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1 Equation 23 of Radiative Transfer rd Meeting of the Atomic and Molecular Data Centres Network Aspects and prospects of KAERI atomic data center Duck-Hee Kwon and Kil-Byoung Chai Nuclear Data Center Korea Atomic Energy Research Institute 4-6 Sept. 2017, IAEA Headquarters, Vienna, Austria 1
2 Outline 1. Research Activities ( ) 2. KAERI Atomic Database Updates 3. Summary and Outlook 2
3 Research Activities 1. State-of-the-art calculations for the electron-impact ionization and recombination, and photoionization data which are essential in modeling for laboratory and astrophysical plasmas Sun Star SNR Galaxy AGN ITER wall design 2. Spectroscopic measurement in plasma devices and collisional radiative modeling for analysis on the measured spectra 3
4 Research Activities 1. Dielectronic recombination (DR) Highly charged W 44+ ~W 46+ Lowly charged W 5+ ~W Photon emissivity coefficient (PEC) W 5+ ~W Spectroscopic measurement & collisional-radiative (CR) modeling Ar 4
5 Spectroscopic Modeling ij n Emissivity ε ij for line transition i j Z r tn r, t PEC ( T, n ), e ij e e Photon Emissivity Coefficient Electron density ij e 0i Charge Z ion density Aik from transport Collisional excitation ki modeling (CE) rate Radiative transition Simple coronal Model for state population density probability CE from 0 to i i Radiative transitions any k below i j 0 Ground state for any charge state of Z ions PEC n T e e T X A Atomic Data 3 8 cm Z 1 3 1/ Z 1 ev exp T e ij with hydrogenic approximation 2 5
6 Transport Modeling 6
7 Photon Emissivity Coefficient (PEC) 7
8 Photon Emissivity Coefficient (PEC) Full J-J coupled level resolved scheme For eg. W 25+ Total levels FAC data vs. ADAS data Configuration average scheme 1+28 states 8
9 Impurity injection experiment in KSTAR On the courtesy of In Woo Song in KAIST and KSTAR team 9
10 Measured spectra in KSTAR Lines of sight, Thomson T e & n e profiles LoS for CAES on KSTAR Channel 1 - Simple 2-D configuration (only the pinhole position and the detector position are considered) - 10 lines of sight (corresponding to 10 channels during #16958) - Sample points are generated on the LoS with equal distance apart Channel 10 - Thomson data at 4.15 s (100 ms averaged) are used - Fitted by using tanh function On the courtesy of In Woo Song in KAIST and KSTAR team 10
11 Measured vs. modeled spectra 11
12 Transport free modeled spectra Fractional abundance from ADAS ca09_w.dat (ionization) and acd50_w.dat (recombination). PEC from FAC calculations 12
13 Ionization data for W W + W 17+ W 25+ FAC level resolved ADAS CADW D.-H. Kwon, Y. S. Cho, and Y. O. Lee, IJMS 356, 7 (2013) D.-H. Zhang and D.-H. Kwon, JPB 47, (2014) A. Kyniene, S. Pakalka, S. Masys, and V. Jonauskas, JPB 49, (2016) ADAS ionization data by CADW ab-initio calculation for W ions is reliable within 30-50% accuracy being compared with other ab-initio calculations and the data set is available for all ionization stages. 13
14 Recombination data for W 14
15 DR data for W IAEA&KAERI Joint CM on DR for W (Sept. 2015) ab-initio calculation t ADAS recombination data based on a simple Burgess formula for W ions quite differ from other ab-initio calculations and the data is not available for many ionization stages. j i B (T) g j A a ji t 1 2g A i 2 4a 0Ry kbt E ij Bj exp kbt A B r r jt tj t j a r A k jk A f jf Burgess formula (T) i j f ji 14 n E A(y) exp T e n Z 3/ 2 B(q)D(q,T) 3/ 2 T 15
16 IAEA-KAERI joint CM on DR for W At KAERI (Sept. 2015) 16
17 New recommended DR data for W ions ADNDT in press, available online 5 June
18 New recommended DR data for W ions ADNDT in press, available online 5 June
19 DR data for W ions (Our calculations) D.-H. Kwon and W. Lee, JQSRT 170, 182 (2016); ibid., 179, 98 (2016) D.-H. Kwon and W. Lee, JQSRT, 179, 98 (2016) 19
20 DR data for W ions (Our calculations) 20
21 DR data for W ions (Our calculations) Threshold energy of resonance for DR of W q+ (q = 5-11) Ion Ground configuration FAC (ev) NIST (ev) % Error W 4+ 4f 14 5s 2 5p 6 5d W 5+ 4f 14 5s 2 5p 6 5d W 6+ 4f 14 5s 2 5p W 7+ 4f 14 5s 2 5p 5 or 4f 13 5s 2 5p W 8+ 4f 14 5s 2 5p W 9+ 4f 14 5s 2 5p W 10+ 4f 14 5s 2 5p W 11+ 4f 14 5s 2 5p 4f 13 5s 2 5p
22 DR data for W ions (Our calculations) 4f 14 5s 2 5p 6 5d Ground level 4f 14 5s 2 5p 6 Ground level 22
23 DR data for W ions (Our calculations) 4f 14 5s 2 5p 5 Ground level 4f 14 5s 2 5p 4 Ground level 23
24 DR data for W ions (Our calculations) 4f 14 5s 2 5p 3 Ground level 4f 14 5s 2 5p 2 Ground level To be submitted. 24
25 DR data for W ions (Our calculations) 4f 13 5s 2 5p 2 Ground level Due to so many resonances of 4f core excitation, DR via 4f transition has been still run. 25
26 Spectroscopy in CCP device Experimental setup Optical Emission Spectroscopy MHz RF CCP Langmuir Probe 26
27 Spectroscopy in CCP device EEPF (m -3 ev -3/2 ) Intensity (a.u.) Langmuir probe diagnostics and OES Langmuir probe data OES data T e = 2.6 ev n i = m mtorr 5 W wavelength (nm) Energy (ev) Spectra measured by Ocean Optics HR4000 (calibrated) EEPF: measured by Impedans Ltd. Langmuir probe 27
28 CR modeling for Ar N N N 0 j1 4 m514 : Ground state : M etastable(j 1, 3) and resonance (j states 1s : Excited 5-2, 3p 5 4s states 2p 3p S1, S 0 P J 3p 5 4p 2S1 L J 2,4) Under construction! 28
29 Equation Experiment Database of Radiative updates Transfer Our website for atomic data and CR modeling 29
30 Equation Experiment Summary of Radiative & Outlook Transfer 1. We have calculated PEC for tungsten (W) ions W q+ (q = 5-48) by parallelizing radiative transition routine of FAC. 2. We had compiled available DR data for W ions and gave the recommended data through IAEA and KAERI joint CM. 3. We have calculated DR for W q+ (q =5-11, 44-46) and will calculate DR for W q+ (q = 30-34). 4. We have installed a CCP device and measured plasma temperature and density for Ar with a Langmoir probe. OES for Ar has also been carried out. CR modeling including detailed collision and radiative processes will be constructed. 5. We have updated the calculated atomic data and implemented the previous CR modeling for He I on our Web DB ( 6. Parallelization for FAC was done for AI routine will be performed. 7. Unitary correction for collisional excitation routine based on distorted wave approximation of FAC will be tried. 30
31 Collaborations Dept. of Physics, Fusion Plasma Transport Research Center ITER Korea VUV Diagnostic Team, KSTAR Team Physical Metrology team: Absolute calibration for spectrometer 31
32 Fractional abundance Nuclear Data Center 32
33 W VUV Spectra measured in KSTAR Main ions emitting nm VUV Transport free spectrum 33
34 New/ADAS Fractional abundance Fractional abundance difference Electron temperature (ev) 34
35 Spectra sensitivity 35
36 Modeling uncertainties Electron temperature & density profiles Transport D & V coefficients Time evolution of impurity Atomic data for ionization and recombination PEC beyond coronal model 36
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