Sensitivity and Uncertainty Analysis of the k eff and b eff for the ICSBEP and IRPhE Benchmarks

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Sensitivity and Uncertainty Analysis of the k eff and b eff for the ICSBEP and IRPhE Benchmarks ANDES Workpackage N : 3, Deliverable D3.3 Ivo Kodeli Jožef Stefan Institute, Slovenia ivan.kodeli@ijs.si ANDES-JEFF Workshop, April.23-25, 2012, NEADB 1

Prepared reports for Deliverable 3.3 Ivan Kodeli, Cyrille De Saint Jean, Yannick Peneliau, ANALYSIS OF THE IRPhE AND ICSBEP EXPERIMENTS: C/E AND SENSITIVITY VECTORS Ivan Kodeli, Cyrille De Saint Jean, Yannick Peneliau, SENSITIVITY PROFILES IN COMPUTER READABLE FORMAT Ivan Kodeli, SENSITIVITY AND UNCERTAINTY IN THE EFFECTIVE DELAYED NEUTRON FRACTION (b eff ), PHYSOR2012 presentation ANDES-JEFF Workshop, April.23-25, 2012, NEADB 2

I. Analysis of benchmarks from ICSBEP and IRPhE SNEAK-7A and -7B fast critical experiments fuel with PuO 2 UO 2 and reflected by metallic depleted uranium. JEZABEL is a bare sphere of plutonium metal FLATTOP-Pu benchmarks included a plutonium sphere reflected by natural uranium ZPPR10A experiment: sodium void effects have been measured in addition to the critical mass 3

DESCRIPTION OF SNEAK-7 ASSEMBLIES Reference: NEA/NSC/DOC(2006)1 March 2009 Edition IRPhE Handbook (Evgeny Ivanov, IRSN, CNAM, IPN) Fuel element lattice pitch was 5.44 cm (square fuel elements tubes), and the cross-section of the platelets 5.077 x 5.077 cm 2. SNEAK-7A core unit cell consisted of one PuO 2 -UO 2 pallet (26,6% PuO 2 and 73,4% UO 2 ) and one graphite platelet. Radial and axial blankets were loaded with depleted UO 2 plates. In SNEAK-7B the graphite platelets were replaced by U nat O 2 platelet resulting in an average Pu-enrichment of ~13%. The effective core radii of SNEAK-7A & 7B were 28.63 cm and 37.84 cm, respectively. 4

SNEAK 7A R-Z Model 5

SNEAK 7B R-Z Model 6

1 2 Model Detailed 3D model with stretched platelets 3D simplified model with homogenized core regions of fuel elements SNEAK 7A SNEAK 7B k eff sk eff k eff sk eff 1.0010 (a) 0.0029 (b) 1.0016 (a) 0.0035 (b) 0.9998 (c) 0.0029 1.0001 (c) 0.0035 3 RZ two-dimensional model 1.0038 (c) 0.0029 1.0028 (c) 0.0035 (a) Measured k eff. (b) Combined experimental uncertainty (c) Equal to experimental value + (calculated simplified model calculated more detailed model) SNEAK 7A SNEAK 7B b eff - 252 Cf source measurements b eff noise analysis b eff benchmark values 0.00395 5% 0.00429 5% 0.00413 6% 0.00450 6% 0.00395 5% 0.00429 6% 7

JSI Computational Methods and Procedures ENDF/B, JEFF, JENDL DANTSYS -SN transport code (1D, 2D, 3D) TRANSX - Processes MATXS format library for SN transport code - Self-shielding factor method Group XS Library Processing (NJOY) Multigroup XS Library Effective XS Generation Self-Shielding Correction, (TRANSX) Multigroup Sn transport calc. (DANTSYS, DOORS, PARTISN, DRAGON) Forward Moment Flux Adjoint Moment Flux SUSD3D - Multi-dimensional, SN based XS sensitivity and uncertainty - First-order perturbation theory Resonance Self- Shielded XS Covariance Matrix Processing (NJOY/ERRORR, ANGELO) Sensitivity Analysis (SUSD3D) All computer codes, XS library (KAFAX, JEFF3.1), and the information on benchmarks publicly available through NEA-DB Sensitivity Coefficient & Uncertainties ANDES-JEFF Workshop, April.23-25, 2012, NEADB 8

CEA Computational Methods and Procedures Neutronic and sensitivity codes : ERANOS and PARIS Cross sections: Ecco+Sn2d with JEFF 3.1.1 and ENDF/B-VII (33 energy groups) Sensitivities to cross sections, total nubar and fission spectra ANDES-JEFF Workshop, April.23-25, 2012, NEADB 9

SNEAK-7A & -7B, JEZEBEL, FLATTOP XS from ENDF/B-VII processed by NJOY (80/33 n groups) SNEAK-7A: TWODANT 2D, r=58.63 cm, z=52.52 cm, 49x52I, P3, S8, k eff =1.00733292 (dir), 1.00732422 (adj) SNEAK-7B: TWODANT 2D, r=67.84 cm, z=65.53 cm, 68x65 I, P3, S8, k eff =1.00213408 (dir), 1.00213277 (adj) JEZEBEL-Pu239: ONEDANT 1D, r=6.3849 cm, 60I, P 5, S 48 k eff =0.998396 (dir), 0.998397 (adj) FLATTOP: ONEDANT 1D, r 1 =4.5332 cm, r 2 =24.1420cm, 725I, P 5, S 48 k eff =1.00143 (dir), 1.00141 (adj) TOPSY: ONEDANT 1D, r 1 =6.1156 cm, r 2 = 24.1242 cm, 237I, P 5, S 48 ZPR 6-7: TWODANT 2D R-Z NEA-1650 ZZ-KAFAX-F22 (80 n groups JEFF 2.2) k eff =0.985169 (P 1 S 4 ) NEA-1815: ZZ-KAFAX-E70 150 n groups ENDF/B-VII.0 ( 238 U data recalculated since k eff ~1.08 was obtained with original 238 U) k eff =1.0009163 (P 1 S 4, direct) k eff =1.0009171 (P 1 S 4, adjoint) k eff =1.0006591 (P 3 S 4, direct) ANDES-JEFF Workshop, April.23-25, 2012, NEADB 10

SNEAK-7A 11

SNEAK-7A Sensitivity plot 12

SNEAK-7B 13

JEZEBEL 14

FLATTOP 15

CONCLUSIONS I (SU Intercomparison) Different approached developed at JSI and CEA, using different computer codes (SUSD3D, ERANOS, PARIS), cross-section libraries, energy group structures and modelisation of the geometry were applied to a series of high quality benchmark experiments, including SNEAK-7A & -7B, JEZEBEL and FLATTOP fast reactor systems. This study confirms good agreement between the sensitivities, both of integral values and sensitivity profiles, calculated using the two approaches and contributes in this way to their validation. SG33 Meeting, Dec.. 1, 2011, NEADB 16

II. Sensitivity / Uncertainty of the Effective Delayed Neutron Fraction SUMMARY RECORD of UAM-4 Evaluate uncertainties in delayed neutron yield and its distribution in six delayed groups. Add SNEAK (fast core problem) as an optional test case to the test problems for Exercise I-3 since it has a unique set of experimental data for βeff uncertainties and can be used as an example on how to calculate uncertainty in βeff. The two high-quality reactor physics benchmark experiments, SNEAK-7A & 7B (Karlsruhe Fast Critical Facility) are part of the International Reactor Physics Benchmark Experiments (IRPhE) database. The objectives of adding SNEAK test problem to Exercise I-3 are as follow: The PWR, BWR & VVER cases are very similar in spectrum, a fast reactor case based on a well evaluated experiment would broaden the verification of methods for Phase I of UAM and is a link to reactors of a next generation; Fast reactor benchmarks are proposed to test and compare state-of-the-art cross section sensitivity and uncertainty codes; Benchmark provides an unique set of experimental data on delayed neutrons effective fraction; it could be useful in analysis of components of a βeff uncertainty; The analysis of the experimental set could bring a better comprehension on validity of covariance matrices to be applied. 17

Effective delayed neutron fraction b-eff b eff P d, eff P eff Pd, eff F ( r, E ', ') d ( E ') de ' d' nd ( E) S f ( r, E) F( r, E, ) deddr P F ( r, E ', ') ( E ') de ' d' n( E) S ( r, E) F( r, E, ) deddr eff f where: F, F + = direct, adjoint angular fluxes, S f = fission cross section, χ d, χ = fission spectra (delayed & total), n d, n = delayed & total nu-bar. 18

Effective delayed neutron fraction b-eff DETERMINISTIC CODES: easy b eff can be obtained e.g. using SUSD3D as a ration of two sensitivity terms: b eff d ( E) de S ( E) S ( E) de n p S n n d 1 S E dr d n d de r E r E E n E s E N r p R ' ' * ' i i ( ) F(,, ) F (, ', ) p( ') p( ) f ( ) ( ) 1 S E dr d n d de r E r E E n E s E N r d R ' ' * ' i i ( ) F(,, ) F (, ', ) d ( ') d ( ) f ( ) ( ) Monte Carlo: M. M. Bretscher b 1 eff k k p 19

Calulated & measured b-eff b-eff (pcm) SUSD3D MCNP Measured SNEAK-7A 373 369 395 5% SNEAK-7B 420 415 429 6% FLATTOP-Pu 277 284 360 9% JEZEBEL 184 186 194 10% 20

Sensitivity & uncertainty in b-eff Hammer & Tuttle (1979): Db eff /b eff 5% (power reactor) (F, F + ~2%, nσ f ~1.5%, d ~0.5%) D Angelo et al. (1987): Db eff /b eff 5% (fast reactors) (n d ~2%, d ~0.5%) Zukeran et al. (1999): Db eff /b eff 4-5% (generalised pert. method) (n d ~2.5%, σ f ~1.6%, d ~0.5%) P. Hammer, Requirements of delayed neutron data for the design, operation, dynamics and safety of fast breeder and thermal power reactors, Proc. Consultants Meeting on Delayed Neutron Properties, Vienna, 26-30 March 1979, INDC (NDS)-107/G+Special D'Angelo A., Vuillemin B. and Cabrillat J.C.: NEACRP-A-766, (1987). A. Zukeran, H. Hanaki, S. Sawada, T. Suzuki, Uncertainty Evaluation of Effecti ve Delayed Neutron Fraction b eff of Typical Proto-type Fast Reactor, J. Nucl. Sci. and Technology, Vol. 36, No.1, p. 61-80 (Jan. 1999). 21

Sensitivity & uncertainty in b-eff Monte Carlo: M. M. Bretscher b eff 1 k k p Sensitivity of b-eff can be obtained as a (properly weighted) difference between two standard sensitivity terms: s beff s k p k pk k p s k p s k k p 2 Sk S beff s beff ks k s k k p k p s k s k k p kp or alternatively: s beff k p b s kb eff eff S k S kp 22

This method was first proposed in: I. Kodeli, Sensitivity and uncertainty in the effective delayed neutron fraction b-eff (method and SNEAK-7A example), proc. UAM-5 Workshop, Stockholm, Apr. 13-15, 2011, NEA-1769/04 package, OECD-NEA Data Bank. I. Kodeli, Sensitivity And Uncertainty in the Effective Delayed Neutron Fraction (b eff ), PHYSOR 2012 Knoxville, Tennessee, USA, April 15-20, 2012, on CD-ROM (2012). In January 2012 a similar method was independently presented in: G. Chiba et al., JENDL-4.0 Benchmarking for Effective Delayed Neutron Fraction of Fast Neutron Systems, J. Nucl. Sci. Technology, Vol. 48, No. 12, p.1471-1477 (2011), available online 5. Jan. 2012. 23

SNEAK-7A: Sensitivity to b-eff 24

SNEAK-7A: Uncertainty in b-eff (JENDL-4) TOTAL=3 % 25

JEZEBEL: Total uncertainty in b-eff: 2.2 % 26

FLATTOP-Pu: Total uncertainty in b-eff: 2.6 % 27

Sensitivity of b-eff to delayed nu-bar of Pu-239 SNEAK7A JEZEBEL FLATTOP 28

Objectives / Conclusions (b eff sensitivities) New and relatively simple method was proposed to evaluate the uncertainty in beta-effective due to the basic nuclear data. It is obtained by deriving the Bretscher s (prompt k-ratio) b eff expression with respect to the basic nuclear data. The method was implemented in SUSD3D and applied to the fast benchmarks SNEAK-7A, JEZEBEL and FLATTOP. seem the method provides reasonable results, in rough agreement with other methods used in the past. According to the JENDL-4 covariance data the uncertainty in b eff is mainly due to the uncertainties in delayed (and prompt) neutron yields, inelastic and elastic scattering and fission cross sections, as well as the prompt and delayed fission spectra. The total uncertainty in b eff was found to be between 2.2 to 3 % for the studied cases. 29