Title to the Late Professor Yoshiaki Uemu.

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Title Elastic Scattering of ¹⁶0 on ⁹Be (M to the Late Professor Yoshiaki Uemu Author(s) Takimoto, Kiyohiko; Fujii, Kazuo; Y Jun; Muto, Jiro Citation Bulletin of the Institute for Chemi University (1974), 52(1): 240-245 Issue Date 1974-07-25 URL http://hdl.handle.net/2433/76523 Right Type Departmental Bulletin Paper Textversion publisher Kyoto University

Bull. Inst. Chem. Res., Kyoto Univ., Vol. 52, No. 1 Elastic Scattering of 160 on 'Be Kiyohiko TAKIMOTO, Kazuo FUJII, ISao YAMANEt, Jun ScHIMIZU, and Jiro MuTO* Received January 8, 1974 Using the tandem Van de Graaff in Kyoto University, excitation functions of the elastic scattering of 160 on Be at 73.7, 90.0 and 148.6 degrees in the center of mass system have been measured in the energy range Elab=11.0-34.0 MeV. The excitation functions are compared with the optical model calculation using the shallow potential values and or the deeper potential values. Those in the lower energy region are fairly well reproduced with the deeper potential calculation. However, the anomalous structures in the higher energy region could not be explained with our optical model calculation. More complex reactions related to the nuclear structure of the projectile and the target nucleu seems to occur in the higher energy region. INTRODUCTION Recently, heavy ions accelerated by tandem Van de Graaff are frequently used in studies on nuclear reactions. Especially, measurements of excitation functions have been actively pursued for elastic scattering and nuclear reactions between light nuclei in the mass region up to sd-shell nuclei. From these studies some special phenomena related to the character of interaction between nuclei have been recognized. At the energy far above Coulomb barrier energy, existence of the gross structure which can not be attributed to black nucleus scattering in excitation function of the elastic scattering was found for the cases of160-160,etc.1) At the energy near by Coulomb barrier energy, existence of quasi molecular state in 12C-12C system was reported.2) However, at the medium energy, above the Coulomb barrier but under the energy ;. of gross structure region, excitation function shows very complicated feature. The excitation function of elastic scattering has quite different feature depended on combinations of nuclei, for example, in 12C-12C system it shows complicated resonancelike structure, while in 14N 14N system has monotonically decreasing character, and in 12C_ 160 system seems to have an intermediate feature between above two cases.3) In this energy region, nuclear reactions also seems to have complicated feature. Examples are the reactions, (7Li, t), (7Li, cc), (6Li, d),. and (6Li, a) on some states of light nuclei, where the angular distributions show forward peaking as if the directreaction process, conversely the excitation functions have resonance-like features.4) The other example is 12C(12C, 0)2ONe* reaction leading to so-called "2a-state" of 2 Ne, which shows the similar feature as in the cases of Li-induced reactions.5) From these examples it seems that in this medium energy region the process of elastic scat- * *Lc, **At, A L:Ari : Department of Physics, Faculty of Science, Kyoto University t Now in Research Center for Nuclear Science and Technology, Tokyo University ( 240 )

Elastic Scattering of 160 on 'Be tering and reaction depends strongly on the structure of nuclei concerned. Some experimental researches on heavy ion nuclear reactions in the medium energy region are undertaken by authors to make clear the dependence of heavy ion interactions nuclear structure. Ex.(MeV) 3He 3He d 20 n d t p P n d ' n t dp Pdt3Hen. t F n a t 1,0 _Ptn n n--ap a a apapnp n d n -- a a p at det "B 14N-------------'2C '9F MO IN MC' a p mr P 7Li 20Nez lg Fig. 1. Particle-decay threshold energies of some light nuclei. In seeking the dependence of the reaction process in medium energy region on the structure of projectile and target,nuclei, it seems to be important fact that in the excitation energycorresponding to incident energy very few particle-decay channels are opened for the projectile or target nucleus (shown: in Fig. 1). Among these decay channels, a-decay channels are situated at low energy, especially those of 4N-nuclei are the lowest channel far from other possible channels. The anomaly observed in reactions above mentioned occurs in the cases of these nuclei being the projectile or the target. When the nucleus as 160 or 20Ne which has the states formed by a+core interaction above a-threshold reacts on the other nucleus at the energy region where only a-channel is open, exchange process of a-particle is possible to have important influence upon the phenomenon. From the point of view above mentioned, interaction between closed core nucleus and closed core +a nucleus are studied. As the former 160 nucleus is used and as the latter 9Be (because, in 9Be nuclei intranuclear a would have a nature not so differing from that in 8Be nuclei) or 20Ne is used. In this report experimental results of elastic scattering of 160 on 9Be are described. EXPERIMENTAL METHODS AND RESULTS A self-supported 9Be foil (30 g/cm2)p was bombarded by 160 ions of the energy (241)

o m -------------------------------------------------------------------------------- K. TAKIMOTO, K. FujII, I. YAMANE, J. SCHIMIZIJ, and J. MUTO from 11.0 MeV to 34.0 MeV accelerated by the Kyoto-University tandem Van de Graaff. 160 ions and 9Be ions emitted after scattering are measured by two 100 it surface barrier solid state detectors respectively. To measure the intensity of incident 160 ions, counts of elastically scattered 160 on Ag which was slightly evaporated (2 3 pg/cm2) on the 9Be target was used. Since elastic scattering of 160 on Ag in this energy region, is almost pure Coulomb scattering, this method gives easily absolute value of the elastic scattering cross sections for 160 + 9Be. 150 _ 9L -29.4108A(160160)108A E. =20 MeV99 > 6 100 160 (16016060X 10 50_9Be(160,60)9Be recoit9be 32s(1601,60)32, / \\.]12C(16o Il0)12C 050100150200 channel number Fig. 2. An example of the energy spectrum of 360 scattering on 'Be. ''AI(160;(0)Al21 6 etc(160 ;60) An example of the measured single energy spectrum is shown in Fig. 2. In heavy ion reactions, background due to contamination in target is large. Especially, the contaminations of C and 0 are troublesome, because quantities of C and 0 in the target vary during the experimental runs. To avoid this background trouble, coincidence counting between the scattered 160 and recoiled 9Be was used. By this method spectra almost without background could be obtained. Measurements were carried on the laboratory energy of 160 between 11.1 MeV and 34.2 MeV (4.0 MeV and 12.3 MeV in the center of mass system respectively) at the center of mass angle 90.0. Also the measurements were carried at the center of mass angles 73.7 and 148.6. Excitation functions were obtained at the laboratory energy step of 100' 500 KeV. These curves show complicated features over the c. m. energy of about 9 MeV beyond which energy a-channels of both 160 and 9Be ire able to be opened. (242)

Elastic Scattering of 160 on 9Be DISCUSSIONS The measured excitation function was compared with optical model calculation. An optical potential of usual volume type Woods-Saxon form: U(r)_+1 V-------------- W 11+exp(r RR I 1 \arjal 1+exp(/r RR was used. Actual calculation* was performed by 4 parameters postulating RR = R1 = R and ar = al= a as usual. Calculation was done with FACOM 230-60 computer facility in Kyoto University. Values of R and a used in the calculation were 6.4 fm and 0.49 fm respectively. Two sorts of potential value have beep tried, one is a shallow potential which gives a fairly good explanation of the excitaiton function of 160 160 elastic scattering,6) and the other is a deep potential') which have frequently used so far for the calculation of angular distribution of heavy ion elastic scattering. Calculated excitation functions derived from the shallow potential are shown in Fig. 3 as well as Fig. 4 with experimental data. I I I I 1 I II = E.Vr-13.0MEVG-V=-14.OMEV W=(-0.4-015E)MEVaW=(-0.4-0.15E)MEV. ec.m-73.7 Rr=Ri ='6.7fmO 6c.m=73.7 Rr=Ri= 6.7 fm _ 700ar=ai=0.49fm100 ar=ai=0.49fm 1390.0' oarn.`b '~f % 6cm90.0d}tf 4i 101}}}i---- 10=fl}} } api ' 6148.6..ec.m 148.6 } 1iiI}f-- _ 1 - i4f _ }} { {Ilii 1 i }}}} } }}{1} I I 11111it 1 5 6 7 89 10` 12 5 6 7 8 9 10 j 12 CENTER OF MASS ENERGY IN MEVCENTER OF MASS ENERGY IN MEV Fig. 3Fig. 4 Fig. 3, Fig. 4. Excitation functions of 9Be+160 elastic scattering at 73.7, 90.0 and 148.6 in C. M. system. Comparison between the experimental values and the optical model calculation using the shallow potential. * We are in debt to Mr. F. Tanabe, Department of Nuclear Engineering in Kyoto University for the program of optical model calculation. (243)

K. TAKIMOTO, K. FUJII, I. YAMANE, J. SCHIMIZU, and J. MUTO Shallow potential seems to be able to reproduce the large bumpy =-150 M EV structure in higher energy part in case V W = -20 MEV of 0=148.6, but it gives a poor fitv,8cm=73.7 RI=.0 R.= 6.7 f m ting for the smooth structure in lower 00a=a. - 0.49fm 100energy part. On the other hand, deep potential reproduce fairly well +1#0 the smooth structure in the lower eni+'+ ;890 +a+1t.ergy part but can not reproduce the bumpy structure in the higher energy 10 }p bw art at 0=148.6 (shown in Fig. 5). +tr f f = Beside this experimental data, an ex- 8 cm=148.6 periment on angular distribution of 9Be+ 160 scattering was reported by }Krubasik et al7) at an energy point ` l } ll f } _ of 30 MeV in laboratory system.' }} _ Their diffraction angular -like structure distribution at backward has no }} 1 + f f angle. Therefore, it seems not to be 5 CENTER 67 OF MASS 8 ENERGY 9 10}12---------reproduced IN MEVIn spite by of shaliow the insufficient potential. para- Fig. 5. Excitation functions of 9Be+160 elastic scat-meter tering at 73.7, 90.0 and 148.6 in C. M.could system. Comparison between the experi-tion mental values and the optical model calculation using the deeper potential.9 search in our calculation, it be said that the excitation funcat the center of mass energy over MeV suggests the possibility of the existence of somekinds of particular structure which can not be reproduced by a simple optical model calculation. This conclusion is supported by the other experimental results. That is, recently Middleton et a!8) have reported the existence of remarkable resonance-like structure in excitation function of 12C(13C, a)21ne* reaction at the energy corresponding to our experiments which gives the same compound nuclei as 160 Be9 system. As far as this preliminary research is concerned, excitation function of elastic scattering of 9Be + 160 seems to have a structure resulting from the openning of a-channels of the concerning nuclei. Experimental research is now in progress on.9be+ 160 system and on 20Ne+ 160 system for the purpose to make clear the characteristic feature of nuclear interactions between heavy ions. This paper is dedicated to the late Professor Yoshiaki Uemura who had contributed to construct the Kyoto University tandem Van de Graaff. REFERENCES (1) R. H. Siemssen, J. V. Maher, A. Weidinger, and D. A. Bromley, Phys. Rev. Lett., 19, 369 (1967). (244)

Elastic Scattering of 016 on 9Be (2) E. Almqvist, D. A. Bromley, J. A. Kuehner, and B. Whalen, Phys. Rev., 130, 1140 (1963). (3) D. A. Bromley, "Nuclear Reactions Induced by Heavy Ions" North-Holland p. 27 (1970). (4) R. R. Carlson and D. J. Johnson, Phys. Rev. Lett., 25, 172 (1970). H. W. Wyborny and R. R. Carlson, Phys. Rev., 03, 2185 (1971). (5) R. Middleton, J. D. Garrett, and H. T. Fortune, Phys. Rev. Lett., 27, 950 (1971). (6) J. V. Maher, M. W. Sachs, R. H. Siemssen, A. Weidinger, and D. A. Bromley, Phys. Rev., 188, 1665 (1969). (7) U. C. Voos, W. V. Oertzen, and R. Bock, Nucl. Phys., A135, 207 (1969). (8) R. Middleton, J. D. Garrett, H. T. Fortune, and R. R. Betts, Phys. Rev. Lett., 27, 1296 (1971). (245)