In-Vessel Tritium Inventory in Fusion DEMO Plant at JAERI

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Japan-US Workshop on Fusion Power Plants and Related Advanced Technologies with participation of EU January 11-13, 2005 at Tokyo, JAPAN In-Vessel Tritium Inventory in Fusion DEMO Plant at JAERI Hirofumi Nakamura and JAERI-DEMO design team Japan Atomic Energy Research Institute(JAERI)

Tritium Issues in Fusion Power Plant Tritium inventory in fusion power plant relates - Tritium inventory control (Accountancy of T production and consumption, Waste management) - Source term for safety assessment (Accidental and normal T release) - Design basis of tritium processing plant (Water detritiation system of cooling system, T removal method from materials) Knowledge on tritium inventory is essential to safety and economical design of the fusion power plant H. Nakamura, Japan-US WS on Fusion Power Plant in participant of EU, 2005,Jan.11-13 2

Objective and Outline OBJECTIVE - To estimate in-vessel tritium inventory in the Fusion DEMO reactor designed by JAERI - To clarify critical tritium issue on inventory reduction or on tritium inventory control in DEMO OUTLINE - Clarification of difference of specification concerning T inventory issues between DEMO and ITER - Evaluation of T inventory in DEMO analytical method analytical conditions analytical results - Characterization of feature of T inventory issues in DEMO H. Nakamura, Japan-US WS on Fusion Power Plant in participant of EU, 2005,Jan.11-13 3

Difference of basic specification between DEMO and ITER on T issues Basic parameters ITER DEMO Reactor operation Fuel cycle Material selection Fusion power 0.5 GW 3 GW(1 GWe) Operation Pulse operation Steady operation (75%/year) Coolant temp. Low (<450K) High (600~700K) T consumption ~17 gt/day ~450 gt/day T production negligible ~500 g/day(tbr=1.1) Site T inventory ~3 kgt <3 kgt PFC W/Be/CFC/Cu W/ Structure SS316/Water /Water BLK various Solid breeder /Water H. Nakamura, Japan-US WS on Fusion Power Plant in participant of EU, 2005,Jan.11-13 4

T Inventory in ITER and DEMO ITER DEMO T in T plant ~1 kgt Same with ITER T in PFC T in coolant ~1 kgt (0.35 kgt) Mainly in Co-deposition layer How much amount of T? Mainly? T in BLK TBD (Maybe negligible) How much amount of T? (There is rough estimation) Key issue on T inventory <2 gt (mainly from Be FW) T concentration <<10 Ci/L* Only the co-deposition of carbon and tritium is a critical problem in ITER. How much amount of T? Where from mainly? (There is rough estimation from BLK region) What is the critical issue on T inventory in DEMO? *Based on the safety handling experience of tritiated water in CANDU reactor. Evaluation of Tritium inventory in DEMO H. Nakamura, Japan-US WS on Fusion Power Plant in participant of EU, 2005,Jan.11-13 5

Evaluation method Tritium inventory evaluation - Classified the DEMO into several in-vessel components - One dimensional analysis for simplification - Combined tritium transport and thermal transport analysis for one-dimensional analytical system (TMAP5 code) Tritium transport Thermal transport C( x, t) J ( x, t) = + γc( x, t) + S( x, t) t x * C( x, t) C( x, t) Q J ( x, t) = Deff ( T )( + ) 2 x kt T ρc = (κ T ) + t p S h C(x,t):T concentration, S:T source J:diffusion flux, γ:decay constant D eff :Effective diffusivity, Q*:heat of transport t, ρ:density, C p :heat capacity, T:temp., κ:thermal conductivity, S h :Heat source To solve tritium inventory using above analytical system - Operational conditions (heat load, particle load,etc.) - Tritium transport properties (Diffusivity, Solubility etc.) are necessary H. Nakamura, Japan-US WS on Fusion Power Plant in participant of EU, 2005,Jan.11-13 6

Classified In vessel components in DEMO for T inventory analysis DEMO components were classified into VV -PFC Divertor (DIV), First wall(fw) - Blanket(BLK) - Structure material (VV) BLK DIV/FW - Coolant In-vessel component in DEMO H. Nakamura, Japan-US WS on Fusion Power Plant in participant of EU, 2005,Jan.11-13 7

DIV Cooling tube Thermal and particle load Detail of classified in-vessel W armor components in DEMO FW 1~2 mm Thermal and particle load FW and BLK W 10 mm 5 mm 1st Multiplier Layer 2nd Breeder Layer 2nd Multiplier Layer 1~2 mm 5 mm W 20 mm 1st Breeding Layer 15 m VV 9 m DT gas 10 mm W armor 6 mm 6.3 mm 1 mm 3 mm W armor 21 mm 10 mm BLK Third Breeder Layer Third Multiplier Layer 1.5mm t Coolant manifold Cooling Tube Coolant T inventory in coolant is evaluated by permeation from the components H. Nakamura, Japan-US WS on Fusion Power Plant in participant of EU, 2005,Jan.11-13 8

Operating conditions of the invessel components of DEMO DIV Thermal load (heat flux/temp.) PFC coolant Flux Particle Load DEMO 7/1273 473 3x10 23 2.5nm FW Thermal load (heat flux/temp.) Range Particle Load PFC coolant Flux Range DEMO 0.6/773 603 3x10 21 2.5nm VV DEMO BLK DEMO Thermal load (heat flux/temp.) Inner surface 0/333 Cooling tube 633~653 Unit of parameters Heat flux: MW/m 2 /s, Temp.: K, Flux:DT/m 2 /s coolant 333 Thermal load (heat flux/temp.) coolant 633~653 Particle Load T Pressure 1 Pa Particle Load T Pressure 1Pa (H 2, T=1%) Surface area and base materials of in-vessel components in DEMO Area/material 200 m 2 DIV W/ VV BLK cooling tube* 700 m FWW/ 2 ~800 m 2 8000 m 2 glass/ * Y.Kosaku et al., Fusion Sci. Technol.,41 958 (2002) H. Nakamura, Japan-US WS on Fusion Power Plant in participant of EU, 2005,Jan.11-13 9

T Transport properties of in- vessel components materials Effective Diffusion coefficient (m 2 /s) Tungsten 6.74 10-8 exp(-0.73ev/kt) *1 10times larger in plasma facing region *2 1.07 10-7 exp(-0.15ev/kt) /(1+2.9x10-8 exp(0.58ev/kt) *5 10times larger in plasma facing region *2 Solubility (atoms/m 3 / Pa) Recombination coefficient (m 4 /s) 1.83 10 24 exp(-1.04ev/kt) *3 6.21 10 23 exp(-0.28ev/kt) *5 7.1 10-18 exp(-0.81ev/kt) *4 9.4 10-26 exp(-0.12ev/kt) *6 * Irradiation effect was not considered in this evaluation *1 H. Nakamura et al., JNM 297(2001)285, *2 H. Nakamura et al., JNM 313-316 (2003) 675 *3 R. Frauenfelder, J. Vac. Sci. Technol. 6 388 (1969), *4 R. A. Anderl et al., Fusion Technol. 21 745 (1992)., *5 E. Serra et al., JNM 245 (1997) 108, *6 M. Enoeda et al., JAERI-tech 2001-078, H. Nakamura, Japan-US WS on Fusion Power Plant in participant of EU, 2005,Jan.11-13 10

Analytical result (1) Transient T inventory in DEMO operation T inventory (gt) 10 2 10 1 10 0 10-1 10-3 10-4 ON OFF DIV Coolant FW In- vessel VV (DIV+FW+VV) 0 500 1000 1500 time (day) Time evolution of tritium inventory in the components and coolant during DEMO operation (except BLK). DIV:1µm W coating on the cooling tube FW: 1mm W coating - Tritium inventory in the components and permeation into the coolant will reach at saturation level and steady state within one year operation of DEMO, respectively, while permeation in ITER will not reach steady state even after 3 years operation* - Tritium inventory and permeation in DEMO is quite faster to reach steady state than the ITER case due to steady state operation, higher operation temp. and ferritic steel () structure. *H. Nakamura et al., JAERI-Research 2003-024 (2003). and JNM 329-333 (2004) 183 H. Nakamura, Japan-US WS on Fusion Power Plant in participant of EU, 2005,Jan.11-13 11

Analytical result (2) T inventory in in-vessel components Tritium inventory in the components at saturation level (Those results didn t include neutron irradiation effect) DIV FW BLK VV ~1.5gT ~0.3gT ~1.2 gt* (Li 2 O case) 100% DIV W 100% FW ~mgt W - Tritium in the components mainly exists in the DIV (armor region) and BLK. - Total T inventory in the invessel components is ~gt. It is negligible smaller than ITER case(1.2kgt) due to carbon free PFC in DEMO. 1.28e- 005% 0.000602% Tritium inventory in the components will not be a critical issue in DEMO Breakdown of T inventory in materials for DIV and FW * M. Enoeda et al., Nuclear Fusion, 43 1837 (2003) H. Nakamura, Japan-US WS on Fusion Power Plant in participant of EU, 2005,Jan.11-13 12

T inventory increse (gt/y) 10 4 10 3 10 2 10 1 PRF =1 Analytical result (3) T inventory in coolant(1) Permeation from BLK* current design PRF =100 PRF =1000 Permeation from PFC W armorw armor =0mm =0.5mm current design W armor =1mm Annual T inventory increase in the coolant from PFC (DIV and FW) and BLK for various permeation reduction barrier PRF:Permeation Reduction Factor W armor: W armor thickness on FW * Y.Kosaku et al., Fusion Sci. Technol.,41 958 (2002) ** M. Enoeda et al., JAERI-tech 2001-078 (By Nakamichi) - T inventory in coolant strongly depends on the permeation reduction effect of coatings on components surface. -Current design of DEMO FW: W coating (~mm) is necessary for the reduction of erosion of ferritic steel BLK: 100 or more PRF is expected by the glassy coating on the cooling tubes** - In current design of DEMO, T in the coolant is mainly attributed to permeation from BLK region. H. Nakamura, Japan-US WS on Fusion Power Plant in participant of EU, 2005,Jan.11-13 13

Analytical result (3) T inventory in coolant(2) T inventory increse (gt/y) 10 4 10 3 10 2 10 1 PRF =1 Permeation from BLK current design PRF =100 PRF =1000 Permeation from PFC W armorw armor =0mm =0.5mm current design W armor =1mm Annual T inventory increase in the coolant from PFC (DIV and FW) and BLK for various permeation reduction barrier * - Without permeation barrier, annual T inventory increase in the coolant will be tens kgt/y. - Water detritiation system (WDS) can not recover such amount of tritium from cooling water even in the R&D target for DEMO. - It means tritium will run out within one month operation of DEMO. - It is not acceptable!! - At least PRF=100 is required to maintain the T concentration in the coolant below 10 Ci/L/year (within R&D target of WDS capacity) Tritium permeation reduction is a critical issue in a viewpoint of the tritium inventory control at DEMO H. Nakamura, Japan-US WS on Fusion Power Plant in participant of EU, 2005,Jan.11-13 14

Analytical result (4) T Inventory in ITER and DEMO T in PFC T in coolant T in BLK ITER ~1.2 kgt Mainly in Co-deposition <2 gt (20 years) mainly from Be FW TBD (Maybe negligible) DEMO ~1.5 gt Mainly in W armor of DIV ~tens kgt/y (worst case) <200 gt/y (target value) ~1.2 gt Mainly in the breeder In ITER, - Only the co-deposition issue is a critical issue In DEMO -Tritium inventory in the component (PFC and BLK) will be negligible, since there are no carbon materials. - Tritium inventory in the coolant will be a critical issue without permeation reduction method. H. Nakamura, Japan-US WS on Fusion Power Plant in participant of EU, 2005,Jan.11-13 15

Uncertainties and Further analysis We could identify the critical issue on T inventory in DEMO. There are still uncertainties, however. Uncertainties - T transport properties in the permeation reduction coating materials (Key issue for PRF in BLK region) - Neutron irradiation effect on T transport properties in the DEMO components materials (Durability of coating and inventory enhancement) - T transport mechanism at the interface between cooling tube and coolant Further analysis - Further evaluation in BLK region - Evaluation of tritium migration into the secondary coolant - Modification of evaluation with resolved uncertainties H. Nakamura, Japan-US WS on Fusion Power Plant in participant of EU, 2005,Jan.11-13 16

Summary - In-vessel tritium inventory in the JAERI-DEMO has been evaluated under the current design and operational conditions - Based on the obtained results, the feature of tritium inventory in DEMO has been characterized by comparing with that in ITER - Analytical results indicated that tritium inventory in in-vessel components will be negligible in DEMO. However, the tritium inventory in the coolant in DEMO is much greater than that in ITER. - Establishment of tritium permeation reduction technique into the coolant is a critical issue in a viewpoint of tritium inventory control. H. Nakamura, Japan-US WS on Fusion Power Plant in participant of EU, 2005,Jan.11-13 17