David Edwards, Jérôme Barré and Helen Worden (NCAR) Arlindo da Silva (NASA GSFC) is sponsored by the National Science Foundation.

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The atmospheric composition geostationary satellite constellation for air quality and climate science: Evaluating performance with Observation System Simulation Experiments (OSSEs) David Edwards, Jérôme Barré and Helen Worden (NCAR) Arlindo da Silva (NASA GSFC) is sponsored by the National Science Foundation.

OSSEs & the GEO constellation The CEOS Atmospheric Composition Constellation activity identified joint OSSEs as a way to promote collaboration between the planned and proposed geostationary Earth orbit (GEO) missions from NASA GEO-CAPE/TEMPO, ESA Sentinel 4 & KARI GEMS OSSEs are extensively used by the NWP community to develop and optimize contemporary meteorological satellite instruments; now increasingly used in other fields of earth observation OSSEs assess the impact of hypothetical observations on a model analysis/forecast/inversion and provide a means to generalize on the conclusions of limited case-studies NASA TEMPO/ GEO-CAPE NOAA GOES R/S ESA, EUMETSAT SENTINEL-4 + IRS KARI, GEMS.

Funded tropospheric chemistry missions Europe Sentinel 4 USA TEMPO Korea GEMS Europe Sentinel 5 Precursor TROPOMI Orbit Geostationary Geostationary Geostationary Low-Earth Launch 2019 ~2018 2018 2015 Domain Europe North America Asia-Pacific Global Resolution 8km x 8km at 40N 8km x 4.5km at 35N 7 km (56 km 2 ) at 38N 7km x 7km nadir Revisit 1 hour 1 hour 1 hour 1 day Payload UV-Vis-NIR 305-500, 750-775 nm UV-Vis 290-740 nm (tbc) UV-Vis 300-500 nm (tbc) UV-Vis-NIR-SWIR 270-500, 675-775, 2305-2385 nm Species O 3, NO 2, SO 2, HCHO, AAI, AOD, heightresolved aerosol O 3 sensitivity to lowest 2km, NO 2, SO 2, HCHO, CHOCHO, AOD, AAOD, AAI O 3, NO 2, SO 2, HCHO, AOD O 3, NO 2, SO 2, HCHO, CO, CH 4, AAI, AOD, height-resolved aerosol.

An OSSE to demonstrate value of a GEO constellation: What is the impact of the constellation observations for improving analysis and forecast of pollutant distributions? First experiments: Build on experience assimilating Terra/MOPITT multispectral tropospheric CO observations that have sensitivity to the lower troposphere, and imagine similar capability for all the members of the GEO constellation Such capability proposed for GEO-CAPE over the USA with EV CHRONOS; Europe currently plans column CO measurements from IRS accompanying Sentinel 4; currently no CO plans for the Korean platform to accompany GEMS OSSE goal Control run: Met Only assimilated Assimilation run: Met + MOPITT

A chemical OSSE framework Nature & Control Runs Instrument Simulator Data Assimilation

Experimental setup Nature Run (NR): GEOS-5 0.5 o Global Mesoscale Simulation for summer 2006 Instrument Simulator: Computationally efficient regression algorithm based on MOPITT multispectral observations (Worden et al., 2010) Control Run (CR): CESM CAM-Chem at 1 o resolution Assimilation Run (AS): DART EAKF Assess the ability to observe impact of emissions over each region Look at importance of long range transport from one region to next Investigate the value of the measurements from each mission individually and together

The Nature Run (NR) Global Mesoscale Simulation: GMAO GEOS-5 7-km high resolution CO total column 15 July 2006 Courtesy Arlindo Da Silva, NASA GSFC

CO anthropogenic emissions budget Nature: Control: Jun Jul Aug 06 GMAO GEOS-5 NR Anth: merge of several inventories with EDGAR (2000) as a base (EPA/NEI, CAC, BRAVO, EMEP); fires: QFED v2.2; biog: MEGAN NCAR CAM-Chem CR Anthro: MACCity; Fires: FINN biog: MEGAN

The Observation Simulator 1. Nature Run Model Required state: 2. The Forward Model Simulated signal: Measurement Sensitivity: Simulated Candidate Observations 4. Retrieved Products: Instrument Description Noise: Radiative Transfer.

Observation Simulator measurement & retrieval characteristics are represented by the Averaging Kernel (AK) and retrieval error However, running the full Observation Simulator in the OSSE is expensive and very involved Previously, CO and O 3 OSSEs have been simplified by assuming all observations can be represented with a few AK cases and these are used to sample the Nature Run model everywhere/all day But AKs vary a lot. Depend on surface characteristics, temperatures, clouds, aerosol loadings, trace gas loadings, viewing and solar angles - realistic OSSEs need to account for this! Retrieval Averaging Kernels Pressure (hpa) MOPITT CO 400 Spread in CONUS AKs for surface & 500 hpa. TES-OMI trop. O 3

Observation simulator: Near-surface CO concentration accounting for scene-dependent measurement sensitivity Scene-dependent retrieval near-surface information content large differences between regions DFS Lower Trop CO 15 July 2006, 3pm local time Barré et al., Atm. Env., accepted, 2015.

Simulated cloud coverage Ratio of cloud free pixels Cloud coverage varies according to region with large differences affecting effective temporal coverage July 2006 cloud coverage ratio Barré et al., Atm. Env., in press, 2015

GMAO GEOS-5 Nature Run Assimilation Run NCAR CAM-Chem Control Run Emissions: Anth: merge of several inventories with EDGAR (2000) as a base (EPA/NEI, CAC, BRAVO, EMEP). Fires: QFED v2.2. Biog: MEGAN Chemistry: Only AeroChem: Global CO and CO2 tracers; GOCART aerosols Resolution: Vertical: 72 levels (Surface - 0.01hPa), Horizontal: 0.5 (0.06 ) Emissions: Anth/Fires: MACCity, Biog: MEGAN Chemistry: MOZART full tropospheric chemistry Aerosols and chemistry (87 species + 16 bulk aerosols) Resolution: Vertical: 30 levels (Surface - 3hPa ) Horizontal: 1 Assimilation run over Summer 2006. Meteorological Spin-up over May. Reduced NR resolution (0.5 ) used Barré et al., Atm. Env., in prep..

The OSSE result for the difference between the Assimilation Run (AS) and Control Run (CR) for June 26, 2006, for CO concentration after the assimilation of Simulated Candidate Observations from GEO over Europe, Asia and USA NR CR AR Lower-troposphere AR-CR.

DA impact relative to nature run (NR): Assimilating all 3 GEOs Monthly 200 1000 hpa average NR-AR Jun Jul Aug Next look at Skill Score = 1 MSE(AR-NR) / MSE(CR-NR) SS < 0 degraded simulation SS > 0 improved simulation SS = 1 perfect simulation

DA impact relative to nature run: Assimilating individual GEOs Monthly 200 1000 hpa average Jun Jul Aug Assimilating US-GEO Assimilating EUR-GEO Assimilating ASIA-GEO

First OSSE results Assimilation of the GEO constellation provides a strong constraint over anthropogenic source locations Global constraint of CO is also strong in remote regions due to long range transport of assimilation increments Impacts are reduced over Asia due to increased cloud coverage limiting the number of clear observations Experiments are being extended with a winter case study when the CO lifetime is longer, and emissions and cloud coverage also change Next steps Expand the experiments to consider LEO (TROPOMI) measurements, AOD, tropospheric ozone and chemical correlations.

Thank You! NCAR is sponsored by the National Science Foundation.

OSSE Infrastructure: Recommendations OSSEs need to account for realistic atmospheric variability: Requires evaluation of NR with observations OSSEs require realistic variability in measurement simulations generated from NR: Requires incorporation of sensitivities due to cloud, aerosol, trace gases, surface UV-visible reflectivity, and IR emissivity Simulated retrievals must include realistic range of sensitivities: Requires generation of scene-dependent AKs and errors OSSEs for relative performance between instruments/observation strategies may provide most reliable conclusions: Difficult to predict absolute performance of future systems compared to the current capability; requires full system evaluation with the existing observing system NWP experience: OSSE-based decisions have international stakeholders and experiments should be developed as joint global projects; community ownership and oversight of OSSE capability is also important for maintaining credibility.

GEO constellation DA increments

DA impact relative to nature run (NR): Assimilating all 3 GEOs Monthly 200 1000 hpa average NR-CR Jun Jul Aug NR-AR

DA impact relative to nature run (NR): Assimilating all 3 GEOs Monthly 200 1000 hpa average NR-AR Skill Score = 1 MSE(AR-NR)/MSE(CR-NR) SS > 0 improved simulation SS < 0 degraded simulation SS = 1 perfect simulation Jun Jul Aug

GEO constellation DA increments RMS surface increments Jun Jul Aug RMS profile increments GEO-US GEO-EU GEO-AS Lower troposphere CO 900hPa

Regional Distribution of the EPA09 Ozone Sensitivity EPA09 N.E. Asia Over 35% of mean surface ozone in EPA09 comes from emissions outside EPA09 Chinese emissions contribute to mean column ozone @ 70% of local emissions 70% 60% 50% 40% 30% India China S.E. Asia Column Surface 20% 10% 0% China India NEAsia SEAsia EPA09 USA-EPA09

GEOCAPE Atmosphere Regional/Urban OSSE Task Participants Institute 1. Urban Nature Run** K. Pickering/C. Loughner NASA/GSFC 2. Regional Nature Run*/DA* B. Pierce/A. Lenzen/T. Schaack NOAA/CIMSS 3. Forward RT Modeling* K. Bowman/V. Natraj/T. Kurosu JPL 4. AK Regression* D. Edwards/H. Worden NCAR 5. Multi-Spectral Retrieval* L. Iraci/S. Kulawik NASA/BAERI 6. Nature Run Verification* M. Newchurch/L. Wang UAH * Completed in FY13 * Completed in FY14 * In preparation Extends previous GEOCAPE OSSE studies by: Utilizing independent modeling systems for generation of the Nature atmosphere and conducting the assimilation impact experiments Accounting for realistic atmospheric variability, which requires evaluation of the nature runs with respect to observations. Inclusion of realistic variability in the synthetic radiances, which requires incorporation of realistic surface UV and visible reflectivities, and IR emissivities. Inclusion of realistic sensitivities, which requires generation of averaging kernels (AK) for each retrieval for use in assimilation studies

The OSSE Components OSSEs are extensively used by the NWP community to develop and optimize contemporary meteorological satellite instruments Now also increasingly used in other fields of earth observation OSSEs assess the impact of hypothetical observations on a model analysis/forecast/inversion and provide a means to generalize on the conclusions of limited case-studies OSSE components: Nature Run (NR): Model representation of truth Simulated Candidate Observations: The Observation Simulator samples the Nature Run Control Run (CR): An alternative model representation of the atmospheric state ( this might represent current capability to provide ground-truth or the a priori best guess) Assimilation Run (AR): Assimilation of the Simulated Candidate Observations in the Control Run Compare: Assess impact of the Candidate Observations - Does the Assimilation Run tend to the Nature Run compared to the Control Run? If so, Candidate Observation may be useful.