis of transverse functions starting with u ( x, ) u ( x, 0 y ) 1 y { u x, y), u ( x, y),..., u ( x, ),...} 0( 1 n y Quantum fluctuations on E(p) come only from mode u ( x, ) 1 y

1) Intensity measurement beyond the SCRB: i mm=0, n Image processor E(p) if E ( p) = dxdyi( x, y, p) g( x, y) then : u x, y) = u ( x, y) g( x, ) 1( 0 y u p For optimum gain :, ) = u ( x, y, ) x y 1( 0 p

non-classical beam for squeezed image processing: i mm=0, n Image processor E(p) Coherent state in mode Squeezed vacuum in mode p min = u0( x, y) u1( x, y) p0 Sq 2 N The superposition of these two modes creates anticorrelated quantum fluctuations on the different pixels, which results in a noise cancellation in E(p)

Example Beyond the SCRB in laser beam nano-positioning

Intensity measurement Noise mode for the optimized image processing: u ( = xtem = TEM 1 x, y) = g( x, y) u0( x, y) 00 10 light beam x l Coherent state Squeezed vacuum

Homodyne measurement E(p) Coherent state Squeezed vacuum Same superposition of coherent state and squeezed state as previously

Experimental implementation M. Lassen, V. Delaubert, J. Janousek, K. Wagner, H-A.Bachor, P.K.Lam, N.Treps, P.Buchhave, C.Fabre, C.C.Harb, Phys. Rev. Letters 98, 083602 (2007) E(p) Coherent state Squeezed vacuum Spectral power of E(p) beam displacement smaller than Standard Cramer Rao bound Standard Cramer Rao bound Reduced noise with squeezed TEM 10

MEASUREMENTS IN THE TIME/FREQUENCY DOMAIN

From spatial quantum effects to temporal quantum effects Trains of pulses of arbitrary shape time «Frequency combs» Can it be used to improve information processing? How to generate entanglement and reduced quantum fluctuations in such systems? frequency

temporal positioning of a train of pulses Mode-locked Laser Cs clock Observer at point A Cs clock Mode-locked Laser Observer at point B time transfer problem Implementation of Einstein s protocol for clock synchronization Space-time positioning of satellites flying in formation

1 Δ S CRb = N ( t) Quantum limit to the accuracy of time transfer B. Lamine, C. Fabre, N. Treps, Quantum improvement of time transfer between remote clocks To be published in Phys. Rev. Letters (2008) It is given by the Cramer Rao Bound in the case of a Gaussian coherent pulse: 2 2 0 1 2 ω + Δω N : total number of photons ω 0 : mean frequency Δω : frequency spread 1 Δω shift of pulse enveloppe maximum shift of oscillation at optical frequency 1 ω 0

Optimal balanced homodyne measurement Optimal Local Oscillator temporal shape to be found w 1 : combination of a quadrature and of Cramer Rao Bound reached: no other measurement can do better on a shot noise limited pulse Ultimate sensitivity of 20 yoctoseconds (10 fs, 1s integration time)

Simplified version of homodyne measurement Simplified version of LO: the «temporal TEM 01 pulse» w 1 : 1 1 Δ S CRb = N 2Δω ( t) optimizesonlythemeasurement of the pulse maximum Sensitivity of 70 yoctoseconds

Beyond the standard quantum limit in optimal time transfer observer A sends a superposition of two modes: Phase squeezed state Squeezed vacuum Better sensitivity than by sharing entangled light between A and B

Beyond the standard quantum limit in simplified configuration observer A sends: Coherent state Squeezed vacuum

How to produce non-classical combs?

Synchronously Pumped OPOs («SPOPOs») femtosecond mode-locked laser Frequency doubler Laser OPO

Twin photon generation Phase matching conditions for degenerate operation ω 0 frequency comb for pump ω frequency comb for signal/idler ω 0 /2 ω Multiple fathers for the twins! Every pair of photons can find a common father

Evolution of modes in the parametric crystal ω j ω i ω d dz aˆ ω i j ( ) + ω, ω A ( ω + ω ) a ω j = χ ˆ i j pump Coupling between the modes : linear, symmetrical i j Diagonalization by a set of specific combinations of modes or frequency combs: «supermodes» b j d bˆ j = Λ j bˆ + dz j Squeezing transformation

Generation of squeezed frequency combs eigen «super modes» ω Gaussian variation of pump*phase matching G. De Valcarcel et al, Phys. Rev A74 061801R (2006) ω ω mode 1 mode 2 Below the oscillation threshold, all modes are squeezed especially the mode 1, with maximum Λ Above threshold, mode 1 oscillates, the others are squeezed

C.F. Nicolas Treps, German de Valcarcel Vincent Delaubert Giuseppe Patera Benoit Chalopin Olivier Pinel Jean-François Morizur Strong and efficient collaboration with Hans Bachor group at ANU Canberra Australia Post doc position available immediately!!