Atmospheric Composition Matters: To Air Quality, Weather, Climate and More

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Atmospheric Composition Matters: To Air Quality, Weather, Climate and More Burkholder et al., ES&T, 2017 2

Overarching Research Need: Improve Prediction Capabilities via Incorporating/Integrating Composition, Weather and Climate Coupled Environmental Models Moderating Influences Impacts Extreme Weather Monitoring Natural & Human-Induced Environmental Change Atmospheric (Weather) Coupled Computer Modelling Models Air-borne Transport Water Cycle Atmospheric Chemistry Land change processes Climate induced Health impacts Toxic, Nuclear & Disease Transport Flooding/Drought...Alerts Water Availability Air Pollution Ecosystems Habitat changes Biodiversity loss Research Adaptation Measures Across Relevant Temporal and Spatial Scales 3

Transformation of the GAW Programme New GAW Data Management strategy New focal area total deposition New Scientific Advisory Group on Applications

Priority Science Area 1: Advance the fundamental atmospheric chemistry knowledge that enables predictive capability for the distribution, reactions, and lifetimes of gases and particles. Actions needed to address key scientific gaps include: Quantify reaction rates and understand detailed chemical mechanisms in multi-pollutant and multi-phase environments that cover the chemical and dynamical regimes from polluted urban to natural remote regions. Identify and quantify important atmospheric oxidants or other reactants that lead to transformation and removal of chemical species from the atmosphere across broad spatial and temporal scales. Develop a stronger understanding of the influences that surface chemistry exerts on tropospheric composition. Understand and quantify the influence of the coupling between chemical and meteorological processes on the distribution of trace constituents in the troposphere. Understand and quantify the influence of the coupling between chemical, dynamical, and radiative processes involving stratospheric chemistry.

Priority Science Area 2: Quantify emissions and deposition of gases and particles in a changing Earth system. Actions needed to address key scientific gaps include: Better determine emissions from both anthropogenic and natural sources and their spatial and temporal variations and trends. Identify mechanisms and measure rates by which wet and dry deposition removes aerosol particles and trace gases from the atmosphere. Determine the role of meteorology, including temperature, precipitation, and extreme events, on emissions and removal of atmospheric species. Determine the role of global change and societal choices (including changes in climate, energy choices, and land use) on the emissions and removal of atmospheric species.

Priority Science Area 3: Advance the integration of atmospheric chemistry within weather and climate models to improve forecasting in a changing Earth system. Actions needed to address key scientific gaps include: The atmospheric chemistry community should expand interactions with the climate and weather research community to address these key scientific gaps: Determine the global distributions and variability of atmospheric trace gases and aerosol particles, and better understand their climate-relevant properties. Understand the role of aerosol particles as a modulator of cloud microphysics and precipitation efficiency in natural and anthropogenically-perturbed environments. Develop accurate descriptions of the complex chemical and physical evolution of atmospheric constituents that can be implemented in models for robust prediction of the impact of the chemical state of the atmosphere on climate and weather.

Priority Science Area 4: Understand the sources and atmospheric processes controlling the species most deleterious to human health. Actions needed to address key scientific gaps include: The atmospheric chemistry community should expand interactions with the exposure, epidemiology, and toxicology research communities to address these key scientific gaps: Develop mechanistic understanding to predict the composition and transformations of atmospheric trace species that contribute to impacts on human health. Quantify the distribution of atmospheric constituents that impact human health. Determine what unique sources and chemical reactions occur in indoor environments that have implications for atmospheric chemistry and human health.

Priority Science Area 5: Understand the feedbacks between atmospheric chemistry and the biogeochemistry of natural and managed ecosystems. Actions needed to address key scientific gaps include: The atmospheric chemistry community should expand interactions with the ocean, land surface, and other Earth science research communities to address these key scientific gaps: Quantify the full suite of trace gases and particles deposited from the atmosphere and connect these to ecosystem responses. Identify and quantify the chemical composition, transformations, bioavailability, and transport of nutrients and contaminants in the global atmosphere and their interactions with the biosphere. Identify important feedbacks between atmospheric chemistry and the biosphere under global change.

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GAW IP: Defining our role in research Burkholder et al., ES&T, 2017 12

GAW IP: Defining our role in research Burkholder et al., ES&T, 2017 13

The Growing Interest in Improving Air Quality Predictions/Services and the Role of Atmospheric Composition in Weather and Climate Applications Offer Great Opportunities for Our Community Improved Forward Models & Assm. Sys. Evolving Obs Systems Continuous Research Improved Predictions Requires Improved Emissions Enhanced Data Management & Discovery Systems 14