GEISA 2013 Ozone and related atmospheric species contents description and assessment
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1 GEISA 2013 Ozone and related atmospheric species contents description and assessment N. Jacquinet-Husson C. Boutammine, R. Armante, L.Crépeau, A. Chédin, N.A. Scott, C. Crevoisier, V.Capelle, A. Bouhdaoui Laboratoire de Météorologie Dynamique Atmospheric Radiation Analysis Group/ABC(t) Ecole Polytechnique Palaiseau, France GEISA: Gestion et Etude des Informations Spectroscopiques Atmosphériques ; Management and Study of Atmospheric Spectroscopic Information
2 OUTLINE [1] GEISA OVERVIEW [2] OZONE GEISA-2013 UPDATED ARCHIVE [3] SPECTROSPIC PARAMETERS ARCHIVE AND ATMOSPHERIC REMOTE SENSING OPERATIONAL MISSIONS [4] GEISA INTERACTIVE DISTRIBUTION
3 GEISA-11 SYSTEM GENERAL CONTEXT The performance of the new generation of hyperspectral Earth atmosphere sounders, such as AIRS in the USA and IASI in Europe, depends ultimately on the accuracy to which the spectroscopic parameters of the optically active atmospheric gases are known, since they constitute an essential input to the forward radiative transfer models that are used to interpret their observations. GEISA is a computer-accessible Spectroscopic Database designed for accurate forward atmospheric radiative transfer calculations using a lineby-line (atmospheric) layer-by-layer approach. spectral range 10-6 _ 35,877 cm _ 0.28 µm GEISA: Gestion et Etude des Informations Spectroscopiques Atmosphériques ; Management and Study of Atmospheric Spectroscopic Information
4 GEISA-11 SYSTEM GENERAL CONTEXT Spectroscopy is at the root of modern planetology, enabling to determine the physical properties of planets remotely Computer-accessible Spectroscopic Database (CASSINI-HUYGENS 29/01/06 TITAN) GEISA Gestion et Etude des Informations Spectroscopiques Atmosphériques ; Management and Study of Atmospheric Spectroscopic Information MANAGEMENT SOFTWARES For each Sub-database spectral range ,877 cm µm Microphysical and optical properties of atmospheric Aerosols sub-database GEISA 2013 UPDATE UNDERWAY
5 Archived Spectroscopic Line Parameters A Wavenumber (cm -1 ) of the line B Intensity of the line in (cm -1 /(molecule.cm -2 ) C Air broadening pressure halfwidth (HWHM)(*) (cm -1 atm -1 ) D Energy of the lower transition level (cm -1 ) E Transition quantum identifications for the lower and upper state of the transition F Temperature dependence coefficient n of the air broadening HWHM G Identification code for isotope as in GEISA I Identification code for molecule as in GEISA J Internal GEISA code for the data identification K Molecule number in HITRAN L Isotope number (1=most abundant. 2= second etc) in HITRAN M Einstein A-coefficient (s -1 ). N Self broadening pressure HWHM (cm -1 atm -1 ) (for water) O Air pressure shift of the line transition (cm -1 atm -1 ) R Temperature dependence coefficient n of the air pressure shift A Estimated accuracy (cm -1 ) on the line position B Estimated accuracy on the intensity of the line in (cm -1 /(molecule.cm -2 ) C Estimated accuracy on the air collision HWHM (cm -1 atm -1 ) F Estimated accuracy on the temperature dependence coefficient n of the air broadening HWHM O Estimated accuracy on the air pressure shift of the line transition (cm -1 atm -1 ) R Estimated accuracy on the temperature dependence coefficient n of the air pressure shift N Estimated accuracy on the self HWHM T Self pressure shift of the line transition (cm -1 atm -1 ) T Estimated accuracy on the self pressure shift of the line transition (cm -1 atm -1 ) U Temperature dependence coefficient n of the self pressure shift U Estimated accuracy on the temperature dependence coefficient n of the self pressure shift broadened HWHM (cm -1 atm -1 ) S Temperature dependence coefficient n of the self broadening HWHM S Estimated accuracy on the temperature dependence coefficient n of the self- broadening (*) HWHM: line half-width at half-maximum Since GEISA-09 Standardized parameter missing values
6 UPDATED IN 2011
7 A. Barbe, A.Campargue GEISA 2013 OZONE UPDATED ARCHIVE A. Chichery GSMA (Reims) LIPHY (Grenoble) LTS (Tomsk) M.-R. De Backer S. Kassi S.N. Mikhailenko D. Mondelain J.J. Plateaux E. Starikova S.A. Tashkun X. Thomas Vl.G. Tyuterev line list for update provided by Semen Mikhaïlenko
8 References for GEISA 2013 ozone updates A. Barbe, M.-R. De Backer, E. Starikova, S.A. Tashkun, X. Thomas, Vl.G. Tyuterev, FTS high resolution spectra of 16O3 in 3500 and 5500 cm-1 regions. First example of new theoretical modelling for a polyad of strongly coupled states, JQSRT, 113, (2012) A. Barbe, Private communication (2011) A. Barbe, J.J. Plateaux, S.N. Mikhailenko, Vl.G. Tyuterev, Infrared spectrum of ozone in the 4600 and 5300 cm-1 regions: High order accidental resonances through the analysis of the ν1+2 ν 2+3 ν3- ν2, ν 1+2 ν 2+3 ν 3, and 4 ν 1+ ν 3 bands, J. Mol. Spectrosc. 185, (1997) A. Barbe, J.J. Plateaux, Vl.G. Tyuterev, S.N. Mikhailenko, Analysis of high resolution measurements of the 2ν1+3ν3 band of ozone: Coriolis interaction with the ν1+3ν2+2ν3 band, JQSRT 59, (1998) A. Barbe, A. Chichery, The 2ν1+ ν2+3ν3 band of 16O3. Line positions and intensities, J. Mol. Spectrosc. 192, (1998). Vibrational assignment of upper state is now change from (213) to (015). A. Barbe, M.-R. De Backer-Barilly, Vl.G. Tyuterev, A. Campargue, D. Romanini, S. Kassi, CW-cavity ring down spectroscopy of ozone molecule in the cm-1 region, J. Mol. Spectrosc. 242, (2007) A. Barbe, M.-R. De Backer-Barilly, Vl.G. Tyuterev, S. Kassi, A. Campargue, CW-cavity ring down spectroscopy of ozone molecule in the cm-1 region, J. Mol. Spectrosc. 246, (2007) A. Barbe, A. Chichery, Vl.G. Tyuterev, J.J. Plateaux, Analysis of high resolution measurements of the ν1+5ν3 band of ozone: Coriolis interactions with the 6ν3 and 3ν1+ ν2+2ν3 bands, Mol. Phys. 94, (1998) A. Campargue, M.-R. De Backer-Barilly, A. Barbe, Vl.G. Tyuterev, S. Kassi, The near infrared spectrum of ozone by CW-cavity ring down spectroscopy between 5850 and 7000 cm-1: New observations and exhaustive review, PCCP, 10, (2008) A. Campargue, S. Kassi, D. Romanini, A. Barbe, M.-R. De Backer-Barilly, Vl.G. Tyuterev, CW-cavity ring down spectroscopy of ozone molecule in the cm-1 region, J. Mol. Spectrosc. 240, 1-13 (2006)
9 List of transitions for O 3 GEISA-2013 Update Lines in the spectral range cm Vib. Transitions
10 GEISA-2013 O3 line list update details (1) Ranking index for transitions corresponding to normal modes strongly mixed
11 GEISA-2013 O3 line list update details (2) 11,374 lines suppressed and replaced 16,541 lines added
12 GEISA-2013 Ozone contents summary 405,919 lines +16,541 lines since GEISA transitions +36 transitions since GEISA-11
13
14
15 Bin average 5 cm -1
16 Bin average 5 cm -1
17 Bin average 5 cm -1
18 Bin average 5 cm -1
19 Bin average 5 cm -1
20 SPECTROSPIC PARAMETERS ARCHIVE AND ATMOSPHERIC REMOTE SENSING OPERATIONAL MISSIONS
21 Monitoring the evolution of the ozone layer has become a subject of major concern both by the scientific community and the general public from a wider perspective, including the close relationship between the ozone layer changes and the global climate change. There are several instruments on board satellites which have been designed for retrieving ozone and other trace gases in the atmosphere, providing daily images of the global total ozone column (TOC) with uniform spatial coverage. In this context, the Meteorological Operational satellite program MetOp from EUMETSAT has foreseen a series of three polar-orbit platforms. Two of them, MetOp-A and MetOp-B have already been launched. Among the instruments aboard Metop s are the Global Ozone Monitoring Experiment 2 (GOME-2) and the Infrared Atmospheric Sounding Interferometer (IASI). Both sensors retrieve total ozone column and ozone profile information with a high spatial and temporal resolution: GOME-2 instrument obtains the total ozone from the backscattered solar ultraviolet visible (UV VIS; 240 to 790 nm) radiance emerging at the top of the atmosphere, the IASI instrument retrieves it from the thermal infrared radiance (TIR)
22 GEISA-11 : UV-Vis Cross Section contents Molecular species selection and data files provided by J. Orphal 17 molecular species, 158 T/P sets
23 [3] GEISA : Effective Use GEISA : Effective Use 3 Spectral Bands [1] cm µm [2] cm µm [3] cm µm Related to IASI Level 1 Cal/Val CNES LMD GEISA/IASI ( cm -1 ) used as the reference spectroscopic database Validation achieved using 4A/OP line by line Radiative Transfer Model [Scott & Chédin, J.Appl.Met (1981); 4A/LMD 4A/OP co-developed by LMD and Noveltis with the support of CNES (2006)]
24 [3] GEISA : Effective Use GEISA and IASI Atmospheric Sounding GEISA/IASI-11 ( cm -1 ) Extraction of GEISA-11 Reference database for IASI Level 1 Cal/Val activities and operattional CNES LMD Individual spectral lines spectroscopic parameters sub-database 20 molecules (66 isotopic species): 14 molecules (53 isotopic species) selected for operational meteorology) H 2 O, CO 2, O 3, N 2 O,CO, CH 4, O 2, NO, SO 2, NO 2, HNO 3, OCS, C 2 H 2, N 2 6 molecules (13 isotopic species) selected for IASI trace gas retrievals HCN, NH 3, HCOOH, C 2 H4, CH 3 OH, H 2 CO IR absorption cross-sections sub-database (mainly CFC s) 6 molecular species: CFC-11, CFC-12, CFC-14, CCl 4,N 2 O 5, HCFC-22; PAN (peroxyacetyl nitrate) Microphysical and optical properties of Basic Atmospheric aerosol components sub-database Validation achieved using 4A/OP line by line Radiative Transfer Model [Scott & Chédin, J.Appl.Met (1981); 4A/LMD 4A/OP co-developed by LMD and Noveltis with the support of CNES (2006)]
25 Transmittance
26 Ozone lines in IASI Band-1: cm -1
27 Ozone lines in IASI Band-2: cm -1
28 Ozone lines in IASI Band-3: cm -1
29
30
31 GEISA INTERACTIVE DISTRIBUTION
32 GEISA SYSTEM COMPREHENSIVE DISTRIBUTION
33 GEISA : ETHER distribution Home page Descriptions of updates and changes related to GEISA Visualization tools for line by line database content NEW Databases access and description content. GEISA publications list
34 GEISA : ETHER distribution Database page 3 Sub-databases : Line by line Cross sections Aerosols Line by line sub-database : Content description
35 General content GEISA : ETHER distribution Description page Format descriptor References Overall description 3 Sub-databases : Line by line Cross sections Aerosols Line by line sub-database : Content description General content Format description Overall description References
36 GEISA : ETHER distribution Database acess page 3 Sub-databases : Line by line Cross sections Aerosols Line by line sub-database : Content description General content Format description Overall description Data access (FTP) Data access (Interactive) Information Content analysis Histogram analysis Database extract Transition analysis Transition list
37 Interactive tools : Examples Database extract option (choices of parameters) Database extract results The histogram option
38 GEISA : ETHER distribution Graphical Tools Descriptions of updates and changes related to GEISA Visualization tools for line by line database content NEW Databases access and description content. GEISA publications list
39 GEISA : ETHER distribution Graphical Tools Global positions of transitions Database content Databases comparison
40 ACKNOWLEDGMENTS to CNES, CNRS/INSU and EUMETSAT for their Encouragements and Supports THANK YOU FOR YOUR ATTENTION
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