Quantum Kinetics in Transport and Optics of Semiconductors

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Springer Series in Solid-State Sciences 123 Quantum Kinetics in Transport and Optics of Semiconductors Bearbeitet von Hartmut Haug, Antti-Pekka Jauho Neuausgabe 2007. Buch. xix, 362 S. Hardcover ISBN 978 3 540 73561 8 Format (B x L): 15,5 x 23,5 cm Gewicht: 1570 g Weitere Fachgebiete > Technik > Technik Allgemein > Physik, Chemie für Ingenieure Zu Leseprobe schnell und portofrei erhältlich bei Die Online-Fachbuchhandlung beck-shop.de ist spezialisiert auf Fachbücher, insbesondere Recht, Steuern und Wirtschaft. Im Sortiment finden Sie alle Medien (Bücher, Zeitschriften, CDs, ebooks, etc.) aller Verlage. Ergänzt wird das Programm durch Services wie Neuerscheinungsdienst oder Zusammenstellungen von Büchern zu Sonderpreisen. Der Shop führt mehr als 8 Millionen Produkte.

Contents Part I Introduction to Kinetics and Many-Body Theory 1 Boltzmann Equation... 3 1.1 Heuristic Derivation ofthesemiclassicalboltzmannequation... 3 1.2 Approach to Equilibrium: H-Theorem................... 5 1.3 Linearization:EigenfunctionExpansion... 8 2 Numerical Solutions of the Boltzmann Equation... 11 2.1 Introduction... 11 2.2 Linearized Coulomb Boltzmann Kinetics ofa2delectrongas... 12 2.3 EnsembleMonteCarloSimulation... 20 2.3.1 GeneralTheory... 20 2.3.2 Simulation of the Relaxation Kinetics ofa2delectrongas... 23 2.4 N + N N + Structure: Boltzmann Equation Analysis...... 29 3 Equilibrium Green Function Theory... 35 3.1 SecondQuantization... 35 3.2 Density Matrix Equations: An Elementary Derivation of a Non-Markovian Quantum Kinetic Equation.......... 38 3.3 GreenFunctions... 41 3.3.1 ExamplesofMeasurableQuantities... 43 3.4 Fluctuation DissipationTheorem... 45 3.5 Perturbation Expansion of the Green Function........... 47 3.6 ExamplesofSimpleSolvableModels... 50 3.6.1 Free-ParticleGreenFunction... 50 3.6.2 Resonant-LevelModel... 50

XVI Contents 3.7 Self-Energy... 52 3.7.1 Electron PhononInteraction... 52 3.7.2 Elastic Impurity System: Impurity Averaging..... 54 3.8 FiniteTemperatures... 58 Part II Nonequilibrium Many-Body Theory 4 Contour-Ordered Green Functions... 63 4.1 GeneralRemarks... 63 4.2 TwoTransformations... 64 4.3 AnalyticContinuation... 69 5 Basic Quantum Kinetic Equations... 75 5.1 IntroductoryRemarks... 75 5.2 TheKadanoff BaymFormulation... 75 5.3 KeldyshFormulation... 77 6 Boltzmann Limit... 79 6.1 GradientExpansion... 79 6.2 QuasiparticleApproximation... 81 6.3 RecoveryoftheBoltzmannEquation... 82 7 Gauge Invariance... 85 7.1 ChoiceofVariables... 85 7.2 GaugeInvariantQuantumKineticEquation... 87 7.2.1 DrivingTerm... 87 7.2.2 Collision Term................................ 90 7.3 RetardedGreenFunction... 91 8 Quantum Distribution Functions... 93 8.1 Relation to Observables, and the Wigner Function........ 93 8.2 GeneralizedKadanoff BaymAnsatz... 94 8.3 SummaryoftheMainFormalResults... 97 Part III Quantum Transport in Semiconductors 9 Linear Transport... 101 9.1 QuantumBoltzmannEquation... 101 9.2 Linear Conductivity ofelectron-elasticimpuritysystems... 104 9.2.1 KuboFormula... 105 9.2.2 QuantumKineticFormulation... 109 9.3 Weak Localization Corrections to Electrical Conductivity.. 111

Contents XVII 10 Field-Dependent Green Functions... 115 10.1 Free Green Functions andspectralfunctionsinanelectricfield... 115 10.2 A Model for Dynamical Disorder: TheGaussianWhiteNoiseModel... 121 10.2.1 Introduction... 121 10.2.2 Determination of the Retarded Green Function.... 121 10.2.3 KineticEquationfortheGWN... 123 10.2.4 OtherTransportProperties... 127 10.3 Introduction to High-Field Transport in Semiconductors... 129 10.4 Resonant-Level Model in High Electric Fields............ 131 10.4.1 Introduction... 131 10.4.2 Retarded Green Function: SingleImpurityProblem... 131 10.4.3 Retarded Green Function: Dilute ConcentrationofImpurities... 133 10.4.4 AnalyticContinuation... 140 10.4.5 QuantumKineticEquation... 141 10.5 Quantum Kinetic Equation forelectron PhononSystems... 144 10.6 An Application: Collision Broadening for a Model Semiconductor......... 148 10.6.1 AnalyticalConsiderations... 148 10.6.2 A Simple Model: Optical Phonon Emission at T =0... 150 10.7 SpatiallyInhomogeneousSystems... 151 11 Optical Absorption in Intense THz Fields... 157 11.1 IntroductoryRemarks... 157 11.2 OpticalAbsorptionasaResponseFunction... 158 11.3 AbsorptionCoefficient... 162 11.4 StaticElectricField... 163 11.5 Harmonically Varying External Electric Fields........... 164 11.5.1 JointDensityofStates,2D... 167 11.5.2 JointDensityofStates,3D... 169 11.6 Dynamical Franz Keldysh Effect: Excitonic Effects....... 171 11.6.1 MatrixTruncation... 172 11.6.2 FloquetSpaceFormulation... 175 12 Transport in Mesoscopic Semiconductor Structures... 181 12.1 Introduction... 181 12.2 Nonequilibrium Techniques in Mesoscopic Tunneling Structures..................... 184 12.3 ModelHamiltonian... 185 12.4 GeneralExpressionfortheCurrent... 186

XVIII Contents 12.5 CurrentConservation... 191 12.6 NoninteractingResonant-LevelModel... 192 12.7 Density Functional Theory andmodelingofmolecularelectronics... 195 12.8 Resonant Tunneling withelectron PhononInteractions... 196 12.9 Transport in a Semiconductor Superlattice............... 198 12.10 Transport in Atomic Gold Wires: SignatureofCouplingtoVibrationalModes... 202 12.11 TransportThroughaCoulombIsland... 205 13 Time-Dependent Phenomena... 213 13.1 Introduction... 213 13.2 Applicability to Experiments........................... 214 13.3 MathematicalFormulation... 215 13.4 AverageCurrent... 217 13.5 Time-DependentResonant-LevelModel... 218 13.5.1 Responseto HarmonicModulation... 221 13.5.2 Responseto Step-LikeModulation... 224 13.6 Linear-Response... 227 13.7 FluctuatingEnergyLevels... 229 13.8 Noise... 230 13.8.1 TheDisconnectedTerms... 235 13.8.2 TheConnectedTerms... 236 Part IV Theory of Ultrafast Kinetics in Laser-Excited Semiconductors 14 Optical Free-Carrier Interband Kinetics in Semiconductors... 243 14.1 Interband Transitions in Direct-Gap Semiconductors...... 243 14.1.1 ReducedDensityMatrices... 243 14.1.2 Nonequilibrium Green Functions................. 245 14.1.3 Calculations of the Two-Time-Dependent Nonequilibrium Green Function................. 245 14.1.4 Replacement of Two-Time Propagators by a One-Time Density Matrix anda Two-TimeSpectralFunction... 246 14.2 Free-Carrier Kinetics Under Laser-PulseExcitation... 251 14.3 TheOpticalFree-CarrierBlochEquations... 255 15 Interband Quantum Kinetics with LO-Phonon Scattering. 259 15.1 Derivation of the Interband Quantum Kinetic Equations... 259 15.2 The Spectral Green Functions G r µν and Ga µν... 266

Contents XIX 15.2.1 Free-ParticleRetardedGreenFunction... 266 15.2.2 Retarded GF in the Mean-Field Approximation... 267 15.2.3 SpectraofRetardedGfs... 269 15.2.4 Dephasing of Retarded Green Functions.......... 274 15.3 IntrabandRelaxation... 279 15.4 Interband-PolarizationDephasing... 281 15.5 NumericalStrategies... 283 16 Two-Pulse Spectroscopy... 287 16.1 IntroductoryRemarks... 287 16.2 ThinSamples... 289 16.3 Low-IntensityTwo-BeamExperiments... 290 16.3.1 LO-PhononRelaxationCascades... 291 16.3.2 LO-Phonon Quantum Beats in FWM............ 292 16.3.3 Two-Time Electron Phonon Quantum Kinetics.... 294 17 Coulomb Quantum Kinetics in a Dense Electron Hole Plasma... 301 17.1 Introduction... 301 17.2 Screening in the Nonequilibrium GF Theory............. 302 17.3 CoulombQuantumKinetics... 306 17.4 Plasmon-Pole Approximation forthetwo-time-dependentpotential... 309 17.4.1 Parametric Plasma Oscillations.................. 311 17.4.2 Instantaneous Static Potential Approximation..... 313 18 The Buildup of Screening... 317 18.1 ScreeningoftheCoulombInteraction... 317 18.1.1 Calculations of the Two-Time-Dependent ScreenedPotential... 318 18.1.2 Femtosecond Optical Pump andthzprobespectroscopy... 320 18.2 Time-Dependent Screening of Phonon-Mediated andcoulombinteractions... 320 18.2.1 Buildup of the Phonon-Plasmon Mixed Modes.... 324 19 Femtosecond Four-Wave Mixing with Dense Plasmas... 331 19.1 Time-ResolvedFour-WaveMixing... 331 19.2 Time-IntegratedFour-WaveMixing... 334 19.3 Four-WaveMixing withcoherentcontrol... 335 References... 341 Index... 353