Small and large Fermi surfaces in metals with local moments

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Small and large Fermi surfaces in metals with local moments T. Senthil (MIT) Subir Sachdev Matthias Vojta (Augsburg) cond-mat/0209144 Transparencies online at http://pantheon.yale.edu/~subir

Luttinger s theorem on a d-dimensional lattice For simplicity, we consider systems with SU(2) spin rotation invariance, which is preserved in the ground state. Let v 0 be the volume of the unit cell of the ground state, n T be the total number of electrons per volume v 0. Then, in a metallic Fermi liquid state with a sharp electron-like Fermi surface: 0 2 Volume enclosed by Fermi surface d v 2 n T mod 2 A large Fermi surface

Our claim There exist topologically ordered ground states in dimensions d > 1with a Fermi surface of sharp electron-like quasiparticles for which v 0 2 Volume enclosed by Fermi surface d 2 n 1 mod 2 T A small Fermi surface

I. Kondo lattice models II. III. IV. Outline Topologically ordered states of quantum antiferromagnets Quantum-disordering transitions of magnetically ordered states with non-collinear spin correlations Models with small Fermi surfaces. Lieb-Schultz-Mattis-Laughlin-Bonesteel-Affleck-Yamanaka- Oshikawa flux-piercing arguments V. Conclusions

I. Kondo lattice models Model Hamiltonian for intermetallic compound with conduction electrons, c i, and localized orbitals, f i H t c c Vc f Vf c n n Un n ij i j i i i i f fi fi fi fi i j i n f f ; n c c fi i i ci i i n n n T For small U, we obtain a Fermi liquid ground state, with a Fermi surface volume determined by n T (mod 2) This is adiabatically connected to a Fermi liquid ground state at large U, where n f =1, and whose Fermi surface volume must also be determined by n T (mod 2)=(1+ n c )(mod 2) f c

The large U limit is also described (after a Schrieffer- Wolf transformation) by a Kondo lattice model of conduction electrons c i and S=1/2 spins on f orbitals H tc c J c c S J i js S ', ij i j K i i fi H fi fj i j i i j This can have a Fermi liquid ground state whose Fermi surface volume is determined by (1+ n c )(mod 2) We will show that for small J K, a ground state with a small electron-like Fermi surface enclosing a volume determined by n c (mod 2) is also possible.

II. Topologically ordered states of quantum antiferromagnets Begin with magnetically ordered states, and consider quantum transitions which restore spin rotation invariance Two classes of ordered states: (A) Collinear spins (B) Non-collinear spins S r NcosQr Q 2, ; N 1 S N N r 1cosQr 2sin Qr 4 4 2 2 Q, ; N1 N2 1; N1N2 0 3 3

(A) Collinear spins, bond order, and confinement Quantum transition restoring spin rotation invariance S r NcosQr Q 2, ; N 1 1 2 Bond-ordered state N. Read and S. Sachdev, Phys. Rev. Lett. 62, 1694 (1989).

k Excitations of bond-ordered paramagnet Stable S=1 spin exciton quanta of 3-component vector particle N ck ck 2 2 2 2 x x y y 2 Spin gap S=1/2 spinons are confined by a linear potential. Transition to Neel state Bose condensation of N

Bond order wave in a frustrated S=1/2 XY magnet A. W. Sandvik, S. Daul, R. R. P. Singh, and D. J. Scalapino, cond-mat/0205270 First large scale numerical study of the destruction of Neel order in S=1/2 antiferromagnet with full square lattice symmetry x x y y i j i j i j k l i j k l H 2J S S S S K S S S S S S S S ij ijkl g=

(B) Non-collinear spins, deconfined spinons, Z 2 gauge theory, and topological order Quantum transition restoring spin rotation invariance S N N r 1cosQr 2sin Qr 4 4 2 2 Q, ; N1 N2 1; N1N2 0 3 3 RVB state with free spinons P. Fazekas and P.W. Anderson, Phil Mag 30, 23 (1974). N. Read and S. Sachdev, Phys. Rev. Lett. 66, 1773 (1991) first discussion of Z 2 gauge theory A.V. Chubukov, T. Senthil and S. Sachdev, Phys. Rev. Lett. 72, 2089 (1994).

Solve constraints by writing: S N N r 1cosQr 2sin Qr 4 4 2 2 Q, ; N1 N2 1; N1N2 0 3 3 N1iN2 ac zc abzb where z are two complex numbers with 1,2 z 2 2 1 z2 3 2 Physical observables are invariant under the Z2 gauge transformation z a z a 1 Order parameter space: Other approaches to a Z 2 gauge theory: R. Jalabert and S. Sachdev, Phys. Rev. B 44, 686 (1991); S. Sachdev and M. Vojta, J. Phys. Soc. Jpn 69, Suppl. B, 1 (2000). X. G. Wen, Phys. Rev. B 44, 2664 (1991). T. Senthil and M.P.A. Fisher, Phys. Rev. B 62, 7850 (2000). R. Moessner, S. L. Sondhi, and E. Fradkin, Phys. Rev. B 65, 024504 (2002). L. B. Ioffe, M.V. Feigel'man, A. Ioselevich, D. Ivanov, M. Troyer and G. Blatter, Nature 415, 503 (2002). S Z

Vortices associated with 1 (S 3 /Z 2 )=Z 2 (A) North pole y (A) (B) (B) South pole S 3 x Can also consider vortex excitation in phase without magnetic order, S r 0 : vison A paramagnetic phase with vison excitations suppressed has topological order

ij ij Model effective action and phase diagram S J z z h.c. K ij i j ij First order transition Z 2 gauge field (Derivation using Schwinger bosons on a quantum antiferromagnet: S. Sachdev and N. Read, Int. J. Mod. Phys. B 5, 219 (1991)). Magnetically ordered L Confined spinons R Impose boundary conditions inducing single vortex on walls of cylinder Free spinons and topological order P. E. Lammert, D. S. Rokhsar, and J. Toner, Phys. Rev. Lett. 70, 1650 (1993) ; Phys. Rev. E 52, 1778 (1995). (For nematic liquid crystals)

Topologically ordered state has a 2 d -fold degeneracy on a d-dimensional torus Vison present or absent S. Kivelson, Phys. Rev. B 39, 259 (1989); N. Read and B. Chakraborty, Phys. Rev. B 40, 7133 (1989). N. E. Bonesteel, Phys. Rev. B 40, 8954 (1989). G. Misguich, C. Lhuillier, M. Mambrini, and P. Sindzingre, Eur. Phys. J. B 26, 167 (2002).

III. Small Fermi surfaces in Kondo lattices Kondo lattice model: H tc c J c c S J i js S ', ij i j K i i fi H fi fj i j i i j Consider, first the case J K =0 and J H chosen so that the spins form a bond ordered paramagnet This system has a Fermi surface of conduction electrons with volume n c (mod 2) However, because n f =2 (per unit cell of ground state) n T = n f + n c = n c (mod 2), and small Fermi volume= large Fermi volume (mod Brillouin zone volume) These statements apply also for a finite range of J K Conventional Luttinger Theorem holds

III. Small Fermi surfaces in Kondo lattices Kondo lattice model: H tc c J c c S J i js S ', ij i j K i i fi H fi fj i j i i j Consider, first the case J K =0 and J H chosen so that the spins form a topologically ordered paramagnet This system has a Fermi surface of conduction electrons with volume n c (mod 2) Now n f =1 (per unit cell of ground state) n n n n mod 2 T f c c This state, and its Fermi volume, survive for a finite range of J K Perturbation theory is J K is free of infrared divergences, and the topological ground state degeneracy is protected. A small Fermi surface which violates conventional Luttinger theorem

Mean-field phase diagram (Sp(N), large N theory) Pairing of spinons in small Fermi surface state induces superconductivity at the confinement transition Small Fermi surface state can also exhibit a secondorder metamagnetic transition in an applied magnetic field, associated with vanishing of a spinon gap.

IV. Lieb-Schultz-Mattis-Laughlin-Bonesteel-Affleck- Yamanaka-Oshikawa flux-piercing arguments Unit cell a x, a y. L x /a x, L y /a y coprime integers L y L x Adiabatically insert flux =2 (units =c=e=1) acting on electrons. 1 State changes from to ', and UH 0 U H, where 2 i U exp xnˆ. Tr Lx r M. Oshikawa, Phys. Rev. Lett. 84, 3370 (2000).

Adiabatic process commutes with the translation operator momentum P is conserved. x 2 i 1 However U TU exp ˆ x Tx n ; T L r x r so shift in momentum P between states U ' and x T x is, so Ly 2 Px nt mod 1. v0 ax Alternatively, we can compute P by assuming it is absorbed by x quasiparticles of a Fermi liquid. Each quasiparticle has its momentum shifted by 2 L x, and so 2 Volume enclosed by Fermi surface 2 Px mod 2. Lx ax 2 2 LL x y From 1 and 2, same argument in y direction, using coprime L a, L a : v 2 n 0 2 Volume enclosed by Fermi surface mod 2 2 T M. Oshikawa, Phys. Rev. Lett. 84, 3370 (2000). x x y y

Effect of flux-piercing on a topologically ordered quantum paramagnet N. E. Bonesteel, Phys. Rev. B 40, 8954 (1989). G. Misguich, C. Lhuillier, M. Mambrini, and P. Sindzingre, Eur. Phys. J. B 26, 167 (2002). D L y a D D D L x -2 L x -1 L x 1 2 3

Effect of flux-piercing on a topologically ordered quantum paramagnet N. E. Bonesteel, Phys. Rev. B 40, 8954 (1989). vison G. Misguich, C. Lhuillier, M. Mambrini, and P. Sindzingre, Eur. Phys. J. B 26, 167 (2002). D a D Number of bonds cutting dashed line L x -2 L x -1 L x 1 2 3 L y D D After flux insertion D 1 D ; Equivalent to inserting a vison inside hole of the torus. Vison carries momentum L v y 0

Flux piercing argument in Kondo lattice Shift in momentum is carried by n T electrons, where n T = n f + n c In topologically ordered, state, momentum associated with n f =1 electron is absorbed by creation of vison. The remaining momentum is absorbed by Fermi surface quasiparticles, which enclose a volume associated with n c electrons. A small Fermi surface. cond-mat/0209144

Conclusions I. Orders characterizing ground states of regular Kondo lattices: II. (A) Spin density wave. (B) Superconductivity. (C) Topological order small Fermi surface, (D) Large Fermi surface. Some orders can co-exist, and this permits a plethora of phase diagrams and quantum critical points. (A) (D) Hertz theory (C) (D) Local quantum criticality? (Small Fermi surfaces in extended DMFT: S. Burdin, D. R. Grempel, and A. Georges, Phys. Rev. B 66, 045111 (2002)).