Ultrafast Spectroscopy of Semiconductors and Semiconductor Nanostructures

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1 Springer Series in Solid-State Sciences 115 Ultrafast Spectroscopy of Semiconductors and Semiconductor Nanostructures Bearbeitet von Jagdeep Shah erweitert Buch. xvi, 522 S. Hardcover ISBN Format (B x L): 15,5 x 23,5 cm Gewicht: 2070 g Weitere Fachgebiete > Technik > Elektronik > Halb- und Supraleitertechnologie schnell und portofrei erhältlich bei Die Online-Fachbuchhandlung beck-shop.de ist spezialisiert auf Fachbücher, insbesondere Recht, Steuern und Wirtschaft. Im Sortiment finden Sie alle Medien (Bücher, Zeitschriften, CDs, ebooks, etc.) aller Verlage. Ergänzt wird das Programm durch Services wie Neuerscheinungsdienst oder Zusammenstellungen von Büchern zu Sonderpreisen. Der Shop führt mehr als 8 Millionen Produkte.

2 Contents 1. Introduction Semiconductors: Basic Concepts Band Structure Excitons Phonons in Semiconductors Scattering Processes in Semiconductors Carrier Relaxation: Four Regimes Carrier Transport Ultrafast Lasers Ultrafast Spectroscopy Techniques Pump-Probe Spectroscopy FWM Spectroscopy Luminescence Spectroscopy Interferometric Techniques Terahertz Spectroscopy Interpretation of Results FWM Spectroscopy Pump-Probe Spectroscopy Raman Spectroscopy Luminescence Spectroscopy Calculation of the Dynamics Current Trends Summary Coherent Spectroscopy of Semiconductors Basic Concepts An Ensemble of Independent Two-Level Systems Semiconductor Bloch Equations Coherence Effects in Other Optical Experiments Concluding Remarks Dephasing of Excitons Exciton-Exciton and Exciton-Free-Carrier Collisions in Quantum Wells Exciton-Phonon Interactions Localized Excitons AC Stark Effect Transient Spectral Oscillations... 60

3 XII Contents 2.5 Exciton Resonance in FWM Quantum Beats of Excitons Beats from Discrete Excitonic Islands HH-LH Beats Quantum Beats of Magneto-Excitons Distinction Between Quantum and Polarization Beats Propagation Quantum Beats Concluding Remarks Interaction-Induced Effects: Beyond the Independent-Level Approximation Exciton-Exciton Interaction Effects Biexcitonic Effects Coherent Oscillations of an Electronic Wavepacket Bloch Oscillations in a Semiconductor Superlattice Semiclassical Picture Tight-Binding Picture Qualitative Quantum-Mechanical Picture Observation of Bloch Oscillations in Semiconductor Superlattices Influence of Excitons Concluding Remarks Coherent Spectroscopy of Free Electron-Hole Pairs Transient Oscillations Free-Carrier Dephasing in Bulk GaAs Free-Carrier Dephasing in Intrinsic Quantum Wells Free-Carrier Dephasing in Modulation-Doped Quantum Wells Time-Resolved FWM from Modulation-Doped Quantum Wells Coherent Phonons Terahertz Spectroscopy of Semiconductor Nanostructures Coherent Oscillations in a-dqws HH-LH Oscillations Bloch Oscillations Coherent Control of Charge Oscillations Summary Conclusions Initial Relaxation of Photoexcited Carriers Non-thermal Distributions in GaAs Pump-Probe Spectroscopy Luminescence Spectroscopy Intervalley Scattering in GaAs Initial Carrier Relaxation in Quantum Wells Spectral Hole-Burning in GaAs Quantum Wells

4 Contents XIII Non-thermal Holes in n-modulation-doped Quantum Wells Intersubband Scattering in Quantum Wells Summary and Conclusions Cooling of Hot Carriers Simple Model of Carrier Energy-Loss Rates and Cooling Curves Cooling Curves: Early Measurements and Analysis Other Factors Influencing the Cooling Curves Pauli Exclusion Principle and Fermi-Dirac Statistics Hot Phonons Screening and Many-Body Aspects Further Experimental Investigations of Energy-Loss Rates Direct Measurement of the Energy-Loss Rates Bulk vs Quasi-2D Semiconductors Conclusions Phonon Dynamics Phonon Dynamics in Bulk Semiconductors Phonon Generation in Bulk Semiconductors Phonon Detection by Raman Scattering Steady-State Results in GaAs Phonon Dynamics in GaAs Coherent Generation and Detection of Phonons Monte-Carlo Simulation of Phonon Dynamics in GaAs Phonon Dynamics in Quantum Wells Phonons in Quantum Wells Phonon Generation in Quantum Wells Phonon Detection by Raman Scattering Monte-Carlo Simulation of Phonon Dynamics in GaAs Quantum Wells Hot-Phonon Dynamics in GaAs Quantum Wells Determination of Phonon Occupation Number Experimental Determination of the Hot-Phonon Occupation Number and Dynamics Conclusions Exciton Dynamics Basic Concepts Exciton States Exciton-Polaritons Exciton Fine Structure Dynamical Processes of Excitons

5 XIV Contents 6.2 Experimental Results: Non-resonant Excitation Exciton-Formation Dynamics in GaAs Quantum Wells Exciton Relaxation Dynamics in Cu 2 O Spin Relaxation Dynamics in GaAs Quantum Wells Recombination Dynamics of Thermalized Excitons in GaAs Quantum Wells Experimental Results: Resonant Excitation Pump-and-Probe Studies Picosecond Luminescence Studies Femtosecond Luminescence Studies Conclusions Carrier Tunneling in Semiconductor Nanostructures Basic Concepts: Optical Markers Basic Concepts: Double-Barrier Structures Basic Concepts: Asymmetric Double-Quantum-Well Structures Optical Markers in a-dqws Non-resonant Tunneling Resonant Tunneling Tunneling in Double-Barrier Structures Dependence on the Barrier Thickness Dependence on Electric Field Summary Non-resonant Tunneling in Asymmetric Double-Quantum-Well Structures Dependence on Barrier Thickness Resonant Phonon-Assisted Tunneling Resonant Tunneling in Asymmetric Double-Quantum-Well Structures Resonant Tunneling of Electrons: Initial Studies Resonant Tunneling of Holes: Initial Studies Resonant Tunneling of Electrons and Holes: Further Studies Unified Picture of Tunneling and Relaxation Summary Conclusions Carrier Transport in Semiconductor Nanostructures Basic Concepts Some Examples Perpendicular Transport in Graded-Gap Superlattices Carrier Sweep-Out in Multiple Quantum Wells Hybrid Technique All-Optical Studies of Carrier Sweep-Out

6 Contents XV 8.4 Carrier Capture in Quantum Wells Theoretical Predictions Experimental Studies Implications for Lasers Summary Conclusions Recent Developments Nanostructures, Lasers and Techniques Semiconductor Nanostructures Ultrafast Lasers Measurement Techniques Coherent Spectroscopy Quantum Kinetics in Semiconductors Beyond the Semiconductor Bloch Equations Coherent Control in Semiconductors Phase Sensitive Measurements Exciton-Continuum Interaction Bloch Oscillations Coherent Phonons Plasmon-Phonon Oscillations HH-LH Resonance in the Continuum Biexcitons Coherent and Nonlinear Phenomena in Semiconductor Microcavities Coherence in Multiple Quantum-Well Structures and Bragg/Anti-Bragg Structures Coherent Properties of Quantum Wires and Dots Ultrafast Emission Dynamics Resonant Secondary Emission from Quantum Wells: Intensity Resonant Secondary Emission from Quantum Wells: Investigation by Phase-Locked Pulses Resonant Secondary Emission from Quantum Wells: Direct Measurement of Amplitude and Phase Microcavities The Incoherent Regime: Dynamics and High-Intensity Effects Carrier Dynamics Exciton Dynamics Quantum Wires: Capture and Relaxation Dynamics Quantum Wires: High-Density Effects Quantum Dots: Relaxation Dynamics Carrier-Transport Dynamics Epilogue

7 XVI Contents References Subject Index

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