GEMS-aerosol work plan

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GEMS-aerosol work plan Met Office, ECMWF, CNRS-LOA, MPI-M, CEA-IPSL-LSCE, NUIG, SA-UPMC, FMI, DWD, RMIB, DLR (no cost) Olivier Boucher Presentation to the GEMS annual assembly Reading, 9 February 2006 Page 1

Aerosol monitoring in GEMS GEIA / ACCENT / RETRO / EMEP PHOENICS / PARTS DAEDALUS / ASSET GlobAER (ESA) Emission maps AER_2 Emissions Aerosol models AER_1 Aerosol model Methodology AER_3 Data assimilation Aerosol satellite data (AOD, radiances) Fire counts ESA EUMETSAT NASA ESA NASA Emissions Global aerosol monitoring system AER_4 validation Various datasets / CREATE RAQ Boundary conditions Heterogeneous chemistry Oxidants GRG GHG Page 2

Objectives of the aerosol breakout session 1/ Review progress from all partners 2/ Make a number of key decisions - model set up for the next year or so - emission datasets - satellite datasets for data assimilation - interfaces with other sub-projects - evaluation strategy 3/ Agree on and polish workplan for months 13 to 30 4/ Decide if interim aerosol meetings are needed Page 3

Constraints PRO workplan Availability and quality of model and satellite data Model cost: choice of the scheme and sensitivity experiments Requirements from other sub-projects (RAQ) Page 4

AER model setup - reanalysis 4-variable scheme in the troposphere -coarse dust and sea-salt calibrated against full ECMWF 10-bin scheme -gas precursor and accumulation mode aerosol from LMDZT -opportunity for upgrades (RAQ) -fudge PM2.5/PM10 variable? 1 moment stratospheric aerosol scheme in the stratosphere - prescribed maps of sigma and r0, OK for background conditions only - to be tested first in LMDZT - to be ported to ECMWF - stratospheric mask: p < 300 mb AND (wv < 7 ppmv OR and O3 > 100 ppbv) potential vorticity 2003, then 2003-2004 Hadley T159L60 Centre (or Crown 91 copyright?) 2004 eq 1.125 Page 5

AER model setup - reanalysis Number of sensitivity runs=function(cpu, evaluation) Sensitivity runs to be performed in the 9 months w/o data assimilation (1-2 year periods) vertical resolution L91 vs L60 wave model on/off w/o and w stratospheric aerosol dust and sea-salt source functions biomass burning emissions (sub-monthly variability) w data assimilation (1-2 week, up to 1 month periods) (possibility of reducing the amount of satellite data assimilated to speed up the system and afford longer test periods) 1/ MODIS total ocean AOD, 2/ MODIS fine/total ocean AOD 3/ MODIS fine/total ocean and total land AOD, 4/ total + SAGE biomass burning emissions (sub-monthly variability) 1 final 2-year experiment with data assimilation (PRO) Page 6

AER model setup - reanalysis Diagnostics list of variables -AOD @ 14 wavelengths (+extra UV and IR to be defined) -fine-mode AOD, absorption AOD, -effective radius of total size spectrum -mass concentrations, fudged PM (?) -profile of extinction coefficient @ 5 wavelengths (strat + trop) -radiation (surface UVB with interactive O3, PAR, SW direct & diffuse, LW) using a second radiation call with aerosols -visibility temporal sampling: 3 hourly (+daily and monthly means) wind-sector sampling (Mace Head, Cape Grim) Page 7

Emissions Fossil-fuel SO2/BC/OC = AEROCOM (updated from EDGAR, ships,...) consult with GRG and Frank first to avoid inconsistencies BC from AEROCOM and CO from RETRO will be compared H2S = scaled to SO2 neglect ammonium and nitrate 2 levels of injection seasonal cycle =paste from RAQ in Europe as possible upgrade weekly cycle = same diurnal cycle = same annual increase rate = projections to 2003/04 from Laxenburg Page 8

Emissions Biomass burning GFEDv2, monthly, 1997-2004, ASCII, 1 x1 SO2 = MS to discuss how to get it BC / OC / PM2.5 / TPM injection height = AEROCOM? MS to review AEROCOM, OB to check MISR products on plumes sub-submonthly variability = F(x,y,t,day,month)=CLIM(month,X,Y) * hotspot(x,y,day) * f(t) hotspot = smooth function from previous days if no data ocean AOD assim, no sub-monthly variability ocean + land AOD assim, some refinements needed some more investigation needed, consistency with GRG Page 9

Emissions Dust YB and PG to provide a benchmark dust source for 2003 development on road dust and arable dust SK to investigate for a further dust source Sea salt YB to provide a benchmark sea-salt source for 2003 Combination of Monahan and Marttensson (T0+16) Source function from Andreas (revised Smith supermicron) Revised source formulation from MAP in the long run Page 10

Emissions Natural VOC Guenther et al monoterpenes DMS check with Sylvia Kloster (JRC) oceanic DMS climatology + transfer function Volcanoes continuous emissions: AEROCOM explosive emissions: TOMS? (SB) Stratospheric source chemical production from OCS prescribed (using correlations with other LL species in the merged system) Page 11

Data assimilation Merged satellite product for validation: - Stefan will provide a document with his comparisons (MODIS,MISR,TOMS,AVHRR,POLDER) - dataset without MODIS for validation of analysis - MSG and GlobAER AOD: under development, will be used for validation and in the future for assimilation if proven good Observations to be used in the first reanalysis: - MODIS data with a bias correction and pixel-by-pixel error estimate over ocean only (AOD to start with, total and fine-mode AOD then) - MODIS data with ocean and land retrievals Observation screening and thinning: - closest pixel - Blacklist problem area Bias correction for MODIS: Page 12 - not recommended to use Remer et al. (need to come up with our own)

Model evaluation No requirement for centralised aerosol data at ECMWF for the moment WDCA, AERONET and other database being maintained already AEROCOM: located at LSCE, ok for daily and monthly point data, 2003-2004 AERONET ok, EMEP?, satellite? Possibility of including more AOD data into AEROCOM (Brewer+PFR) List of case events for 2003/2004 (HB+SK, link to GRG) Need for some headroom for evaluation using DLR data & EARLINET Need for a few common diagnostics with RAQ and GRG Future need for verification data at ECMWF in the operational phase using the MetPy tools. Need to secure NRT access to AERONET. Scoring against AERONET gridded data Need Hadleyto Centre account Crownfor copyright data 2004 error. Page 13

Practical details Minutes and list of actions to be circulated asap Workplan for months 13-30 OB to send revised workplan draft with placeholders Partners to send revised version with track changes by Feb 20. OB to send TH by 28 Feb. First year activity report Partners to send their contribution to WP leaders by 10 March WP leaders to send to OB by 20 March OB to send to TH by 31 March 2 potential interim meetings in the autumn Satellite data (GlobAER, MSG, ATSR) Evaluation (scores, link to GRG and RAQ) Page 14