Magnetism, Rotons, and Beyond: Engineering atomic systems with lattice shaking.

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Magnetism, Rotons, and Beyond: Engineering atomic systems with lattice shaking. Colin V. Parker James Franck Institute and Dept. of Physics University of Chicago

Quantum simulation with cold atoms Chin Lab Nuclear Physics: Efimov Trimers (see PRL 113 240402) Cosmology: Sakharov Oscillations (see Science 341 1213) Condensed Matter: Superfluids, Magnets and more (current topic) Image Credit: Wikipedia/Chin Lab

Variety in condensed matter systems Superconductivity Multiferroics Topological Insulation Image Credit: Wikipedia Density wave (charge/spin) Magnetism (ferro-/anti-ferro)

Where does the variety come from???? 4 Single Particle Dispersion Particle-Particle Interactions Lattice Phonons Image Credit: Wikipedia

Where does the variety come from???? 5 Single Particle Dispersion Particle-Particle Interactions V(q) = V Image Credit: Wikipedia

Dispersion Simple Cases V(q) = V Free Particle: Normal Gas, Superfluid, BEC-BCS crossover Anderson et al Science 269 198 (1995) Davis et al PRL 75 3969 (1995) Square/Cubic Lattice: Mott Insulator Greiner et al Nature 415 39 (2002)

How to create a designer dispersion Simple optical lattices have only one parameter (depth of potential) More complicated lattices require higher spatial frequencies Accessing the time domain of the lattice is a convenient alternative

Outline Intro Ferromagnetism in a single component Bose gas Excitations in the ferromagnetic state (roton/maxon) Optical control of scattering NEW! length

In situ Imaging Trap/lattice beams Microscope objective Vertical compress. beams Imaging beam Gemelke et al., Nature (2009) Single site resolution: M. Greiner Nature (2009), I. Bloch Nature (2010)

Shaking Lattice Ferromagnetism

Near resonant shaking with low heating Bandstructure at 7 E R depth E/E R k/k L

Near resonant shaking with low heating Parker, Ha, Chin - Nat. Phys. (2013) c.f. Gemelke (PRL 170404 2005), Lignier (PRL 220403 2007), Struck (Science 2011) Other driven lattices: ETH, MPQ, MIT

Observation of two minima Cs density 0 50 µm -2 30 nm 13 nm 30 ms TOF No shaking 100 µm

Observation of two minima Lattice Spacing: 532 nm Calculation

Why does the system avoid pseudo-spin mixtures? Momentum Space Real Space U = <n 2 > = (3/2)<n> 2 <n> 2k * π/k *

Can we still prepare a multi-state mixture? 30 ms TOF 20 µm Parker, Ha, Chin - Nature Physics (2013)

Domain reconstruction - + = j z

Domain gallery Geometry: 10 µm Parker, Ha, Chin - Nature Physics (2013)

Domain size and ramping speed 100 ms ramping 10 µm 10 ms ramping Parker, Ha, Chin - Nature Physics (2013)

Correlation length 100 ms G( r) j z (r) j z (r r)dr n(r)n(r r)dr Fidelity 10 ms

Summary - Ferromagnetism Modifying only the dispersion we create an effective ferromagnet in a single-component gas. Domain formation at long length scales (of order the system size) Dynamics considerably faster than heating timescales

Excitations: Roton/Maxon

Excitations of the double-well dispersion Lowest Excitations: Pseudospin Flips (gapped) Lowest Excitations: Phonons

Roton-maxon excitations (He II) E=pv s Phonon mode Maxon maximum Landau (1941, 47) Roton minimum Neutron Scattering: Henshaw and Woods (1961) Reference: Glyde, H. R. Excitations in Liquid and Solid Helium (Clarendon, 1994)

Similar Proposals/Experiments Theory proposals: Resonantly-interacting gases: Yunomae, Yamamoto, Danshita, Yokoshi, Tsuchiya, PRA (09); Cormack, Schumayer, Hutchinson, PRL (11); Rota, Tramonto, Galli, Giorgini, PRB (13). Dipolar gases: Santos, Shlyapnikov, Lewenstein, PRL (03); O'Dell, Giovanazzi, Kurizki, PRL (03); Wilson, Ronen, Bohn, Pu, PRL (08). Rydberg-excited condensates: Henkel, Nath, Pohl, PRL (10). Dilute 2D Bose gases: Fischer PRA(06), Nogueira, Kleinert, PRB (06). Spinor condensates: Cherng, Demler, PRL (09); M. Matuszewski, PRL (10). Spin-orbit coupled condensates: Higbie, Stamper-Kurn, PRL (02); Zheng, Li, PRA (12); Martone, Li, Pitaevskii, Stringari, PRA (12); Zheng, Yu, Cui, Zhai, J. Phys. B (13). Experimental observation: Cavity mediated systems (Roton-type mode softening): Mottl et. al., Science (12)

Digital Micromirror Device Projection 789 nm gravity Projection optics: Heinzen group (UTexas), Greiner group (Harvard), Bloch group (Munich), Esslinger group (ETH), Hadzibabic group(cambridge), Dalibard group (ENS)

DMD/Imaging Cs condensate: 20,000~40,000 atoms Imaging resolution: 1.0 µm Pixel size: 0.54 µm µmirror (mirror pixel) size: 0.21 µm

(Raman) Bragg Spectroscopy Momentum transfer: P=h/d Energy transfer: E=pv v d

Typical frequency (energy) spectrum

Warm-up exercise (w/o shaking) Bogoliubov theory Regular BEC BEC in a stationary lattice Ha, Clark, Parker, Anderson, Chin PRL 114 055301 (2015)

Roton dispersion measurement Ha, Clark, Parker, Anderson, Chin PRL (2015) (soon)

Dispersion Calculations Parker, Ha, Chin - Nature Physics (2013) Ha, Clark, Parker, Anderson, Chin PRL 114 055301 (2015)

Dispersion Calculations Parker, Ha, Chin - Nature Physics (2013) Ha, Clark, Parker, Anderson, Chin PRL 114 055301 (2015)

Roton depends on interactions a = 3.5 nm (70 a 0 ) a = 0.25 nm (5 a 0 ) Ha, Clark, Parker, Anderson, Chin PRL 114 055301 (2015)

Interaction scales as expected m C a 2/5 r ~ a 2/5 Ha, Clark, Parker, Anderson, Chin PRL 114 055301 (2015)

Critical Velocity Measurement Digital aperture Depth U/h ~ 1.1 Hz Ha, Clark, Parker, Anderson, Chin PRL 114 055301 (2015)

Asymmetric critical velocity! Non-roton direction Roton direction condensate number fraction 1.0 0.9 0.8-400 -200 0 200 speckle velocity v ( m/s)

Superfluid critical velocity 400 critical velocity v c ( m/s) 300 200 100 non-roton roton 0 0 10 20 30 modulation amplitude x (nm) Ha, Clark, Parker, Anderson, Chin PRL 114 055301 (2015)

Superfluid critical velocity critical velocity v c ( m/s) 400 300 200 100 non-roton roton 0 0 10 20 30 modulation amplitude x (nm) v Landau v Landau Ha, Clark, Parker, Anderson, Chin PRL 114 055301 (2015)

Summary - Roton Excitations of the effective ferromagnetism turn out to be phonon-maxon-roton Roton properties driven by interaction Landau criterion qualitatively explains critical velocity (strong suppression with roton) Exotic behavior, but still a single component gas with simple interactions

Optical Control of Scattering Length

Motivation For Cs, already good control of scattering length Want optical control for: Spatially varying interactions Fast modulation of interactions

New Approach: Vector Light Shift Cs ideal: Large 6p 1/2-6p 3/2 fine structure splitting Allows vector light shift at large detuning Many Feshbach resonances available Can choose sensitivity in terms of a(b) B = B physical + B eff σ +

New Approach: Vector Light Shift Cs ideal: Large 6p 1/2-6p 3/2 fine structure splitting Allows vector light shift at large detuning Many Feshbach resonances available Can choose sensitivity in terms of a(b) B = B physical + B eff σ + 6p 3/2 6p 1/2 6s 1/2

Caveat: We want minimal scalar shift Adjust detuning so that polarizability is zero for the entrance channel 3,3> state Molecular state still experiences a light shift, which changes scattering length Polarization is very sensitive

Scattering Length Change Near 48 G

Heating Rate: Low Condensate Lifetime: 600 ms @ 200 a 0 shift Scattering Rate: 0.4 s -1

Cloud Size Change

Rich Dynamics

Chicago cold atom group: Collaborators: PI Postdoc Undergrad Brandon Anderson Jason Ho (Ohio State) Cheng Chin CVP Paloma Ocola Sayan Choudhury, Erich Mueller (Cornell Univ.) Hui Zhai (Tsinghua Univ.) Graduate Students Li-Chung Ha Logan Clark Jacob Johansen Gustaf Downs Lei Feng