2012 NCTS Workshop on Dynamical Systems
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1 Barbara Gentz gentz 2012 NCTS Workshop on Dynamical Systems National Center for Theoretical Sciences, National Tsing-Hua University Hsinchu, Taiwan, May 2012 The Effect of Gaussian White Noise on Dynamical Systems: Diffusion Exit from a Domain Barbara Gentz University of Bielefeld, Germany
2 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Introduction: A Brownian particle in a potential
3 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Small random perturbations Gradient dynamics (ODE) ẋ det t = V (x det t ) Random perturbation by Gaussian white noise (SDE) dxt ε (ω) = V (xt ε (ω)) dt + 2ε db t (ω) Equivalent notation ẋt ε (ω) = V (xt ε (ω)) + 2εξ t (ω) x z y with V : R d R : confining potential, growth condition at infinity {B t (ω)} t 0 : d-dimensional Brownian motion {ξ t (ω)} t 0 : Gaussian white noise, ξ t = 0, ξ t ξ s = δ(t s)
4 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Fokker Planck equation Stochastic differential equation (SDE) of gradient type dx ε t (ω) = V (x ε t (ω)) dt + 2ε db t (ω) Kolmogorov s forward or Fokker Planck equation Solution {x ε t (ω)} t is a (time-homogenous) Markov process Densities (x, t) p(x, t y, s) of the transition probabilities satisfy t p = L εp = [ V (x)p ] + ε p If {x ε t (ω)} t admits an invariant density p 0, then L ε p 0 = 0 Easy to verify (for gradient systems) p 0 (x) = 1 e V (x)/ε with Z ε = e V (x)/ε dx Z ε R d
5 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Equilibrium distribution Invariant measure or equilibrium distribution µ ε (dx) = 1 Z ε e V (x)/ε dx System is reversible w.r.t. µ ε (detailed balance) p(y, t x, 0) e V (x)/ε V (y)/ε = p(x, t y, 0) e For small ε, invariant measure µ ε concentrates in the minima of V ε = 1/4 ε = 1/10 ε = 1/
6 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Timescales Let V double-well potential as before, start in x0 ε = x = left-hand well How long does it take until xt ε is well described by its invariant distribution? For ε small, paths will stay in the left-hand well for a long time xt ε first approaches a Gaussian distribution, centered in x, T relax = 1 V (x ) = 1 curvature at the bottom of the well (d=1) With overwhelming probability, paths will remain inside left-hand well, for all times significantly shorter than Kramers time T Kramers = e H/ε, where H = V (z ) V (x ) = barrier height Only for t T Kramers, the distribution of x ε t approaches p 0 The dynamics is thus very different on the different timescales
7 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Diffusion exit from a domain
8 The more general picture: Diffusion exit from a domain dx ε t = b(x ε t ) dt + 2εg(x ε t ) dw t, x 0 R d General case: b not necessarily derived from a potential Consider bounded domain D x 0 (with smooth boundary) First-exit time: τ = τd ε = inf{t > 0: x t ε D} First-exit location: xτ ε D Questions Does xt ε leave D? If so: When and where? Expected time of first exit? Concentration of first-exit time and location? Distribution of τ and xτ ε? Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30
9 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 First case: Deterministic dynamics leaves D If x t leaves D in finite time, so will x ε t. Show that deviation x ε t x t is small: Assume b Lipschitz continuous and g = Id By Gronwall s lemma x ε t x t L t 0 x ε s x s ds + 2ε W t sup xs ε x s 2ε sup W s e Lt 0 s t 0 s t d = 1: Use André s reflection principle { } { } P sup W s r 2 P sup W s r 4 P { W t r } 2 e r 2 /2t 0 s t 0 s t d > 1: Reduce to d = 1 using independence General case: Use large-deviation principle
10 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Second case: Deterministic dynamics does not leave D Assume D positively invariant under deterministic flow: Study noise-induced exit dxt ε = b(xt ε ) dt + 2εg(xt ε ) dw t, x 0 R d b, g Lipschitz continuous, bounded-growth condition a(x) = g(x)g(x) T 1 M Id (uniform ellipticity) Infinitesimal generator A ε of diffusion x ε t A ε v(t, x) = ε d i,j=1 a ij (x) 2 x i x j v(t, x) + b(x), v(t, x) Compare to Fokker Planck operator: L ε is the adjoint operator of A ε Approaches to the exit problem Mean first-exit times and locations via PDEs Exponential asymptotics via Wentzell Freidlin theory
11 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Diffusion exit from a domain: Relation to PDEs Theorem Poisson problem: { E x {τd ε } is the unique solution of A ε u = 1 u = 0 Dirichlet problem: { E x {f (xτ ε )} is the unique solution of A ε w = 0 D ε w = f (for f : D R continuous) in D on D in D on D Remarks Expected first-exit times and distribution of first-exit locations obtained exactly from PDEs
12 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Diffusion exit from a domain: Relation to PDEs Theorem Poisson problem: { E x {τd ε } is the unique solution of A ε u = 1 u = 0 Dirichlet problem: { E x {f (xτ ε )} is the unique solution of A ε w = 0 D ε w = f (for f : D R continuous) in D on D in D on D Remarks Expected first-exit times and distribution of first-exit locations obtained exactly from PDEs In principle...
13 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Diffusion exit from a domain: Relation to PDEs Theorem Poisson problem: { E x {τd ε } is the unique solution of A ε u = 1 u = 0 Dirichlet problem: { E x {f (xτ ε )} is the unique solution of A ε w = 0 D ε w = f (for f : D R continuous) in D on D in D on D Remarks Expected first-exit times and distribution of first-exit locations obtained exactly from PDEs In principle... Smoothness assumption for D can be relaxed to exterior-ball condition
14 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 An example in d = 1 Motion of a Brownian particle in a quadratic single-well potential dx ε t = b(x ε t ) dt + 2ε dw t where b(x) = V (x), V (x) = ax 2 /2 with a > 0 Drift pushes particle towards bottom Probability of x ε t leaving D = (α 1, α 2 ) 0 through α 1? Solve the (one-dimensional) Dirichlet problem { A ε w = 0 in D with f (x) = w = f on D { 1 for x = α 1 0 for x = α 2 { } α2 P x x ε τ ε D = α 1 = Ex f (xτ ε ) = w(x) = D ε x e V (y)/ε dy / α2 α 1 e V (y)/ε dy
15 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 An example in d = 1: Small noise limit? { } α2 P x x ε τ ε D = α 1 = x e V (y)/ε dy / α2 α 1 e V (y)/ε dy What happens in the small-noise limit? lim ε 0 P x{x ε τ ε D = α 1} = 1 if V (α 1) < V (α 2) lim P x{xτ ε = α 1} = 0 ε 0 D ε if V (α 2) < V (α 1) /( ) lim P x{xτ ε = α 1 1 1} = ε 0 D ε V (α 1 ) V (α 1 ) + 1 V if V (α 1) = V (α 2) (α 2 )
16 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Large deviations: Wentzell Freidlin theory
17 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Exponential asymptotics via large deviations Probability of observing sample paths being close to a given function ϕ : [0, T ] R d behaves like exp{ 2I (ϕ)/ε} Large-deviation rate function I (ϕ) = I [0,T ] (ϕ) = { 1 2 T 0 ϕ s b(ϕ s ) 2 ds for ϕ H 1 + otherwise Large deviation principle reduces est. of probabilities to variational principle: For any set Γ of paths on [0, T ] inf Γ ε 0 I lim inf 2ε log P{(x ε t ) t Γ} lim sup ε 0 2ε log P{(xt ε ) t Γ} inf I Γ Assume domain D has unique asymptotically stable equilibrium point x Quasipotential with respect to x = cost to reach z against the flow V (x, z) := inf t>0 inf{i [0,t](ϕ): ϕ C([0, t], D), ϕ 0 = x, ϕ t = z}
18 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Wentzell Freidlin theory Theorem [Wentzell & Freidlin, , 1984] For arbitrary initial condition in D Mean first-exit time: EτD ε e V /2ε as ε 0 Concentration of first-exit times { P e (V δ)/2ε τd ε e (V +δ)/2ε} 1 as ε 0 (for arbitrary δ > 0) Concentration of exit locations near minima of quasipotential Gradient case (reversible diffusion) b = V, g = Id Quasipotential V (x, z) = 2[V (z) V (x )] Cost for leaving potential well is V = inf z D V (x, z) = 2[V (z ) V (x )] = 2H Attained for paths going against the flow: ϕ t = + V (ϕ t ) H
19 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Remarks Arrhenius Law [van t Hoff 1885, Arrhenius 1889] follows as a corollary E x τ + const e [V (z ) V (x )]/ε where τ + = first-hitting time of small ball B δ (x+) around other minimum x+ τ + = τx ε (ω) = inf{t 0: x ε + t (ω) B δ (x+)} Exponential asymptotics depends only on barrier height LDP also leads information on optimal transition paths Only 1-saddles are relevant for transitions between wells Multiwell case described by hierarchy of cycles Nongradient case: Work with variational problem Prefactor cannot be obtained by this approach
20 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Subexponential asymptotics
21 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Refined results in the gradient case: Kramers law First-hitting time of a small ball B δ (x +) around minimum x + τ + = τ ε x + (ω) = inf{t 0: x ε t (ω) B δ (x +)}
22 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Refined results in the gradient case: Kramers law First-hitting time of a small ball B δ (x +) around minimum x + τ + = τ ε x + (ω) = inf{t 0: x ε t (ω) B δ (x +)} Arrhenius Law [van t Hoff 1885, Arrhenius 1889] see previous slide E x τ + const e [V (z ) V (x )]/ε
23 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Refined results in the gradient case: Kramers law First-hitting time of a small ball B δ (x +) around minimum x + τ + = τ ε x + (ω) = inf{t 0: x ε t (ω) B δ (x +)} Arrhenius Law [van t Hoff 1885, Arrhenius 1889] see previous slide E x τ + const e [V (z ) V (x )]/ε Eyring Kramers Law [Eyring 35, Kramers 40] 2π d = 1: E x τ + V (x ) V (z ) e[v (z ) V (x )]/ε
24 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Refined results in the gradient case: Kramers law First-hitting time of a small ball B δ (x +) around minimum x + τ + = τ ε x + (ω) = inf{t 0: x ε t (ω) B δ (x +)} Arrhenius Law [van t Hoff 1885, Arrhenius 1889] see previous slide E x τ + const e [V (z ) V (x )]/ε Eyring Kramers Law [Eyring 35, Kramers 40] 2π d = 1: E x τ + V (x ) V (z ) e[v (z ) V (x )]/ε d 2: E x τ + 2π det 2 V (z ) (z ) V (x λ 1 (z ) det 2 V (x ) e[v )]/ε where λ 1(z ) is the unique negative eigenvalue of 2 V at saddle z
25 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Proving Kramers law (multiwell potentials) Low-lying spectrum of generator of the diffusion (analytic approach) [Helffer & Sjöstrand 85, Miclo 95, Mathieu 95, Kolokoltsov 96,... ] Potential theoretic approach [Bovier, Eckhoff, Gayrard & Klein 04] E x τ + = 2π det 2 V (z ) (z ) V (x λ 1 (z ) det 2 V (x ) e[v )]/ε [1 + O ( (ε log ε ) 1/2) ] Full asymptotic expansion of prefactor [Helffer, Klein & Nier 04] Asymptotic distribution of τ + [Day 83, Bovier, Gayrard & Klein 05] lim P x {τ ε 0 + > t E x τ + } = e t
26 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Generalizations: Non-quadratic saddles What happens if det 2 V (z ) = 0? det 2 V (z ) = 0 At least one vanishing eigenvalue at saddle z Saddle has at least one non-quadratic direction Kramers Law not applicable Why do we care about this non-generic situation? Parameter-dependent systems may undergo bifurcations Quartic unstable direction Quartic stable direction
27 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Example: Two harmonically coupled particles V γ (x 1, x 2 ) = U(x 1 ) + U(x 2 ) + γ 2 (x 1 x 2 ) 2 Change of variable: Rotation by π/4 yields U(x) = x4 V γ (y 1, y 2 ) = 1 2 y γ y y 4 2 8( 1 + 6y1 2 y2 2 + y2 4 ) Note: det 2 Vγ (0, 0) = 1 2γ Pitchfork bifurcation at γ = 1/2 x2 4 2 γ > > γ > > γ > 0
28 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Transition times for non-quadratic saddles Assume x is a quadratic local minimum of V (non-quadratic minima can be dealt with) Assume x + is another local minimum of V Assume z = 0 is the relevant saddle for passage from x to x + Normal form near saddle V (y) = u 1 (y 1 ) + u 2 (y 2 ) Assume growth conditions on u 1, u 2 Theorem [Berglund & G, 2010)] d j=3 λ j y 2 j +... E x τ + = (2πε)d/2 e V (x )/ε det 2 V (x ) / [ 1 + O((ε log ε ) α ) ] ε e u2(y2)/ε dy 2 e u1(y1)/ε dy 1 d j=3 2πε λ j where α > 0 depends on the growth conditions and is explicitly known
29 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Corollary: Pitchfork bifurcation Pitchfork bifurcation: V (y) = 1 2 λ 1 y λ 2y C 4 y For λ 2 > 0 (possibly small wrt. ε): (λ 2 + 2εC 4 )λ 3... λ d E x τ + = 2π λ 1 det 2 V (x ) where α(1 + α) ( α Ψ + (α) = e α2 /16 2 ) K 1/4 8π 16 lim Ψ +(α) = 1 α d j=3 e [V (z ) V (x )]/ε Ψ + (λ 2 / [1 + R(ε)] 2εC 4 ) λ j y 2 j K 1/4 = modified Bessel fct. of 2nd kind For λ 2 < 0: Similar, involving I ±1/4 λ 2 prefactor 2 1 ε = 0.5, ε = 0.1, ε = 0.01
30 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Cycling
31 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 New phenomena in non-gradient case: Cycling Simplest situation of interest: Nontrivial invariant set which is a single periodic orbit Assume from now on: d = 2, D = unstable periodic orbit Eτ D e V /2ε still holds Quasipotential V (Π, z) V is constant on D: Exit equally likely anywhere on D (on exp. scale) Phenomenon of cycling [Day 92]: Distribution of x τd on D does not converge as ε 0 Density is translated along D proportionally to log ε. In stationary regime: (obtained by reinjecting particle) Rate of escape d dt P{ x t D } has log ε -periodic prefactor [Maier & Stein 96]
32 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Universality in cycling Theorem ([Berglund & G 04, 05, work in progress) There exists an explicit parametrization of D s.t. the exit time density is given by p(t, t 0 ) = f trans(t, t 0 ) N Q λt (y) is a universal λt -periodic function Q λt ( θ(t) 1 2 log ε ) θ (t) λt K (ε) e (θ(t) θ(t0)) / λt K(ε) θ(t) is a natural parametrisation of the boundary: θ (t) > 0 is explicitely known model-dependent, T -periodic fct.; θ(t + T ) = θ(t) + λt T K (ε) is the analogue of Kramers time: T K (ε) = C ε e V /2ε f trans grows from 0 to 1 in time t t 0 of order log ε
33 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 y Q λt (λty)/2λt The universal profile Profile determines concentration of first-passage times within a period Shape of peaks: Gumbel distribution P(z) = 1 2 e 2z exp { 1 2 e 2z} The larger λt, the more pronounced the peaks s For smaller values of λt, the peaks overlap more
34 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Density of the first-passage time for V = 0.5, λ = 1 (a) (b) ε = 0.4, T = 2 ε = 0.4, T = 20 (c) (d) ε = 0.5, T = 2 ε = 0.5, T = 5
35 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 References Large deviations and Wentzell Freidlin theory (textbooks) M. I. Freidlin, and A. D. Wentzell, Random Perturbations of Dynamical Systems, Springer (1998) A. Dembo and O. Zeitouni, Large deviations techniques and applications, Springer (1998) Kramers law H. Eyring, The activated complex in chemical reactions, Journal of Chemical Physics 3 (1935), pp H. A. Kramers, Brownian motion in a field of force and the diffusion model of chemical reactions, Physica 7 (1940), pp A. Bovier, M. Eckhoff, V. Gayrard, and M. Klein, Metastability in reversible diffusion processes. I. Sharp asymptotics for capacities and exit times, J. Eur. Math. Soc. 6 (2004), pp A. Bovier, V. Gayrard, and M. Klein, Metastability in reversible diffusion processes. II. Precise asymptotics for small eigenvalues, J. Eur. Math. Soc. 7 (2005), pp
36 Diffusion Exit from a Domain Barbara Gentz NCTS, 16 May / 30 Kramers law (cont.) References (cont.) B. Helffer, M. Klein, and F. Nier, Quantitative analysis of metastability in reversible diffusion processes via a Witten complex approach, Mat. Contemp. 26 (2004), pp N. Berglund and B. Gentz, The Eyring Kramers law for potentials with nonquadratic saddles, Markov Processes Relat. Fields 16 (2010), pp Cycling M. V. Day, Conditional exits for small noise diffusions with characteristic boundary, Ann. Probab. 20 (1992), pp N. Berglund and B. Gentz, On the noise-induced passage through an unstable periodic orbit I: Two-level model, J. Statist. Phys. 114 (2004), pp N. Berglund and B. Gentz, Universality of first-passage- and residence-time distributions in non-adiabatic stochastic resonance, Europhys. Lett. 70 (2005), pp. 1 7
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