Ultra clean layers and low albedo ( grey ) clouds in CSET

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CSET RF11, near Hawaii Ultra clean layers and low albedo ( grey ) clouds in CSET Robert Wood, University of Washington Paquita Zuidema, Chris Bretherton, Kuan Ting (Andy) O, Hans Mohrmann, Isabel McCoy, Ryan Eastman, Bob Charlson, Louise Leahy, Bruce Albrecht, Virendra Ghate, Mampi Sarkar, Ed Eloranta, Susanne Glienke, Raymond Shaw, and Jacob Fugal, Matt Lebsock Special thanks to EOL staff who worked to ensure a successful project VOCALS RF06, SE Pacific CSET RF11, near Hawaii

Pathways by which cloud droplet concentration and precipitation impact albedo

Intense drizzle associated with optically thin cloud layers SW Reflectance Closed cells Almost twice as reflective Rain rate @ cloud base [mm d-1] 0.1 1 10 100 Open cells More heavy drizzle More optically thin cloud Column max reflectivity [dbz] Cloud optical depth Muhlbauer et al. (Atmos. Chem. Phys., 2014)

Ultra clean layers and optically thin clouds Strong depletions of N d /CCN associated with optically thin gray clouds in all VOCALS open cell cases VOCALS RF06 profile Schematic figure of decoupled remote marine boundary layer

Gray layers and bright Cu CSET RF04 50 km 300 km MODIS Terra visible imagery Photo: Bruce Albrecht

A Train example of gray clouds CMIP5 Models - Obs Albedo Cloud fraction Too few, too bright pathology from Bender et al. (2016), Nam et al. (2012)

Prevalence of optically thin clouds in trade PBL MODIS perspective In regions with 50% low cloud (e.g., Hawaii), 50% of clouds have optical thickness <3 CALIOP lidar perspective In regions with 50% low cloud (e.g., Hawaii), the surface can be detected through >50% of low clouds [Leahy et al. 2012] Optically thin fraction of low cloud

Optically thin layer clouds in open cells CSET RF07 (19 Jul 2015) 1 z [km] 0 1.5 3.0 HSRL backscatter [G-V] 10 km UCL optically thin cloud layers No clear drizzle below cloud km -1 sr -1 0.1 0.01 10-3 10-4 10-5

Gray clouds in ultra clean layers (UCLs) RF07 Photo from GV aircraft 17:42 UTC (Paquita Zuidema) MODIS Aqua RGB image, 22:15 UTC Cold pools seen in sunglint

View angle dependence of perceived gray cloud morphology RF07 Photo: Paquita Zuidema

What is an Ultra Clean Layer? A horizontally extensive layer that can contain either clear air, cloud, or both cloudy/clear air with very low concentrations N a of accumulation mode aerosol particles (diameters > 0.1 m), or very low cloud droplet concentrations N d (when the layer is cloudy) Here, we define a UCL as having: N a < 10 cm 3 [CLEAR SAMPLES] N d < 10 cm 3 [CLOUDY SAMPLES, q L,CDP > 0.01 g m 3, RH > 0.95]

UCL coverage clear UCL coverage determined separately for clear and cloudy samples. Aggregate data flight byflight into 5 o longitude boxes and 100 m altitude bins Level with maximum UCL frequency sets coverage on any given day. Average daily coverage to give overall UCL coverage for all flights/longitude boxes cloudy RH

Ultra clean layers (UCLs) are common over NE Pacific Cloud System Evolution in the Trades (CSET) project, NCAR G-V, Jul-Aug 2015 CALIOP cloud top height [km] Frequency Increase with z frequency UCLs defined as samples with N d (cloudy) or N a (clear) < 10 cm -3

Low N d Low N a Clear and cloudy UCLs tend to occur near the top of the PBL, with higher concentrations below.

Liquid water contents and particle concentrations in UCLs height [km] 3 2 1 Mean cloud q L,cld and drizzle q L,driz liquid water contents of cloudy UCLs q L,cld (CDP) q L,cld (King) q L,driz (2DC) height [km] 3 2 1 Median aerosol or cloud droplet concentrations for UCL samples (b) (a) 0 0.00 0.05 0.10 0.15 0.20 Mean q L [g m -3 ] 0 cloudy samples clear samples 0 2 4 6 8 10 Median N a or N d in UCLs [cm -3 ] (a) Mean liquid water contents in UCLs partitioned into condensate in cloud droplets (r<20 mm) and drizzle drops (r>20 mm). Cloud liquid water contents are shown for two different measurements (CDP and King hotwire probe); (b) Median concentrations of cloud droplets (for cloudy UCL samples) and accumulation mode aerosols (for clear UCL samples).

UCL Gray Cloud Microphysics Droplet size distribution RF07 - July 19th Concentrations and condensate Droplet concentration [cm -3, left axis] Liquid Water Content [g m -3, right axis] Drizzle Drop Conc. [liter -1, left axis] Height [km] 0 1.5 3 4.5 High Spectral Resolution Lidar dbz 19:10 19:11 19:12 19:13 19:14 19:15

UCL clouds and vertical turbulent motions w'w' Example from RF02 shows positive correlation between Nd and vertical wind variance (using Chris Bretherton s derived whi2 variable) UCL clouds associated with low values of whi2

UCL clouds and vertical turbulent motions Statistical analysis from all CSET flights UCL clouds have much lower turbulence than non UCL clouds Clear UCLs also much less turbulent than non clear UCLs? Consistent with UCLs tending to occur in the upper PBL away from surface driven mixing w'w'

Hypothesis for UCL gray cloud formation Active trade Cu towers driven by surface and latent heating loft condensate into the upper PBL, but the strong trade inversion quickly decelerates the rising column, which must therefore spread by continuity of mass. Turbulence in the spreading Cu anvils dissipates, resulting in relatively long in cloud residence times, and an opportunity for cloud microphysical processes to act to broaden drop size distribution and deplete droplets. Upon evaporation of UCL clouds, few accumulation mode particles are returned to the clear sky, leaving horizontally extensive layers strongly depleted in aerosol. The long overturning timescale ( 12 hr) for the upper trade PBL means that numerous Cu events can result in UCLs extending many hundreds of km

GOES: evolution of cloud fraction and retrieved N d along CSET Lagrangian trajectories During CSET, only trajectories starting with extensive cloud cover (CF > 0.8) had N d > 40 cm 3 Transition to lower CF along Lagrangian trajectories was associated with N d values < 40 cm 3 Is the formation of low N d (UCLs) a requirement of Sc to Cu transition?

Potential for retrieval of droplet size in UCL clouds with radar lidar In-situ DSD in UCL cloud UCL clouds in CSET MODIS r e [micron] O Connor et al. (2005) radar-lidar method to estimate effective radius Maddux et al (2010)

Next steps Complete UCL analysis of CSET in situ data Further examination of cloud and aerosol size distributions Examination of thermodynamic PBL structure associated with cloudy and clear UCLs Turbulence analysis Remote sensing investigation of UCL clouds How to characterize gray clouds using CSET remote sensing (radar, lidar, radiometry) and satellites? Evaluate how well satellites measure N d in UCL clouds Acknowledgements Many thanks to the staff of EOL and RAF for ensuring a successful project and for producing a unique dataset of high quality