Variational Calculation of Eective Classical. November 12, Abstract
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1 Variational Calculation of Eective Classical Potential at T to Higher Orders H.Kleinert H.Meyer November, 99 Abstract Using the new variational approach proposed recently for a systematic improvement of the locally harmonic Feynman{Kleinert approximation to path integrals we calculate the partition function of the anharmonic oscillator for all temperatures and coupling strength with high accuracy. HEP-TH-9578 ) Some time ago, Feynman and Kleinert [] extended the variational approach to euclidean path integrals developed earlier by Feynman in his textbook on statistical mechanics [], improving greatly the accuracy at low temperatures. A similar extension was found independently by Giacetti and Tognetti [] who applied this method to several statistical systems []. The approach is particularly successful in systems in which the quantum eects do not produce essentially new phenomena, their main result being a modication of the quasi-harmonic properties of a system. This happens in quantum crystals [5] where experimental data can now be explained very well. The approach yields a good approximation to the eective classical potential V e ;cl at all temperatures and serves to calculate the free energy of the system as well as particle distributions at all coupling strength, including the strong coupling limit. The purpose of this note is to present results of a recently proposed systematic improvement [] of this method for the anharmonic oscillator carried out to third order in the coupling strength. The results turn out to be in excellent agreement with a precise numerical values of the free energy [7] at all temperatures and coupling strengths available in the literature. ) Let us briey review the Feynman{Kleinert approach. The aim is to write the partition function as a classical conguration space integral over a Boltzmann factor involving an eective classical potential V e ;cl (x ): Z Z dx q e V e;cl(x ) h M ()
2 with k B T. The variable x is equal to the time-averaged position x R h d x() of the uctuating path. The eective potential V e ;cl (x ) is dened by the path integral ZZ exp f V e ;cl g Z x Dx (x x ) exp f Ahg ; () with the euclidean action A d M _x V (x) where (x x ) q h M(x x ) restricts the path average x to the value x. The paths are periodic in h. We shall refer to Z x as a restricted partition function. The usefulness of separating out x derives from the fact that at any temperature the uctuations rarely carry x() far away from x. This allows approximating the deviations from x in a quasi-harmonic way. One reexpresses the local partition function as an expectation value within a harmonic trial system whose action is, for each x, A x M d _x (x )(x x ) () and chooses (x ) optimally. With the help of A x, the dening expression () can be rewritten as exp f V e ;cl (x )g (Z x ) hexp f (A A x )hgix () for any (x ). The subscript stands for the trial system in which the expectation is calculated and the superscript x indicates the restricted value of x. The expectation value on the right-hand side of () cannot be calculated exactly. A lowest-order approximation is found with the help of the Jensen-Peierls inequality hexp f (A A x )hgix exp ha A x ix h : The harmonic expectation value in the exponent of the right-hand side yields the approximation W for the eective classical potential V e ;cl (x ) W (x )V x (x )V a (x ) M (x )a (x ): (5) The rst term is the logarithm of the restricted partition function of the trial system ln f(h(x )) sinh(h(x ))g, the last two terms are the restricted expectations hv (x)i x V (x a )
3 and M (x ) (x x ) x M (x )a (x ): In the last equation we have abbreviated the restricted square deviation h(x x ) i x by a (x ) h coth h M : () The rst term is the usual thermal expectation <x ()>; the second term subtracts from this the square deviations of the temporal average x from x. The restricted expectation of the potential is obtained by a simple gaussian smearing process of a width a (x ) Z dx V a (x ) p V (x)e (x x ) a : (7) a The best approximation is obtained by minimizing the function W (x ) with respect to (x ) which yields the V a (x ): (8) The resulting W (x ) is always slightly larger than the exact eective classical potential V e ;cl (x ). Eqs. () and (8) are solved numerically. The resulting approximation to the partition function Z dx Z q e W (x ) h M leads to the free energy F k B T ln Z which describes the true free energy F k B T ln Z of the system quite well at all temperatures. Ref. [8] explains why this is so. For the anharmonic oscillator potential V (x)! x g x ; Eq. (8) leads to the following equation for the optimal : gx g h coth h : (9) The resulting free energies are listed in Tab. for comparison with the improved results to be derived in this note. ) To gobeyond the above approximation we split the action into a free part A and an interacting part A x int. The rst contains all classical terms depending on x plus the
4 trial action A x be rewritten as Z of Eq. (), the second term all the rest. The partition function can then Z Z dx q Z x dx D E q e V (x )h e Ax x int h : () h M h M In the previous section, the Jensen{Peierls inequality was used to approximate the expectation value on the right-hand side of (). Now weevaluate this expectation perturbatively, expanding the exponential function in a Taylor series Z x e V (x ) Z x h hax int ix (A x!h ) x int (A x!h ) x int : and going over to the connected parts by a reexpansion into cumulants n Z x exp V (x ) V x The truncated exponents W N (x ) V (x )V x h hax int ix h hax int ix (A x h ) x int ;c h (A x int ) x ;c o: () h (A x ) x int ;c (A x h int ) x ;c ( )N (A x N!h N int )N x () are optimized in (x ) and yield the successive approximations to the eective classical potential V e ;cl (x ). The lowest approximation W (x )obviously coincides with the Feynman-Kleinert approximation. We study the behavior of W N (x )upton. The condition of an optimal (x ) cannot always be met by an extremum of W N (x ), since for higher N>the N (x )@(x ) does not always have real solutions (x ). This happens for example at N. In such cases, an optimal result is obtained by enforcing a minimal dependence on via the disappearance of the second derivative ofw N (x ) with respect to (x ). To calculate the restricted expectation values in equation () we consider polynomiallike potentials in view of the intended quantum eld theoretic applications. The interaction A x int is expanded around x A x d int dening the coupling constants n g! (x x ) g! (x x ) g o! (x x ) ; () g i V (i) (x ) i; : ()
5 5 Then () is obtained by calculating all connected vacuum diagrams formed with vertices g n n!h and lines which stand for the correlation function ( G () (; ) h cosh[ h ( ) j j )] h ; (5) M sinh h in which the rst term is the usual Green function hx()x( )i of the harmonic oscillator while the second term subtracts from this the zero-frequency part hx i. The number of Feynman integrals to be calculated is reduced in three ways. First, only one-particle irreducible vacuum graphs contribute (i.e., there are no tadpole diagrams) due to the absence of the zero-frequency modes in x() x() x. Second, Feynman integrals of subdiagrams which touch the rest in one vertex can be factored out. Third, diagrams with vertices g (mass insertions) can be obtained from those without these vertices by replacing the frequency by p g and expanding the result in powers of g. ) We now turn to the application to an anharmonic oscillator with the potential The interaction is A x int Z d V (x)! x g x : n g! (x) () g! (x) () g o! (x) () (we use natural units with h M ), with the coupling constants g (! )gx g gx () g g: The quadratic coupling g (x) () isnow included into the harmonic trial potential term by changing it to (x x ) with the modied frequency introduced above. The third-order approximation W ( ) V (x )V x h hax int ix has the diagrammatic expansion ( W ( ) V (x )! h (A x ) x int ;c (A x h int ) x (7) ;c 7!
6 !)! : The number under each diagram count in how many Wick contractions it appears; this number multiplies the prefactors. Only ve integrals corresponding to the diagrams ; ; ; ; need to be evaluated explicitly. The remaining diagrams follow by dierentiation with respect to and factorization into subdiagrams touching each other at a point. In quantum eld theory one is used to calculate Feynman diagrams in momentum space. At a nite temperature this requires performing multiple sums over Matsubara frequencies. To higher order, they are hard to do in closed form. In the present case of a D -dimensional quantum eld theory it is more convenient to evaluate the diagrams in -space as integrals over products of the Green function (5). For example, the diagrams ; require the integrals (before replacing! ). h ha a G () (;) d; G () ( ; )G () ( ; )G () ( ; ) d d d ; respectively. The factors h are due to an overall -integral, the powers of arise from the remaining ones. The parameters a m have the dimension of a length, the subscript indicating the number of vertices in the diagram (dening a a ). In terms of these two Feynman integrals, the integral associated with the last diagram in (8) is given by the product ^ h a (a )
7 7 The symbol ^ indicates that the right-hand side is only the Feynman integral of the diagram without the factors g n n!h associated with the vertices. The explicit expressions for the dierent Feynman integrals are, with the abbreviation x h, Tr log G () V x ^ h a h a x sinh x ^ h a 8 a a 8 log sinh(x) x x cosh x x cosh x 9 x sinh x h 78x sinh x 8 8 x 5 cosh x x cosh x 88 cosh x x cosh x 88 x sinh x x sinh x x sinh x x sinh x ^ h a h 5 x sinh x 5 x x 8 cosh x 9 x cosh x 5 cosh x 8 x cosh x 8 x sinh x x sinh x 5 x sinh x 5x sinh x ^ h a h a 95x sinh x 75 7 x x 9x 8 cosh x x cosh x 777 x cosh x x cosh x 5 cosh x 595 x cosh x x cosh x 75 cosh x x cosh x 9x cosh x 88 x sinh x x sinh x x 5 sinh x x sinh x x sinh x 57 x sinh x x sinh x (8) To obtain the diagrams involving g we replace, as explained above, by and expand
8 8 in powers of g h: ; 7 8 ; ; : Note that the dot being associated with the vertex g is equal to half a mass insertion. The numbers underneath the diagrams are their multiplicities; they act as factors. The expansion of the trace log follows a dierent pattern since the one-loop diagram requires a reexpansion of the logarithm pictured by it: 8 : As an example, consider the Feynman diagram g h h a: It is obtained from the second-order Taylor expansion term of the trace log as follows: The dierentiation yields g h h h (@ ) V x i ( ) : a h 8x sinh x corresponding to the Feynman integral x cosh x x sinh x ; h a G ( ) d d :
9 9 Similarly we nd the Feynman integrals ^ h a a h x sinh x x cosh x x cosh x xcosh x (9) 8 sinh x x sinh x sinh x a 8 ^ h h a 8 88x sinh x 5 x cosh x x cosh x 5 x cosh x () sinh x 5 x sinh x sinh x x sinh x ^ h a 5 h a n 9x sinh x 7 x cosh x 5 8 x cosh x x5 cosh x 8 x cosh x x cosh x x cosh 5x 5x cosh 5x 78 sinh x 5 x sinh x 7x sinh x 8 sinh x x sinh x x sinh x 78 sinh 5x x sinh 5x obtain the graphical expansion for W (x ) (the multiplicities of the diagrams have been canceled by the n!-denominators of the couplings g n hn!; now the vertices represent only g n h): W (x )V(x ) " 8 8 ()
10 ! 8! 8!# : corresponding to the analytic expression (in the same order) W V (x )V x g a g 8 a!h!h g a g g a a g g a g g a8 g g a8 a g g g g a g a8 g g g g a (a ) g 8 a a g a a (a ) a g g a g g a a (a a ) g a a g 8 a g 8 a a () The best (x ) is found numerically by searching for the roots of the rst derivate of W with respect to. There are many solutions and we must pick the right one, which we take to be the one closest to the unique solution found at the lowest order (where the Jensen-Peierls inequality ensured its existence). Fig. shows the approximations W ;; over the variational parameter for g and atx. The new extremum lies indeed near the old one. Note that W has no extremum as remarked before, but the curve has a very small slope and the point of smallest -dependence is easily identied. In fact, the -dependence decreases rapidly with increasing order reecting the fact that the exact W is completely independent of the choice of. The corresponding results for the free energy F ln Z are listed in Tab. and compared with the precise numbers F ex of Ref. [7]. To third order, the new approximation gives energies which are better than the lowest order results by a factor of to 5. They dier from the exact results only in the forth digit.
11 W Ω Figure : Eective potential V e versus for g and atx. The curves,, show the approximations W ;; respectively. While W and W have an extremum at ; 7, the second-order approximation W has only extrema in the complex plane.
12 g F F F ex Table : Free energy of the anharmonic oscillators with the potential V (x) x gx for dierent g and kt.
13 W 8 β Figure : The approximations W ;; for the eective classical potential V e versus for g and x with optimized. The curves,, shows the approximations W ;; respectively. The dotted line is the asymptote of W. In the high-temperature limit, all W N tend to the classical results (which, in turn, becomes exact). It is therefore not astonishing that for small, the approximations W and W are practically indistinguishable. Fig. shows the dependence of W ;; on. For increasing, the dierence between the rst approximation and the other curves increases. The worst possible case is T, where the diagrams become most simple and have been given before []. Conclusion We have presented a systematic improvement of the Feynman-Kleinert approximation up to third-order. For the anharmonic oscillator the free energy was obtained with an error less than. % for all coupling constants g and all temperatures. In comparison with the previously available lowest-order approximation, the accuracy is increased by about a factor. The virtue of the improved variational approach lies in the ability to yield very precise results for all coupling constants and temperatures. This is in contrast to other
14 g g Figure : The eective dimensionless coupling constant g h gh (g) of the new perturbation series versus gh in the rst and third approximation W and W, respectivly (axes are labeled setting h ). methods which are applicable only in selected limiting temperature or coupling constant regimes. The improvement with respect to the ordinary perturbation expansion is due to the fact that the new perturbative expansion has an eective coupling constant g h gh (g), which remains small even for g!(see Figure ). Certainly, the accuracy can be increased by calculating higher-order terms. The complexity, however, increases rapidly with increasing orders. Thus higher-order calculations will require much more work. In this note, we have presented only the free energy of the anharmonic oscillator. Other quantities like particle distributions can be obtained quite similarly. This will be done in future work. References [] R.P. Feynman and H. Kleinert, Phys. Rev. A,58 (98). see also
15 5 H. Kleinert, Phys. Lett. B 8, (98); A 8, 95, 7 (98). W. Janke and H. Kleinert, Phys. Lett A 8, 7 (98); Chem. Phys. Lett. 7, (987). W. Janke and B.K. Chang, Phys. Lett. B 9, (988). [] R.P. Feynman, Statistical Mechanics, Frontiers in Physics, Addison Wesley, Redwood City, California, Eleventh Printing (988). [] R. Giachetti and V. Tognetti, Phys. Rev. Lett. 55, 9 (985); Intern. J. Magn. Mater. 5-57, 8 (98). R. Giachetti, V. Tognetti and R. Vaia, Phys. Rev. B, 77 (98); [] R. Giachetti, V. Tognetti and R. Vaia, Phys. Rev. A 7, 5 (988);A 8, 5,8 (988). A. Cuccoli, V. Tognetti and R. Vaia Phys. Rev. B, 9588 (99); see also review R. Giachetti, V. Tognetti, A. Cuccoli and R. Vaia, lecture presented at XXVI Karpacz School of Theoretical Physics (Karpacz, Poland, 99) [5] A. Cuccoli, A. Maradudin, A. R. Mc Gurn, V. Tognetti, R. Vaia, Phys. Rev. B, 889 (99), S. Liu, G.K. Horton and E.R. Cowly, Phys. Lett. A 5, 79 (99). A. Cuccoli, A. Macci, M. Neumann, V. Tognetti and R. Vaia, Phys. Rev. B 5(5), 88 (99). [] H. Kleinert, Phys Lett. A 7(-5), (99) [7] S. Srivastava and Vishvarmittar, Phys. Rev. A (), 8 (99). [8] H. Kleinert, Path Integrals in Quantum Mechanics, Statistics and Polymer Physics, World Scientic, Singapore (99). A considerably extended discussion can be found in the second edition of the book which has appeared rst in German with B.I.- Wissenschaftsverlag, Mannheim, 99.
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