Clusters in granular flows : elements of a non-local rheology

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CEA-Saclay/SPEC; Group Instabilities and Turbulence Clusters in granular flows : elements of a non-local rheology Olivier Dauchot together with many contributors: D. Bonamy, E. Bertin, S. Deboeuf, B. Andreotti, O. Pouliquen, (GDR MIDI) Geneve, November 2003

Introduction: Granular materials Three typical behaviours, depending on the stress/strain imposed to the material Specific properties Complex interactions : solid friction Inelastic collision => dissipative dynamics Rather large number of particles => statistical description

Overview Dense flows : The need for a non-local rheology Experimental evidence of clusters : a first step towards a non-local rheology Dynamical Clusters in stationnary flow (rapidly) Intermittent clusters during relaxation towards mechanical equilibrium (in more details)

Studying dense flows rheology Several configurations given state of stress /strain measure the kinematic properties extract the rheology Questions are Relevant timescales? Dependance on microscopic properties? Dimensionless parameters? Influence of the geometry?

Relevant parameters (I) Three scales of different natures: The microscopic scale : the contact scale The grain scale The flow scale At the microscopic scale: The roughness and the interparticle friction: fully encoded into some effective friction During a collision : a collision time (elastic properties) and a dissipation timescale (internal elastic vibrations damping rate) => For slow enough flows, the grains are equivalent to rigid inelastic spheres

the effective friction coefficient µ eff = τ /P => The rheological relation is given by the relation between τ /P and I Relevant parameters (II) At the grain level : Natural length scale : grain diameter d In homogeneous shear flows : Strain tensor reduces to shear rate γ& Stress tensor reduces to normal stress P and shear stress τ Two independant dimensionless numbers the rescaled shear rate I = &d γ P ρ

Flow down an inclined plane (O. Pouliquen) Flow thresholds :the flow starts at θ start (h) and is sustained above θ stop (h)< θ start (h) => hysteretic The velocity profile is Bagnold like : V( y) gd ( h = A( θ) 3/ 2 ( h 3/ 2 d y) 3/ 2 A scaling law is obtained : < V > gh β h stop h (θ)

Flow down a heap (D. Bonamy) Flow thresholds :the flow starts at θ start and is sustained above θ stop => hysteretic V ( y) ( h y) The velocity profile is linear : = γ& gd d A scaling law is obtained : h d Q* < V > gh h d in agreement with the direct observation on the profiles of a

Rheology In both flows τ P( y) = ρg( h y)cosθ ; = P tanθ Assuming a local rheology : τ/p=µ(i), integrating I = & γ y) d = µ P( y) / ρ ( 1 (tanθ ) leads to the Bagnold profile with 2 A ( θ ) = I( θ ) cosθ 3 V( y) gd ( h = A( θ) 3/ 2 ( h 3/ 2 d y) 3/ 2 ) Integrating the profile on the flow thickness leads to the scaling < V > 3 h gh = 5 d A( θ )

First Conclusion: At the first order, a local rheology is compatible with the kinematic properties of a dense granular flow down an inclined plane On the contrary, it is incompatible with the observations made in the case of the flow down a heap! As a matter of fact, a closer inspection of the inclined plane case reveals that the boundary layers escape the Bagnold type profile and therefore also escape the local rheology assumption.

Experimental evidence of clusters : a first step towards a non-local rheology Rotating drum D = 450 mm δ = 3 to 22 mm Steel beads d = 3 mm m = 0.11 g Angular velocity Ω

Dynamical clusters in steady flow Ω h (2D flow) Local density field at the grain scale Voronoï cells around each grain 0,7 0,9 A priori, rather weak variation

Rigid clusters induced by the Reynolds dilatancy property Reynolds dilatancy V 0 < V1 > V2 V0 V1 V2 Very intermittent rigid clusters of all sizes 0,7 ρ > ρc no shear (in 2D, ρc = π/4=0,78) 0,9

Clusters during relaxation The drum is rotated for a while, stopped and the pile slope is set to θ i < θ stop at t=0, (θ stop = 19.2 ) The pile relaxes towards mechanical equilibrium: Average images (25 im at 5 Hz) are recorded every 15 s. Image differences allows to observe where displacements occur. θ i = 0.3 after 15s after 75s after 165s

An intermittent relaxation dynamics θ i = 16.5 First a rapid relaxation of the bulk An intermittent relaxation of the surface layer

Intermittent bursts relates to correlated displacements. θ i = 15 θ i = 16.5 A dynamics composed of exponential decay short intermittent burst Exponential decay : Individual displacements Intermittent bursts : Correlated displacements

Further characterization : characteristic times Exponential decay rate : τ increases with θ i. Bursts intervals distribution essentially invariant, with characteristic time : τ b =100s.

Exponential decay : rapid saturation and average number of move smaller than one In the presence of bursts : no saturation and average number of move larger than one. Further characterization: two-time relaxation function t = w t, t) + N ( δa( u) du w t w t

An over-simplified model Beads can be in active (1->n) or inactive (0) states active state : the bead transits to another active state with rate α and to inactive state with rate α resulting in a global rate of transition from an active state γ=α +(n-1)α. These transition are assimilated to actual individual move of the beads and thus contribute to N(t w, t). inactive state : the bead do not evolve spontaneously. the reactivation process : randomly chosen beads are instantaneously set in the active state with probability ν independently of their state. This process is assumed not to involve displacement of the bead but rather a rearrangement of its environment and thus do not contribute to N(t w, t).

Model : results The fraction of active beads is given by : P = m( t) Pi ( t) 1 where is the probability of being in active state i. P i (t) n Accordingly, t = w N ( t, t) +t γp ( t) dt w t w m The dynamics is given by dp dt = α P + νp = α P + ν (1 0 m m where the key ingredient of the model is now introduced: ν = ν ( P ) = µ m P m γ g( t w + t) After some calculations, one finds: N( t = w, t) ln µ with a reparametrization of time: g( tw) ( α µ ) g( t) = ( α µ ) + µ P t m (0)1 e m m P [ ] ).

Model discussion : applying to experimental data A scaling function is proposed for N(t w,t): It is valid It provides experimental (a) (b) values for the parameters. 1/α 1/(α-µ) 56 s 75 s 294 s 1250 s γ/α 1 4.7

+saturation Model discussion: interpretation A correlation function can be defined as the probability not to have changed state between t w and t w +t. It reads : C( t w, t) = P m ( t w ) e γt rapid relaxation + (1 P m ( t w g( t ) w + t )) g( tw) 1 relaxation on time t 0 (t w ) t 0 1/α t 0 t w t 0 1/δ t 0 1/α t 0 t w t 0 1/δ

Conclusion The kinematic properties of dense granular flows are incompatible with a simple local reology Experimental evidence of clusters support the need for a non-local rheology: In steady flows : rigid clusters induced by the Reynold s dilatancy property In relaxation processes : intermittent bursts of correlated displacement Investigating clusters has driven us towards the description of long term but finite aging behaviours Granular rheology, in very dense or slow flow may have a lot to do with glassy dynamics.