Exploring long-range interacting quantum many-body systems with Rydberg atoms

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Exploring long-range interacting quantum many-body systems with Rydberg atoms Christian Groß Max-Planck-Institut für Quantenoptik Hannover, November 2015

Motivation: Quantum simulation Idea: Mimicking one quantum system by another which is: cleaner, more controlled, better observable Motivation: Study fundamental questions of many-body physics. (Quantum) phase transitions, topology, quantum magnetism, out-of-equilibrium physics, thermalization, disorder,. in 1, 2 or 3 dimensions. Challenge: Design experiments to be described by a specific Hamiltonian: Theory and experiment often go hand-in-hand Feynman, Int. J. Theor. Phys. 1982 Georgescu, Rev. Mod. Phys. 2014 2

Simulating solid-state systems Prime example: Optical lattices Solid-state Mott insulator (V2O3) Ultracold atomic Mott insulator Quantum simulators can explore fundamentally new many-body settings! 3

Why Rydberg atoms? Controlled long-range interactions Neutral ground state atoms state of the art: Feshbach tunable contact interactions Weak magnetic dipolar interactions Rydberg atoms: Strong dipolar interactions Interactions laser controlled and state selective Designable spatial dependence Applications in Q-simulation, Q-information and Q-metrology! 4

Examples of Rydberg Q-sim experiments Excitation transport Dissipative systems Günter, Science 2013 Malossi, PRL 2014 Spin chain dynamics Rydberg crystals Barredo, PRL 2015 Schauß, Science 2015 Note: List not complete 5

Outline Increasing complexity One lonely excitation: A scalable superatom Multiple excitations: Dynamics and spatial order Ground state physics: Dynamical crystallization The future: Rydberg dressing 6

The setting Single 2d sample Uniform laser coupling In-situ detection

The machine Laser table Main table Pictures: C. Lünig

The experimental setup Prepare atoms in single 2d plane Engineer initial density distribution Rydberg excitation Image the atoms Sherson, Nature 2010 9

Site resolved imaging of ground state atoms Freeze the atomic distribution (ramp lattices to ~300 μk) 10

Site resolved imaging of ground state atoms Freeze the atomic distribution (ramp lattices to ~300 μk) 11 Use laser cooling (molasses) to induce fluorescence cool the atoms

Site resolved imaging of ground state atoms Freeze the atomic distribution (ramp lattices to ~300 μk) Use laser cooling (molasses) to induce fluorescence cool the atoms Imaging of Rydberg atoms: Be patient for a few more slides... 12

Local control of the atoms Focus laser beam on selected sites Use microwave to drive the spin flip Weitenberg, Nature 2011 13

Writing atomic patterns Digital mirror device (DMD) to objective and atoms 14

Writing atomic patterns Digital mirror device (DMD) to objective and atoms 15

Ultimate initial state control Engineering the density distribution Initial Mott insulator DMD mask 16

Ultimate initial state control Engineering the density distribution Initial Mott insulator DMD mask 17 An atom cookie

Ultimate initial state control Engineering the density distribution Initial Mott insulator DMD mask 18 An atom cookie Precisely defined edge Total atom number 6dB below shot-noise

Rydberg superatoms Rb 68S J. Zeiher, P. Schauß, S. Hild, T. Macrì, I. Bloch, and C. Gross, Phys. Rev. X 5, 031015 (2015)

A normal atom (0.5 μm)

A normal atom (0.5 μm)

A Rydberg atom (250 μm)

Rydberg atoms Highly excited atoms Hydrogen-like wavefunction Saffman, Rev. Mod. Phys. 2010 23

Rydberg atoms Highly excited atoms Hydrogen-like wavefunction Extreme interactions (huge polarizability) (van der Waals: dipole-dipole: ) Saffman, Rev. Mod. Phys. 2010 24

Rydberg atoms Highly excited atoms Hydrogen-like wavefunction Extreme interactions (huge polarizability) (van der Waals: dipole-dipole: ) Tunability! Saffman, Rev. Mod. Phys. 2010 25

The dipole blockade Two photon laser coupling Laser parameters: Rabi frequency: Detuning Jaksch, PRL 2000 Lukin, PRL 2001 26

The dipole blockade Two photon laser coupling Interaction exceeds all relevant Laser parameters: Rabi frequency: Detuning energy scales on μm scales! Blockade radius: Jaksch, PRL 2000 Lukin, PRL 2001 27

Driving a superatom Extreme nonlinearity: At most one excitation Symmetry! Coupling to W-state 28

Driving a superatom Extreme nonlinearity: At most one excitation Symmetry! Coupling to W-state Signature of a superatom scaling of the Rabi frequency 29

Many experiments already... Paris (Browaeys, Grangier) Gaetan, Nat. Phys. 2009 Atlanta (Kuzmich) Dudin, Nat. Phys. 2012 30 Madison (Saffman) Ebert, PRL 2014

Imaging single Rydberg atoms Quantum gas microscope 31

Imaging single Rydberg atoms Coupling Quantum gas microscope 32

Imaging single Rydberg atoms Coupling Blowout Quantum gas microscope 33

Imaging single Rydberg atoms Coupling Blowout De-pumping Quantum gas microscope Detection efficiency: 65% 34

Rabi oscillations 1 atom 35

Rabi oscillations 1 atom 8 atoms 36

Rabi oscillations 1 atom 8 atoms 18 atoms 37

Rabi oscillations 1 atom 8 atoms 18 atoms 41 atoms 38

Rabi oscillations 1 atom 8 atoms 18 atoms 41 atoms 85 atoms 39

Rabi oscillations 1 atom 8 atoms 18 atoms 41 atoms 85 atoms 130 atoms 40

Rabi oscillations 1 atom 8 atoms 18 atoms 41 atoms 85 atoms 130 atoms 186 atoms 41

Scaling the superatom Fitted exponent 0.48±0.10 W-state scaling between 1 and 190 atoms 42

Breaking the dipole blockade Largest system 15x15 sites (186 atoms) Decay time: 0.34μs 43

Breaking the dipole blockade Largest system 15x15 sites (186 atoms) Decay time: 0.34μs Double Rydberg events 44

Breaking the dipole blockade Largest system 15x15 sites (186 atoms) Decay time: 0.34μs Only single Rydberg events Decay time: 0.91μs Double Rydberg events 45

Exploring the transverse Ising Model with long-range interactions Rb 43S P. Schauß, M. Cheneau, M. Endres, T. Fukuhara, S. Hild, A. Omran, T. Pohl, C. Gross, S. Kuhr, and I. Bloch, Nature 491, 87 (2012)

Seriously breaking the blockade Let's drive Rabi oscillations. 47

Frozen gas Rydberg physics Dynamics on sub-μs timescales no atomic motion 48

Long-range interacting transverse Ising model 49

A closer look to the data Superposition of different many-body states 50

A closer look to the data Superposition of different many-body states 51

Emerging spatial order Post select according to the number of excitations Single shot Ensemble ne=2 ne=3 ne=4 ne=5 52

Emerging spatial order Post select according to the number of excitations Single shot Ensemble Ensemble aligned Theory ne=2 ne=3 ne=4 ne=5 53

The blockade radius Distance correlations between Rydberg atoms Imperfections: 54 Hopping during detection: 1% Hopping before detection: 0.5μm Finite blow out: 0.2 atoms/image

Sweeped excitation: Adiabatic ground-state preparation Picture: van Bijnen, J. Phys. B: At., Mol. Opt. Phys. 2011 P. Schauß, J. Zeiher, T. Fukuhara, S. Hild, M. Cheneau, T. Macrì, T. Pohl, I. Bloch, and C. Gross, Science 347, 1455 1458 (2015)

The ground state phase diagram 56

Dynamical crystallization Coherent control of many-body systems through adiabatic sweeps 57

Tracking the crystallization 1D chains 58

Tracking the crystallization 1D chains 59

Tracking the crystallization 1D chains 60

Tracking the crystallization 1D chains 61

1D Rydberg chains: Different lengths Goal: measure crystal compressibility Excitations vs. detuning: Excitations vs. length: 62

1D Rydberg chains: Different lengths Goal: measure crystal compressibility Excitations vs. detuning: Excitations vs. length: DMD cutting: Keep 3xN sites 63

1D Rydberg chains: Different lengths Goal: measure crystal compressibility Excitations vs. detuning: Excitations vs. length: DMD cutting: Keep 3xN sites 64

Rydberg crystals compressibility Rydberg excittion number vs. chain length 65

Rydberg crystals compressibility Rydberg excittion number vs. chain length Plateaus of equal height Vanishing compressibility on the plateaus 66

2D Rydberg crystals Sweeped excitation localizes the excitations! No sweep Sweep, small cloud 67 Sweep, large cloud

2D Rydberg crystals Sweeped excitation localizes the excitations! No sweep Sweep, small cloud Sweep, large cloud Some single shots 68

2D Rydberg crystals Sweeped excitation localizes the excitations! No sweep Sweep, small cloud Sweep, large cloud Some single shots 69

The future: Rydberg dressing New directions for quantum simulations Flexible spin models Supersolids Glaetzle, PRL 2015 van Bijnen, PRL 2015 Henkel, PRL 2010 Pupillo, PRL 2010... And more: Dipolar Fermions Dauphin, PRA 2012 Xiong, PRA 2014 Li, Nat. Comm. 2015 Quantum metrology Bouchoule, PRA 2002 Gil, PRL 2014

Rydberg dressing concepts Admix a little bit of Rydberg to the ground state Admixture Lifetime Interaction Bouchoule, PRA 2002 Henkel, PRL 2010 Pupillo, PRL 2010 Honer, PRL (2010) Johnson, PRA (2010) 71

Rydberg dressing concepts Admix a little bit of Rydberg to the ground state Admixture Lifetime Interaction Requires high Rabi frequency! Bouchoule, PRA 2002 Henkel, PRL 2010 Pupillo, PRL 2010 Honer, PRL (2010) Johnson, PRA (2010) 72

Rydberg dressing concepts Admix a little bit of Rydberg to the ground state Admixture Lifetime Interaction Direct UV coupling! Requires high Rabi frequency! Bouchoule, PRA 2002 Henkel, PRL 2010 Pupillo, PRL 2010 Honer, PRL (2010) Johnson, PRA (2010) 73

Revealing the interaction potential Probing via Ramsey interferometry Rel. pulse height 1 0.8 At short times: phase ~ interactions Directly image the dressing potential 0.6 0.4 0.2 0 0 40 80 Time (μs) 120 74 state feels pair potential Ising Hamiltonian

Rydberg dressing first signs Correlation map Raw image Vert. shift (pix) 5 2 0-5 9-5 0 1 Hor. shift (pix) 5 PRELIMINARY 75

Rydberg dressing first signs Correlation map Raw image Vert. shift (pix) 5 2 0-5 9-5 0 1 Hor. shift (pix) 5 Dressing time (μs) 0 4 7 PRELIMINARY 18 Inducing a long range potential works! 76

Summary Scalable superatoms Multiple excitations Dynamics Rydberg crystals Rydberg dressing First steps The team Theory T. Yefsah J. Zeiher S. Hild R.v.Bijnen J.-Y. Choi S. Hollerith I. Bloch T.Pohl P. Schauß T. Fukuhara M. Cheneau

Starting 2016: RyD-QMB (= Rydberg dressed quantum many-body physics) Starting Grant 2015 Developing a new Q-sim platform: Rydberg dressing with potassium Goals: Flexible spin models Supersolids Glaetzle, PRL 2015 van Bijnen, PRL 2015 Henkel, PRL 2010 Pupillo, PRL 2010... 78

Starting 2016: RyD-QMB (= Rydberg dressed quantum many-body physics) Starting Grant 2015 Developing a new Q-sim platform: Rydberg dressing with potassium Interested in a PhD project? Contact me! Goals: Flexible spin models Supersolids Glaetzle, PRL 2015 van Bijnen, PRL 2015 Henkel, PRL 2010 Pupillo, PRL 2010... 79