Perovskite solar cells
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1 IMO - IMOMEC INSTITUUT VOOR MATERIAALONDERZOEK Perovskite solar cells dr. ir. Bert Conings bert.conings@uhasselt.be
2 state-of-the-art
3 outline! introduction! planar heterojunction perovskite solar cells! low-temperature processing! intrinsic stability! conclusions
4 introduction Published on Web 04/14/2009 Organometal Halide Perovskites as Visible-Light Sensitizers for Photovoltaic Cells Akihiro Kojima, Kenjiro Teshima, Yasuo Shirai, and Tsutomu Miyasaka*,,, Graduate School of Arts and Sciences, The UniVersity of Tokyo, Komaba, Meguro-ku, Tokyo , Figure 1. (a) Crystal structures of perovskite compounds. (b) SEM image of particles of nanocrystalline CH 3 NH 3 PbBr 3 deposited on the TiO 2 surface. The arrow indicates a particle, and the scale bar shows 10 nm. η = 3.8%
5 introduction Cite this: Nanoscale, 2011, 3, % efficient perovskite quantum-dot-sensitized solar cell Jeong-Hyeok Im, Chang-Ryul Lee, Jin-Wook Lee, Sang-Won Park and Nam-Gyu Park* COMMUNICATION
6 introduction 2 : 591 DOI: /srep00591 Lead Iodide Perovskite Sensitized All-Solid-State Submicron Thin Film Mesoscopic Solar Cell with Efficiency Exceeding 9% Hui-Seon Kim 1, Chang-Ryul Lee 1, Jeong-Hyeok Im 1, Ki-Beom Lee 1, Thomas Moehl 2, Arianna Marchioro 2, Soo-Jin Moon 2, Robin Humphry-Baker 2, Jun-Ho Yum 2, Jacques E. Moser 2, Michael Grätzel 2 & Nam-Gyu Park 1
7 introduction C Ag Efficient Hybrid Solar Cells Based on Meso-Superstructured Organometal Halide Perovskites Michael M. Lee et al. Science 338, 643 (2012); DOI: /science Spiro-OMeTAD Photoactive Layer FTO Perovskite Mesoporous Oxide Compact TiO 2 Glass A IPCE (%) B Current density (ma cm -2 ) η 10.9% Wavelength (nm) Voltage (V)
8 introduction c Counts Efficiency (%) Science 2012, 338, 643 Energy Environ. Sci. 2013, 6, 1739 Energy Environ. Sci. 2013, 6, 3249 Nat. Photonics 2013, 7, 486
9 porous layers; infiltration issues; fluctuation in results ambipolar perovskite planar heterojunction perovskite solar cells
10 planar heterojunction perovskite solar cells 100 C CH 3 NH 3 I PbCl 2 CH 3 NH 3 PbI 2 Cl
11 planar heterojunction perovskite solar cells B. Conings, L. Baeten, C. De Dobbelaere, J. D Haen, J. Manca, H.-G. Boyen, Adv. Mater. 2014, 26,
12 planar heterojunction perovskite solar cells absorbance / arb. units V / V λ / nm perovskite precursor concentration (wt%) efficiency (%) ± ± ± ± 0.5 J sc / ma cm % ± B. Conings, L. Baeten, C. De Dobbelaere, J. D Haen, J. Manca, H.-G. Boyen, Adv. Mater. 2014, 26,
13 low temperature processing TiO 2 layer typically requires ~500 C to sinter bottleneck towards large-scale / roll-to-roll processes necessity for low(er) temperature fabrication intensity particle diameter (nm) B. Conings, L. Baeten, T. Jacobs, R. Dera, J. D Haen, J. Manca, H.-G. Boyen, submitted
14 low temperature processing & performance improvement P3HT Ag CH 3 NH 3 PbI 2 Cl TiO 2 ITO glass 0 full device stack prepared <150 C V (V) J (ma/cm 2 ) J sc = 21.0 ma/cm 2 V oc = V FF = η = 13.6 % 20 B. Conings, L. Baeten, T. Jacobs, R. Dera, J. D Haen, J. Manca, H.-G. Boyen, submitted
15 intrinsic stability the$holy$trinity$of$photovoltaic$technology$ efficiency perovskite? lifetime cost
16 intrinsic stability - it will get hot up there perovskite is easily created at slightly elevated temperature we should be suspicious about its stability at slightly elevated temperature
17 intrinsic stability 85 C as in IEC test
18 intrinsic stability impact of atmosphere C$ O 2$ 24h$@$85 C$ N 2$ 24h$@$85 C$ air $
19 intrinsic stability - crystalline properties upon degradation pristine C in O 2 O θ ( ) pristine C in N 2 N θ ( ) PbI 2 2θ ( ) pristine C in ambient air θ ( )
20 intrinsic stability - Friday night experiment H 2 O
21 conclusions! perovskite solar cells possess many of the desirable features for next (4 th?) generation photovoltaics! high efficiencies with simple planar device structure! low temperature fabrication; towards roll-to-roll! questionable intrinsic stability! presence of Pb might or might not be a problem
22 acknowledgements! IMO/IMOMEC dr. Linny Baeten prof. Hans-Gerd Boyen prof. Jean Manca prof. Jan D Haen dr. Christopher de Dobbelaere prof. Marlies K. Van Bael dr. Anitha Ethirajan Lien D Olieslaeger Tanya Jacobs Rafael Dera Bart Ruttens Thijs Vandenreijt Johnny Baccus Bijzonder$Onderzoeksfonds$
23 Thank you for your attention! IMO - IMOMEC INSTITUUT VOOR MATERIAALONDERZOEK Institute for Materials Research Hasselt University Division IMOMEC, IMEC vzw Wetenschapspark Diepenbeek Belgium Tel Fax bert.conings@uhasselt.be
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