Searching for high-spin toroidal isomers in collisions induced by α-conjugate nuclei

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Searching for high-spin toroidal isomers in collisions induced by α-conjugate nuclei X.G. Cao, K. Schmidt, E.-J. Kim, K. Hagel, M. Barbui, J. Gauthier, M. Huang, J.B. Natowitz, R. Wada, S. Wuenschel, G.Q. Zhang, H. Zheng, N. Blando, A. Bonasera, G. Giuliani, M. Rodrigues, C. Botosso, and G. Liu Nuclei in the valley of stability are usually treated as a fluid made of nucleons with sphere-like geometry in their ground states. However, correlations between nucleons and cluster formation play more important roles in excited nuclei. For light excited α-conjugate (even-even N=Z) nuclei, the importance of α clusters is apparent in both theoretical calculations and experimental observables. Wheeler suggested that nuclear liquid can assume toroidal shapes under certain conditions [1]. Wong et al. quantitatively discussed where the existence of a toroidal nucleus and its stability against sausage deformation [2, 3]. In light α-conjugate nuclei the α particle can be expected to be important in the toroidal configuration which leads to a reduced nuclear density. Heavy ion collisions induced by light α-conjugate nuclei may provide the appropriate conditions to access toroidal isomers with high angular momentum and excitation energy. The toroidal isomer may manifest itself by decaying into α particles or α-like fragments (where the α-like fragments refer to α, 12 C, 16, and 20 Ne etc.). Therefore, an experimental exploration with special attention and methodology into observing α-like decays is indicated and very intriguing. A series of experiments were carried out at Texas A&M University Cyclotron Institute with 40 Ca and 28 Si beams at 10, 25, 35 MeV/u provided by the K500 superconducting cyclotron incident on 28 Si, 12 C, 40 Ca, and 181 Ta targets [4], respectively. The combinations with different α-conjugate projectiles ( 28 Si and 40 Ca) and targets ( 12 C, 28 Si, and 40 Ca) may favor population of different α cluster states. The reaction products were detected using a 4π array, NIMROD-ISiS (Neutron Ion Multidetector for Reaction Oriented Dynamics with the Indiana Silicon Sphere), which consisted of 14 concentric rings covering from 3.6 to 167 in the laboratory frame. In addition, the neutron ball surrounding the NIMROD-ISiS charged particle array provided information on average neutron multiplicities for different selected event groups. The preliminary analysis of parts of the raw data was accomplished by C. Bottosso, E-J Kim, and K. Schmidt et al. [4] and some interesting preliminary results about the α-like mass (Almass) emission have been obtained for 40 Ca+ 40 Ca [5]. Here we focus on cluster decay from 28 Si and check its dependence on 12 C, 28 Si and 181 Ta targets [6]. For the 28 Si+ 12 C reaction, a total of 17 million events were recorded and a significant proportion of events have significant alpha-like mass emission. Half a million events have Almass=28. There are 7 alpha-like decay channels with Almass=28 as shown in Fig. 1. For the most interesting event group: 7 α decay channels, more than 10 thousand events are obtained. II-16

FIG. 1. The proportion of decay channels for Almass=28 from 28Si+12C @ 35MeV/u. The hierarchy effect, which refers to a correspondence between fragment mass and parallel velocity, was found for α-like fragments from 40Ca decay [5]. For most of the 28Si channels this hierarchy effect is also observed. The angles between α and heavier fragments are shown in Fig. 2. The αs tend to FIG. 2. The emission angle between α and heavier fragment for the α-like decay channels. For the 7 α channel, the angle is calculated between center-of-mass velocity and the velocity of α particles. II-17

be emitted backward relative to the large fragment, indicating they mainly come from the neck region. This means absence of complete equilibrium of the α-like emission source. In order to explore the configuration of the possible toroid formed in the dynamical stage, we utilize a shape analysis technique to diagnose the source shape in momentum space [7]. Shape analysis is a popular method to study emission patterns of sources, dynamical aspects of multifragmentation and collective flows of particles in relativistic heavy ion collisions. A tensor constructed on the momenta can be written as: T "# = of ν th ' p " & ()* p # &,where N is the total nucleon number, p " & is the momentum component nucleon in the center-of-mass and i refers to the Cartesian coordinate. The tensor can be diagonalized to reduce the event shape to an ellipsoid. The eigenvalues of the tensor: λ *, λ., and λ 0, normalized by: λ * + λ. + λ 0 = 1 and ordered according to: λ * λ. λ 0, can quantitatively give shape information of the events. The sphericity is defined as: S = 0. (1 λ 0), and coplanarity is defined as: S = 0. (λ. λ * ). In the sphericity-coplanarity plane, the ideal rod, disk and sphere events exactly locate at the three vertexes of the triangle: (0,0) (3/4, of shape analysis is shown by Fig. 3. 3/4), and (1,0), respectively. A schematic figure FIG. 3. A schematic figure illustrating the shape analysis method, where the δ and distance definitions are used in Fig. 5. The results of the shape analysis are shown in Fig. 4. events. Two fragments will always have a rod shape in momentum space while three fragments can form a plane or rod shape. We can see there are always some events located around the disk point, which may be the toroidal candidates, especially for the 7 α channel. II-18

FIG. 4. Shape analysis of sources decaying by Almass. We extract the excitation energy of source decaying by Almass by scanning around the rod-disk line. The extracted excitation energy is shown in Fig. 5, with cut labeled: δ 0,0.05 and distance 0.4,0.6, where the δ and distance are defined in Fig. 3. For our most interesting channel: 7 α, there are several peaks near the 143.18 MeV energy predicted by Staszczak and Wong s [3]. They predicted this to be a 44 ħ 28 Si isomer corresponding to a toroidal configuration. The 6 α and 8 α channels are included for comparison. For the 6 α channel, there are no obvious peaks. For the 8 α channel, at least one α would have to come from the target-like fragment (TLF). The statistics are low and this suggests that the 7 α we analyzed may be relatively free of contributions from decay of the target-like fragment (TLF). FIG. 5. Excitation energy of Almass source with cut on sphericity-coplanarity plane. A determination of the angular momentum of Almass source is necessary to pin down the toroidal candidate. Such a determination is difficult. Antisymmetrized molecular dynamics (AMD) simulations are in progress. II-19

Similar results are seen for the 28 S+ 28 Si, and 28 Si+ 181 Ta systems at 35MeV/u. However, the statistics for the 28 Si+ 181 Ta reaction is much lower than for the other two systems. [1] G. Gamow, Biography of Physics, Harper & Brothers Publishers, New York, 1961, 297 pp. [2] C.Y. Wong, Phys. Lett. 41B, 446 (1972); C.Y. Wong, Phys. Rev. C 17, 331 (1978). [3] A. Staszczak, C.Y. Wong, Phys. Lett. B 738, 401 (2014). [4] K. Schmidt et al., Progress in Research, Cyclotron Institute, Texas A&M University (2010-2011), p. II-8; C. Bottosso et al., Progress in Research, Cyclotron Institute, Texas A&M University (2008-2009), p.ii-7. [5] K. Schmidt et al., Progress in Research, Cyclotron Institute, Texas A&M University (2011-2012), p. II-7; Progress in Research, Cyclotron Institute, Texas A&M University (2012-2013), p. II-17; Progress in Research, Cyclotron Institute, Texas A&M University (2013-2014), p. II-18. [6] X.G. Cao et al., Progress in Research, Cyclotron Institute, Texas A&M University (2014-2015), p. II- 16. [7] J. P. Bondorf et al., Phys. Lett. B 240, 28 (1990). II-20