How Can We Eliminate Radiation from Radioactive Materials?

Transcription

1 Seventh Annual Conference on the Physics, Chemistry and Biology of Water, Grand Summit, 2012, Oct How Can We Eliminate Radiation from Radioactive Materials? S.Sugihara Research Institute of Engineering Kanagawa University Yokohama, Japan

2 Content I II Introduction Scenario ( Ideas ) for elimination of radioactivity Experiments and Theory short & more than 6 months follow-up and theoretical approaches III IV Results and Discussions Summaries

3 INTRODUCTION Polices from each prefecture in Japan guard to go into the hot spot May

4 INTRODUCTION 346 S v/h Namie machi in May 5 th, km from Fukushima 1 st nuclear plant Max. 420 S v/h in this day Sugihara

5 INTRODUCTION General methods for reduction (?) of radioactivity 1 Only wash by water 2 Adsorption by zeolites Size of ion (pm) ; contaminated matter? Efficiency of absoption? Cs + Cs 1.65 > K 1.33 > Na 0.98 cesium potassium sodium Oxidation-reduction potential (volts) Na; > Cs; K; As the results, Cs must compete with Na and K 3 Reaction with bacteria & plants Practical use? zeolite S-ist

6 INTRODUCTION what is elimination of radioactivity? ---- genuine method / be true to Nature --- Shield : coolant water just like in the reactor how to shield ray and electron beam change Cs to non-radioactive matter Various kinds of elements have been formed as stable ones since the earth was born. S-ist

7 Te I Xe U Periodic table 周期 率表 の一 部 Emitted elements ; Pu Cm 32 from Fuku.1st

8 Elements including a various short half life 7 kinds of Ba

9 INTRODUCTION hydroxyl (surface activity Chemical aspects H 3 O 2 - H 3 O + Hydronium pasteurizing, Elimination of active oxygen Hydogen bond Physics Dissociation of hydrogen bond and movement of electron are important involving light electromagnetic wave Sugihara, Water.J, 2009

10 Computer simulation of water molecule (DV-X Bond Overlap Population Even after braking hydrogen bonds, molecules are still stable Bond Overlap Population in Bond Overlap Population in Ground State Excited State B.O.P.v.s. xin2h2o xiðj Distance vs energy - x H O H O z x H H x Bond Overlap Population Infoton B.O.P.v.s.No.ex.elec.in2H2O H O Numberofexcitedelectrons No. of excited electron 0.5 ~1 vs enegry H H O z itinerant <H + -e - > H Sugihara, Water J x

11 NMR,and water molecule can be smaller Relaxation time & Half -width of spectral 1 City water Value of Active water Active water City water Image of water molecule Distance between collisions Measurement Prof. Takayama 2010 T 2

12 What is the Infoton? Dissociated hydrogen bonds generate the Infoton(s) Registered to Japanese Patent Office, 2008 Infoton H + --e - Similar to EZ water? Symbol mark; <H 2 O = h > bra & ket vector a plasma-like state ( looks like in a metal surface=plasmon) Emit radiation of Far Infrared to THz (10 13 ~ Hz) Long wave length Extended particle like an elementary particle, and described in wave function

13 INTRODUCTION i Wave function of Infoton (r,t ) t H ( r,t ) < H + e > p/e Infoton Cs r r' H * i c grad e A 2 mc d 2 c 2 P (curl A) 2 d 1 2 (r, t) r (r r ' ', t ' ) d d ' momentum transverse wave longitudinal wave P ; momentum, A ; electromagnetic potential, ; electrical charge r r' ; the distance between the nucleus and the Infoton < H + e > p/e.

14 INTRODUCTION low frequency Macro scopic aspects for shielding high frequency longer wavelength shorter wavelength such as Infoton (ex. Far Infrared and/or THz) (radiation ) -ray ( photon ) is absorbed by Infoton <H + --e - > (left hand side) Shielding=resonance =like resonance circuit in the devices ( Transition of energy is accompanied with an absorption of one quantum )

15 Is it possible the reaction between Cs and Infoton < H + --e - > Radiation ; energy as follows; Cs Infoton < H + -e - > Hyperboloid potential Cs 137 energy 662keV Cs ~1365 kev Kobe Univ. Hyperboloid and Gauss curvature 3 2 r K ( p) lim r 0 r 3 L p ( r) L p ( r ); circumference of geodesic line r ; distance between Cs & infoton m ) Larger curvature differential Momentum of Infoton becomes larger

16 Cs137 How can Cs interact with Infoton? infoton Pommel shape potential Ba 138 etc.

17 Synthesis of elements from Cs application of group theory A + 1 = Ba Z + 1 = 56 A+ 2 = La Z + 2 = 57 A + 3 = Ce Z + 3 = 58 A mass Z charge example Cs 3 <H+e> 2 <H+e> + 1 <H+e> 4 <H+e> 2 <H+e> + 2 <H+e>

18 Another Mathematical Postulation Local field theory with operator math. (D,t ) P ; proton field in Cs, (D,T ) I ; Infoton field model; < Cs >--<H + --e - > spin is regarded 1) Overlap on two operators Simultaneouly 2) Separation on two operators be formed! Now requirement are ; Operator (X, t) occupies field D p annihilation operator ; Cs Operator (X, t) occupies field D I creation operator ; Ba conjugate

19 H+--e- e Application of Multiplication method in Group Theory Cs H+--e- p/e 2 < > 3 < > Ba 52%, La 32 %, Ce 16%

20 Exp. 1 Radioactivity changed Place : 23km from Fukushima N.P.site 2011/4/3-4 半減期からの計算 from half life 250 S/h S/h S/h /4/3 12: /4/3 12: /4/3 12: /4/3 17: /4/4 9: /4/7 9:40 線量 (μsv/h) 通常低減線量 After an hour After 7 hours The soil was placed in activated pot (1.9 L ).

21 Exp. 2 Radioactivity changed residual radioactivity up to one month Residual (%) 100 From half life 残量放射能 (%) X 半 log One month Time/log ;17,22,42 時間後 ; 別の計測機関による値 X;9 6 時間後点線は活性化容器内で放置した場合の減衰の推測曲線 1 年 30 年 30 years

22 Exp. 3 Radioactivity changed μsv /h day Follow-up of radiation reduction for 3 months. Soils at 23km from Fukushima N.P.P.

23 Exp. 4 Radioactivity changed μ Sv/ start tim e/h 6 m onths

24 Exp. 5 Radioactivity changed Reduction rate (%) Measurement: high purity Ge detector@ Kobe Univ. Sample 134 Cs (Bq/g) (sample/control ratio) 137 Cs (Bq/g) (sample/control ratio) 40 K (Bq/g) (sample/control ratio) Dry C W et C (0.504) 272 (0.50) GP5-F 111 (0.786) 116 (0.787) 1.35 (0.577) 1)Dry C (20g) Control soil mr/h (0.57 μsv/h ) 2)Wet C (20g) placed in the activated pot with 50 cc water, measured after 6 months. 3)GP5-F (20g) measured at 7 days after Wet C

25 Radiation of elimination due to Synthesis of new elements Analysis by ICP MS method sample/control ratio Ba La C e log scale sample/control ratio for Cs B a La C e M IC A100 M O U 5 M O U 10 M IC A 100 M O U 5 M O U 10 For the control, city water was mixed with the soil. The levels of Ba, La, and Ce detected after the treatment were markedly different from those usually present in soil. Soil + water filtered, then solutions are analyzed.

26 Results of another experimental methods Ba 52%, La 32 %, Ce 16% Experimental results close to theoretical, although they have some discrepancy. Exper. theory

27 Summary We found new idea and experimental results for elimination of radioactivity. Theoretical approaches was proposed; 1) To utilize quantum effect of Infoton from treated water. 2) To apply Group theory for reaction between Cs nuclei and Infoton. Confirmed by experimental way 1) Reduction of radioactivity of soils from the nuclear power plant. 2) Stable elements; Ba, La and Ce were confirmed in analysis

28 Acknowledgements; Mr. K.Hatanaka for Water treatment to get activated devices, And also Mr. S. Katanahara for 100 L transportable-facility to get activated water and instrument of radioactivity (GM counter, Inspector ) Measurement of radioactivity (identification and energy; HPGe ); Professor A. Kobe University Mr. K. Kanagawa University for measurement of ICP mass, and Mrs. ACR Co. for ICP AES. Measurement and sampling of contaminated soil etc.; Mr. Brighton Inc. Mr. M. Emoto for Instrument of radioactivity (GM counter, - Scout )and for financial support.

29 Thank you for your attention